High efficiency warm white organic light-emitting diodes with precise confinement of charge carriers and excitons in the exciplex host system

2019 ◽  
Vol 7 (23) ◽  
pp. 7114-7120 ◽  
Author(s):  
Shian Ying ◽  
Jiakun Yuan ◽  
Shuai Zhang ◽  
Qian Sun ◽  
Yanfeng Dai ◽  
...  

A high-performance WOLED with stable spectrum emission was achieved by the ratio regulation between the HTM and ETM in the exciplex host system.

Materials ◽  
2020 ◽  
Vol 13 (9) ◽  
pp. 2029
Author(s):  
Tianyu Zhang ◽  
Asu Li ◽  
Ren Sheng ◽  
Mingyang Sun ◽  
Ping Chen

High-efficiency single-layer organic light-emitting diodes (OLEDs) based on a simple structure doped with iridium(III) bis(4-phenylthieno[3,2-c]pyridinato-N,C2′) acetylacetonate (PO-01) as emission dyes are realized, achieving maximum current efficiency (CE) and power efficiency (PE) of 37.1 cd A−1 and 33.3 lm W−1 as well as low turn-on voltage of 3.31 V. Such superior performance is mainly attributed to the employment of a uniform co-host structure and assisted charge transport property of phosphors dyes, which were in favor of the balance of charge carrier injection and transport in the single emitting layer (EML). Moreover, systematic researches on the position of exciton recombination region and the dopant effect on charge carriers were subsequently performed to better understand the operational mechanism. It could be experimentally found that the orange emitting dopants promoted the acceleration of the charge carriers transport and raised the exciton recombination efficiency, eventually leading to an excellent performance of single-layer OLEDs.


2018 ◽  
Vol 6 (40) ◽  
pp. 10793-10803 ◽  
Author(s):  
Shian Ying ◽  
Dezhi Yang ◽  
Xianfeng Qiao ◽  
Yanfeng Dai ◽  
Qian Sun ◽  
...  

High-performance WOLEDs realizing high efficiency and low efficiency roll-off simultaneously were achieved by strategically managing triplet excitons in the emission layer.


2020 ◽  
Vol 8 (36) ◽  
pp. 12450-12456 ◽  
Author(s):  
Yuwen Chen ◽  
Yibing Wu ◽  
Chengwei Lin ◽  
Yanfeng Dai ◽  
Qian Sun ◽  
...  

High performance hybrid WOLEDs have been realized by precisely inserting ultrathin red/green phosphorescent layers in a blue exciplex emitter.


2020 ◽  
Vol 976 ◽  
pp. 110-115
Author(s):  
Fei Yang Liu ◽  
Bin Wei ◽  
Guo Chen

Recently the phosphorescent organic light-emitting diodes (PhOLEDs) have attracted tremendous attention owing to their extremely high performance. However, PhOLEDs always suffer from the annihilation and quenching of excitons due to higher guest doping concentration. In this work, to obtain a high efficiency red PhOLED, a gradient-doped emitting layer (EML) was employed in the device to improve the device efficiency and suppress the annihilation of excitons. A significant enhancement in terms of current efficiency (CE) and power efficiency (PE) of PhOLEDs with optimized gradient-doped EML was realized with the maximum CE of 13.84 cd A-1 and PE of 18.11 lm W−1, which are 33.9% and 60.7% higher than that of the control device, respectively. The enhanced performance of the PhOLEDs is attributed to the lower guest doping concentration in gradient-doped EML and balanced hole/electron recombination, leading to the reduced triplet-triplet annihilation and triplet-polaron quenching. The simple strategy opens a new avenue for fabricating high-performance PhOLEDs.


2019 ◽  
Vol 33 (24) ◽  
pp. 1950284
Author(s):  
Nan Zhang ◽  
Yang Chen ◽  
Yan-Hui Wang

It has been demonstrated that high efficiency and brightness can be achieved in phosphorescent organic light-emitting diodes (PHOLEDs) by using molybdenum oxide (MoO3)/poly(3,4-ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS) as dual hole injection layers (HILs) on indium tin oxide (ITO) substrate. The dual HILs were simply fabricated by spin-coating PEDOT:PSS solution on a thin MoO3 layer deposited by vacuum thermal evaporation. This work reveals that PEDOT:PSS coating on MoO3 resulted in a smoother surface, simultaneously MoO3 lamella prevented acid corrosion of PEDOT:PSS on ITO. Meanwhile, with the insertion of PEDOT:PSS and MoO3 as HILs between anode and hole transporting layer (HTL), the energy barrier has been reduced and gave rise to effective hole injection. OLEDs with dual HILs resulted in the maximum current efficiency (CE) of 61.3 cd A[Formula: see text] and maximum luminance of 112200 cd cm[Formula: see text], which showed a superior performance compared to those devices with single HIL of PEDOT:PSS or MoO3. Our results proved the composition of PEDOT:PSS and MoO3 as HILs were beneficial for high performance OLEDs.


RSC Advances ◽  
2018 ◽  
Vol 8 (71) ◽  
pp. 40883-40893 ◽  
Author(s):  
Yuwen Chen ◽  
Shian Ying ◽  
Qian Sun ◽  
Yanfeng Dai ◽  
Xianfeng Qiao ◽  
...  

High performance hybrid WOLEDs based on a blue fluorescent EML and inserted an exciton regulation layer of ultrathin green phosphor.


2019 ◽  
Vol 3 (4) ◽  
pp. 640-649 ◽  
Author(s):  
Shian Ying ◽  
Qian Sun ◽  
Yanfeng Dai ◽  
Dezhi Yang ◽  
Xianfeng Qiao ◽  
...  

Ultra-high performance WOLEDs were achieved by solving the trade-off between charge carrier trapping and energy transfer in electroluminescence processes.


2021 ◽  
Vol 9 (10) ◽  
pp. 3626-3634
Author(s):  
Jingwen Yao ◽  
Wei Liu ◽  
Chengwei Lin ◽  
Qian Sun ◽  
Yanfeng Dai ◽  
...  

The positions of the phosphor-sensitized yellow EML from the exciton recombination zone were controlled to strategically utilize singlet and triplet excitons for blue and yellow emissions to realize high-performance fluorescent WOLEDs.


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