Continuous ozone depletion over Antarctica after 2000 and its relationship with the polar vortex

2014 ◽  
Vol 28 (1) ◽  
pp. 162-171 ◽  
Author(s):  
Libo Zhou ◽  
Yu Zhang ◽  
Shupo Ma
Keyword(s):  
2021 ◽  
Author(s):  
Ramina Alwarda ◽  
Kristof Bognar ◽  
Kimberly Strong ◽  
Martyn Chipperfield ◽  
Sandip Dhomse ◽  
...  

<p>The Arctic winter of 2019-2020 was characterized by an unusually persistent polar vortex and temperatures in the lower stratosphere that were consistently below the threshold for the formation of polar stratospheric clouds (PSCs). These conditions led to ozone loss that is comparable to the Antarctic ozone hole. Ground-based measurements from a suite of instruments at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Canada (80.05°N, 86.42°W) were used to investigate chemical ozone depletion. The vortex was located above Eureka longer than in any previous year in the 20-year dataset and lidar measurements provided evidence of polar stratospheric clouds (PSCs) above Eureka. Additionally, UV-visible zenith-sky Differential Optical Absorption Spectroscopy (DOAS) measurements showed record ozone loss in the 20-year dataset, evidence of denitrification along with the slowest increase of NO<sub>2</sub> during spring, as well as enhanced reactive halogen species (OClO and BrO). Complementary measurements of HCl and ClONO<sub>2</sub> (chlorine reservoir species) from a Fourier transform infrared (FTIR) spectrometer showed unusually low columns that were comparable to 2011, the previous year with significant chemical ozone depletion. Record low values of HNO<sub>3</sub> in the FTIR dataset are in accordance with the evidence of PSCs and a denitrified atmosphere. Estimates of chemical ozone loss were derived using passive ozone from the SLIMCAT offline chemical transport model to account for dynamical contributions to the stratospheric ozone budget.</p>


2018 ◽  
Vol 45 (4) ◽  
pp. 2115-2124 ◽  
Author(s):  
M. H. Denton ◽  
R. Kivi ◽  
T. Ulich ◽  
M. A. Clilverd ◽  
C. J. Rodger ◽  
...  

Polar Science ◽  
2019 ◽  
Vol 22 ◽  
pp. 100469 ◽  
Author(s):  
Vladimir V. Zuev ◽  
Ekaterina Savelieva

2014 ◽  
Vol 14 (23) ◽  
pp. 12855-12869 ◽  
Author(s):  
K. Sagi ◽  
D. Murtagh ◽  
J. Urban ◽  
H. Sagawa ◽  
Y. Kasai

Abstract. The Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) on board the International Space Station observed ozone in the stratosphere with high precision from October 2009 to April 2010. Although SMILES measurements only cover latitudes from 38° S to 65° N, the combination of data assimilation methods and an isentropic advection model allows us to quantify the ozone depletion in the 2009/2010 Arctic polar winter by making use of the instability of the polar vortex in the northern hemisphere. Ozone data from both SMILES and Odin/SMR (Sub-Millimetre Radiometer) for the winter were assimilated into the Dynamical Isentropic Assimilation Model for OdiN Data (DIAMOND). DIAMOND is an off-line wind-driven transport model on isentropic surfaces. Wind data from the operational analyses of the European Centre for Medium- Range Weather Forecasts (ECMWF) were used to drive the model. In this study, particular attention is paid to the cross isentropic transport of the tracer in order to accurately assess the ozone loss. The assimilated SMILES ozone fields agree well with the limitation of noise induced variability within the SMR fields despite the limited latitude coverage of the SMILES observations. Ozone depletion has been derived by comparing the ozone field acquired by sequential assimilation with a passively transported ozone field initialized on 1 December 2009. Significant ozone loss was found in different periods and altitudes from using both SMILES and SMR data: The initial depletion occurred at the end of January below 550 K with an accumulated loss of 0.6–1.0 ppmv (approximately 20%) by 1 April. The ensuing loss started from the end of February between 575 K and 650 K. Our estimation shows that 0.8–1.3 ppmv (20–25 %) of O3 has been removed at the 600 K isentropic level by 1 April in volume mixing ratio (VMR).


2005 ◽  
Vol 62 (3) ◽  
pp. 860-870 ◽  
Author(s):  
Jens-Uwe Grooß ◽  
Paul Konopka ◽  
Rolf Müller

Abstract In September 2002, the Antarctic polar vortex was disturbed, and it split into two parts caused by an unusually early stratospheric major warming. This study discusses the chemical consequences of this event using the Chemical Lagrangian Model of the Stratosphere (CLaMS). The chemical initialization of the simulation is based on Halogen Occultation Experiment (HALOE) measurements. Because of its Lagrangian nature, CLaMS is well suited for simulating the small-scale filaments that evolve during this period. Filaments of vortex origin in the midlatitudes were observed by HALOE several times in October 2002. The results of the simulation agree well with these HALOE observations. The simulation further indicates a very rapid chlorine deactivation that is triggered by the warming associated with the split of the vortex. Correspondingly, the ozone depletion rates in the polar vortex parts rapidly decrease to zero. Outside the polar vortex, where air masses of midlatitude origin were transported to the polar region, the simulation shows high ozone depletion rates at the 700-K level caused mainly by NOx chemistry. Owing to the major warming in September 2002, ozone-poor air masses were transported into the midlatitudes and caused a decrease of midlatitude ozone by 5%–15%, depending on altitude. Besides this dilution effect, there was no significant additional chemical effect. The net chemical ozone depletion in air masses of vortex origin was low and did not differ significantly from that of midlatitude air, in spite of the different chemical composition of the two types of air masses.


2013 ◽  
Vol 70 (12) ◽  
pp. 3977-3994 ◽  
Author(s):  
John R. Albers ◽  
Terrence R. Nathan

Abstract A mechanistic chemistry–dynamical model is used to evaluate the relative importance of radiative, photochemical, and dynamical feedbacks in communicating changes in lower-stratospheric ozone to the circulation of the stratosphere and lower mesosphere. Consistent with observations and past modeling studies of Northern Hemisphere late winter and early spring, high-latitude radiative cooling due to lower-stratospheric ozone depletion causes an increase in the modeled meridional temperature gradient, an increase in the strength of the polar vortex, and a decrease in vertical wave propagation in the lower stratosphere. Moreover, it is shown that, as planetary waves pass through the ozone loss region, dynamical feedbacks precondition the wave, causing a large increase in wave amplitude. The wave amplification causes an increase in planetary wave drag, an increase in residual circulation downwelling, and a weaker polar vortex in the upper stratosphere and lower mesosphere. The dynamical feedbacks responsible for the wave amplification are diagnosed using an ozone-modified refractive index; the results explain recent chemistry–coupled climate model simulations that suggest a link between ozone depletion and increased polar downwelling. The effects of future ozone recovery are also examined and the results provide guidance for researchers attempting to diagnose and predict how stratospheric climate will respond specifically to ozone loss and recovery versus other climate forcings including increasing greenhouse gas abundances and changing sea surface temperatures.


2017 ◽  
Vol 2017 ◽  
pp. 1-12 ◽  
Author(s):  
Yu Zhang ◽  
Jing Li ◽  
Libo Zhou

As the most prominent feature of the polar stratosphere, polar vortex results in widespread changes in the climate system, especially in the ozone variation. In this study, the linkage between polar vortex and ozone depletion in Antarctic stratosphere during the period 1979–2016 is investigated; we calculated the averaged total column ozone within the polar vortex based on the vortex edge (−28.8 PVU PV contour) instead of the geographical region defined by latitude and longitude. Results from the spatial patterns of ozone and polar vortex suggest that the morphological changes of polar vortex can impact the horizontal distribution of ozone and the ozone within the polar vortex experiences a severe depletion in spring. The negative relationship between ozone and polar vortex in terms of vortex area, strength, and breakup time is significant with the correlation coefficients of −0.57, −0.68, and −0.76, respectively. The breakup time of polar vortex plays an important role in the relation between polar vortex and ozone depletion with the highest-value correlation coefficient among three polar vortex parameters. Furthermore, the possible mechanism for this relationship is also discussed in this article.


Science ◽  
1990 ◽  
Vol 248 (4956) ◽  
pp. 721-724 ◽  
Author(s):  
Y. Yung ◽  
M Allen ◽  
D Crisp ◽  
R. Zurek ◽  
S. Sander

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