scholarly journals Variability and trends in surface solar spectral ultraviolet irradiance in Italy: on the influence of geopotential height and lower-stratospheric ozone

2021 ◽  
Vol 21 (24) ◽  
pp. 18689-18705
Author(s):  
Ilias Fountoulakis ◽  
Henri Diémoz ◽  
Anna Maria Siani ◽  
Alcide di Sarra ◽  
Daniela Meloni ◽  
...  

Abstract. The short- and long-term variability of the surface spectral solar ultraviolet (UV) irradiance is investigated across Italy using high-quality ground-based measurements from three locations: Aosta (45.7∘ N, 7.4∘ E, 570 m a.s.l.), Rome (41.9∘ N, 12.5∘ E, 15 75 m a.s.l.), and Lampedusa (35.5∘ N, 12.6∘ E, 50 m a.s.l.). The three sites are characterized by different environmental conditions and represent almost the full latitudinal extent of the Italian territory. Data of two periods were analysed: 2006–2020 (all sites) and 1996–2020 (Rome only). The main objective of this study is to quantify the effect of the geopotential height (GPH) at 250 hPa on total ozone, and spectral irradiance at 307.5 and 324 nm. We first show that monthly anomalies in GPH, total ozone, and spectral irradiances are correlated amongst the three sites, suggesting that Italy is often affected by the same synoptical weather systems. We further find statistically significant anticorrelations between GPH and monthly anomalies in total ozone for all stations and months. Conversely, we identify positive correlations between GPH and monthly anomalies in spectral irradiance at 307.5 nm for most months. The influence of GPH on short-term variability also hold for long-term trends. For example, long-term changes in total ozone over the period 2006–2020 were associated with changes in GPH for all stations. This suggests that observed negative trends in total ozone were mainly driven by changes in lower-stratospheric ozone as upper-stratospheric ozone was increasing over this period. For several months of the year, positive trends in UV irradiance were observed, and we found that these trends were predominantly caused by changes in clouds and/or aerosols instead of total ozone. For the longer period of 1996–2020, a statistically significant annualized decrease in total ozone of ∼ 0.1 % per year was identified for Rome and could subsequently be attributed to decreasing lower-stratospheric ozone. While positive trends in spectral irradiance at 307.5 nm were observed for several months of this extended period, the negative trend in total ozone did not lead to a positive trend in the spectral irradiance at 307.5 nm in the deseasonalized data. Our study provides evidence that dynamical processes taking place in the troposphere lead to significant variability in total ozone and surface solar UV irradiance.

2021 ◽  
Author(s):  
Ilias Fountoulakis ◽  
Henri Diémoz ◽  
Anna Maria Siani ◽  
Alcide di Sarra ◽  
Daniela Meloni ◽  
...  

Abstract. In this study the short- and long-term variability of the surface spectral solar ultraviolet (UV) irradiance are investigated over Italy using high quality ground based measurements from three sites located at quite different environmental conditions, and covering the full latitudinal extent of the Italian territory: Aosta (45.7° N, 7.4°  E, 570 m a.s.l.), Rome (41.9° N, 12.5° E, 75 m a.s.l.), and Lampedusa (35.5° N, 12.6° E, 50 m a.s.l.). The variability of the irradiances at 307.5 nm, 324 nm, and of the ratio between the 307.5 nm and the 324 nm irradiances were investigated with respect to the corresponding variability in total ozone and the geopotential height at 250 hPa (GPH). The study was performed for two periods: 2006–2020 for all stations, and 1996–2020 only for Rome. A statistically significant correlation between the GPH and total ozone monthly anomalies was found for all stations and all seasons of the year. A corresponding statistically significant correlation was also found in most cases between the GPH and the 307.5 nm irradiance monthly anomalies. The correlation between GPH anomalies at different sites was statistically significant, possibly explaining the strong and significant correlation between the total ozone monthly anomalies at the three sites. A statistically significant decrease of total ozone, of ~0.1 %/year was found for Rome for the period 1996–2020, which however did not induce increasing trends in irradiance at 307.5 nm (neither increasing trends in the ratio between the 307.5 nm and the 324 nm irradiances) at SZA = 67°. Further analyses revealed positive trends in the ratio and the 307.5 nm irradiance at smaller solar zenith angles (SZA), which can be attributed to the fact that total ozone decrease is driven by a decrease in the lower stratosphere while upper stratospheric ozone increases, and the effect of changes of upper stratospheric ozone becoming disproportionately larger for increasing SZA. It was also showed that long-term changes in total ozone follow changes in GPH, which is an additional indication that negative trends in total ozone are mainly driven by changes in lower stratospheric ozone. An anti-correlation between the GPH long-term changes and total ozone was also evident for all stations in 2006–2020. Positive trends in UV irradiance for this latter period which were possibly driven by changes in clouds and/or aerosols were found for Rome and Aosta. This study clearly points out the significance of dynamical processes which take place in the troposphere for the variability of total ozone and surface solar UV irradiance.


2020 ◽  
Vol 645 ◽  
pp. A2
Author(s):  
M. Meftah ◽  
M. Snow ◽  
L. Damé ◽  
D. Bolseé ◽  
N. Pereira ◽  
...  

Context. Solar spectral irradiance (SSI) is the wavelength-dependent energy input to the top of the Earth’s atmosphere. Solar ultraviolet (UV) irradiance represents the primary forcing mechanism for the photochemistry, heating, and dynamics of the Earth’s atmosphere. Hence, both temporal and spectral variations in solar UV irradiance represent crucial inputs to the modeling and understanding of the behavior of the Earth’s atmosphere. Therefore, measuring the long-term solar UV irradiance variations over the 11-year solar activity cycle (and over longer timescales) is fundamental. Thus, each new solar spectral irradiance dataset based on long-term observations represents a major interest and can be used for further investigations of the long-term trend of solar activity and the construction of a homogeneous solar spectral irradiance record. Aims. The main objective of this article is to present a new solar spectral irradiance database (SOLAR-v) with the associated uncertainties. This dataset is based on solar UV irradiance observations (165−300 nm) of the SOLAR/SOLSPEC space-based instrument, which provides measurements of the full-disk SSI during solar cycle 24. Methods. SOLAR/SOLSPEC made solar acquisitions between April 5, 2008 and February 10, 2017. During this period, the instrument was affected by the harsh space environment that introduces instrumental trends (degradation) in the SSI measurements. A new method based on an adaptation of the Multiple Same-Irradiance-Level (MuSIL) technique was used to separate solar variability and any uncorrected instrumental trends in the SOLAR/SOLSPEC UV irradiance measurements. Results. A new method for correcting degradation has been applied to the SOLAR/SOLSPEC UV irradiance records to provide new solar cycle variability results during solar cycle 24. Irradiances are reported at a mean solar distance of 1 astronomical unit (AU). In the 165−242 nm spectral region, the SOLAR/SOLSPEC data agrees with the observations (SORCE/SOLSTICE) and models (SATIRE-S, NRLSSI 2) to within the 1-sigma error envelope. Between 242 and 300 nm, SOLAR/SOLSPEC agrees only with the models.


2016 ◽  
Vol 16 (4) ◽  
pp. 2493-2505 ◽  
Author(s):  
Ilias Fountoulakis ◽  
Alkiviadis F. Bais ◽  
Konstantinos Fragkos ◽  
Charickleia Meleti ◽  
Kleareti Tourpali ◽  
...  

Abstract. In this study, we discuss the short- and the long-term variability of spectral UV irradiance at Thessaloniki, Greece, using a long, quality-controlled data set from two Brewer spectrophotometers. Long-term changes in spectral UV irradiance at 307.5, 324 and 350 nm for the period 1994–2014 are presented for different solar zenith angles and discussed in association with changes in total ozone column (TOC), aerosol optical depth (AOD) and cloudiness observed in the same period. Positive changes in annual mean anomalies of UV irradiance, ranging from 2 to 6 % per decade, have been detected both for clear- and all-sky conditions. The changes are generally greater for larger solar zenith angles and for shorter wavelengths. For clear-skies, these changes are, in most cases, statistically significant at the 95 % confidence limit. Decreases in the aerosol load and weakening of the attenuation by clouds lead to increases in UV irradiance in the summer, of 7–9 % per decade for 64° solar zenith angle. The increasing TOC in winter counteracts the effect of decreasing AOD for this particular season, leading to small, statistically insignificant, negative long-term changes in irradiance at 307.5 nm. Annual mean UV irradiance levels are increasing from 1994 to 2006 and remain relatively stable thereafter, possibly due to the combined changes in the amount and optical properties of aerosols. However, no statistically significant corresponding turning point has been detected in the long-term changes of AOD. The absence of signatures of changes in AOD in the short-term variability of irradiance in the UV-A may have been caused by changes in the single scattering albedo of aerosols, which may counteract the effects of changes in AOD on irradiance. The anti-correlation between the year-to-year variability of the irradiance at 307.5 nm and TOC is clear and becomes clearer as the AOD decreases.


Environments ◽  
2019 ◽  
Vol 7 (1) ◽  
pp. 1 ◽  
Author(s):  
Ilias Fountoulakis ◽  
Henri Diémoz ◽  
Anna-Maria Siani ◽  
Gudrun Laschewski ◽  
Gianluca Filippa ◽  
...  

Review of the existing bibliography shows that the direction and magnitude of the long-term trends of UV irradiance, and their main drivers, vary significantly throughout Europe. Analysis of total ozone and spectral UV data recorded at four European stations during 1996–2017 reveals that long-term changes in UV are mainly driven by changes in aerosols, cloudiness, and surface albedo, while changes in total ozone play a less significant role. The variability of UV irradiance is large throughout Italy due to the complex topography and large latitudinal extension of the country. Analysis of the spectral UV records of the urban site of Rome, and the alpine site of Aosta reveals that differences between the two sites follow the annual cycle of the differences in cloudiness and surface albedo. Comparisons between the noon UV index measured at the ground at the same stations and the corresponding estimates from the Deutscher Wetterdienst (DWD) forecast model and the ozone monitoring instrument (OMI)/Aura observations reveal differences of up to 6 units between individual measurements, which are likely due to the different spatial resolution of the different datasets, and average differences of 0.5–1 unit, possibly related to the use of climatological surface albedo and aerosol optical properties in the retrieval algorithms.


2015 ◽  
Vol 15 (24) ◽  
pp. 35753-35785
Author(s):  
I. Fountoulakis ◽  
A. F. Bais ◽  
K. Fragkos ◽  
C. Meleti ◽  
K. Tourpali ◽  
...  

Abstract. In this study, we discuss the short- and the long-term variability of spectral UV irradiance at Thessaloniki, Greece using a long, quality-controlled data set from two Brewer spectrophotometers. Long-term changes in spectral UV irradiance at 307.5, 324 and 350 nm for the period 1994–2014 are presented for different solar zenith angles and discussed in association to changes in total ozone column (TOC), aerosol optical depth (AOD) and cloudiness observed in the same period. Positive changes in annual mean anomalies of UV irradiance, ranging from 2 to 6 % per decade, have been detected both for clear- and all-sky conditions. The changes are generally greater for larger solar zenith angles and for shorter wavelengths. For clear skies, these changes are, in most cases, statistically significant at the 95 % confidence limit. Decreases in the aerosol load and weakening of the attenuation by clouds lead to increases in UV irradiance in the summer, of 7–9 % per decade for 64° solar zenith angle. The increasing TOC in winter counteracts the effect of decreasing AOD for this particular season, leading to small, statistically insignificant, negative long-term changes in irradiance at 307.5 nm. Annual mean UV irradiance levels are increasing from 1994 to 2006 and remain relatively stable thereafter, possibly due to the combined changes in the amount and optical properties of aerosols. However, no statistically significant corresponding turning point has been detected in the long-term changes of AOD. Trends in irradiance during the two sub-periods are not discussed, because the length of the two datasets is too short for deriving statistically significant estimates. The absence of signatures of changes in AOD in the short-term variability of irradiance in the UV-A may have been caused by changes in the single scattering albedo of aerosols, which may counteract the effects of changes in AOD on irradiance. The anti-correlation between the year-to-year variability of the irradiance at 307.5 nm and TOC is clear and becomes clearer as the AOD decreases.


Author(s):  
Ilias Fountoulakis ◽  
Henri Diémoz ◽  
Annamaria Siani ◽  
Gudrun Laschewski ◽  
Gianluca Filippa ◽  
...  

Review of the existing bibliography shows that the direction and magnitude of the long-term trends of UV irradiance, and their main drivers, vary significantly throughout Europe. Analysis of total ozone and spectral UV data recorded at four European stations during 1996 – 2017 reveals that long-term changes in UV are mainly driven by changes in aerosols, cloudiness, and surface albedo, while changes in total ozone play a less significant role. The variability of UV irradiance is large throughout Italy due to the complex topography and large latitudinal extension of the country. Analysis of the spectral UV records of the urban site of Rome, and the alpine site of Aosta reveals that differences between the two sites follow the annual cycle of the differences in cloudiness and surface albedo. Comparisons between the noon UV index measured at the ground at the same stations and the corresponding estimates from the DWD forecast model and OMI/Aura observations reveal differences of up to 6 units between individual measurements, which are likely due to the different spatial resolution of the different datasets, and average differences of 0.5 – 1 unit, possibly related to the use of climatological surface albedo and aerosol optical properties in the retrieval algorithms.


2008 ◽  
Vol 8 (23) ◽  
pp. 7033-7043 ◽  
Author(s):  
S. Simic ◽  
P. Weihs ◽  
A. Vacek ◽  
H. Kromp-Kolb ◽  
M. Fitzka

Abstract. The influence of variability of atmospheric parameters on short- and long-term changes of spectral UV irradiance measured at the Sonnblick observatory (47.03° N, 12.57° E, 3106 m) during the period from 1994 to 2006 is studied. Measurements were performed with the Brewer #093 single-monochromator spectrophotometer and with a Bentham DM 150 spectroradiometer (double-monochromator). The influence of ozone, albedo, snowline and clouds on UV variability is evaluated for each parameter separately using 10-year climatology. It is found that the effect of total ozone on short-term variability of UV irradiance at 305 nm can be more than 200% and on average more than 50%. Clouds can cause variability of 150% or more and on average 35%. Variability caused by albedo reaches a maximum of 32% in April (6% on average). In summer and autumn, total ozone and clouds strongly influence the variability of UV radiation, whereas in winter and spring ozone has the more pronounced effect. A decrease in snowline height from 3000 m to 800 m a.s.l. enhances the UV irradiance by a factor of 1.24 for clear sky conditions and by a factor of 1.7 for 8/8 cloud cover. Long-term trends are investigated for the time period from 1994 to 2006 based on clear-sky measurements, using the non-parametric Mann-Kendall trend test. Significant downward trends (99% confidence level) are found for solar zenith angle 55° at wavelengths from 305 nm to 324 nm and erythemally weighted irradiance according to CIE, which are caused by an increase in sunshine duration during periods of high total column ozone. Significant trends (90% confidence level) were also found for other combinations of wavelength and SZA.


2016 ◽  
Vol 9 (4) ◽  
pp. 1553-1567 ◽  
Author(s):  
Luca Egli ◽  
Julian Gröbner ◽  
Gregor Hülsen ◽  
Luciano Bachmann ◽  
Mario Blumthaler ◽  
...  

Abstract. The reliable quantification of ultraviolet (UV) radiation at the earth's surface requires accurate measurements of spectral global solar UV irradiance in order to determine the UV exposure to human skin and to understand long-term trends in this parameter. Array spectroradiometers (ASRMs) are small, light, robust and cost-effective instruments, and are increasingly used for spectral irradiance measurements. Within the European EMRP ENV03 project “Solar UV”, new devices, guidelines and characterization methods have been developed to improve solar UV measurements with ASRMs, and support to the end user community has been provided. In order to assess the quality of 14 end user ASRMs, a solar UV intercomparison was held on the measurement platform of the World Radiation Center (PMOD/WRC) in Davos, Switzerland, from 10 to 17 July 2014. The results of the blind intercomparison revealed that ASRMs, currently used for solar UV measurements, show a large variation in the quality of their solar UV measurements. Most of the instruments overestimate the erythema-weighted UV index – in particular at large solar zenith angles – due to stray light contribution in the UV-B range. The spectral analysis of global solar UV irradiance further supported the finding that the uncertainties in the UV-B range are very large due to stray light contribution in this wavelength range. In summary, the UV index may be detected by some commercially available ASRMs within 5 % compared to the world reference spectroradiometer, if well characterized and calibrated, but only for a limited range of solar zenith angles. Generally, the tested instruments are not yet suitable for solar UV measurements for the entire range between 290 and 400 nm under all atmospheric conditions.


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