scholarly journals The atmospheric chemistry general circulation model ECHAM5/MESSy1: consistent simulation of ozone from the surface to the mesosphere

2006 ◽  
Vol 6 (4) ◽  
pp. 6957-7050 ◽  
Author(s):  
P. Jöckel ◽  
H. Tost ◽  
A. Pozzer ◽  
C. Brühl ◽  
J. Buchholz ◽  
...  

Abstract. The new Modular Earth Submodel System (MESSy) describes atmospheric chemistry and meteorological processes in a modular framework, following strict coding standards. It has been coupled to the ECHAM5 general circulation model, which has been slightly modified for this purpose. A 90-layer model version up to 0.01 hPa was used at T42 resolution (~2.8 latitude and longitude) to simulate the lower and middle atmosphere. The model meteorology has been tested to check the influence of the changes to ECHAM5 and the radiation interactions with the new representation of atmospheric composition. A Newtonian relaxation technique was applied in the tropospheric part of the domain to weakly nudge the model towards the analysed meteorology during the period 1998–2005. It is shown that the tropospheric wave forcing of the stratosphere in the model suffices to reproduce the Quasi-Biennial Oscillation and major stratospheric warming events leading e.g. to the vortex split over Antarctica in 2002. Characteristic features such as dehydration and denitrification caused by the sedimentation of polar stratospheric cloud particles and ozone depletion during winter and spring are simulated accurately, although ozone loss in the lower polar stratosphere is slightly underestimated. The model realistically simulates stratosphere-troposphere exchange processes as indicated by comparisons with satellite and in situ measurements. The evaluation of tropospheric chemistry presented here focuses on the distributions of ozone, hydroxyl radicals, carbon monoxide and reactive nitrogen compounds. In spite of minor shortcomings, mostly related to the relatively coarse T42 resolution and the neglect of interannual changes in biomass burning emissions, the main characteristics of the trace gas distributions are generally reproduced well. The MESSy submodels and the ECHAM5/MESSy1 model output are available through the internet on request.

2006 ◽  
Vol 6 (12) ◽  
pp. 5067-5104 ◽  
Author(s):  
P. Jöckel ◽  
H. Tost ◽  
A. Pozzer ◽  
C. Brühl ◽  
J. Buchholz ◽  
...  

Abstract. The new Modular Earth Submodel System (MESSy) describes atmospheric chemistry and meteorological processes in a modular framework, following strict coding standards. It has been coupled to the ECHAM5 general circulation model, which has been slightly modified for this purpose. A 90-layer model setup up to 0.01 hPa was used at spectral T42 resolution to simulate the lower and middle atmosphere. With the high vertical resolution the model simulates the Quasi-Biennial Oscillation. The model meteorology has been tested to check the influence of the changes to ECHAM5 and the radiation interactions with the new representation of atmospheric composition. In the simulations presented here a Newtonian relaxation technique was applied in the tropospheric part of the domain to weakly nudge the model towards the analysed meteorology during the period 1998–2005. This allows an efficient and direct evaluation with satellite and in-situ data. It is shown that the tropospheric wave forcing of the stratosphere in the model suffices to reproduce major stratospheric warming events leading e.g. to the vortex split over Antarctica in 2002. Characteristic features such as dehydration and denitrification caused by the sedimentation of polar stratospheric cloud particles and ozone depletion during winter and spring are simulated well, although ozone loss in the lower polar stratosphere is slightly underestimated. The model realistically simulates stratosphere-troposphere exchange processes as indicated by comparisons with satellite and in situ measurements. The evaluation of tropospheric chemistry presented here focuses on the distributions of ozone, hydroxyl radicals, carbon monoxide and reactive nitrogen compounds. In spite of minor shortcomings, mostly related to the relatively coarse T42 resolution and the neglect of inter-annual changes in biomass burning emissions, the main characteristics of the trace gas distributions are generally reproduced well. The MESSy submodels and the ECHAM5/MESSy1 model output are available through the internet on request.


2019 ◽  
Vol 77 (1) ◽  
pp. 149-165 ◽  
Author(s):  
Yixiong Lu ◽  
Tongwen Wu ◽  
Weihua Jie ◽  
Adam A. Scaife ◽  
Martin B. Andrews ◽  
...  

Abstract It is well known that the stratospheric quasi-biennial oscillation (QBO) is forced by equatorial waves with different horizontal/vertical scales, including Kelvin waves, mixed Rossby–gravity (MRG) waves, inertial gravity waves (GWs), and mesoscale GWs, but the relative contribution of each wave is currently not very clear. Proper representation of these waves is critical to the simulation of the QBO in general circulation models (GCMs). In this study, the vertical resolution in the Beijing Climate Center Atmospheric General Circulation Model (BCC-AGCM) is increased to better represent large-scale waves, and a mesoscale GW parameterization scheme, which is coupled to the convective sources, is implemented to provide unresolved wave forcing of the QBO. Results show that BCC-AGCM can spontaneously generate the QBO with realistic periods, amplitudes, and asymmetric features between westerly and easterly phases. There are significant spatiotemporal variations of parameterized convective GWs, largely contributing to a great degree of variability in the simulated QBO. In the eastward wind shear of the QBO at 20 hPa, forcing provided by resolved waves is 0.1–0.2 m s−1 day−1 and forcing provided by parameterized GWs is ~0.15 m s−1 day−1. On the other hand, westward forcings by resolved waves and parameterized GWs are ~0.1 and 0.4–0.5 m s−1 day−1, respectively. It is inferred that the eastward forcing of the QBO is provided by both Kelvin waves and mesoscale convective GWs, whereas the westward forcing is largely provided by mesoscale GWs. MRG waves barely contribute to the formation of the QBO in the model.


2013 ◽  
Vol 13 (4) ◽  
pp. 11395-11425 ◽  
Author(s):  
C. Brühl ◽  
J. Lelieveld ◽  
M. Höpfner ◽  
H. Tost

Abstract. A multiyear study with the atmospheric chemistry general circulation model EMAC with the aerosol module GMXe at high altitude resolution demonstrates that the sulfur gases COS and SO2, the latter from low-latitude volcanic eruptions, predominantly control the formation of stratospheric aerosol. The model consistently uses the same parameters in the troposphere and stratosphere for 7 aerosol modes applied. Lower boundary conditions for COS and other long-lived trace gases are taken from measurement networks, while estimates of volcanic SO2 emissions are based on satellite observations. We show comparisons with satellite data for aerosol extinction (e.g. SAGE) and SO2 in the middle atmosphere (MIPAS on ENVISAT). This corroborates the interannual variability induced by the Quasi-Biennial Oscillation, which is internally generated by the model. The model also realistically simulates the radiative effects of stratospheric and tropospheric aerosol including the effects on the model dynamics. The medium strength volcanic eruptions of 2005 and 2006 exerted a nonnegligible radiative forcing of up to −0.6 W m−2 in the tropics, while the large Pinatubo eruption caused a maximum though short term tropical forcing of about −10 W m−2. The study also shows that observed upper stratospheric SO2 can be simulated accurately only when a sulphur sink on meteoritic dust is included and the photolysis of gaseous H2SO4 in the near infrared is higher than assumed previously.


2001 ◽  
Vol 19 (4) ◽  
pp. 435-457 ◽  
Author(s):  
R. Hein ◽  
M. Dameris ◽  
C. Schnadt ◽  
C. Land ◽  
V. Grewe ◽  
...  

Abstract. The coupled climate-chemistry model ECHAM4.L39(DLR)/CHEM is presented which enables a simultaneous treatment of meteorology and atmospheric chemistry and their feedbacks. This is the first model which interactively combines a general circulation model with a chemical model, employing most of the important reactions and species necessary to describe the stratospheric and upper tropospheric ozone chemistry, and which is computationally fast enough to allow long-term integrations with currently available computer resources. This is possible as the model time-step used for the chemistry can be chosen as large as the integration time-step for the dynamics. Vertically the atmosphere is discretized by 39 levels from the surface up to the top layer which is centred at 10 hPa, with a relatively high vertical resolution of approximately 700 m near the extra-tropical tropopause. We present the results of a control simulation representing recent conditions (1990) and compare it to available observations. The focus is on investigations of stratospheric dynamics and chemistry relevant to describe the stratospheric ozone layer. ECHAM4.L39(DLR)/CHEM reproduces main features of stratospheric dynamics in the arctic vortex region, including stratospheric warming events. This constitutes a major improvement compared to earlier model versions. However, apparent shortcomings in Antarctic circulation and temperatures persist. The seasonal and interannual variability of the ozone layer is simulated in accordance with observations. Activation and deactivation of chlorine in the polar stratospheric vortices and their inter-hemispheric differences are reproduced. Considering methane oxidation as part of the dynamic-chemistry feedback results in an improved representation of the spatial distribution of stratospheric water vapour concentrations. The current model constitutes a powerful tool to investigate, for instance, the combined direct and indirect effects of anthropogenic trace gas emissions.Key words. Atmospheric composition and structure (middle atmosphere – composition and chemistry) – Meteorology and atmospheric dynamics (general circulation; middle atmosphere dynamics)


2020 ◽  
Vol 12 (5) ◽  
pp. 803-815
Author(s):  
B. N. Chetverushkin ◽  
I. V. Mingalev ◽  
E. A. Fedotova ◽  
K. G. Orlov ◽  
V. M. Chechetkin ◽  
...  

2005 ◽  
Vol 5 (1) ◽  
pp. 961-1006 ◽  
Author(s):  
M. K. van Aalst ◽  
J. Lelieveld ◽  
B. Steil ◽  
C. Brühl ◽  
P. Jöckel ◽  
...  

Abstract. We have performed a 4-year simulation with the Middle Atmosphere General Circulation Model MAECHAM5/MESSy, while slightly nudging the model’s meteorology in the free troposphere (below 113 hPa) towards ECMWF analyses. We show that the nudging 5 technique, which leaves the middle atmosphere almost entirely free, enables comparisons with synoptic observations. The model successfully reproduces many specific features of the interannual variability, including details of the Antarctic vortex structure. In the Arctic, the model captures general features of the interannual variability, but falls short in reproducing the timing of sudden stratospheric warmings. A 10 detailed comparison of the nudged model simulations with ECMWF data shows that the model simulates realistic stratospheric temperature distributions and variabilities, including the temperature minima in the Antarctic vortex. Some small (a few K) model biases were also identified, including a summer cold bias at both poles, and a general cold bias in the lower stratosphere, most pronounced in midlatitudes. A comparison 15 of tracer distributions with HALOE observations shows that the model successfully reproduces specific aspects of the instantaneous circulation. The main tracer transport deficiencies occur in the polar lowermost stratosphere. These are related to the tropopause altitude as well as the tracer advection scheme and model resolution. The additional nudging of equatorial zonal winds, forcing the quasi-biennial oscillation, sig20 nificantly improves stratospheric temperatures and tracer distributions.


2007 ◽  
Vol 7 (1) ◽  
pp. 127-202 ◽  
Author(s):  
A. Pozzer ◽  
P. Jöckel ◽  
H. Tost ◽  
R. Sander ◽  
L. Ganzeveld ◽  
...  

Abstract. The atmospheric-chemistry general circulation model ECHAM5/MESSy1 is evaluated with observations of different organic ozone precursors. This study continues a prior analysis which focused primarily on the representation of atmospheric dynamics and ozone. We use the results of the same reference simulation and apply a statistical analysis using data from numerous field campaigns. The results serve as a basis for future improvements of the model system. ECHAM5/MESSy1 generally reproduces the spatial distribution and the seasonal cycle of carbon monoxide (CO) very well. However, for the background in the northern hemisphere we obtain a negative bias (mainly due to an underestimation of emissions from fossil fuel combustion), and in the high latitude southern hemisphere a yet unexplained positive bias. The model results agree well with observations of alkanes, whereas severe problems in the simulation of alkenes are present. For oxygenated compounds the results are ambiguous: The model results are in good agreement with observations of formaldehyde, but systematic biases are present for methanol and acetone. The discrepancies between the model results and the observations are explained (partly) by means of sensitivity studies.


2016 ◽  
Vol 73 (8) ◽  
pp. 3213-3226 ◽  
Author(s):  
Alvaro de la Cámara ◽  
François Lott ◽  
Valérian Jewtoukoff ◽  
Riwal Plougonven ◽  
Albert Hertzog

Abstract The austral stratospheric final warming date is often predicted with substantial delay in several climate models. This systematic error is generally attributed to insufficient parameterized gravity wave (GW) drag in the stratosphere around 60°S. A simulation with a general circulation model [Laboratoire de Météorologie Dynamique zoom model (LMDZ)] with a much less pronounced bias is used to analyze the contribution of the different types of waves to the dynamics of the final warming. For this purpose, the resolved and unresolved wave forcing of the middle atmosphere during the austral spring are examined in LMDZ and reanalysis data, and a good agreement is found between the two datasets. The role of parameterized orographic and nonorographic GWs in LMDZ is further examined, and it is found that orographic and nonorographic GWs contribute evenly to the GW forcing in the stratosphere, unlike in other climate models, where orographic GWs are the main contributor. This result is shown to be in good agreement with GW-resolving operational analysis products. It is demonstrated that the significant contribution of the nonorographic GWs is due to highly intermittent momentum fluxes produced by the source-related parameterizations used in LMDZ, in qualitative agreement with recent observations. This yields sporadic high-amplitude GWs that break in the stratosphere and force the circulation at lower altitudes than more homogeneously distributed nonorographic GW parameterizations do.


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