Volcanic aerosol and ozone depletion within the Antarctic polar vortex during the austral spring of 1991

Abstract In September 2002, the Antarctic polar vortex was disturbed, and it split into two parts caused by an unusually early stratospheric major warming. This study discusses the chemical consequences of this event using the Chemical Lagrangian Model of the Stratosphere (CLaMS). The chemical initialization of the simulation is based on Halogen Occultation Experiment (HALOE) measurements. Because of its Lagrangian nature, CLaMS is well suited for simulating the small-scale filaments that evolve during this period. Filaments of vortex origin in the midlatitudes were observed by HALOE several times in October 2002. The results of the simulation agree well with these HALOE observations. The simulation further indicates a very rapid chlorine deactivation that is triggered by the warming associated with the split of the vortex. Correspondingly, the ozone depletion rates in the polar vortex parts rapidly decrease to zero. Outside the polar vortex, where air masses of midlatitude origin were transported to the polar region, the simulation shows high ozone depletion rates at the 700-K level caused mainly by NOx chemistry. Owing to the major warming in September 2002, ozone-poor air masses were transported into the midlatitudes and caused a decrease of midlatitude ozone by 5%–15%, depending on altitude. Besides this dilution effect, there was no significant additional chemical effect. The net chemical ozone depletion in air masses of vortex origin was low and did not differ significantly from that of midlatitude air, in spite of the different chemical composition of the two types of air masses.

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Energetic particle induced intra-seasonal variability of ozone inside the Antarctic polar vortex observed in satellite data

Atmospheric Chemistry and Physics ◽

10.5194/acp-15-3327-2015 ◽

2015 ◽

Vol 15 (6) ◽

pp. 3327-3338 ◽

Cited By ~ 19

Author(s):

T. Fytterer ◽

M. G. Mlynczak ◽

H. Nieder ◽

K. Pérot ◽

M. Sinnhuber ◽

...

Keyword(s):

Geomagnetic Activity ◽

Seasonal Variability ◽

Transport Model ◽

Three Dimensional ◽

Polar Vortex ◽

Quiet Time ◽

Significance Level ◽

Antarctic Polar Vortex ◽

Ap Index ◽

The Antarctic

Abstract. Measurements from 2002 to 2011 by three independent satellite instruments, namely MIPAS, SABER, and SMR on board the ENVISAT, TIMED, and Odin satellites are used to investigate the intra-seasonal variability of stratospheric and mesospheric O3 volume mixing ratio (vmr) inside the Antarctic polar vortex due to solar and geomagnetic activity. In this study, we individually analysed the relative O3 vmr variations between maximum and minimum conditions of a number of solar and geomagnetic indices (F10.7 cm solar radio flux, Ap index, ≥ 2 MeV electron flux). The indices are 26-day averages centred at 1 April, 1 May, and 1 June while O3 is based on 26-day running means from 1 April to 1 November at altitudes from 20 to 70 km. During solar quiet time from 2005 to 2010, the composite of all three instruments reveals an apparent negative O3 signal associated to the geomagnetic activity (Ap index) around 1 April, on average reaching amplitudes between −5 and −10% of the respective O3 background. The O3 response exceeds the significance level of 95% and propagates downwards throughout the polar winter from the stratopause down to ~ 25 km. These observed results are in good qualitative agreement with the O3 vmr pattern simulated with a three-dimensional chemistry-transport model, which includes particle impact ionisation.

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The Life Cycle and Variability of Antarctic Weak Polar Vortex Events

Journal of Climate ◽

10.1175/jcli-d-21-0500.1 ◽

2022 ◽

pp. 1-63

Keyword(s):

Life Cycle ◽

Polar Vortex ◽

Southern Annular Mode ◽

Austral Spring ◽

Stratospheric Polar Vortex ◽

Temperature And Precipitation ◽

Scale Temperature ◽

Precipitation Anomalies ◽

Polar Stratosphere ◽

The Antarctic

Abstract Motivated by the strong Antarctic sudden stratospheric warming (SSW) in 2019, a survey on the similar Antarctic weak polar events (WPV) is presented, including their life cycle, dynamics, seasonality, and climatic impacts. The Antarctic WPVs have a frequency of about four events per decade, with the 2002 event being the only major SSW. They show a similar life cycle to the SSWs in the Northern Hemisphere but have a longer duration. They are primarily driven by enhanced upward-propagating wavenumber 1 in the presence of a preconditioned polar stratosphere, i.e., a weaker and more contracted Antarctic stratospheric polar vortex. Antarctic WPVs occur mainly in the austral spring. Their early occurrence is preceded by an easterly anomaly in the middle and upper equatorial stratosphere besides the preconditioned polar stratosphere. The Antarctic WPVs increase the ozone concentration in the polar region and are associated with an advanced seasonal transition of the stratospheric polar vortex by about one week. Their frequency doubles after 2000 and is closely related to the advanced Antarctic stratospheric final warming in recent decades. The WPV-resultant negative phase of the southern annular mode descends to the troposphere and persists for about three months, leading to persistent hemispheric scale temperature and precipitation anomalies.

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Erratum: Spatial Variation of Ozone Depletion Rates in the Springtime Antarctic Polar Vortex

Science ◽

10.1126/science.844-d ◽

1990 ◽

Vol 249 (4971) ◽

pp. 844-844

Keyword(s):

Spatial Variation ◽

Ozone Depletion ◽

Polar Vortex ◽

Antarctic Polar Vortex

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Long-range transport of volcanic aerosol from the 2010 Merapi tropical eruption to Antarctica

10.5194/acp-2018-332 ◽

2018 ◽

Author(s):

Xue Wu ◽

Sabine Griessbach ◽

Lars Hoffmann

Keyword(s):

Long Range ◽

Lower Stratosphere ◽

Polar Vortex ◽

Volcanic Eruptions ◽

Long Range Transport ◽

Volcanic Plume ◽

Volcanic Aerosol ◽

The South ◽

Range Transport ◽

The Antarctic

Abstract. Volcanic sulfate aerosol is an important source of sulfur for Antarctica where other local sources of sulfur are rare. Mid- and high latitude volcanic eruptions can directly influence the aerosol budget of the polar stratosphere. However, tropical eruptions can also enhance polar aerosol load following long-range transport. In the present work, we analyze the volcanic plume of a tropical eruption, Mount Merapi in October 2010, using the Lagrangian particle dispersion model Massive-Parallel Trajectory Calculations (MPTRAC), Atmospheric Infrared Sounder (AIRS) SO2 observations and Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) aerosol observations. We investigate the pathway and transport efficiency of the volcanic aerosol from the tropical tropopause layer (TTL) to the lower stratosphere over Antarctica. We first estimated the time- and height-resolved SO2 injection time series over Mount Merapi during the explosive eruption using the AIRS SO2 observations and a backward trajectory approach. Then the SO2 injections were tracked for up to 6 months using the MPTRAC model. The Lagrangian transport simulation of the volcanic plume was compared to MIPAS aerosol observations and showed good agreement. Both of the simulation and the observations presented in this study suggest that a significant amount of aerosols of the volcanic plume from the Merapi eruption was transported from the tropics to the south of 60 °S within one month after the eruption and even further to Antarctica in the following two months. This relatively fast meridional transport of volcanic aerosol was mainly driven by quasi-horizontal mixing from the TTL to the extratropical lower stratosphere, which was facilitated by the weakening of the subtropical jet during the seasonal transition from austral spring to summer and linked to the westerly phase of the quasi-biennial oscillation (QBO). When the plume went to southern high latitudes, the polar vortex was displaced from the south pole, so the volcanic plume was carried to the south pole without penetrating the polar vortex. Based on the model results, the most efficient pathway for the quasi-horizontal mixing was in between the isentropic surfaces of 360 and 430 K. Although only 4 % of the initial SO2 load was transported into the lower stratosphere south of 60 °S, the Merapi eruption contributed about 8800 tons of sulfur to the Antarctic lower stratosphere. This indicates that the long-range transport under favorable meteorological conditions enables tropical volcanic eruptions to be an important remote source of sulfur for the Antarctic stratosphere.

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A quasi-Lagrangian coordinate system based on high resolution tracer observations: implementation for the Antarctic polar vortex

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-8-16123-2008 ◽

2008 ◽

Vol 8 (4) ◽

pp. 16123-16173 ◽

Cited By ~ 3

Author(s):

E. V. Ivanova ◽

C. M. Volk ◽

O. Riediger ◽

H. Klein ◽

N. M. Sitnikov ◽

...

Keyword(s):

High Resolution ◽

Coordinate System ◽

Vortex Core ◽

Polar Vortex ◽

Mixing Ratio ◽

Lagrangian Coordinate ◽

Antarctic Polar Vortex ◽

The Antarctic ◽

Lagrangian Coordinate System

Abstract. In order to quantitatively analyse the chemical and dynamical evolution of the polar vortex it has proven extremely useful to work with coordinate systems that follow the vortex flow. We propose here a two-dimensional quasi-Lagrangian coordinate system {χi, Δχi}, based on the mixing ratio of a long-lived stratospheric trace gas i, and its systematic use with i = N2O, in order to describe the structure of a well-developed Antarctic polar vortex. In the coordinate system {χi, Δχi} the mixing ratio χi is the vertical coordinate and Δχi = χi(Θ)−χivort(Θ) is the meridional coordinate (χivort(Θ) being a vertical reference profile in the vortex core). The quasi-Lagrangian coordinates {χi, Δχi} persist for much longer time than standard isentropic coordinates, potential temperature Θ and equivalent latitude φe, do not require explicit reference to geographic space, and can be derived directly from high-resolution in situ measurements. They are therefore well-suited for studying the evolution of the Antarctic polar vortex throughout the polar winter with respect to the relevant chemical and microphysical processes. By using the introduced coordinate system {χN2O, ΔχN2O} we analyze the well-developed Antarctic vortex investigated during the APE-GAIA (Airborne Polar Experiment – Geophysica Aircraft in Antarctica – 1999) campaign (Carli et al., 2000). A criterion, which uses the local in-situ measurements of χi=χi(Θ) and attributes the inner vortex edge to a rapid change (δ-step) in the meridional profile of the mixing ratio χi, is developed to determine the (Antarctic) inner vortex edge. In turn, we suggest that the outer vortex edge of a well-developed Antarctic vortex can be attributed to the position of a local minimum of the χH2O gradient in the polar vortex area. For a well-developed Antarctic vortex, the ΔχN2O-parametrization of tracer-tracer relationships allows to distinguish the tracer inter-relationships in the vortex core, vortex boundary region and surf zone and to examine their meridional variation throughout these regions. This is illustrated by analyzing the tracer-tracer relationships χi : χN2O obtained from the in-situ data of the APE-GAIA campaign for i = CFC-11, CFC-12, H-1211 and SF6. A number of solitary anomalous points in the CFC-11 : N2O correlation, observed in the Antarctic vortex core, are interpreted in terms of small-scale cross-isentropic dispersion.

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