Validation of nuclear reaction models for incident α-particles

Two different models allowing the calculation of reaction products are confronted with data from α-particle induced reactions. Both models contain a pre-equilibrium part and an equilibrium or compound nucleus part. The models are the exciton model in form of a code written by the author and TALYS. The other model is the intranuclear cascade model in form of the Liege-Saclay formulation incorporated in the PHITS code. The data are angle-integrated proton spectra from reactions with α-particle energies below 720 MeV and excitation functions from multi neutron emission with α-particle energies below 200 MeV.

Theoretical calculation and evaluation of neutron inducedreactions on Pu isotopes

The nuclear data on n+239,240,242,244Pu reactions for the incident energy up to 200 MeV are consistently calculated and evaluated in order to meet the design requirements of Generation-IV reactors and accelerator driven systems. The optical model, the distorted wave Born approximation theory, the Hauser-Feshbach theory, the fission model, the evaporation model, the exciton model and the intranuclear cascade model are used in the calculation, and new experimental data are taken into account. Our data are compared with experimental data and the evaluated data from JENDL-4/HE and TENDL. In addition, the variation tendency of reaction cross sections related to the target mass numbers is obtained, which is very important for the prediction of nuclear data on neutron-actinides reactions because the experimental data are lacking.

Cross-section measurement in the reactions of 136Xe on proton, deuteron and carbon

The isotopic production cross sections for the reactions of 136Xe induced by proton, deuteron and carbon at 168 MeV/u were obtained by using the inverse kinematics technique at RIKEN Radioactive Isotope Beam Factory. The target dependence of the cross sections was investigated systematically. It was found that for the light-mass products, the cross sections on carbon are larger than those on deuteron and proton. The measured cross sections on proton were compared with the previous data at higher reaction energies to study the energy dependence. The experimental results were compared with the theoretical calculations including both the intranuclear cascade and evaporation processes using PHITS and with the EPAX and SPACS empirical parameterizations.

Spallation reaction study for long-lived fission products in nuclear waste

Spallation reaction for the long-lived fission product 107Pd has been studied for the purpose of nuclear waste transmutation. The isotopic-distribution cross sections on both proton and deuteron were obtained at 118 MeV/nucleon in inverse kinematics at the RIKEN Radioactive Isotope Beam Factory. A large cross-section difference was found between the proton and deuteron results for the light-mass products. The data were compared with the SPACS semi-empirical parameterization and the PHITS calculations including both the intranuclear cascade and evaporation processes. In addition, the potential of spallation reaction for transmutation of 107Pd is discussed.