scholarly journals Ion tracks in silicon formed by much lower energy deposition than the track formation threshold

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
H. Amekura ◽  
M. Toulemonde ◽  
K. Narumi ◽  
R. Li ◽  
A. Chiba ◽  
...  

AbstractDamaged regions of cylindrical shapes called ion tracks, typically in nano-meters wide and tens micro-meters long, are formed along the ion trajectories in many insulators, when high energy ions in the electronic stopping regime are injected. In most cases, the ion tracks were assumed as consequences of dense electronic energy deposition from the high energy ions, except some cases where the synergy effect with the nuclear energy deposition plays an important role. In crystalline Si (c-Si), no tracks have been observed with any monomer ions up to GeV. Tracks are formed in c-Si under 40 MeV fullerene (C60) cluster ion irradiation, which provides much higher energy deposition than monomer ions. The track diameter decreases with decreasing the ion energy until they disappear at an extrapolated value of ~ 17 MeV. However, here we report the track formation of 10 nm in diameter under C60 ion irradiation of 6 MeV, i.e., much lower than the extrapolated threshold. The diameters of 10 nm were comparable to those under 40 MeV C60 irradiation. Furthermore, the tracks formed by 6 MeV C60 irradiation consisted of damaged crystalline, while those formed by 40 MeV C60 irradiation were amorphous. The track formation was observed down to 1 MeV and probably lower with decreasing the track diameters. The track lengths were much shorter than those expected from the drop of Se below the threshold. These track formations at such low energies cannot be explained by the conventional purely electronic energy deposition mechanism, indicating another origin, e.g., the synergy effect between the electronic and nuclear energy depositions, or dual transitions of transient melting and boiling.

1993 ◽  
Vol 316 ◽  
Author(s):  
Timothy E. Levine ◽  
Emmanuel P. Giannelis ◽  
Padma Kodali ◽  
Joseph Tesmer ◽  
Michael Nastasi ◽  
...  

ABSTRACTWe have investigated the densification behavior of sol-gel zirconia films resulting from ion irradiation. Three sets of films were implanted with neon, krypton, or xenon. The ion energies were chosen to yield approximately constant energy loss through the film and the doses were chosen to yield similar nuclear energy deposition. Ion irradiation of the sol-gel films resulted in carbon and hydrogen loss as indicated by Rutherford backscattering spectrometry and forward recoil energy spectroscopy. Although the densification was hypothesized to result from target atom displacement, the observed densification exhibits a stronger dependence on electronic energy deposition.


MRS Bulletin ◽  
1995 ◽  
Vol 20 (12) ◽  
pp. 29-34 ◽  
Author(s):  
A. Barbu ◽  
H. Dammak ◽  
A. Dunlop ◽  
D. Lesueur

When an energetic ion penetrates a target, it loses its energy via two nearly independent processes: (1) elastic collisions with the nuclei (nuclear-energy loss (dE/dx)n), which dominate the ion slowing down in the low energy range (i.e., in the stopping region); (2) electronic excitation and ionization (electronic-energy loss (dE/dx)e), which strongly overwhelm (dE/dx)n in the high energy range (typically above 1 MeV/nucleon). Until the 1980s, researchers considered that electronic-energy deposition could participate in damaging creation in many insulators, but the effects observed in bulk metals were solely ascribed to elastic nuclear collisions. This widely held opinion was due to the fact that in metallic systems the numerous very mobile conduction electrons allow a fast spreading of the deposited energy and an efficient screening of the space charge created in the projectile wake so that it seemed unreasonable to hope for damage creation or track formation in metallic targets following high levels of electronic-energy deposition.A particular case is the observation more than 30 years ago of damage in thin or discontinuous. metallic films after fission fragment irradiation or MeV heavy ion bombardment. The spreading of the deposited energy is then strongly limited by the close vicinity of surfaces and interfaces.


2021 ◽  
Vol 11 (8) ◽  
pp. 3473
Author(s):  
Yedong Guan ◽  
Peng Lv ◽  
Zuojiang Wang ◽  
Yuzhe Jiang ◽  
Zhao Sun ◽  
...  

Investigating the irradiation effects on borosilicate glass is of great significance for understanding the long-term evolutions of this substance in radioactive environments. In the present study, the hardness and modulus of conventional and ion-irradiated borosilicate glass were investigated through nanoindentation measurements. The obtained results show that the maximum decrease of the mean hardness after He and Ar ion irradiation was 8.4% and 17.0%, respectively, when the fluence reached 1.1 × 1015. It was found that the hardness reduction had a significant ionic correlation. Meanwhile, it was observed that the mean modulus increased by less than 5.0%, while there was no meaningful ionic correlation. The variation in hardness and modulus were primarily the consequence of nuclear energy deposition. The hardness recovery was observed under Ar-irradiated and He-irradiated Ar pre-damaged samples. It was concluded that the hardness recovery mainly originates from electronic energy deposition induced by ion irradiation.


2013 ◽  
Vol 781-784 ◽  
pp. 357-361 ◽  
Author(s):  
Igor V. Khromushin ◽  
Taтiana I. Aksenova ◽  
Turgora Tuseyev ◽  
Karlygash K. Munasbaeva ◽  
Yuri V. Ermolaev ◽  
...  

The effect of irradiation with heavy ions Ne, Ar, and Kr of various energies on the structure and properties of ceramic barium cerate doped with neodymium and annealed in air at 650°C for 7 hours is studied. It is noted that blistering was observed on cerate surface during its irradiation by low energy Ne ions, whereas it was not observed under low-energy Ar and Kr ions irradiation. Irradiation of the cerate with high energy ions caused partial amorphization of the irradiated surface of the material, while the structure of the non-irradiated surface did not change. In addition, the irradiated surface of the cerate endured solid-phase structural changes. Thus, upon high-energy ions irradiation in the range of Ne, Ar, Kr the cerate surface resembled the stages of spherulite formation - nucleation, growth (view of cauliflower), formation of spherulitic crust, respectively. The increase in water molecules release and reduction of molecular oxygen release from the barium cerate, irradiated by high-energy ions is found during vacuum constant rate heating. It is concluded that cerates undergo changes to the distances significantly exceeding the ion ranges in these materials. Features of high-energy ions influence on thermal desorption of carbon dioxide from cerates show, apparently, the formation of weakly bound carbonate compounds on the cerate surface in the irradiation process.


1985 ◽  
Vol 45 ◽  
Author(s):  
T. Venkatesan ◽  
R. Levi ◽  
T. C. Banwell ◽  
T. Tombrello ◽  
M. Nicolet ◽  
...  

ABSTRACTWe have explored the origin of the ion-induced conductivity in polymer films and the distinction between low energy ion-implantation and high-energy ion irradiation. In experiments involving irradiation of polymer and carbon films with ions of energy from 200 keV to 25 MeV we have established that with both low and high energy ions the polymers undergo carbonization. However, the saturation resistivity obtained with low energy implantation is four to six orders of magnitude larger than those obtained by high energy ion irradiation. In experiments on irradiation of carbon films low energy ions caused a two orders of magnitude increase in the resistivity while high energy ion caused a two orders of magnitude decrease. This implies that the structure of the carbonized polymer is different for the low and the high energy ion irradiation. While in the former case there may be no crystalline order in the films; in the latter case, a microcrystalline graphitic structure is obtained (with four orders of magnitude larger conductivity than in the former case). The formation of graphitic crystalline order with increasing high energy ion dose was verified by electron energy loss spectroscopy. This is an interesting example of crystallization induced by electronic excitation alone with no macroscopic thermal effect.


2009 ◽  
Vol 86 (4-6) ◽  
pp. 910-912 ◽  
Author(s):  
Th. Gischkat ◽  
H. Hartung ◽  
F. Schrempel ◽  
E.B. Kley ◽  
A. Tünnermann ◽  
...  

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