Altitude-resolved shortwave and longwave radiative effects of desert dust in the Mediterranean during the GAMARF campaign: Indications of a net daily cooling in the dust layer

2015 ◽  
Vol 120 (8) ◽  
pp. 3386-3407 ◽  
Author(s):  
D. Meloni ◽  
W. Junkermann ◽  
A. di Sarra ◽  
M. Cacciani ◽  
L. De Silvestri ◽  
...  
2013 ◽  
Vol 13 (11) ◽  
pp. 5489-5504 ◽  
Author(s):  
C. Spyrou ◽  
G. Kallos ◽  
C. Mitsakou ◽  
P. Athanasiadis ◽  
C. Kalogeri ◽  
...  

Abstract. Mineral dust aerosols exert a significant effect on both solar and terrestrial radiation. By absorbing and scattering, the solar radiation aerosols reduce the amount of energy reaching the surface. In addition, aerosols enhance the greenhouse effect by absorbing and emitting outgoing longwave radiation. Desert dust forcing exhibits large regional and temporal variability due to its short lifetime and diverse optical properties, further complicating the quantification of the direct radiative effect (DRE). The complexity of the links and feedbacks of dust on radiative transfer indicate the need for an integrated approach in order to examine these impacts. In order to examine these feedbacks, the SKIRON limited area model has been upgraded to include the RRTMG (Rapid Radiative Transfer Model – GCM) radiative transfer model that takes into consideration the aerosol radiative effects. It was run for a 6 year period. Two sets of simulations were performed, one without the effects of dust and the other including the radiative feedback. The results were first evaluated using aerosol optical depth data to examine the capabilities of the system in describing the desert dust cycle. Then the aerosol feedback on radiative transfer was quantified and the links between dust and radiation were studied. The study has revealed a strong interaction between dust particles and solar and terrestrial radiation, with several implications on the energy budget of the atmosphere. A profound effect is the increased absorption (in the shortwave and longwave) in the lower troposphere and the induced modification of the atmospheric temperature profile. These feedbacks depend strongly on the spatial distribution of dust and have more profound effects where the number of particles is greater, such as near their source.


2018 ◽  
Vol 18 (7) ◽  
pp. 4911-4934 ◽  
Author(s):  
Jonathan Guth ◽  
Virginie Marécal ◽  
Béatrice Josse ◽  
Joaquim Arteta ◽  
Paul Hamer

Abstract. In the frame of the Chemistry-Aerosol Mediterranean Experiment (ChArMEx), we analyse the budget of primary aerosols and secondary inorganic aerosols over the Mediterranean Basin during the years 2012 and 2013. To do this, we use two year-long numerical simulations with the chemistry-transport model MOCAGE validated against satellite- and ground-based measurements. The budget is presented on an annual and a monthly basis on a domain covering 29 to 47° N latitude and 10° W to 38° E longitude. The years 2012 and 2013 show similar seasonal variations. The desert dust is the main contributor to the annual aerosol burden in the Mediterranean region with a peak in spring, and sea salt being the second most important contributor. The secondary inorganic aerosols, taken as a whole, contribute a similar level to sea salt. The results show that all of the considered aerosol types, except for sea salt aerosols, experience net export out of our Mediterranean Basin model domain, and thus this area should be considered as a source region for aerosols globally. Our study showed that 11 % of the desert dust, 22.8 to 39.5 % of the carbonaceous aerosols, 35 % of the sulfate and 9 % of the ammonium emitted or produced into the study domain are exported. The main sources of variability for aerosols between 2012 and 2013 are weather-related variations, acting on emissions processes, and the episodic import of aerosols from North American fires. In order to assess the importance of the anthropogenic emissions of the marine and the coastal areas which are central for the economy of the Mediterranean Basin, we made a sensitivity test simulation. This simulation is similar to the reference simulation but with the removal of the international shipping emissions and the anthropogenic emissions over a 50 km wide band inland along the coast. We showed that around 30 % of the emissions of carbonaceous aerosols and 35 to 60 % of the exported carbonaceous aerosols originates from the marine and coastal areas. The formation of 23, 27 and 27 %, respectively of, ammonium, nitrate and sulfate aerosols is due to the emissions within the marine and coastal area.


2017 ◽  
Author(s):  
Antonis Gkikas ◽  
Vincenzo Obiso ◽  
Carlos Pérez García-Pando ◽  
Oriol Jorba ◽  
Nikos Hatzianastassiou ◽  
...  

2016 ◽  
Vol 16 (13) ◽  
pp. 8609-8642 ◽  
Author(s):  
Antonis Gkikas ◽  
Sara Basart ◽  
Nikos Hatzianastassiou ◽  
Eleni Marinou ◽  
Vassilis Amiridis ◽  
...  

Abstract. The main aim of the present study is to describe the vertical structure of the intense Mediterranean dust outbreaks, based on the use of satellite and surface-based retrievals/measurements. Strong and extreme desert dust (DD) episodes are identified at 1°  ×  1° spatial resolution, over the period March 2000–February 2013, through the implementation of an updated objective and dynamic algorithm. According to the algorithm, strong DD episodes occurring at a specific place correspond to cases in which the daily aerosol optical depth at 550 nm (AOD550 nm) exceeds or equals the long-term mean AOD550 nm (Mean) plus two standard deviations (SD), which is also smaller than Mean+4 × SD. Extreme DD episodes correspond to cases in which the daily AOD550 nm value equals or exceeds Mean+4 × SD. For the identification of DD episodes, additional optical properties (Ångström exponent, fine fraction, effective radius and aerosol index) derived by the MODIS-Terra & Aqua (also AOD retrievals), OMI-Aura and EP-TOMS databases are used as inputs. According to the algorithm using MODIS-Terra data, over the period March 2000–February 2013, strong DD episodes occur more frequently (up to 9.9 episodes year−1) over the western Mediterranean, while the corresponding frequencies for the extreme ones are smaller (up to 3.3 episodes year−1, central Mediterranean Sea). In contrast to their frequency, dust episodes are more intense (AODs up to 4.1), over the central and eastern Mediterranean Sea, off the northern African coasts. Slightly lower frequencies and higher intensities are found when the satellite algorithm operates based on MODIS-Aqua retrievals, for the period 2003–2012. The consistency of the algorithm is successfully tested through the application of an alternative methodology for the determination of DD episodes, which produced similar features of the episodes' frequency and intensity, with just slightly higher frequencies and lower intensities. The performance of the satellite algorithm is assessed against surface-based daily data from 109 sun-photometric (AERONET) and 22 PM10 stations. The agreement between AERONET and MODIS AOD is satisfactory (R = 0.505 − 0.750) and improves considerably when MODIS level 3 retrievals with higher sub-grid spatial representativeness and homogeneity are considered. Through the comparison against PM10 concentrations, it is found that the presence of dust is justified in all ground stations with success scores ranging from 68 to 97 %. However, poor agreement is evident between satellite and ground PM10 observations in the western parts of the Mediterranean, which is attributed to the desert dust outbreaks' vertical extension and the high altitude of dust presence. The CALIOP vertical profiles of pure and polluted dust observations and the associated total backscatter coefficient at 532 nm (β532 nm), indicate that dust particles are mainly detected between 0.5 and 6 km, though they can reach 8 km between the parallels 32 and 38° N in warm seasons. An increased number of CALIOP dust records at higher altitudes is observed with increased latitude, northwards to 40° N, revealing an ascending mode of the dust transport. However, the overall intensity of DD episodes is maximum (up to 0.006 km−1 sr−1) below 2 km and at the southern parts of the study region (30–34° N). Additionally, the average thickness of dust layers gradually decreases from 4 to 2 km, moving from south to north. In spring, dust layers of moderate-to-high β532 nm values ( ∼  0.004 km−1 sr−1) are detected over the Mediterranean (35–42° N), extending from 2 to 4 km. Over the western Mediterranean, dust layers are observed between 2 and 6 km, while their base height is decreased down to 0.5 km for increasing longitudes underlying the role of topography and thermal convection. The vertical profiles of CALIOP β532 nm confirm the multilayered structure of the Mediterranean desert dust outbreaks on both annual and seasonal bases, with several dust layers of variable geometrical characteristics and intensities. A detailed analysis of the vertical structure of specific DD episodes using CALIOP profiles reveals that the consideration of the dust vertical structure is necessary when attempting comparisons between columnar MODIS AOD retrievals and ground PM10 concentrations.


2017 ◽  
Vol 148 ◽  
pp. 16-29 ◽  
Author(s):  
A. Valenzuela ◽  
M.J. Costa ◽  
J.L. Guerrero-Rascado ◽  
D. Bortoli ◽  
F.J. Olmo

2014 ◽  
Vol 141 (690) ◽  
pp. 1634-1645 ◽  
Author(s):  
A. Gkikas ◽  
E. E. Houssos ◽  
C. J. Lolis ◽  
A. Bartzokas ◽  
N. Mihalopoulos ◽  
...  

2016 ◽  
Author(s):  
Umberto Rizza ◽  
Francesca Barnaba ◽  
Mario Marcello Miglietta ◽  
Gian Paolo Gobbi ◽  
Cristina Mangia ◽  
...  

Abstract. In this study, the Weather Research and Forecasting (WRF) Model with online coupled chemistry (WRF-Chem) is applied to simulate an intense Saharan dust outbreak event that took place over the Mediterranean in May 2014. The dust outbreak was generated in correspondence with an omega-like pressure configuration associated with a cyclogenesis in the Atlantic coasts of Spain. This pattern has been recognized as one of the three major cyclogenesis situations responsible for the transport of Saharan dust towards the Central and Western Mediterranean. In fact, in the case investigated here, a cyclone near the Atlantic coasts of Spain is responsible for strong westerly Atlantic winds (about 20 m s−1) reaching the northern Sahara and leading to the lifting of mineral dust. The northward transport is made possible by a ridge over the central Mediterranean associated with the omega-like pressure configuration. WRF-Chem simulations are able to reproduce the synoptic meteorological conditions and the transport outline of the dust outbreak that was in fact characterized by multiple, superimposed dust impulses. The model performances in reproducing the atmospheric desert dust load were evaluated using a multi-platform observational dataset of aerosol and desert dust properties, including optical properties from satellite and ground-based sun-photometers and lidars, plus in situ PM10 data. This comparison allowed us to investigate the model ability in reproducing both the horizontal and the vertical displacement of the dust plume, and its evolution in time. Results show a good agreement between the model and the AERONET-AOD in six sites in the Mediterranean. Comparison with the MODIS-AOD retrieval shows that WRF-Chem satisfactorily resolves the arrival, the time evolution and the horizontal pattern of the dust storm over Central Mediterranean. Comparison with lidar data confirms the desert dust advection to occur in several, superimposed ‘pulses’, as simulated by the model. In most cases the desert dust is shown to arrive above the PBL and then to descend and mix with the local aerosols within it. The vertical displacement of the dust was in good agreement with the lidar soundings with a mean discrepancy along the aerosol extinction of about 40–60 %. The model-measurements comparison for the PM10 and PM2.5 shows a good temporal matching, although there is a clear overestimation of PM10 and PM2.5, of the order of 70 % during the dust peak. This tendency is reduced or even inverted in weak-dust or no-dust conditions, in which model and measured PM10 and PM2.5 are within 30 % and 10–60 %, respectively. For the PM10 metrics it was also possible to investigate the accordance between the model-based and the measurements-based dust-PM10. This comparison confirmed the PM10 model overestimation to be related to over-predicted dust mass by a factor of 140 %.


2004 ◽  
Vol 4 (9/10) ◽  
pp. 2367-2391 ◽  
Author(s):  
F. Barnaba ◽  
G. P. Gobbi

Abstract. The one-year (2001) record of aerosol data from the space borne Moderate Resolution Imaging Spectroradiometer (MODIS) is analyzed focusing on the Mediterranean region. The MODIS aerosol optical thickness standard product (AOT at 550nm) provided over both land and ocean is employed to evaluate the seasonal and spatial variability of the atmospheric particulate over the region. Expected accuracy of the MODIS AOT is (±0.05±0.2xAOT) over land and (±0.03±0.05xAOT) over ocean. The seasonal analysis reveals a significant AOT variability all over the region, with minimum values in Winter (AOT<0.15) and maximum in Summer (AOT>0.2). The spatial variability is also found to be considerable, particularly over land. The impact of some major urban sites and industrialized areas is detectable. For the sole Mediterranean basin, a method (aerosol mask) was implemented to separate the contribution of maritime, continental and desert dust aerosol to the total AOT. Input of both continental and desert dust particles is well captured, showing North-to-South and South-to-North AOT gradients, respectively. A quantitative summary of the AOT seasonal and regional variability is given for different sectors of the Mediterranean basin. Results of this summary were also used to test the aerosol mask assumptions and indicate the method adopted to be suitable for the aerosol type selection. Estimates of the atmospheric aerosol mass load were performed employing specifically-derived mass-to-extinction efficiencies (α). For each aerosol type, a reliable mean α value was determined on the basis of both lidar measurements of extinction and aerosol models. These estimates indicate a total of 43Mtons of desert dust suspended over the basin during 2001. A comparable value is derived for maritime aerosol. Opposite to the dust case, a minor seasonal variability (within 15%) of maritime aerosol mass is found. This latter result is considered a further check of the suitability of the methodology adopted to separate, on the basis of MODIS data, the three aerosol types which dominate the Mediterranean region.


2017 ◽  
Author(s):  
Antonis Gkikas ◽  
Vincenzo Obiso ◽  
Carlos Pérez García-Pando ◽  
Oriol Jorba ◽  
Nikos Hatzianastassiou ◽  
...  

Abstract. The direct radiative effect (DRE) of 20 intense and widespread dust outbreaks that affected the broader Mediterranean basin during the period March 2000 – February 2013, has been calculated with the regional NMMB-MONARCH model. The DREs have been calculated based on short-term simulations (84 hours) for a domain covering the Sahara and most part of the European continent. At midday, desert dust outbreaks induce locally a NET (shortwave plus longwave) strong atmospheric warming (DREATM values up to 285 Wm−2), a strong surface cooling (DRENETSURF values down to −337 Wm−2) whereas they strongly reduce the downward radiation at the ground (DRESURF values down to −589 Wm−2). During nighttime, reverse effects of smaller magnitude are found. At the top of the atmosphere (TOA), positive (planetary warming) DREs up to 85 Wm−2 are found over highly reflective surfaces while negative (planetary cooling) DREs down to −184 Wm−2 are computed over dark surfaces at noon. Desert dust outbreaks significantly affect the regional radiation budget, with regional clear-sky NET DRE values ranging from −13.9 to 2.6 Wm−2, from −43.6 to 4 Wm−2, from −26.3 to 3.9 Wm−2 and from −3.7 to 28 Wm−2 for TOA, SURF, NETSURF and ATM, respectively. Although the shortwave (SW) DREs are larger than the longwave (LW) ones, the latter are comparable or even larger at TOA, particularly over the Sahara at midday. As a response to the strong surface cooling during daytime, dust outbreaks cause a reduction of the regional sensible and latent heat fluxes by up to 45 Wm−2 and 4 Wm−2, respectively, averaged over land areas of the simulation domain. Dust outbreaks reduce the temperature at 2 meters by up to 4 K during day, whereas a reverse tendency of similar magnitude is found during night. Depending on the vertical distribution of dust loads and time, mineral particles heat (cool) the atmosphere by up to 0.9 K (0.8 K) during daytime (nighttime) within atmospheric dust layers. Beneath and above the dust clouds, mineral particles cool (warm) the atmosphere by up to 1.3 K (1.2 K) at noon (night). When dust radiative effects are taken into account in numerical simulations, the total emitted dust and dust AOD, computed on a regional mean basis, are decreased (negative feedback) by 19.5 % and 6.9 %. The consideration of dust radiative effects in numerical simulations improves the model predictive skills. More specifically, it reduces the model positive and negative biases for the downward surface SW and LW radiation, respectively, with respect to Baseline Surface Radiation Network (BSRN) measurements. In addition, they also reduce the model near-surface (at 2 meters) nocturnal cold biases by up to 0.5 K (regional averages), as well as the model warm biases at 950 and 700 hPa, where the dust concentration is maximized, by up to 0.4 K.


2015 ◽  
Vol 15 (6) ◽  
pp. 3303-3326 ◽  
Author(s):  
P. Nabat ◽  
S. Somot ◽  
M. Mallet ◽  
M. Michou ◽  
F. Sevault ◽  
...  

Abstract. The present study investigates the radiative effects of dust aerosols in the Mediterranean region during summer 2012 using a coupled regional aerosol–atmosphere–ocean model (CNRM-RCSM5). A prognostic aerosol scheme, including desert dust, sea salt, organic, black-carbon and sulphate particles, has been integrated to CNRM-RCSM5 in addition to the atmosphere, land surface and ocean components. An evaluation of this aerosol scheme of CNRM-RCSM5, and especially of the dust aerosols, has been performed against in situ and satellite measurements, showing its ability to reproduce the spatial and temporal variability of aerosol optical depth (AOD) over the Mediterranean region in summer 2012. The dust vertical and size distributions have also been evaluated against observations from the TRAQA/ChArMEx campaign. Three simulations have been carried out for summer 2012 with CNRM-RCSM5, including the full prognostic aerosol scheme, only monthly-averaged AOD means from the aerosol scheme or no aerosols at all, in order to focus on the radiative effects of dust particles and the role of the prognostic scheme. Surface short-wave aerosol radiative forcing variability is found to be more than twice as high over regions affected by dust aerosols, when using a prognostic aerosol scheme instead of monthly AOD means. In this case downward surface solar radiation is also found to be better reproduced according to a comparison with several stations across the Mediterranean. A composite study over 14 stations across the Mediterranean, designed to identify days with high dust AOD, also reveals the improvement of the representation of surface temperature brought by the use of the prognostic aerosol scheme. Indeed the surface receives less radiation during dusty days, but only the simulation using the prognostic aerosol scheme is found to reproduce the observed intensity of the dimming and warming on dusty days. Moreover, the radiation and temperature averages over summer 2012 are also modified by the use of prognostic aerosols, mainly because of the differences brought in short-wave aerosol radiative forcing variability. Therefore this first comparison over summer 2012 highlights the importance of the choice of the representation of aerosols in climate models.


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