High resolution plutonium-239/240 mixture alpha spectroscopy using centrifugally tensioned metastable fluid detector sensor technology

Author(s):  
Catalin Harabagiu ◽  
Nathan Boyle ◽  
Brian Archambault ◽  
David DiPrete ◽  
Rusi Taleyarkhan

This paper presents a novel and rapid, wet chemistry technique for spectroscopically detecting trace (∼10−3 Bq mL−1) level alpha emitting radionuclides mixtures with under 10 keV alpha energy resolution – with 100% gamma–beta rejection.

1998 ◽  
Vol 5 (3) ◽  
pp. 515-517 ◽  
Author(s):  
M. Frank ◽  
C. A. Mears ◽  
S. E. Labov ◽  
L. J. Hiller ◽  
J. B. le Grand ◽  
...  

Experimental results are presented obtained with a cryogenically cooled high-resolution X-ray spectrometer based on a 141 × 141 µm Nb-Al-Al2O3-Al-Nb superconducting tunnel junction (STJ) detector in an SR-XRF demonstration experiment. STJ detectors can operate at count rates approaching those of semiconductor detectors while still providing a significantly better energy resolution for soft X-rays. By measuring fluorescence X-rays from samples containing transition metals and low-Z elements, an FWHM energy resolution of 6–15 eV for X-rays in the energy range 180–1100 eV has been obtained. The results show that, in the near future, STJ detectors may prove very useful in XRF and microanalysis applications.


2021 ◽  
Vol 28 (5) ◽  
Author(s):  
Takayuki Muro ◽  
Tomohiro Matsushita ◽  
Kazumi Sawamura ◽  
Jun Mizuno

A wide-acceptance-angle spherical grid composed of numerous micro cylindrical holes was developed to be used for the retarding grid of a display-type retarding field analyzer (RFA) and to enhance the energy resolution (E/ΔE). Each cylindrical hole with a diameter of 50 µm and a depth of 80 µm is directed to the spherical center. The inner radius of the spherical grid is 40 mm. The holed area corresponds to an acceptance angle of ±52°. The E/ΔE of an RFA equipped with the developed holed grid was estimated to be 2000 from a measured Au 4f photoemission spectrum. A clear photoelectron hologram was observed in the Mo 4p core-level region of MoS2, indicating that the RFA with the holed grid is effective for photoelectron holography.


2014 ◽  
Vol 21 (4) ◽  
pp. 762-767 ◽  
Author(s):  
Ari-Pekka Honkanen ◽  
Roberto Verbeni ◽  
Laura Simonelli ◽  
Marco Moretti Sala ◽  
Ali Al-Zein ◽  
...  

Wavelength-dispersive high-resolution X-ray spectrometers often employ elastically bent crystals for the wavelength analysis. In a preceding paper [Honkanenet al.(2014).J. Synchrotron Rad.21, 104–110] a theory for quantifying the internal stress of a macroscopically large spherically curved analyser crystal was presented. Here the theory is applied to compensate for the corresponding decrease of the energy resolution. The technique is demonstrated with a Johann-type spectrometer using a spherically bent Si(660) analyser in near-backscattering geometry, where an improvement in the energy resolution from 1.0 eV down to 0.5 eV at 9.7 keV incident photon energy was observed.


2010 ◽  
Vol 19 (12) ◽  
pp. 2487-2496 ◽  
Author(s):  
◽  
F. Garibaldi ◽  
E. Cisbani ◽  
F. Cusanno ◽  
S. Frullani ◽  
...  

The characteristics of the Jefferson LAB electron beam, together with those of the experimental equipments, offer a unique opportunity to study hypernuclear spectroscopy via electromagnetic induced reactions. Experiment 94-107 started a systematic study on 1p-shell targets, 12 C , 9 Be and 16 O . We present the results from 12 C , 16 O and very preliminary results from 9 Be . For 12 C for the first time measurable strength in the core-excited part of the spectrum between the ground state and the pΛ state was shown in [Formula: see text] for the first time. A high-quality 16Λ N spectrum was produced for the first time with sub-MeV Energy resolution. A very precise B Λ value for 16Λ N , calibrated against the elementary ( e , e ′ K +) reaction on hydrogen, has also been obtained. Final data on 9 Be will be available soon. The missing energy resolution is the best ever obtained in hypernuclear production experiments.


1971 ◽  
Vol 49 (4) ◽  
pp. 483-485 ◽  
Author(s):  
C. Doekes ◽  
D. C. Kean ◽  
R. V. Elliott ◽  
R. H. Spear

The energy levels of the nucleus 27Al have been studied with an energy resolution of about 6 keV by magnetic analysis of the protons from the 27Al(p, p′)27Al reaction. A number of previously unreported levels have been observed.


2010 ◽  
Vol 19 (12) ◽  
pp. 2480-2486 ◽  
Author(s):  
Y. Fujii ◽  
A. Chiba ◽  
D. Doi ◽  
T. Gogami ◽  
O. Hashimoto ◽  
...  

Hypernuclear spectroscopy with electron beam at JLab Hall C has been studied since 2000. The first experiment, JLab E89-009, demonstrated the possibility of the (e, e′ K+) reaction for hypernuclear spectroscopy by achieving an energy resolution of better than 1 MeV (FWHM). The second experiment, JLab E01-011 employed a newly constructed high resolution kaon spectrometer and introduced a vertically tilted electron arm setup to avoid electrons from bremsstrahlung and Moeller scattering. The setup allowed us to have 10 times yield rate and 4 times better signal to accidental ratio with expected energy resolution of 400 keV (FWHM). The third experiment, JLab E05-115 will be performed in 2009 with employing newly constructed high resolution electron spectrometer and a new charge-separation magnet. With the fully customized third generation experimental setup, we can study a variety of targets up to medium-heavy ones such as 52 Cr .


2019 ◽  
Author(s):  
Meghana Mahaveer Patil ◽  
Michele Caselle ◽  
Lorenzo Rota ◽  
Alexander Dierlamm ◽  
Marta Baselga Bacardit ◽  
...  

2018 ◽  
Vol 33 (12) ◽  
pp. 2070-2082 ◽  
Author(s):  
Le Pape Pierre ◽  
Blanchard Marc ◽  
Juhin Amélie ◽  
Rueff Jean-Pascal ◽  
Ducher Manoj ◽  
...  

To improve our knowledge of arsenic local environment in sulfide minerals, Resonant Inelastic X-Ray Scattering (RIXS) maps and High-Energy Resolution Fluorescence Detected (HERFD) XANES measurements are performed at the As K-edge. In addition, the spectra are compared to XANES modelled through first-principles calculations.


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