scholarly journals Light helicity detector based on 2D magnetic semiconductor CrI3

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Xing Cheng ◽  
Zhixuan Cheng ◽  
Cong Wang ◽  
Minglai Li ◽  
Pingfan Gu ◽  
...  

AbstractTwo-dimensional magnetic semiconductors provide a platform for studying physical phenomena at atomically thin limit, and promise magneto-optoelectronic devices application. Here, we report light helicity detectors based on graphene-CrI3-graphene vdW heterostructures. We investigate the circularly polarized light excited current and reflective magnetic circular dichroism (RMCD) under various magnetic fields in both monolayer and multilayer CrI3 devices. The devices exhibit clear helicity-selective photoresponse behavior determined by the magnetic state of CrI3. We also find abnormal negative photocurrents at higher bias in both monolayer and multilayer CrI3. A possible explanation is proposed for this phenomenon. Our work reveals the interplay between magnetic and optoelectronic properties in CrI3 and paves the way to developing spin-optoelectronic devices.

2013 ◽  
Vol 59 ◽  
pp. 359-382 ◽  
Author(s):  
Andrew J. Thomson ◽  
Laurence D. Barron

Philip J. Stephens was a theoretical chemist who brought to fruition two new forms of optical spectroscopy, using circularly polarized light, for the determination of electronic structure and molecular stereochemistry. The first was magnetic circular dichroism (MCD), the wavelength dependence of the differential absorption of left and right circularly polarized light induced by a magnetic field applied parallel to the light beam. Stephens established a methodology for extracting from MCD spectra the angular momentum characteristics of ground and excited electronic states and demonstrated applications to the assignment of the optical spectra of coordination complexes of transition metals and to metalloproteins. In the second half of his career Stephens led the field of vibrational circular dichroism (VCD), the measurement of the natural circular dichroism (CD) arising from the vibrational transitions of chiral molecules. He developed instrumental techniques to measure this weak dichroism over a wide frequency range with high sensitivity. Subsequently he developed a quantum-mechanical method that yielded reliable calculations of VCD spectra by using density functional theory. Thus absolute configurations of all the chiral centres in an organic molecule are readily established. Given the increasing importance of enantiomerically pure chiral drugs, VCD has found widespread application in the pharmaceutical industry. Philip had not only a deep understanding of chemical theory but also a thorough grasp of experiments. His lectures on theoretical topics were models of clarity. He was also an accomplished pianist in demand, when a student at Oxford University, as an accompanist and for chamber concerts.


2000 ◽  
Vol 07 (05n06) ◽  
pp. 643-647 ◽  
Author(s):  
K. ENOMOTO ◽  
Y. MIYATAKE ◽  
K. FUKUMOTO ◽  
A. KOBAYASHI ◽  
K. HATTORI ◽  
...  

Circular dichroism has been measured in the photoelectron diffraction of bulk W 4f photoelectrons from the W(110)(1×1) clean surface. The forward focusing peaks along the symmetric axis in the diffraction pattern showed an azimuthal rotation similar to those reported in a prior experiment on Si(001) and chemically shifted W 4f photoelectrons from the W(110)(1×1)-O surface. The emission angle dependence of the rotation angles has been measured and analyzed for the first time and the angles observed are in good agreement with those calculated using the formula Δ ϕ=m/kR sin 2θ derived previously by Daimon et al. [Jpn. J. Phys.32, L1480 (1993)] considering the angular dependence of m. This property gives a basis for the analysis of structure or various magnetic and electronic properties on surfaces.


Sensors ◽  
2021 ◽  
Vol 21 (13) ◽  
pp. 4381
Author(s):  
Joohoon Kim ◽  
Ahsan Sarwar Rana ◽  
Yeseul Kim ◽  
Inki Kim ◽  
Trevon Badloe ◽  
...  

Chiral materials, which show different optical behaviors when illuminated by left or right circularly polarized light due to broken mirror symmetry, have greatly impacted the field of optical sensing over the past decade. To improve the sensitivity of chiral sensing platforms, enhancing the chiroptical response is necessary. Metasurfaces, which are two-dimensional metamaterials consisting of periodic subwavelength artificial structures, have recently attracted significant attention because of their ability to enhance the chiroptical response by manipulating amplitude, phase, and polarization of electromagnetic fields. Here, we reviewed the fundamentals of chiroptical metasurfaces as well as categorized types of chiroptical metasurfaces by their intrinsic or extrinsic chirality. Finally, we introduced applications of chiral metasurfaces such as multiplexing metaholograms, metalenses, and sensors.


2004 ◽  
Vol 84 (26) ◽  
pp. 5440-5442 ◽  
Author(s):  
Kenji Miyakawa ◽  
Hiroto Adachi ◽  
Yoshinori Inoue

Hyomen Kagaku ◽  
2005 ◽  
Vol 26 (12) ◽  
pp. 746-751 ◽  
Author(s):  
Fumihiko MATSUI ◽  
Yukako KATO ◽  
Fang Zhun GUO ◽  
Tomohiro MATSUSHITA ◽  
Hiroshi DAIMON

Author(s):  
Marcos F. Maestre

Recently we have developed a form of polarization microscopy that forms images using optical properties that have previously been limited to macroscopic samples. This has given us a new window into the distribution of structure on a microscopic scale. We have coined the name differential polarization microscopy to identify the images obtained that are due to certain polarization dependent effects. Differential polarization microscopy has its origins in various spectroscopic techniques that have been used to study longer range structures in solution as well as solids. The differential scattering of circularly polarized light has been shown to be dependent on the long range chiral order, both theoretically and experimentally. The same theoretical approach was used to show that images due to differential scattering of circularly polarized light will give images dependent on chiral structures. With large helices (greater than the wavelength of light) the pitch and radius of the helix could be measured directly from these images.


2021 ◽  
Author(s):  
Zhaoming Zhang ◽  
Takunori Harada ◽  
Adriana Pietropaolo ◽  
Yuting Wang ◽  
Yue Wang ◽  
...  

Preferred-handed propeller conformation was induced by circularly polarized light irradiation to three amorphous molecules with trigonal symmetry, and the molecules with induced chirality efficiently exhibited blue circularly polarized luminescence. In...


Sign in / Sign up

Export Citation Format

Share Document