scholarly journals Experimental and modeled UV erythemal irradiance under overcast conditions: the role of cloud optical depth

2012 ◽  
Vol 12 (8) ◽  
pp. 21241-21266
Author(s):  
M. Antón ◽  
L. Alados-Arboledas ◽  
J. L. Guerrero-Rascado ◽  
M. J. Costa ◽  
J. C. Chiu ◽  
...  

Abstract. This paper evaluates the relationship between the cloud modification factor (CMF) in the ultraviolet erythemal range and the cloud optical depth (COD) retrieved from the Aerosol Robotic Network (AERONET) "cloud mode" algorithm under overcast cloudy conditions (confirmed with sky images) at Granada (Spain). Empirical CMF showed a clear exponential dependence on experimental COD values, decreasing approximately from 0.7 for COD = 10 to 0.25 for COD = 50. In addition, these COD measurements were used as input in the LibRadtran radiative transfer code allowing the simulation of CMF values for the selected overcast cases. The modeled CMF exhibited a dependence on COD similar to the empirical CMF, but modeled values present a strong underestimation with respect to the empirical factors (mean bias of 22%). To explain this high bias, an exhaustive comparison between modeled and experimental UV erythemal irradiance (UVER) data was performed. This exercise revealed that a significant part of the bias (~8%) may be related to code's overestimation of the experimental data for clear-sky conditions. The rest of the bias (~14%) may be attributed to the substantial underestimation of modeled UVER with respect to experimental UVER under overcast conditions, although the correlation between both dataset was high (R2 ~0.93). A sensitive test showed that the main responsible for that underestimation is the experimental AERONET COD used as input in the simulations, which has been retrieved from zenith radiances in the visible range. In this sense, effective COD in the erythemal interval were derived from an iteration procedure based on searching the best match between modeled and experimental UVER values for each selected overcast case. These effective COD values were smaller than AERONET COD data in about 80% of the overcast cases with a mean relative difference of 22%.

2012 ◽  
Vol 12 (23) ◽  
pp. 11723-11732 ◽  
Author(s):  
M. Antón ◽  
L. Alados-Arboledas ◽  
J. L. Guerrero-Rascado ◽  
M. J. Costa ◽  
J. C Chiu ◽  
...  

Abstract. This paper evaluates the relationship between the cloud modification factor (CMF) in the ultraviolet erythemal range and the cloud optical depth (COD) retrieved from the Aerosol Robotic Network (AERONET) "cloud mode" algorithm under overcast cloudy conditions (confirmed with sky images) at Granada, Spain, mainly for non-precipitating, overcast and relatively homogenous water clouds. Empirical CMF showed a clear exponential dependence on experimental COD values, decreasing approximately from 0.7 for COD = 10 to 0.25 for COD = 50. In addition, these COD measurements were used as input in the LibRadtran radiative transfer code allowing the simulation of CMF values for the selected overcast cases. The modeled CMF exhibited a dependence on COD similar to the empirical CMF, but modeled values present a strong underestimation with respect to the empirical factors (mean bias of 22%). To explain this high bias, an exhaustive comparison between modeled and experimental UV erythemal irradiance (UVER) data was performed. The comparison revealed that the radiative transfer simulations were 8% higher than the observations for clear-sky conditions. The rest of the bias (~14%) may be attributed to the substantial underestimation of modeled UVER with respect to experimental UVER under overcast conditions, although the correlation between both dataset was high (R2 ~ 0.93). A sensitive test showed that the main reason responsible for that underestimation is the experimental AERONET COD used as input in the simulations, which has been retrieved from zenith radiances in the visible range. In this sense, effective COD in the erythemal interval were derived from an iteration procedure based on searching the best match between modeled and experimental UVER values for each selected overcast case. These effective COD values were smaller than AERONET COD data in about 80% of the overcast cases with a mean relative difference of 22%.


2017 ◽  
Vol 17 (9) ◽  
pp. 5991-6001 ◽  
Author(s):  
Antti Arola ◽  
Thomas F. Eck ◽  
Harri Kokkola ◽  
Mikko R. A. Pitkänen ◽  
Sami Romakkaniemi

Abstract. AERONET (AErosol RObotic NETwork), which is a network of ground-based sun photometers, produces a data product called the aerosol spectral deconvolution algorithm (SDA) that utilizes spectral total aerosol optical depth (AOD) data to infer the component fine- and coarse-mode optical depths at 500 nm. Based on its assumptions, SDA identifies cloud optical depth as the coarse-mode AOD component and therefore effectively computes the fine-mode AOD also in mixed cloud–aerosol observations. Therefore, it can be argued that the more representative AOD for fine-mode fraction should be based on all direct sun measurements and not only on those cloud screened for clear-sky conditions, i.e., on those from level 1 (L1) instead of level 2 (L2) in AERONET. The objective of our study was to assess, including all the available AERONET sites, how the fine-mode AOD is enhanced in cloudy conditions, contrasting SDA L1 and L2 in our analysis. Assuming that the cloud screening correctly separates the cloudy and clear-sky conditions, then the increases in fine-mode AOD can be due to various cloud-related processes, mainly by the strong hygroscopic growth of particles in the vicinity of clouds and in-cloud processing leading to growth of accumulation mode particles. We estimated these cloud-related enhancements in fine-mode AOD seasonally and found, for instance, that in June–August season the average over all the AERONET sites was 0.011, when total fine-mode AOD from L2 data was 0.154; therefore, the relative enhancement was 7 %. The enhancements were largest, both absolutely and relatively, in East Asia; for example, in June–August season the absolute and relative differences in fine-mode AOD, between L1 and L2 measurements, were 0.022 and 10 %, respectively. Corresponding values in North America and Europe were about 0.01 and 6–7 %. In some highly polluted areas, the enhancement is greater than these regional averages, e.g., in Beijing region and in June–July–August (JJA) season the corresponding absolute values were about 0.1. It is difficult to separate the fine-mode AOD enhancements due to in-cloud processing and hygroscopic growth, but we attempted to get some understanding by conducting a similar analysis for SDA-based fine-mode Ångström exponent (AE) patterns. Moreover, we exploited a cloud parcel model, in order to understand in detail the relative role of different processes. We found that in marine conditions, were aerosol concentration are low and cloud scavenging is efficient, the AE changes in opposite direction than in the more polluted conditions, were hygroscopic growth of particles leads to a negative AE change.


2016 ◽  
Author(s):  
Iolanda Ialongo ◽  
Jay Herman ◽  
Nick Krotkov ◽  
Lok Lamsal ◽  
Folkert Boersma ◽  
...  

Abstract. We present the comparison of satellite-based OMI (Ozone Monitoring Instrument) NO2 products with ground-based observations in Helsinki. OMI NO2 total columns, available from standard product (SP) and DOMINO algorithm, are compared with the measurements performed by the Pandora spectrometer in Helsinki in 2012. The relative difference between Pandora #21 and OMI SP retrievals is 4 % and −6 % for clear sky and all sky conditions, respectively. DOMINO NO2 retrievals showed slightly lower total columns with median differences about −5 % and −14 % for clear sky and all sky conditions, respectively. Large differences often correspond to cloudy autumn-winter days with solar zenith angles above 65°. Nevertheless, the differences remain within the retrieval uncertainties. Furthermore, the weekly and seasonal cycles from OMI, Pandora and NO2 surface concentrations are compared. Both satellite- and ground-based data show a similar weekly cycle, with lower NO2 levels during the weekend compared to the weekdays as result of reduced emissions from traffic and industrial activities. Also the seasonal cycle shows a similar behaviour, even though the results are affected by the fact that most of the data are available during spring-summer because of cloud cover in other seasons. This is one of few works in which OMI NO2 retrievals are evaluated in a urban site at high latitudes (60° N). Despite the city of Helsinki having relatively small pollution sources, OMI retrievals have proved to be able to describe air quality features and variability similar to surface observations. This adds confidence in using satellite observations for air quality monitoring also at high latitudes.


2020 ◽  
Vol 12 (24) ◽  
pp. 4171
Author(s):  
Xinlu Xia ◽  
Xiaolei Zou

The Hyperspectral Infrared Atmospheric Sounder (HIRAS) onboard the Feng Yun-3D (FY-3D) satellite is the first Chinese hyperspectral infrared instrument. In this study, an improved cloud detection scheme using brightness temperature observations from paired HIRAS long-wave infrared (LWIR) and short-wave infrared (SWIR) channels at CO2 absorption bands (15-μm and 4.3-μm) is developed. The weighting function broadness and a set of height-dependent thresholds of cloud-sensitive-level differences are incorporated into pairing LWIR and SWIR channels. HIRAS brightness temperature observations made under clear-sky conditions during a training period are used to develop a set of linear regression equations between paired LWIR and SWIR channels. Moderate-resolution Imaging Spectroradiometer (MODIS) cloud mask data are used for selecting HIRAS clear-sky observations. Cloud Emission and Scattering Indices (CESIs) are defined as the differences in SWIR channels between HIRAS observations and regression simulations from LWIR observations. The cloud retrieval products of ice cloud optical depth and cloud-top pressure from the Atmospheric Infrared Sounder (AIRS) are used to illustrate the effectiveness of the proposed cloud detection scheme for FY-3D HIRAS observations. Results show that the distributions of modified CESIs at different altitudes can capture features in the distributions of AIRS-retrieved ice cloud optical depth and cloud-top pressure better than the CESIs obtained by the original method.


2008 ◽  
Vol 8 (17) ◽  
pp. 5393-5401 ◽  
Author(s):  
A. Pribullová ◽  
M. Chmelík

Abstract. Maps of solar erythemal ultraviolet (EUV) irradiance daily doses were created for every month with a horizontal resolution of 500 m at the geographical domain 47.15 N–49.86 N×16.94 E–22.81 E covering the territory of Slovakia. The cloud modification factor for the EUV radiation (cmfUV) was modeled utilizing the relation between the cloud modification factor of global and EUV radiation. The maps of the cmfUV factor were created by utilizing measurements of global irradiance performed at nine observatories during the period 1995–2004 and modeling of the cmfUV dependence on altitude. Maps of the EUV irradiance daily dose corresponded to clear-sky conditions and EUV irradiance daily dose affected by average cloudiness were constructed for mean monthly total ozone, its upper and lower monthly limits, for two probability levels of snow cover occurrence as criteria for the snow effect incorporation in the model and for one day representing typical values for every month. The map-set can be regarded as an atlas of solar EUV radiation over Slovakia.


2011 ◽  
Vol 11 (7) ◽  
pp. 3281-3289 ◽  
Author(s):  
J. Xu ◽  
C. Li ◽  
H. Shi ◽  
Q. He ◽  
L. Pan

Abstract. This study investigated the decadal variation of the direct surface solar radiation (DiSR) and the diffuse surface solar radiation (DfSR) during 1961–2008 in the Shanghai megacity as well as their relationships to Aerosol Optical Depth (AOD) under clear-sky conditions. Three successive periods with unique features of long term variation of DiSR were identified for both clear-sky and all-sky conditions: a "dimming" period from the late 1960s to the mid 1980s, a "stabilization"/"slight brightening" period from the mid 1980s to the mid 1990s, and a "renewed dimming" period thereafter. During the two dimming periods of DiSR, DfSR brightened significantly under clear-sky conditions, indicating that change in atmospheric transparency resulting from aerosol emission has an important role on decadal variation of surface solar radiation (SSR) over this area. The analysis on the relationship between the Moderate-resolution Imaging Spectroradiometer (MODIS) retrieved AOD and the corresponding hourly measurements of DiSR and DfSR under clear-sky conditions clearly revealed that AOD is significantly correlated and anti-correlated with DfSR and DiSR, respectively, both above 99% confidence in all seasons, indicating the great impact of aerosols on SSR through absorption and/or scattering in the atmosphere. In addition, both AOD and the corresponding DiSR and DfSR measured during the satellite passage over Shanghai show obvious weekly cycles. On weekends, AOD is lower than the weekly average, corresponding to higher DiSR and lower DfSR, while the opposite pattern was true for weekdays. Less AOD on weekends due to the reduction of transportation and industrial activities results in enhancement of atmospheric transparency under cloud free conditions so as to increase DiSR and decrease DfSR simultaneously. Results show that aerosol loading from the anthropogenic emissions is an important modulator for the long term variation of SSR in Shanghai.


2012 ◽  
Vol 29 (6) ◽  
pp. 857-866 ◽  
Author(s):  
Wilawan Kumharn ◽  
John S. Rimmer ◽  
Andrew R. D. Smedley ◽  
Toh Ying Ying ◽  
Ann R. Webb

Abstract Aerosols play an important role in attenuating solar radiation reaching the earth's surface and are thus important inputs to climate models. Aerosol optical depth is routinely measured in the visible range but little data in the ultraviolet (UV) are available. In the UV range it can be determined from Langley plots of direct-sun measurements from the Brewer spectrophotometer (where conditions allow) and can also be determined as the residual once the ozone and sulfur dioxide have been accounted for in the extinction observed during a normal Brewer direct-sun measurement. By comparing aerosol optical depth derived from Brewer direct-sun data in both the United Kingdom and Malaysia, two very different locations, it is determined that while most of the existing global Brewer network could contribute to aerosol optical depth data, further analysis, such as calculation of the Ångström parameter, would be dependent on latitude and sky conditions.


2012 ◽  
Vol 5 (11) ◽  
pp. 2675-2688 ◽  
Author(s):  
T. Manninen ◽  
A. Riihelä ◽  
G. de Leeuw

Abstract. Ground-based pyranometer measurements of the (clear-sky) broadband surface albedo are affected by the atmospheric conditions (mainly by aerosol particles, water vapour and ozone). A new semi-empirical method for estimating the magnitude of the effect of atmospheric conditions on surface albedo measurements in clear-sky conditions is presented. Global and reflected radiation and/or aerosol optical depth (AOD) at two wavelengths are needed to apply the method. Depending on the aerosol optical depth and the solar zenith angle values, the effect can be as large as 20%. For the cases we tested using data from the Cabauw atmospheric test site in the Netherlands, the atmosphere caused typically up to 5% overestimation of surface albedo with respect to corresponding black-sky surface albedo values.


2014 ◽  
Vol 7 (10) ◽  
pp. 3509-3527 ◽  
Author(s):  
C. Gielen ◽  
M. Van Roozendael ◽  
F. Hendrick ◽  
G. Pinardi ◽  
T. Vlemmix ◽  
...  

Abstract. We present a cloud-screening method based on differential optical absorption spectroscopy (DOAS) measurements, more specifically using intensity measurements and O4 differential slant-column densities (DSCDs). Using the colour index (CI), i.e. the ratio of the radiance at two wavelengths, we define different sky conditions including clear, thin clouds/polluted, fully-cloudy, and heavily polluted. We also flag the presence of broken and scattered clouds. The O4 absorption is a good tracer for cloud-induced light-path changes and is used to detect clouds and discriminate between instances of high aerosol optical depth (AOD) and high cloud optical depth (COD). We apply our cloud screening to MAX-DOAS (multi-axis DOAS) retrievals at three different sites with different typical meteorological conditions, more specifically suburban Beijing (39.75° N, 116.96° E), Brussels (50.78° N, 4.35° E) and Jungfraujoch (46.55° N, 7.98° E). We find that our cloud screening performs well characterizing the different sky conditions. The flags based on the colour index are able to detect changes in visibility due to aerosols and/or (scattered) clouds. The O4-based multiple-scattering flag is able to detect optically thick clouds, and is needed to correctly identify clouds for sites with extreme aerosol pollution. Removing data taken under cloudy conditions results in a better agreement, in both correlation and slope, between the MAX-DOAS AOD retrievals and measurements from other co-located instruments.


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