scholarly journals Airborne observation during KORUS-AQ show aerosol optical depth are more spatially self-consistent than aerosol intensive properties

2022 ◽  
Author(s):  
Samuel E. LeBlanc ◽  
Michal Segal-Rozenhaimer ◽  
Jens Redemann ◽  
Connor J. Flynn ◽  
Roy R. Johnson ◽  
...  
Keyword(s):  
Air Quality ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Variability ◽  
Spatial Scales ◽  
Aerosol Emission ◽  
Fine Mode ◽  
Predominant Factor ◽  
Spatio Temporal ◽  
Microphysical Processes

Abstract. Aerosol particles can be emitted, transported, removed, or transformed, leading to aerosol variability at scales impacting the climate (days to years and over hundreds of kilometers) or the air quality (hours to days and from meters to hundreds of kilometers). We present the temporal and spatial scales of changes in AOD (Aerosol Optical Depth), and aerosol size (using Angstrom Exponent; AE, and Fine-Mode-Fraction; FMF) over Korea during the 2016 KORUS-AQ (KORea-US Air Quality) atmospheric experiment. We use measurements and retrievals of aerosol optical properties from airborne instruments for remote sensing (4STAR; Spectrometers for Sky-Scanning Sun Tracking Atmospheric Research) and in situ (LARGE; NASA Langley Aerosol Research Group Experiment) on board the NASA DC-8, geostationary satellite (GOCI; Geostationary Ocean Color Imager; Yonsei aerosol retrieval (YAER) version 2) and reanalysis (MERRA-2; Modern-Era Retrospective Analysis for Research and Applications, version 2). Measurements from 4STAR when flying below 500 m, show an average AOD at 501 nm of 0.43 and an average AE of 1.15 with large standard deviation (0.32 and 0.26 for AOD and AE respectively) likely due to mixing of different aerosol types (fine and coarse mode). The majority of AODs due to fine mode aerosol is observed at altitudes lower than 2 km. Even though there are large variations, for 18 out of the 20 flight days, the column AOD measurements by 4STAR along the NASA DC-8 flight trajectories matches the south-Korean regional average derived from GOCI. We also observed that, contrary to prevalent understanding, AE and FMF are more spatially variable than AOD during KORUS-AQ, even when accounting for potential sampling biases by using Monte Carlo resampling. Averaging between measurements and model for the entire KORUS-AQ period, a reduction in correlation by 15 % is 65.0 km for AOD and shorter at 22.7 km for AE. While there are observational and model differences, the predominant factor influencing spatial-temporal homogeneity is the meteorological period. High spatio-temporal variability occur during the dynamic period (25–31 May), and low spatio-temporal variability occur during blocking Rex pattern (01–07 June). The changes in spatial variability scales between AOD and FMF/AE, while inter-related, indicate that microphysical processes that impact mostly the dominant aerosol size, like aerosol particle formation, growth, and coagulation, vary at shorter scales than the aerosol concentration processes that mostly impact AOD, like aerosol emission, transport, and removal.

scholarly journals A low-cost monitor for measurement of fine particulate matter and aerosol optical depth – Part 2: Citizen-science pilot campaign in northern Colorado

2019 ◽  
Vol 12 (12) ◽  
pp. 6385-6399 ◽  
Author(s):  
Bonne Ford ◽  
Jeffrey R. Pierce ◽  
Eric Wendt ◽  
Marilee Long ◽  
Shantanu Jathar ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
Aerosol Optical Depth ◽  
Citizen Science ◽  
Optical Depth ◽  
Spatial Scales ◽  
Fine Particulate Matter ◽  
Optical Measurements ◽  
Fine Particulate ◽  
Northern Colorado

Abstract. A pilot field campaign was conducted in the fall and winter of 2017 in northern Colorado to test the deployment of the Aerosol Mass and Optical Depth (AMOD) instrument as part of the Citizen-Enabled Aerosol Measurements for Satellites (CEAMS) network. Citizen scientists were recruited to set up the device to take filter and optical measurements of aerosols in their backyards. The goal of the network is to provide more surface particulate matter and aerosol optical depth (AOD) measurements to increase the spatial and temporal resolution of ratios of fine particulate matter (PM2.5) to AOD and to improve satellite-based estimates of air quality. Participants collected 65 filters and 160 multi-wavelength AOD measurements, from which 109 successful PM2.5 : AOD ratios were calculated. We show that PM2.5, AOD, and their ratio (PM2.5 : AOD) often vary substantially over relatively short spatial scales; this spatial variation is not typically resolved by satellite- and model-based PM2.5 exposure estimates. The success of the pilot campaign suggests that citizen-science networks are a viable means for providing new insight into surface air quality. We also discuss lessons learned and AMOD design modifications, which will be used in future wider deployments of the CEAMS network.

scholarly journals Spatio-Temporal Variability of Aerosol Components, Their Optical and Microphysical Properties over North China during Winter Haze in 2012, as Derived from POLDER/PARASOL Satellite Observations

2021 ◽  
Vol 13 (14) ◽  
pp. 2682
Author(s):  
Yang Ou ◽  
Lei Li ◽  
Zhengqiang Li ◽  
Ying Zhang ◽  
Oleg Dubovik ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Air Quality ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Mass Concentration ◽  
North China ◽  
Satellite Observations ◽  
Fine Mode ◽  
The Mean ◽  
Fine Mode Aerosol

Pollution haze is a frequent phenomenon in the North China Plain (NCP) appearing during winter when the aerosol is affected by various pollutant sources and has complex distribution of the aerosol properties, while different aerosol components may have various critical effects on air quality, human health and radiative balance. Therefore, large-scale and accurate aerosol components characterization is urgently and highly desirable but hardly achievable at the regional scale. In this respect, directional and polarimetric remote sensing observations have great potential for providing information about the aerosol components. In this study, a state-of-the-art GRASP/Component approach was employed for attempting to characterize aerosol components in the NCP using POLDER/PARASOL satellite observations. The analysis was done for January 2012 in Beijing (BJ) and Shanxi (SX). The results indicate a peak of the BC mass concentration in an atmospheric column of 82.8 mg/m2 in the SX region, with a mean of 29.2 mg/m2 that is about four times higher than one in BJ (8.9 mg/m2). The mean BrC mass concentrations are, however, higher in BJ (up to ca. 271 mg/m2) than that in SX, which can be attributed to a higher anthropogenic emission. The mean amount of fine ammonium sulfate-like particles observed in the BJ region was three times lower than in SX (131 mg/m2). The study also analyzes meteorological and air quality data for characterizing the pollution event in BJ. During the haze episode, the results suggest a rapid increase in the fine mode aerosol volume concentration associated with a decrease of a scale height of aerosol down to 1500 m. As expected, the values of aerosol optical depth (AOD), absorbing aerosol optical depth (AAOD) and fine mode aerosol optical depth (AODf) are much higher on hazy days. The mass fraction of ammonium sulfate-like aerosol increases from about 13% to 29% and mass concentration increases from 300 mg/m2 to 500 mg/m2. The daily mean PM2.5 concentration and RH independently measured during these reported pollution episodes reach up to 425 g/m3 and 80% correspondingly. The monthly mean mass concentrations of other aerosol components in the BJ are found to be in agreement with the results of previous research works. Finally, a preliminary comparison of these remote sensing derived results with literature and in situ PM2.5 measurements is also presented.

scholarly journals Spatio-Temporal Variability of Aerosol Optical Depth, Total Ozone and NO2 Over East Asia: Strategy for the Validation to the GEMS Scientific Products

2020 ◽  
Vol 12 (14) ◽  
pp. 2256
Author(s):  
Sang Seo Park ◽  
Sang-Woo Kim ◽  
Chang-Keun Song ◽  
Jong-Uk Park ◽  
Kang-Ho Bae
Keyword(s):  
Seasonal Variation ◽  
East Asia ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Validation Study ◽  
Temporal Variability ◽  
Total Column Ozone ◽  
The North ◽  
Spatio Temporal ◽  
Total Column

In this study, the spatio-temporal variability of aerosol optical depth (AOD), total column ozone (TCO), and total column NO2 (TCN) was identified over East Asia using long-term datasets from ground-based and satellite observations. Based on the statistical results, optimized spatio-temporal ranges for the validation study were determined with respect to the target materials. To determine both spatial and temporal ranges for the validation study, we confirmed that the observed datasets can be statistically considered as the same quantity within the ranges. Based on the thresholds of R2>0.95 (temporal) and R>0.95 (spatial), the basic ranges for spatial and temporal scales for AOD validation was within 30 km and 30 min, respectively. Furthermore, the spatial scales for AOD validation showed seasonal variation, which expanded the range to 40 km in summer and autumn. Because of the seasonal change of latitudinal gradient of the TCO, the seasonal variation of the north-south range is a considerable point. For the TCO validation, the north-south range is varied from 0.87° in spring to 1.05° in summer. The spatio-temporal range for TCN validation was 20 min (temporal) and 20–50 km (spatial). However, the nearest value of satellite data was used in the validation because the spatio-temporal variation of TCN is large in summer and autumn. Estimation of the spatio-temporal variability for respective pollutants may contribute to improving the validation of satellite products.

scholarly journals A low-cost monitor for measurement of fine particulate matter and aerosol optical depth – Part 2: Citizen science pilot campaign in northern Colorado

2019 ◽  
Author(s):  
Bonne Ford ◽  
Jeffrey R. Pierce ◽  
Eric Wendt ◽  
Marilee Long ◽  
Shantanu Jathar ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
Aerosol Optical Depth ◽  
Citizen Science ◽  
Optical Depth ◽  
Spatial Scales ◽  
Low Cost ◽  
Lessons Learned ◽  
Optical Measurements ◽  
Northern Colorado

Abstract. A pilot field campaign was conducted in the fall and winter of 2017 in northern Colorado to test the deployment of the Aerosol Mass and Optical Depth (AMOD) instrument as part of the Citizen-Enabled Aerosol Measurements for Satellites (CEAMS) network. Citizen scientists were recruited to set up the device to take filter and optical measurements of aerosols in their backyards. The goal of the network is to provide more surface particulate matter and aerosol optical depth (AOD) measurements to increase the spatial and temporal resolution of PM2.5 to AOD ratios and to improve satellite-based estimates of air quality. Participants collected 65 filters and 160 multi-wavelength AOD measurements from which 109 successful PM2.5 to AOD ratios were calculated. We show that PM2.5, AOD, and their ratio (PM2.5:AOD) often vary substantially over relatively short spatial scales; this spatial variation is not typically resolved by satellite- and model-based PM2.5 exposure estimates. The success of the pilot campaign suggests that citizen-science networks are a viable means for providing new insight into surface air quality. We also discuss lessons learned and AMOD design modifications, which will be used in future, wider deployments of the CEAMS network.

scholarly journals Monitoring the Spatial Variation of Aerosol Optical Depth and Its Correlation with Land Use/Land Cover in Wuhan, China: A Perspective of Urban Planning

2021 ◽  
Vol 18 (3) ◽  
pp. 1132
Author(s):  
Qijiao Xie ◽  
Qi Sun
Keyword(s):  
Land Use ◽  
Air Quality ◽  
Urban Planning ◽  
Land Cover ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Water Bodies ◽  
Landsat 8 ◽  
Land Use Land Cover ◽  
The Impact

Aerosols significantly affect environmental conditions, air quality, and public health locally, regionally, and globally. Examining the impact of land use/land cover (LULC) on aerosol optical depth (AOD) helps to understand how human activities influence air quality and develop suitable solutions. The Landsat 8 image and Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol products in summer in 2018 were used in LULC classification and AOD retrieval in this study. Spatial statistics and correlation analysis about the relationship between LULC and AOD were performed to examine the impact of LULC on AOD in summer in Wuhan, China. Results indicate that the AOD distribution expressed an obvious “basin effect” in urban development areas: higher AOD values concentrated in water bodies with lower terrain, which were surrounded by the high buildings or mountains with lower AOD values. The AOD values were negatively correlated with the vegetated areas while positively correlated to water bodies and construction lands. The impact of LULC on AOD varied with different contexts in all cases, showing a “context effect”. The regression correlations among the normalized difference vegetation index (NDVI), normalized difference built-up index (NDBI), normalized difference water index (NDWI), and AOD in given landscape contexts were much stronger than those throughout the whole study area. These findings provide sound evidence for urban planning, land use management and air quality improvement.

scholarly journals Aerosol optical depth in the European Brewer Network

2017 ◽  
Author(s):  
Javier López-Solano ◽  
Alberto Redondas ◽  
Thomas Carlund ◽  
Juan J. Rodriguez-Franco ◽  
Henri Diémoz ◽  
...  
Keyword(s):  
Real Time ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Variability ◽  
Input Data ◽  
Spatial And Temporal Variability ◽  
Ultraviolet Range ◽  
Using Data ◽  
Better Than

Abstract. The high spatial and temporal variability of aerosols make networks capable of measuring their properties in near real time of high scientific interest. In this work we present and discuss results of an aerosol optical depth algorithm to be used in the European Brewer Network, which provides data in near real time of more than 30 spectrophotometers located from Tamanrasset (Algeria) to Kangerlussuaq (Greenland). Using data from the Brewer Intercomparison Campaigns in the years 2013 and 2015, and the period in between, plus comparisons with Cimel sunphotometers and UVPFR instruments, we check the precision, stability, and uncertainty of the Brewer AOD in the ultraviolet range from 300 to 320 nm. Our results show a precision better than 0.01, an uncertainty of less than 0.05, and a stability similar to that of the ozone measurements for well-maintained instruments. We also discuss future improvements to our algorithm with respect to the input data, their processing, and the characterization of the Brewer instruments for the measurement of aerosols.

Sign in / Sign up

Export Citation Format

Share Document