scholarly journals A new study of sea spray optical properties from multi-sensor spaceborne observations

2014 ◽  
Vol 14 (1) ◽  
pp. 213-244
Author(s):  
K. W. Dawson ◽  
N. Meskhidze ◽  
D. Josset ◽  
S. Gassó

Abstract. Retrievals of aerosol optical depth (AOD) from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite sensor require the assumption of an extinction-to-backscatter ratio, also known as the lidar ratio. This paper evaluates a new method to calculate the lidar ratio of sea spray aerosol using two independent sources: the AOD from the Synergized Optical Depth of Aerosols (SODA) algorithm and the integrated attenuated backscatter from CALIOP. With this method, the particulate lidar ratio can be derived for individual CALIOP retrievals in single aerosol layer columns over the ocean. Global analyses are carried out using CALIOP level 2, 5 km sea spray aerosol layer products and the collocated SODA nighttime data from December 2007 to December 2009. The global mean lidar ratio for sea spray aerosols was found to be 26 sr, roughly 30% higher than the current value prescribed by CALIOP standard retrieval algorithm. Data analysis also showed considerable spatiotemporal variability in the calculated lidar ratio over the remote oceans. The calculated aerosol lidar ratios are shown to be inversely related to the mean ocean surface wind speed: increase in ocean surface wind speed (U10) from 0 to >15 m s−1 reduces the mean lidar ratios for sea spray particles from 32 sr (for 015 m s−1). Such changes in the lidar ratio are expected to have a corresponding effect on the sea spray AOD. The outcomes of this study are relevant for future improvements of the SODA and CALIOP operational product and could lead to more accurate retrievals of sea spray AOD.

2020 ◽  
Vol 12 (12) ◽  
pp. 2034 ◽  
Author(s):  
Hongsu Liu ◽  
Shuanggen Jin ◽  
Qingyun Yan

Ocean surface wind speed is an essential parameter for typhoon monitoring and forecasting. However, traditional satellite and buoy observations are difficult to monitor the typhoon due to high cost and low temporal-spatial resolution. With the development of spaceborne GNSS-R technology, the cyclone global navigation satellite system (CYGNSS) with eight satellites in low-earth orbit provides an opportunity to measure the ocean surface wind speed of typhoons. Though observations are made at the extremely efficient spatial and temporal resolution, its accuracy and reliability are unclear in an actual super typhoon case. In this study, the wind speed variations over the life cycle of the 2018 Typhoon Mangkhut from CYGNSS observations were evaluated and compared with European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Analysis-5 (ERA-5). The results show that the overall root-mean-square error (RMSE) of CYGNSS versus ECMWF was 4.12 m/s, the mean error was 1.36 m/s, and the correlation coefficient was 0.96. For wind speeds lower and greater than 15 m/s, the RMSE of CYGNSS versus ECMWF were 1.02 and 4.36 m/s, the mean errors were 0.05 and 1.61 m/s, the correlation coefficients were 0.91 and 0.90, and the average relative errors were 9.8% and 11.6%, respectively. When the typhoon reached a strong typhoon or super typhoon, the RMSE of CYGNSS with respect to ERA-5 from ECMWF was 5.07 m/s; the mean error was 3.57 m/s; the correlation coefficient was 0.52 and the average relative error was 11.0%. The CYGNSS estimation had higher precision for wind speeds below 15 m/s, but degraded when the wind speed was above 15 m/s.


2011 ◽  
Vol 11 (16) ◽  
pp. 8777-8790 ◽  
Author(s):  
B. Gantt ◽  
N. Meskhidze ◽  
M. C. Facchini ◽  
M. Rinaldi ◽  
D. Ceburnis ◽  
...  

Abstract. For oceans to be a significant source of primary organic aerosol (POA), sea spray aerosol (SSA) must be highly enriched with organics relative to the bulk seawater. We propose that organic enrichment at the air-sea interface, chemical composition of seawater, and the aerosol size are three main parameters controlling the organic mass fraction of sea spray aerosol (OMSSA). To test this hypothesis, we developed a new marine POA emission function based on a conceptual relationship between the organic enrichment at the air-sea interface and surface wind speed. The resulting parameterization is explored using aerosol chemical composition and surface wind speed from Atlantic and Pacific coastal stations, and satellite-derived ocean concentrations of chlorophyll-a, dissolved organic carbon, and particulate organic carbon. Of all the parameters examined, a multi-variable logistic regression revealed that the combination of 10 m wind speed and surface chlorophyll-a concentration ([Chl-a]) are the most consistent predictors of OMSSA. This relationship, combined with the published aerosol size dependence of OMSSA, resulted in a new parameterization for the organic mass fraction of SSA. Global emissions of marine POA are investigated here by applying this newly-developed relationship to existing sea spray emission functions, satellite-derived [Chl-a], and modeled 10 m winds. Analysis of model simulations shows that global annual submicron marine organic emission associated with sea spray is estimated to be from 2.8 to 5.6 Tg C yr−1. This study provides additional evidence that marine primary organic aerosols are a globally significant source of organics in the atmosphere.


2015 ◽  
Vol 15 (6) ◽  
pp. 3241-3255 ◽  
Author(s):  
K. W. Dawson ◽  
N. Meskhidze ◽  
D. Josset ◽  
S. Gassó

Abstract. Retrievals of aerosol optical depth (AOD) from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite sensor require the assumption of the extinction-to-backscatter ratio, also known as the lidar ratio. This paper evaluates a new method to calculate the lidar ratio of marine aerosols using two independent sources: the AOD from the Synergized Optical Depth of Aerosols (SODA) project and the integrated attenuated backscatter from CALIOP. With this method, the particulate lidar ratio can be derived for individual CALIOP retrievals in single aerosol layer, cloud-free columns over the ocean. Global analyses are carried out using CALIOP level 2, 5 km marine aerosol layer products and the collocated SODA nighttime data from December 2007 to November 2010. The global mean lidar ratio for marine aerosols was found to be 26 sr, roughly 30% higher than the current value prescribed by the CALIOP standard retrieval algorithm. Data analysis also showed considerable spatiotemporal variability in the calculated lidar ratio over the remote oceans. The calculated marine aerosol lidar ratio is found to vary with the mean ocean surface wind speed (U10). An increase in U10 reduces the mean lidar ratio for marine regions from 32 ± 17 sr (for 0 < U10 < 4 m s−1) to 22 ± 7 sr (for U10 > 15 m s−1). Such changes in the lidar ratio are expected to have a corresponding effect on the marine AOD from CALIOP. The outcomes of this study are relevant for future improvements of the SODA and CALIOP operational product and could lead to more accurate retrievals of marine AOD.


2011 ◽  
Vol 11 (22) ◽  
pp. 11401-11413 ◽  
Author(s):  
V. P. Kiliyanpilakkil ◽  
N. Meskhidze

Abstract. The relationship between "clean marine" aerosol optical properties and ocean surface wind speed is explored using remotely sensed data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the CALIPSO satellite and the Advanced Microwave Scanning Radiometer (AMSR-E) on board the AQUA satellite. Detailed data analyses are carried out over 15 regions selected to be representative of different areas of the global ocean for the time period from June 2006 to April 2011. Based on remotely sensed optical properties the CALIPSO algorithm is capable of discriminating "clean marine" aerosols from other types often present over the ocean (such as urban/industrial pollution, desert dust and biomass burning). The global mean optical depth of "clean marine" aerosol at 532 nm (AOD532) is found to be 0.052 ± 0.038 (mean plus or minus standard deviation). The mean layer integrated particulate depolarization ratio of marine aerosols is 0.02 ± 0.016. Integrated attenuated backscatter and color ratio of marine aerosols at 532 nm were found to be 0.003 ± 0.002 sr−1 and 0.530 ± 0.149, respectively. A logistic regression between AOD532 and 10-m surface wind speed (U10) revealed three distinct regimes. For U10 ≤ 4 m s−1 the mean CALIPSO-derived AOD532 is found to be 0.02 ± 0.003 with little dependency on the surface wind speed. For 4 < U10 ≤ 12 m s−1, representing the dominant fraction of all available data, marine aerosol optical depth is linearly correlated with the surface wind speed values, with a slope of 0.006 s m−1. In this intermediate wind speed region, the AOD532 vs. U10 regression slope derived here is comparable to previously reported values. At very high wind speed values (U10 > 18 m s−1), the AOD532-wind speed relationship showed a tendency toward leveling off, asymptotically approaching value of 0.15. The conclusions of this study regarding the aerosol extinction vs. wind speed relationship may have been influenced by the constant lidar ratio used for CALIPSO-derived AOD532. Nevertheless, active satellite sensor used in this study that allows separation of maritime wind induced component of AOD from the total AOD over the ocean could lead to improvements in optical properties of sea spray aerosols and their production mechanisms.


2020 ◽  
Vol 12 (2) ◽  
pp. 155-164
Author(s):  
He Fang ◽  
William Perrie ◽  
Gaofeng Fan ◽  
Tao Xie ◽  
Jingsong Yang

2010 ◽  
Vol 10 (14) ◽  
pp. 6711-6720 ◽  
Author(s):  
Y. Lehahn ◽  
I. Koren ◽  
E. Boss ◽  
Y. Ben-Ami ◽  
O. Altaratz

Abstract. Six years (2003–2008) of satellite measurements of aerosol parameters from the Moderate Resolution Imaging Spectroradiometer (MODIS) and surface wind speeds from Quick Scatterometer (QuikSCAT), the Advanced Microwave Scanning Radiometer (AMSR-E), and the Special Sensor Microwave Imager (SSM/I), are used to provide a comprehensive perspective on the link between surface wind speed and marine aerosol optical depth over tropical and subtropical oceanic regions. A systematic comparison between the satellite derived fields in these regions allows to: (i) separate the relative contribution of wind-induced marine aerosol to the aerosol optical depth; (ii) extract an empirical linear equation linking coarse marine aerosol optical depth and wind intensity; and (iii) identify a time scale for correlating marine aerosol optical depth and surface wind speed. The contribution of wind induced marine aerosol to aerosol optical depth is found to be dominated by the coarse mode elements. When wind intensity exceeds 4 m/s, coarse marine aerosol optical depth is linearly correlated with the surface wind speed, with a remarkably consistent slope of 0.009±0.002 s/m. A detailed time scale analysis shows that the linear correlation between the fields is well kept within a 12 h time frame, while sharply decreasing when the time lag between measurements is longer. The background aerosol optical depth, associated with aerosols that are not produced in-situ through wind driven processes, can be used for estimating the contributions of terrestrial and biogenic marine aerosol to over-ocean satellite retrievals of aerosol optical depth.


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