scholarly journals Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter

2021 ◽  
Vol 21 (11) ◽  
pp. 9173-9199
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishna Moorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda Madhab Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Equatorial Indian Ocean ◽  
Mixing State ◽  
The South ◽  
Air Masses ◽  
Continental Outflow ◽  
Mass Concentrations

Abstract. Regional climatic implications of aerosol black carbon (BC), which has a wide variety of anthropogenic sources in large abundance, are well recognized over South Asia. Significant uncertainties remain in its quantification due to a lack of sufficient information on the microphysical properties (its concentration, size, and mixing state with other aerosol components) that determine the absorption potential of BC. In particular, the information on the mixing state of BC is extremely sparse over this region. In this study, the first observations of the size distribution and mixing state of individual refractory black carbon (rBC) particles in the South Asian outflow to the south-eastern Arabian Sea and the northern and equatorial Indian Ocean regions are presented based on measurements using a single particle soot photometer (SP2) aboard the Integrated Campaign for Aerosols, gases, and Radiation Budget (ICARB-2018) ship during winter 2018 (16 January to 13 February). The results revealed significant spatial heterogeneity of BC characteristics. The highest rBC mass concentrations (∼938±293 ng m−3) with the highest relative coating thickness (RCT; the ratio of BC core to its coating diameters) of ∼2.16±0.19 are found over the south-east Arabian Sea (SEAS) region, which is in the proximity of the continental outflow. As we move to farther oceanic regions, though the mass concentrations decreased by nearly half (∼546±80 ng m−3), BC still remained thickly coated (RCT∼2.05±0.07). The air over the remote equatorial Indian Ocean, which received considerable marine air masses compared to the other regions, showed the lowest rBC mass concentrations (∼206±114 ng m−3) with a moderately thick coating (RCT∼1.73±0.16). Even over oceanic regions far from the landmass, regions that received the outflow from the more industrialized east coast/the Bay of Bengal had a thicker coating (∼104 nm) compared to regions that received outflow from the west coast and/or peninsular India (∼86 nm). Although different regions of the ocean depicted contrasting concentrations and mixing state parameters due to the varied extent and nature of the continental outflow as well as the atmospheric lifetime of air masses, the modal parameters of rBC mass–size distributions (mean mass median diameters ∼ 0.19–0.20 µm) were similar over all regions. The mean fraction of BC-containing particles (FBC) varied in the range of 0.08–0.12 (suggesting significant amounts of non-BC particles), whereas the bulk mixing ratio of coating mass to rBC mass was highest (8.31±2.40) over the outflow regions compared to the remote ocean (4.24±1.45), highlighting the role of outflow in providing condensable material for coatings on rBC. These parameters, along with the information on the size-resolved mixing state of BC cores, throw light on the role of sources and secondary processing of their complex mixtures for coatings on BC under highly polluted conditions. Examination of the non-refractory sub-micrometre aerosol chemical composition obtained using the aerosol chemical speciation monitor (ACSM) suggested that the overall aerosol system was sulfate-dominated over the far-oceanic regions. In contrast, organics were equally prominent adjacent to the coastal landmass. An association between the BC mixing state and aerosol chemical composition suggested that sulfate was the probable dominant coating material on rBC cores.

scholarly journals Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter

2020 ◽  
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishnamoorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda M. Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Arabian Sea ◽  
Equatorial Indian Ocean ◽  
Mixing State ◽  
Air Masses ◽  
Continental Outflow ◽  
Mass Concentrations

Abstract. Regional climatic implications of aerosol black carbon (BC) are well recognized over South Asia, which has a wide variety of anthropogenic sources in a large abundance. Significant uncertainties remain in its quantification due to lack of sufficient information on the microphysical properties (its concentration, size, and mixing state with other aerosol components), which determine the absorption potential of BC. Especially the information on mixing state of BC is extremely sparse over this region. In this study, first-ever observations of the size distribution and mixing state of individual refractory black carbon (rBC) particles in the south Asian outflow to Southeastern Arabian Sea, northern and equatorial Indian Ocean regions are presented based on measurements using a single particle soot photometer (SP2) aboard the ship cruise of the Integrated Campaign for Aerosols, gases, and Radiation Budget (ICARB-2018) during winter-2018 (16 January to 13 February). The results revealed significant spatial heterogeneity of BC characteristics. Highest rBC mass concentrations (~ 938 ± 293 ng m−3) with the highest relative coating thickness (RCT; the ratio of BC core to its coating diameters) of ~ 2.16 ± 0.19 are found over the Southeast Arabian Sea (SEAS) region, which is in the proximity of the continental outflow. As we move to farther oceanic regions, though the mass concentrations decreased by nearly half (~ 546 ± 80 ng m−3), BC still remained thickly coated (RCT ~ 2.05 ± 0.07). The air over the remote equatorial Indian Ocean, which received considerable marine air masses compared to the other regions, showed the lowest rBC mass concentrations (~ 206 ± 114 ng m−3), with a moderately thick coating (RCT ~ 1.73 ± 0.16). Even over oceanic regions far from the landmass, regions which received the outflow from more industrialized east coast/the Bay of Bengal had thicker coating (~ 104 nm) compared to regions that received outflow from the west coast/peninsular India (~ 86 nm). Although different regions of the ocean depicted contrasting concentrations and mixing state parameters due to varying extent and nature of the continental outflow as well as the atmospheric lifetime of air masses, the modal parameters of rBC mass-size distributions were similar over all the regions. The observed mono-modal distribution with mean mass median diameters (MMD) in the range of 0.19–0.20 μm suggested mixed sources of BC. The mean fraction of BC containing particles (FBC) varied in the range 0.20–0.28 (suggesting significant amounts of non-BC particles), whereas the bulk mixing ratio of coating mass to rBC mass was highest (8.77 ± 2.77) over the outflow regions compared to the remote ocean (4.29 ± 1.54) highlighting the role of outflow in providing condensable material for coating on rBC. These parameters, along with the information on size-resolved mixing state of BC cores, throw light on the role of sources and secondary processing of their complex mixtures for coating on BC under highly polluted conditions. Examination of the non-refractory sub-micrometre aerosol chemical composition obtained using the aerosol chemical speciation monitor (ACSM) suggested that the overall aerosol system was sulfate dominated over the far-oceanic regions. In contrast, organics were equally prominent adjacent to the coastal landmass. Association between the BC mixing state and aerosol chemical composition suggested that sulfate was the probable dominant coating material on rBC cores.

scholarly journals Supplementary material to "Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter"

2020 ◽  
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishnamoorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda M. Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Mixing State ◽  
The South ◽  
Northern Indian Ocean ◽  
Supplementary Material ◽  
Black Carbon Aerosol

Arabic as a Language of the South Asian Chancery: Bahmani Communications to the Mamluk Sultanate

Arabica ◽  
2020 ◽  
Vol 67 (4) ◽  
pp. 409-435
Author(s):  
Meia Walravens
Keyword(s):  
Indian Ocean ◽  
Fifteenth Century ◽  
Red Sea ◽  
South Asian ◽  
Cultural Exchange ◽  
The South ◽  
Growing Body ◽  
The Indian Ocean

Abstract A growing body of literature on trade and cultural exchange between the Indian Ocean regions has already contributed significantly to our understanding of these processes and the role of language and writing within them. Yet, the question remains how Arabic correspondence played a part in communications between South Asian powers and the rulers in the Red Sea region. In order to begin filling this lacuna, this article studies epistolary writings from the Bahmani Sultanate (748/1347-934/1528) to the Mamluk Sultanate (648/1250-922/1517) during the second half of the ninth/fifteenth century. The contextualisation and discussion of three letters render insight both into the (up to now unstudied) issues at play in Bahmani-Mamluk relations and into the nature of these Arabic texts.

scholarly journals Cloud Condensation Nuclei properties of South Asian outflow over the northern Indian Ocean during winter

2019 ◽  
Author(s):  
Vijayakumar S. Nair ◽  
Jayachandran Venugopalan Nair ◽  
Sobhan Kumar Kompalli ◽  
Mukunda M. Gogoi ◽  
S. Suresh Babu
Keyword(s):  
Indian Ocean ◽  
South Asian ◽  
Cloud Condensation Nuclei ◽  
Geometric Mean ◽  
Equatorial Indian Ocean ◽  
Radiation Budget ◽  
Condensation Nuclei ◽  
The South ◽  
Northern Indian Ocean ◽  
Activation Efficiency

Abstract. Extensive measurements of cloud condensation nuclei (CCN) and condensation nuclei (CN) concentrations in the South Asian outflow to the northern Indian Ocean were carried out on board an instrumented research vessel, as part of the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB) during winter season (January–February 2018). Measurements include a north-south transect across the South Asian plume over the northern Indian Ocean and east–west transect over the equatorial Indian Ocean (~ 2° S), which is far away from the continental sources. South Asian outflow over the northern Indian Ocean is characterized by the high values of CCN number concentration (~ 5000 cm−3), low CCN activation efficiency (~ 25 %) and steep increase in CCN concentration with an increase in supersaturation. In contrast, low CCN concentration (~ 1000 cm−3) with flat supersaturation spectra was found over the equatorial Indian Ocean. The CCN properties exhibited significant dependence on the geometric mean diameter (GMD) of the aerosol number size distribution and CCN activation efficiency decreased to low values (

scholarly journals Secular and orbital-scale variability of equatorial Indian Ocean summer monsoon winds during the late Miocene

2021 ◽  
Author(s):  
Clara T. Bolton ◽  
Emmeline Gray ◽  
Wolfgang Kuhnt ◽  
Ann E. Holbourn ◽  
Julia Lübbers ◽  
...  
Keyword(s):  
Indian Ocean ◽  
South Asian ◽  
Summer Monsoon ◽  
Late Miocene ◽  
Asian Monsoon ◽  
Equatorial Indian Ocean ◽  
South Asian Monsoon ◽  
The South ◽  
Near Surface ◽  
Monsoon Winds

Abstract. In the modern northern Indian Ocean, biological productivity is intimately linked to near-surface oceanographic dynamics forced by the South Asian, or Indian, monsoon. In the late Pleistocene, this strong seasonal signal is transferred to the sedimentary record as strong variance in the precession band (19–23 kyr) because precession dominates low-latitude insolation variations and drives seasonal contrast in oceanographic conditions. In addition, internal climate system feedbacks (e.g. ice-sheet albedo, carbon cycle, topography) play a key role in monsoon variability. Little is known about orbital-scale variability of the monsoon in the pre-Pleistocene, when atmospheric CO2 levels and global temperatures were higher. In addition, many questions remain open regarding the timing of the initiation and intensification of the South Asian monsoon during the Miocene, an interval of significant global climate change that culminated in bipolar glaciation. Here, we present new high-resolution (< 1 kyr) records of export productivity and sediment accumulation from International Ocean Discovery Program Site U1443 in the southernmost Bay of Bengal spanning the late Miocene and earliest Pliocene (9 to 5 million years ago). Underpinned by a new orbitally-tuned benthic isotope stratigraphy, we use X-Ray Fluorescence-derived biogenic barium variations to discern productivity trends and rhythms. Our data show strong eccentricity-modulated precession-band productivity variations throughout the late Miocene, interpreted to reflect insolation forcing of summer monsoon wind strength in the equatorial Indian Ocean. On long timescales, our data support the interpretation that South Asian monsoon winds were already established by 9 Ma, with no apparent intensification over the late Miocene.

scholarly journals Systematic Errors in South Asian Monsoon Simulation: Importance of Equatorial Indian Ocean Processes

2017 ◽  
Vol 30 (20) ◽  
pp. 8159-8178 ◽  
Author(s):  
H. Annamalai ◽  
Bunmei Taguchi ◽  
Julian P. McCreary ◽  
Motoki Nagura ◽  
Toru Miyama
Keyword(s):  
Indian Ocean ◽  
South Asia ◽  
South Asian ◽  
Coupled Model ◽  
Equatorial Indian Ocean ◽  
Coupled Processes ◽  
Cmip5 Models ◽  
Model Errors ◽  
Bjerknes Feedback ◽  
Sst Bias

Abstract Forecasting monsoon rainfall using dynamical climate models has met with little success, partly due to models’ inability to represent the monsoon climatological state accurately. In this article the nature and dynamical causes of their biases are investigated. The approach is to analyze errors in multimodel-mean climatological fields determined from CMIP5, and to carry out sensitivity experiments using a coupled model [the Coupled Model for the Earth Simulator (CFES)] that does represent the monsoon realistically. Precipitation errors in the CMIP5 models persist throughout the annual cycle, with positive (negative) errors occurring over the near-equatorial western Indian Ocean (South Asia). Model errors indicate that an easterly wind stress bias Δτ along the equator begins during April–May and peaks during November; the severity of the Δτ is that the Wyrtki jets, eastward-flowing equatorial currents during the intermonsoon seasons (April–May and October–November), are almost eliminated. An erroneous east–west SST gradient (warm west and cold east) develops in June. The structure of the model errors indicates that they arise from Bjerknes feedback in the equatorial Indian Ocean (EIO). Vertically integrated moisture and moist static energy budgets confirm that warm SST bias in the western EIO anchors moist processes that cause the positive precipitation bias there. In CFES sensitivity experiments in which Δτ or warm SST bias over the western EIO is artificially introduced, errors in the EIO are similar to those in the CMIP5 models; moreover, precipitation over South Asia is reduced. An overall implication of these results is that South Asian rainfall errors in CMIP5 models are linked to errors of coupled processes in the western EIO, and in coupled models correct representation of EIO coupled processes (Bjerknes feedback) is a necessary condition for realistic monsoon simulation.

scholarly journals Trapping, chemistry and export of trace gases in the South Asian summer monsoon observed during CARIBIC flights in 2008

2015 ◽  
Vol 15 (5) ◽  
pp. 6967-7018 ◽  
Author(s):  
A. Rauthe-Schöch ◽  
A. K. Baker ◽  
T. J. Schuck ◽  
C. A. M. Brenninkmeijer ◽  
A. Zahn ◽  
...  
Keyword(s):  
South Asian ◽  
Summer Monsoon ◽  
Asian Summer Monsoon ◽  
Trace Gases ◽  
Particle Dispersion ◽  
Atmospheric Pollutants ◽  
South Asian Summer Monsoon ◽  
The South ◽  
Air Masses ◽  
Asian Summer

Abstract. The CARIBIC (Civil Aircraft for the Regular Investigation of the Atmosphere Based on an Instrument Container) passenger aircraft observatory performed in situ measurements at 10–12 km altitude in the South Asian summer monsoon anticyclone between June and September 2008. These measurements enable us to investigate this atmospheric region, which so far has mostly been observed from satellites, using the broad suite of trace gases and aerosols measured by CARIBIC. Elevated levels of a range of atmospheric pollutants were recorded e.g. carbon monoxide, total reactive nitrogen oxides, aerosol particles and several volatile organic compounds. The measurements provide detailed information about the chemical composition of air in different parts of the monsoon anticyclone, particularly of ozone precursors. While covering a range of 3500 km inside the monsoon anticyclone, CARIBIC observations show remarkable consistency, i.e. with regular latitudinal patterns of trace gases during the entire monsoon period. Trajectory calculations indicate that these air masses originated mainly from South Asia and Mainland Southeast Asia. Using the CARIBIC trace gas and aerosol measurements in combination with the Lagrangian particle dispersion model FLEXPART we investigated the characteristics of monsoon outflow and the chemical evolution of air masses during transport. Estimated photochemical ages of the air were found to agree well with transport times from a source region east of 95° E. The photochemical ages of the air in the southern part of the monsoon anticyclone were consistently younger (less than 7 days) and the air masses mostly in an ozone forming chemical regime. In its northern part the air masses were older (up to 13 days) and had unclear ozone formation or destruction potential. Based on analysis of forward trajectories several receptor regions were identified. In addition to predominantly westward transport, we found evidence for efficient transport (within 10 days) to the Pacific and North America, particularly during June and September, and also of cross-tropopause exchange, which was strongest during June and July. Westward transport to Africa and further to the Mediterranean was the main pathway during July.

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