scholarly journals Revisiting ocean carbon sequestration by direct injection: A global carbon budget perspective

Author(s):  
Fabian Reith ◽  
David P. Keller ◽  
Andreas Oschlies

Abstract. In this study we look beyond the previously studied effects of oceanic CO2 injections on atmospheric and oceanic reservoirs, and also account for carbon cycle and climate feedbacks between the atmosphere and the terrestrial biosphere. Considering these additional feedbacks is important since backfluxes from the terrestrial biosphere to the atmosphere in response to reducing atmospheric CO2 can further offset the targeted reduction. To quantify these dynamics we use an Earth-system model of intermediate complexity to simulate direct injection of CO2 into the deep ocean as a means of emissions mitigation during a high CO2 emission scenario. In three sets of experiments with different injection depths, we simulate a 100-year injection period of a total of 70 GtC and follow global carbon cycle dynamics over another 900 years. Simulated seawater chemistry changes and marine carbon storage effectiveness are similar to previous studies. As expected, by the end of the injection period avoided emissions fall short of the targeted 70 GtC by 16 % to 30 % as a result of carbon cycle feedbacks and backfluxes in both land and ocean reservoirs. An unexpected feature are effects of the model's internal variability of deep-water formation in the Southern Ocean, which, in some model runs, causes additional oceanic carbon uptake after injection termination relative to a control run without injection and therefore with slightly different atmospheric CO2 and climate. These results of a model that has very low internal climate variability illustrate that attribution of carbon fluxes and accounting for injected CO2 may be very challenging in the real climate system with its much larger internal variability.

2016 ◽  
Vol 7 (4) ◽  
pp. 797-812 ◽  
Author(s):  
Fabian Reith ◽  
David P. Keller ◽  
Andreas Oschlies

Abstract. In this study we look beyond the previously studied effects of oceanic CO2 injections on atmospheric and oceanic reservoirs and also account for carbon cycle and climate feedbacks between the atmosphere and the terrestrial biosphere. Considering these additional feedbacks is important since backfluxes from the terrestrial biosphere to the atmosphere in response to reducing atmospheric CO2 can further offset the targeted reduction. To quantify these dynamics we use an Earth system model of intermediate complexity to simulate direct injection of CO2 into the deep ocean as a means of emissions mitigation during a high CO2 emission scenario. In three sets of experiments with different injection depths, we simulate a 100-year injection period of a total of 70 GtC and follow global carbon cycle dynamics over another 900 years. In additional parameter perturbation runs, we varied the default terrestrial photosynthesis CO2 fertilization parameterization by ±50 % in order to test the sensitivity of this uncertain carbon cycle feedback to the targeted atmospheric carbon reduction through direct CO2 injections. Simulated seawater chemistry changes and marine carbon storage effectiveness are similar to previous studies. As expected, by the end of the injection period avoided emissions fall short of the targeted 70 GtC by 16–30 % as a result of carbon cycle feedbacks and backfluxes in both land and ocean reservoirs. The target emissions reduction in the parameter perturbation simulations is about 0.2 and 2 % more at the end of the injection period and about 9 % less to 1 % more at the end of the simulations when compared to the unperturbed injection runs. An unexpected feature is the effect of the model's internal variability of deep-water formation in the Southern Ocean, which, in some model runs, causes additional oceanic carbon uptake after injection termination relative to a control run without injection and therefore with slightly different atmospheric CO2 and climate. These results of a model that has very low internal climate variability illustrate that the attribution of carbon fluxes and accounting for injected CO2 may be very challenging in the real climate system with its much larger internal variability.


2018 ◽  
Vol 14 (8) ◽  
pp. 1229-1252 ◽  
Author(s):  
Carlye D. Peterson ◽  
Lorraine E. Lisiecki

Abstract. We present a compilation of 127 time series δ13C records from Cibicides wuellerstorfi spanning the last deglaciation (20–6 ka) which is well-suited for reconstructing large-scale carbon cycle changes, especially for comparison with isotope-enabled carbon cycle models. The age models for the δ13C records are derived from regional planktic radiocarbon compilations (Stern and Lisiecki, 2014). The δ13C records were stacked in nine different regions and then combined using volume-weighted averages to create intermediate, deep, and global δ13C stacks. These benthic δ13C stacks are used to reconstruct changes in the size of the terrestrial biosphere and deep ocean carbon storage. The timing of change in global mean δ13C is interpreted to indicate terrestrial biosphere expansion from 19–6 ka. The δ13C gradient between the intermediate and deep ocean, which we interpret as a proxy for deep ocean carbon storage, matches the pattern of atmospheric CO2 change observed in ice core records. The presence of signals associated with the terrestrial biosphere and atmospheric CO2 indicates that the compiled δ13C records have sufficient spatial coverage and time resolution to accurately reconstruct large-scale carbon cycle changes during the glacial termination.


Author(s):  
Corinne Le Quéré ◽  
Robbie M. Andrew ◽  
Pierre Friedlingstein ◽  
Stephen Sitch ◽  
Julia Pongratz ◽  
...  

Abstract. Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere – the "global carbon budget" – is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. CO2 emissions from fossil fuels and industry (EFF) are based on energy statistics and cement production data, respectively, while emissions from land-use change (ELUC), mainly deforestation, are based on land-cover change data and bookkeeping models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) and terrestrial CO2 sink (SLAND) are estimated with global process models constrained by observations. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of our imperfect data and understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the last decade available (2007–2016), EFF was 9.4 ± 0.5 GtC yr−1, ELUC 1.3 ± 0.7 GtC yr−1, GATM 4.7 ± 0.1 GtC yr−1, SOCEAN 2.4 ± 0.5 GtC yr−1, and SLAND 3.0 ± 0.8 GtC yr−1, with a budget imbalance BIM of 0.6 GtC yr−1 indicating overestimated emissions and/or underestimated sinks. For year 2016 alone, the growth in EFF was approximately zero and emissions remained at 9.9 ± 0.5 GtC yr−1. Also for 2016, ELUC was 1.3 ± 0.7 GtC yr−1, GATM was 6.1 ± 0.2 GtC yr−1, SOCEAN was 2.6 ± 0.5 GtC yr−1 and SLAND was 2.7 ± 1.0 GtC yr−1, with a small BIM of −0.3 GtC. GATM continued to be higher in 2016 compared to the past decade (2007–2016), reflecting in part the higher fossil emissions and smaller SLAND for that year consistent with El Niño conditions. The global atmospheric CO2 concentration reached 402.8 ± 0.1 ppm averaged over 2016. For 2017, preliminary data indicate a renewed growth in EFF of +2.0 % (range of 0.8 % to 3.0 %) based on national emissions projections for China, USA, and India, and projections of Gross Domestic Product corrected for recent changes in the carbon intensity of the economy for the rest of the world. For 2017, initial data indicate an increase in atmospheric CO2 concentration of around 5.3 GtC (2.5 ppm), attributed to a combination of increasing emissions and receding El Niño conditions. This living data update documents changes in the methods and data sets used in this new global carbon budget compared with previous publications of this data set (Le Quéré et al., 2016; 2015b; 2015a; 2014; 2013). All results presented here can be downloaded from https://doi.org/10.18160/GCP-2017.


2021 ◽  
Author(s):  
Pierre Friedlingstein

<p>Human activities have an unprecedented impact on the global carbon cycle.  Atmospheric CO2 concentrations have been continuously monitored since 1958, and show a 30% increase, from 315 ppm in 1958 to 412 ppm in 2020. Anthropogenic emissions, primarily from fossil fuel combustion, but also from land-use changes, are the drivers of these changes, with global emissions almost tripling over that period, from 4GtC per year in 1958 to almost 12 GtC per year at present. Although fossil fuel emission declined by about 7% in 2020 due to response to the COVID-19 pandemic, there are no long-term sign of global emissions declining yet, despite climate policies being put in places in many countries.</p><p>The atmospheric CO2 increase induces land and ocean carbon uptake, respectively driven by enhanced photosynthesis, leading to larger land biomass and soil carbon; and by enhanced air-sea CO2 exchange, leading to larger carbon content in the surface ocean and export to the deep ocean. These mechanisms are negative feedbacks in the Earth system and are removing about 50% of the CO2 emitted in the atmosphere. Without these land and ocean carbon sinks, current atmospheric CO2 would already be around 600 ppm.</p><p>However, modelling studies show that climate change reduces land and ocean carbon sinks, hence amplifying the warming. Although there is agreement that such positive feedback will develop over the course of the century, there are not yet clear evidence of a major climate driven reduction of the carbon sinks.  So far, observations and modelling studies of the historical carbon cycle do not show any sign of a tipping point in the global carbon cycle.</p>


2018 ◽  
Vol 10 (1) ◽  
pp. 405-448 ◽  
Author(s):  
Corinne Le Quéré ◽  
Robbie M. Andrew ◽  
Pierre Friedlingstein ◽  
Stephen Sitch ◽  
Julia Pongratz ◽  
...  

Abstract. Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere – the global carbon budget – is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. CO2 emissions from fossil fuels and industry (EFF) are based on energy statistics and cement production data, respectively, while emissions from land-use change (ELUC), mainly deforestation, are based on land-cover change data and bookkeeping models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) and terrestrial CO2 sink (SLAND) are estimated with global process models constrained by observations. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the last decade available (2007–2016), EFF was 9.4 ± 0.5 GtC yr−1, ELUC 1.3 ± 0.7 GtC yr−1, GATM 4.7 ± 0.1 GtC yr−1, SOCEAN 2.4 ± 0.5 GtC yr−1, and SLAND 3.0 ± 0.8 GtC yr−1, with a budget imbalance BIM of 0.6 GtC yr−1 indicating overestimated emissions and/or underestimated sinks. For year 2016 alone, the growth in EFF was approximately zero and emissions remained at 9.9 ± 0.5 GtC yr−1. Also for 2016, ELUC was 1.3 ± 0.7 GtC yr−1, GATM was 6.1 ± 0.2 GtC yr−1, SOCEAN was 2.6 ± 0.5 GtC yr−1, and SLAND was 2.7 ± 1.0 GtC yr−1, with a small BIM of −0.3 GtC. GATM continued to be higher in 2016 compared to the past decade (2007–2016), reflecting in part the high fossil emissions and the small SLAND consistent with El Niño conditions. The global atmospheric CO2 concentration reached 402.8 ± 0.1 ppm averaged over 2016. For 2017, preliminary data for the first 6–9 months indicate a renewed growth in EFF of +2.0 % (range of 0.8 to 3.0 %) based on national emissions projections for China, USA, and India, and projections of gross domestic product (GDP) corrected for recent changes in the carbon intensity of the economy for the rest of the world. This living data update documents changes in the methods and data sets used in this new global carbon budget compared with previous publications of this data set (Le Quéré et al., 2016, 2015b, a, 2014, 2013). All results presented here can be downloaded from https://doi.org/10.18160/GCP-2017 (GCP, 2017).


2018 ◽  
Author(s):  
Carlye Peterson ◽  
Lorraine Lisiecki

Abstract. We present a compilation of 117 time series δ13C records from Cibicides wuellerstorfi spanning the last deglaciation (20–6 kyr) and well-suited for reconstructing large-scale carbon cycle changes, especially for comparison with isotope-enabled carbon cycle models. The age models for the δ13C records are derived from regional planktic radiocarbon compilations (Stern and Lisiecki, 2014). The δ13C records were stacked in nine different regions and then combined using volume-weighted averages to create intermediate, deep, and global δ13C stacks. These benthic δ13C stacks are used to reconstruct mean changes in the size of the terrestrial biosphere and deep ocean carbon storage. The timing of change in global mean δ13C is interpreted to indicate terrestrial biosphere expansion from 19–6 ka. The δ13C gradient between the intermediate and deep ocean, which we interpret as a proxy for deep ocean carbon storage, matches the pattern of atmospheric CO2 change observed in ice core records. The presence of signals associated with the terrestrial biosphere and atmospheric CO2 indicates that the compiled δ13C records have sufficient spatial coverage and time resolution to accurately reconstruct large-scale carbon cycle changes during the glacial termination.


2021 ◽  
Author(s):  
Guilherme Torres Mendonça ◽  
Julia Pongratz ◽  
Christian Reick

<p>The increase in atmospheric CO2 driven by anthropogenic emissions is the main radiative forcing causing climate change. But this increase is not only a result from emissions, but also from changes in the global carbon cycle. These changes arise from feedbacks between climate and the carbon cycle that drive CO2 into or out of the atmosphere in addition to the emissions, thereby either accelerating or buffering climate change. Therefore, understanding the contribution of these feedbacks to the global response of the carbon cycle is crucial in advancing climate research. Currently, this contribution is quantified by the α-β-γ framework (Friedlingstein et al., 2003). But this quantification is only valid for a particular perturbation scenario and time period. In contrast, a recently proposed generalization (Rubino et al., 2016) of this framework for weak perturbations quantifies this contribution for all scenarios and at different time scales. </p><p>Thereby, this generalization provides a systematic framework to investigate the response of the global carbon cycle in terms of the climate-carbon cycle feedbacks. In the present work we employ this framework to study these feedbacks and the airborne fraction in different CMIP5 models. We demonstrate (1) that this generalization of the α-β-γ framework consistently describes the linear dynamics of the carbon cycle in the MPI-ESM; and (2) how by this framework the climate-carbon cycle feedbacks and airborne fraction are quantified at different time scales in CMIP5 models. Our analysis shows that, independently of the perturbation scenario, (1) the net climate-carbon cycle feedback is negative at all time scales; (2) the airborne fraction generally decreases for increasing time scales; and (3) the land biogeochemical feedback dominates the model spread in the airborne fraction at all time scales. This last result therefore emphasizes the need to improve our understanding of this particular feedback.</p><p><strong>References:</strong></p><p>P. Friedlingstein, J.-L. Dufresne, P. Cox, and P. Rayner. How positive is the feedback between climate change and the carbon cycle? Tellus B, 55(2):692–700, 2003.</p><p>M. Rubino, D. Etheridge, C. Trudinger, C. Allison, P. Rayner, I. Enting, R. Mulvaney, L. Steele, R. Langenfelds, W. Sturges, et al. Low atmospheric CO2 levels during the Little Ice Age due to cooling-induced terrestrial uptake. Nature Geoscience, 9(9):691–694, 2016.</p>


2016 ◽  
Author(s):  
G. J. Schürmann ◽  
T. Kaminski ◽  
C. Köstler ◽  
N. Carvalhais ◽  
M. Voßbeck ◽  
...  

Abstract. We describe the Max Planck Institute Carbon Cycle Data Assimilation System (MPI-CCDAS) built around the tangent-linear version of the land surface scheme of the MPI-Earth System Model v1 (JSBACH). The simulated terrestrial biosphere processes (phenology and carbon balance) were constrained by observations of the fraction of photosynthetically active radiation (TIP-FAPAR product) and by observations of atmospheric CO2 at a global set of monitoring stations for the years 2005–2009. The system successfully, and computationally efficiently, improved average foliar area and northern extra-tropical seasonality of foliar area when constrained by TIP-FAPAR. Global net and gross carbon fluxes were improved when constrained by atmospheric CO2, although the system tended to underestimate tropical productivity. Assimilating both data streams jointly allowed the MPI-CCDAS to match both observations (TIP-FAPAR and atmospheric CO2) equally well as the single data stream assimilation cases, therefore overall increasing the appropriateness of the resultant parameter values and biosphere dynamics. Our study thus highlights the role of the TIP-FAPAR product in stabilising the underdetermined atmospheric inversion problem and demonstrates the value of multiple-data stream assimilation for the simulation of terrestrial biosphere dynamics. The constraint on regional gross and net CO2 flux patterns is limited through the parametrisation of the biosphere model. We expect improvement on that aspect through a refined initialisation strategy and inclusion of further biosphere observations as constraints.


2013 ◽  
Vol 4 (2) ◽  
pp. 869-873
Author(s):  
M. Heimann

Abstract. Becker et al. (2013) argue that an afforestation of 0.73 109 ha with Jatropha curcas plants would generate an additional terrestrial carbon sink of 4.3 PgC yr−1, enough to stabilise the atmospheric mixing ratio of carbon dioxide (CO2) at current levels. However, this is not consistent with the dynamics of the global carbon cycle. Using a well established global carbon cycle model, the effect of adding such a hypothetical sink leads to a reduction of atmospheric CO2 levels in the year 2030 by 25 ppm compared to a reference scenario. However, the stabilisation of the atmospheric CO2 concentration requires a much larger additional sink or corresponding reduction of anthropogenic emissions.


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