Temporal disparity of the atmospheric systems contributing to interannual variation of wintertime haze pollution in the North China Plain

2019 ◽  
Vol 40 (1) ◽  
pp. 128-144 ◽  
Author(s):  
Shangfeng Chen ◽  
Jianping Guo ◽  
Linye Song ◽  
Jason B. Cohen ◽  
Yong Wang
Keyword(s):  
Interannual Variation ◽  
North China Plain ◽  
North China ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Atmospheric Systems ◽  
Temporal Disparity

Intra-seasonal differences in the atmospheric systems contributing to interannual variations of autumn haze pollution in the North China Plain

2020 ◽  
Vol 141 (1-2) ◽  
pp. 389-403
Author(s):  
Shangfeng Chen ◽  
Jianping Guo ◽  
Linye Song ◽  
Jason Blake Cohen ◽  
Yong Wang
Keyword(s):  
North China Plain ◽  
North China ◽  
Interannual Variations ◽  
Seasonal Differences ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Atmospheric Systems

scholarly journals Assessment of Meteorological Impact and Emergency Plan for a Heavy Haze Pollution Episode in a Core City of the North China Plain

2020 ◽  
Vol 20 (1) ◽  
pp. 26-42 ◽  
Author(s):  
Simeng Ma ◽  
Zhimei Xiao ◽  
Yufen Zhang ◽  
Litao Wang ◽  
Min Shao
Keyword(s):  
North China Plain ◽  
North China ◽  
Emergency Plan ◽  
The North ◽  
The North China Plain ◽  
Pollution Episode ◽  
Haze Pollution ◽  
Meteorological Impact

scholarly journals Supplementary material to "Nitrate-driven haze pollution during summertime over the North China Plain"

2018 ◽  
Author(s):  
Haiyan Li ◽  
Qiang Zhang ◽  
Bo Zheng ◽  
Chunrong Chen ◽  
Nana Wu ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Supplementary Material

scholarly journals Aerosol optical depth thresholds as a tool to assess diffuse radiation fertilization of the land carbon uptake in China

2017 ◽  
Vol 17 (2) ◽  
pp. 1329-1342 ◽  
Author(s):  
Xu Yue ◽  
Nadine Unger
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
North China Plain ◽  
North China ◽  
Carbon Uptake ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Aerosol Pollution ◽  
Sky Conditions

Abstract. China suffers from frequent haze pollution episodes that alter the surface solar radiation and influence regional carbon uptake by the land biosphere. Here, we apply combined vegetation and radiation modeling and multiple observational datasets to assess the radiative effects of aerosol pollution in China on the regional land carbon uptake for the 2009–2011 period. First, we assess the inherent sensitivity of China's land biosphere to aerosol pollution by defining and calculating two thresholds of aerosol optical depth (AOD) at 550 nm, (i) AODt1, resulting in the maximum net primary productivity (NPP), and (ii) AODt2, such that if local AOD < AODt2, the aerosol diffuse fertilization effect (DFE) always promotes local NPP compared with aerosol-free conditions. Then, we apply the thresholds, satellite data, and interactive vegetation modeling to estimate current impacts of aerosol pollution on land ecosystems. In the northeast, observed AOD is 55 % lower than AODt1, indicating a strong aerosol DFE on local NPP. In the southeastern coastal regions, observed AOD is close to AODt1, suggesting that regional NPP is promoted by the current level of aerosol loading, but that further increases in AOD in this region will weaken the fertilization effects. The North China Plain experiences limited enhancement of NPP by aerosols because observed AOD is 77 % higher than AODt1 but 14 % lower than AODt2. Aerosols always inhibit regional NPP in the southwest because of the persistent high cloud coverage that already substantially reduces the total light availability there. Under clear-sky conditions, simulated NPP shows widespread increases of 20–60 % (35.0 ± 0.9 % on average) by aerosols. Under all-sky conditions, aerosol pollution has spatially contrasting opposite sign effects on NPP from −3 % to +6 % (1.6 ± 0.5 % on average), depending on the local AOD relative to the regional thresholds. Stringent aerosol pollution reductions motivated by public health concerns, especially in the North China Plain and the southwest, will help protect land ecosystem functioning in China and mitigate long-term global warming.

scholarly journals Aerosol–radiation feedback deteriorates the wintertime haze in the North China Plain

2019 ◽  
Vol 19 (13) ◽  
pp. 8703-8719 ◽  
Author(s):  
Jiarui Wu ◽  
Naifang Bei ◽  
Bo Hu ◽  
Suixin Liu ◽  
Meng Zhou ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Air Pollutants ◽  
North China Plain ◽  
North China ◽  
Near Surface ◽  
The North ◽  
The North China Plain ◽  
Incoming Solar Radiation ◽  
Haze Pollution ◽  
Pm2.5 Concentration

Abstract. Atmospheric aerosols scatter or absorb a fraction of the incoming solar radiation to cool or warm the atmosphere, decreasing surface temperature and altering atmospheric stability to further affect the dispersion of air pollutants in the planetary boundary layer (PBL). In the present study, simulations during a persistent and heavy haze pollution episode from 5 December 2015 to 4 January 2016 in the North China Plain (NCP) were performed using the Weather Research and Forecasting model with Chemistry (WRF-Chem) to comprehensively quantify contributions of aerosol shortwave radiative feedback (ARF) to near-surface (around 15 m above the ground surface) PM2.5 mass concentrations. The WRF-Chem model generally performs well in simulating the temporal variations and spatial distributions of air pollutants concentrations compared to observations at ambient monitoring sites in the NCP, and the simulated diurnal variations of aerosol species are also consistent with the measurements in Beijing. Additionally, the model simulates the aerosol radiative properties, the downward shortwave flux, and the PBL height against observations in the NCP well. During the episode, ARF deteriorates the haze pollution, increasing the near-surface PM2.5 concentrations in the NCP by 10.2 µg m−3 or with a contribution of 7.8 % on average. Sensitivity studies have revealed that high loadings of PM2.5 attenuate the incoming solar radiation reaching the surface to cool the low-level atmosphere, suppressing the development of the PBL, decreasing the surface wind speed, further hindering the PM2.5 dispersion, and consequently exacerbating the haze pollution in the NCP. Furthermore, when the near-surface PM2.5 mass concentration increases from around 50 to several hundred µg m−3, ARF contributes to the near-surface PM2.5 by more than 20 % during daytime in the NCP, substantially aggravating the heavy haze formation. However, when the near-surface PM2.5 concentration is less than around 50 µg m−3, ARF generally reduces the near-surface PM2.5 concentration due to the consequent perturbation of atmospheric dynamic fields.

scholarly journals Aerosol chemistry and particle growth events at an urban downwind site in the North China Plain

2018 ◽  
Author(s):  
Yingjie Zhang ◽  
Wei Du ◽  
Yuying Wang ◽  
Qingqing Wang ◽  
Haofei Wang ◽  
...  
Keyword(s):  
Growth Rates ◽  
North China Plain ◽  
North China ◽  
Particle Growth ◽  
Early Morning ◽  
Scanning Mobility Particle Sizer ◽  
Average Mass ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution

Abstract. The North China Plain (NCP) has experienced frequent severe haze pollution events in recent years. While extensive measurements have been made in megacities, aerosol sources, processes, and particle growth at urban downwind sites remain less understood. Here, an Aerosol Chemical Speciation Monitor and a Scanning Mobility Particle Sizer, along with a suite of collocated instruments, were deployed at the downwind site of Xingtai, a highly polluted city in the NCP, for real-time measurements of submicron aerosol (PM1) species and particle number size distributions during May and June 2016. The average mass concentration of PM1 was 30.5 (±19.4) μg m−3, which is significantly lower than that during wintertime. Organic aerosols (OA) constituted the major fraction of PM1 (38 %) followed by sulfate (25 %) and nitrate (14 %). Positive matrix factorization with the Multilinear Engine version 2 showed that oxygenated OA (OOA) was the dominant species in OA throughout the study, on average accounting for 78 % of OA, while traffic and cooking emissions both accounted for 11 % of OA. Our results highlight that aerosol particles at the urban downwind site were highly aged and mainly from secondary formation. However, the diurnal cycle also illustrated the substantial influence of urban emissions on downwind sites, which are characterized by similar pronounced early morning peaks for most aerosol species. New particle formation and growth events were also frequently observed (58 % of the time) on both clean and polluted days. Particle growth rates varying from 1.2 to 4.9 nm h−1 were positively related to the condensation sink during periods with high OOA contributions and also to sulfate concentrations during relatively clean periods. Our results showed that sulfate and OOA played important roles in particle growth during clean periods, while OOA was more important than sulfate during polluted events. Further analyses showed that particle growth rates have no clear dependence on air mass trajectories.

scholarly journals Wintertime aerosol chemistry and haze evolution in an extremely polluted city of the North China Plain: significant contribution from coal and biomass combustion

2017 ◽  
Vol 17 (7) ◽  
pp. 4751-4768 ◽  
Author(s):  
Haiyan Li ◽  
Qi Zhang ◽  
Qiang Zhang ◽  
Chunrong Chen ◽  
Litao Wang ◽  
...  
Keyword(s):  
Air Pollution ◽  
Biomass Burning ◽  
Coal Combustion ◽  
North China Plain ◽  
North China ◽  
Biomass Combustion ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Haze Episode

Abstract. The North China Plain (NCP) frequently experiences heavy haze pollution, particularly during wintertime. In winter 2015–2016, the NCP region suffered several extremely severe haze episodes with air pollution red alerts issued in many cities. We have investigated the sources and aerosol evolution processes of the severe pollution episodes in Handan, a typical industrialized city in the NCP region, using real-time measurements from an intensive field campaign during the winter of 2015–2016. The average (±1σ) concentration of submicron aerosol (PM1) during 3 December 2015–5 February 2016 was 187.6 (±137.5) µg m−3, with the hourly maximum reaching 700.8 µg m−3. Organic was the most abundant component, on average accounting for 45 % of total PM1 mass, followed by sulfate (15 %), nitrate (14 %), ammonium (12 %), chloride (9 %) and black carbon (BC, 5 %). Positive matrix factorization (PMF) with the multilinear engine (ME-2) algorithm identified four major organic aerosol (OA) sources, including traffic emissions represented by a hydrocarbon-like OA (HOA, 7 % of total OA), industrial and residential burning of coal represented by a coal combustion OA (CCOA, 29 % of total OA), open and domestic combustion of wood and crop residuals represented by a biomass burning OA (BBOA, 25 % of total OA), and formation of secondary OA (SOA) in the atmosphere represented by an oxygenated OA (OOA, 39 % of total OA). Emissions of primary OA (POA), which together accounted for 61 % of total OA and 27 % of PM1, are a major cause of air pollution during the winter. Our analysis further uncovered that primary emissions from coal combustion and biomass burning together with secondary formation of sulfate (mainly from SO2 emitted by coal combustion) are important driving factors for haze evolution. However, the bulk composition of PM1 showed comparatively small variations between less polluted periods (daily PM2. 5  ≤  75 µg m−3) and severely polluted periods (daily PM2. 5  >  75 µg m−3), indicating relatively synchronous increases of all aerosol species during haze formation. The case study of a severe haze episode, which lasted 8 days starting with a steady buildup of aerosol pollution followed by a persistently high level of PM1 (326.7–700.8 µg m−3), revealed the significant influence of stagnant meteorological conditions which acerbate air pollution in the Handan region. The haze episode ended with a shift of wind which brought in cleaner air masses from the northwest of Handan and gradually reduced PM1 concentration to  <  50 µg m−3 after 12 h. Aqueous-phase reactions under higher relative humidity (RH) were found to significantly promote the production of secondary inorganic species (especially sulfate) but showed little influence on SOA.

scholarly journals Impact of the Green Light Program on haze pollution in the North China Plain, China

2019 ◽  
Author(s):  
Xin Long ◽  
Xuexi Tie ◽  
Jiamao Zhou ◽  
Wenting Dai ◽  
Xueke Li ◽  
...  
Keyword(s):  
Power Generation ◽  
Emission Reduction ◽  
North China Plain ◽  
North China ◽  
Thermal Power ◽  
Coal Consumption ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Pm2.5 Concentration

Abstract. As the world's largest developing country, China undergoes the ever-increasing demand for electricity during the past few decades. In 1996, China launched the Green Lights Program (GLP), which becomes a national energy conservation activity for saving lighting electricity, as well as an effective reduction of the coal consumption for power generation. Despite of the great success of the GLP, its effects on haze pollution have not been investigated and well understood. This study focused to assess the potential coal-saving induced by the GLP and to estimate the consequent improvements of the haze pollutions in the North China Plain (NCP), because severe haze pollutions often occur in the NCP and a large amount of power plants locate in this region. The estimated potential coal-saving induced by the GLP can reach a massive value of 120–323 million tons, accounting for 6.7–18.0 % of the total coal consumption for thermal power generation in China. In December 2015, there was a massive potential emission reduction of air pollutants from thermal power generation in the NCP, which was estimated to be 20.0–53.8 Gg for NOx and 6.9–18.7 Gg for SO2. The potential emission reductions induced by the GLP played important roles in the haze formation, because the NOx and SO2 are important precursors for the formation of particles. To assess the impact of the GLP on haze pollution, sensitive studies were conducted by applying a regional chemical/dynamical model (WRF-CHEM). The model results suggest that in the lower limit case of emission reduction, the PM2.5 concentration decreases by 2–5 µg m−3 in large areas of the NCP. In the upper limit case of emission reduction, there was much more remarkable decrease in PM2.5 concentration (4–10 µg m−3). This study is a good example to illustrate that scientific innovation can induce important benefits on environment issues, such as haze pollution.

scholarly journals Nitrate-driven urban haze pollution during summertime over the North China Plain

2018 ◽  
Vol 18 (8) ◽  
pp. 5293-5306 ◽  
Author(s):  
Haiyan Li ◽  
Qiang Zhang ◽  
Bo Zheng ◽  
Chunrong Chen ◽  
Nana Wu ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
Organic Aerosol ◽  
Control Measures ◽  
Public Attention ◽  
The North ◽  
The North China Plain ◽  
Nitrate Production ◽  
Haze Pollution ◽  
Aerosol Pollution

Abstract. Compared to the severe winter haze episodes in the North China Plain (NCP), haze pollution during summertime has drawn little public attention. In this study, we present the highly time-resolved chemical composition of submicron particles (PM1) measured in Beijing and Xinxiang in the NCP region during summertime to evaluate the driving factors of aerosol pollution. During the campaign periods (30 June to 27 July 2015, for Beijing and 8 to 25 June 2017, for Xinxiang), the average PM1 concentrations were 35.0 and 64.2 µg m−3 in Beijing and Xinxiang. Pollution episodes characterized with largely enhanced nitrate concentrations were observed at both sites. In contrast to the slightly decreased mass fractions of sulfate, semivolatile oxygenated organic aerosol (SV-OOA), and low-volatility oxygenated organic aerosol (LV-OOA) in PM1, nitrate displayed a significantly enhanced contribution with the aggravation of aerosol pollution, highlighting the importance of nitrate formation as the driving force of haze evolution in summer. Rapid nitrate production mainly occurred after midnight, with a higher formation rate than that of sulfate, SV-OOA, or LV-OOA. Based on observation measurements and thermodynamic modeling, high ammonia emissions in the NCP region favored the high nitrate production in summer. Nighttime nitrate formation through heterogeneous hydrolysis of dinitrogen pentoxide (N2O5) enhanced with the development of haze pollution. In addition, air masses from surrounding polluted areas during haze episodes led to more nitrate production. Finally, atmospheric particulate nitrate data acquired by mass spectrometric techniques from various field campaigns in Asia, Europe, and North America uncovered a higher concentration and higher fraction of nitrate present in China. Although measurements in Beijing during different years demonstrate a decline in the nitrate concentration in recent years, the nitrate contribution in PM1 still remains high. To effectively alleviate particulate matter pollution in summer, our results suggest an urgent need to initiate ammonia emission control measures and further reduce nitrogen oxide emissions over the NCP region.

scholarly journals Response of Early Winter Haze Days in the North China Plain to Autumn Beaufort Sea Ice

2018 ◽  
Author(s):  
Zhicong Yin ◽  
Yuyan Li ◽  
Huijun Wang
Keyword(s):  
North China Plain ◽  
North China ◽  
Beaufort Sea ◽  
Gulf Of Alaska ◽  
Sea Surface ◽  
Early Winter ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
The Bering Sea

Abstract. Recently, early winter haze pollution in the North China Plain has been serious and disastrous, dramatically damaging human health and the social economy. In this study, we emphasized the close connection between early winter haze days in the North China Plain and the September-October sea ice in the west of the Beaufort Sea (R = 0.51). Due to efficient radiative cooling, the responses of atmospheric circulations partially manifested as reductions of surface wind speed over the Beaufort Sea and Gulf of Alaska, resulting in a warmer sea surface in the subsequent November. The sea surface temperature anomalies over the Bering Sea and Gulf of Alaska acted as a bridge. The warmer sea surface efficiently heated the above air and led to suitable atmospheric backgrounds to enhance the potential of haze weather (e.g., a weaker East Asia jet stream and a Rossby wave-like train propagated from North China and the Japan Sea, through the Bering Sea and Gulf of Alaska, to the Cordillera Mountains). Near the surface, the weakening sea level pressure gradient stimulated anomalous southerlies over the coastal area of China and brought about a calm and moist environment for haze formation. The thermal inversion was also enhanced to restrict the underswing of clear and dry upper air. Thus, the horizontal and vertical dispersion were both limited, and the fine particles were apt to accumulate and cause haze pollution.

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