scholarly journals Classification of aerosols using multiple clustering techniques over Zanjan, Iran, during 2010-2014

2019 ◽  
Vol 99 ◽  
pp. 02007
Author(s):  
Maryam Gharibzadeh ◽  
Khan Alam ◽  
Yousefali Abedini ◽  
Abbasali Aliakbari Bidokhti

A more detailed study and identification of aerosol types can help to better understand the sources and effects of aerosols. In the present study, a number of optical properties of aerosols have been investigated seasonal for discrimination of aerosol types during 2010-2014 over Zanjan, Iran. Also using AERosol RObotic NETwork (AERONET) data, aerosol was classified by multiple clustering techniques. Both fine and coarse modes particles were seen in seasonal averaged of Aerosol Volume Size Distribution (AVSD). Single Scattering Albedo (SSA) variations indicate the presence of scattering aerosol like dust in the spring, summer and fall, and dominance of absorbing type aerosols in the winter. The maximum value of the phase function was observed in the summer and in small scattering angle which can be due to presence of coarse mode dust particles. The scatter plot of Aerosol Optical Depth (AOD) versus Angstrom Exponent (AE) is one of the most effective methods to find aerosol types. Extinction Angstrom exponent (EAE) versus SSA and EAE versus absorption Angstrom exponent (AAE) are other ways to classification of aerosol types. Graphs show abundance of dust in the spring, summer and fall in Zanjan's atmosphere. Also presence of urban/industrial aerosols is in all seasons, especially in the fall and winter. In addition mixed aerosols exist in all seasons. On the other hand, no biomass burning aerosols found in Zanjan's atmosphere.

2013 ◽  
Vol 6 (10) ◽  
pp. 2659-2669 ◽  
Author(s):  
A. Bayat ◽  
H. R. Khalesifard ◽  
A. Masoumi

Abstract. The polarized phase function of atmospheric aerosols has been investigated for the atmosphere of Zanjan, a city in northwest Iran. To do this, aerosol optical depth, Ångström exponent, single-scattering albedo, and polarized phase function have been retrieved from the measurements of a Cimel CE 318-2 polarized sun-photometer from February 2010 to December 2012. The results show that the maximum value of aerosol polarized phase function as well as the polarized phase function retrieved for a specific scattering angle (i.e., 60°) are strongly correlated (R = 0.95 and 0.95, respectively) with the Ångström exponent. The latter has a meaningful variation with respect to the changes in the complex refractive index of the atmospheric aerosols. Furthermore the polarized phase function shows a moderate negative correlation with respect to the atmospheric aerosol optical depth and single-scattering albedo (R = −0.76 and −0.33, respectively). Therefore the polarized phase function can be regarded as a key parameter to characterize the atmospheric particles of the region – a populated city in the semi-arid area and surrounded by some dust sources of the Earth's dust belt.


2021 ◽  
Vol 14 (10) ◽  
pp. 6419-6441
Author(s):  
Krista Luoma ◽  
Aki Virkkula ◽  
Pasi Aalto ◽  
Katrianne Lehtipalo ◽  
Tuukka Petäjä ◽  
...  

Abstract. We present a comparison between three absorption photometers that measured the absorption coefficient (σabs) of ambient aerosol particles in 2012–2017 at SMEAR II (Station for Measuring Ecosystem–Atmosphere Relations II), a measurement station located in a boreal forest in southern Finland. The comparison included an Aethalometer (AE31), a multi-angle absorption photometer (MAAP), and a particle soot absorption photometer (PSAP). These optical instruments measured particles collected on a filter, which is a source of systematic errors, since in addition to the particles, the filter fibers also interact with light. To overcome this problem, several algorithms have been suggested to correct the AE31 and PSAP measurements. The aim of this study was to research how the different correction algorithms affected the derived optical properties. We applied the different correction algorithms to the AE31 and PSAP data and compared the results against the reference measurements conducted by the MAAP. The comparison between the MAAP and AE31 resulted in a multiple-scattering correction factor (Cref) that is used in AE31 correction algorithms to compensate for the light scattering by filter fibers. Cref varies between different environments, and our results are applicable to a boreal environment. We observed a clear seasonal cycle in Cref, which was probably due to variations in aerosol optical properties, such as the backscatter fraction and single-scattering albedo, and also due to variations in the relative humidity (RH). The results showed that the filter-based absorption photometers seemed to be rather sensitive to the RH even if the RH was kept below the recommended value of 40 %. The instruments correlated well (R≈0.98), but the slopes of the regression lines varied between the instruments and correction algorithms: compared to the MAAP, the AE31 underestimated σabs only slightly (the slopes varied between 0.96–1.00) and the PSAP overestimated σabs only a little (the slopes varied between 1.01–1.04 for a recommended filter transmittance >0.7). The instruments and correction algorithms had a notable influence on the absorption Ångström exponent: the median absorption Ångström exponent varied between 0.93–1.54 for the different algorithms and instruments.


2019 ◽  
Vol 99 ◽  
pp. 01003
Author(s):  
Athina Avgousta Floutsi ◽  
Marios Bruno Korras Carraca ◽  
Christos Matsoukas ◽  
Nikos Hatzianastassiou ◽  
George Biskos

Central and South Asia are regions of particular interest for studying atmospheric aerosols, being among the largest sources of desert dust aerosols globally. In this study we use the newest collection (C061) of MODIS - Aqua aerosol optical depth (AOD) at 550 nm and Ångström exponent (a) at 412/470 nm over the 15-year period between 2002 and 2017, providing the longest analyzed dataset for this region. According to our results, during spring and summer, high aerosol load (AOD up to 1.2) consisting of coarse desert dust particles, as indicated by a values as low as 0.15, is observed over the Taklamakan, Thar and Registan deserts and the region between the Aral and Caspian seas. The dust load is much lower during winter and autumn (lower AOD and higher a values compared to the other seasons). The interannual variation of AOD and a suggests that the dust load exhibits large decreasing trends (AOD slopes down to -0.22, a slopes up to 0.47 decade-1) over the Thar desert and large increasing trends between the Aral and Caspian seas (AOD and a slopes up to 0.23 decade-1 and down to -0.61 decade-1, respectively.) The AOD data are evaluated against AERONET surface-based measurements. Generally, MODIS and AERONET data are in good agreement with a correlation coefficient (R) equal to 0.835.


Atmosphere ◽  
2020 ◽  
Vol 11 (10) ◽  
pp. 1103
Author(s):  
Jie Luo ◽  
Yongming Zhang ◽  
Qixing Zhang

In this work, the absorption Ångström exponent (AAE), extinction Ångström exponent (EAE), and single-scattering albedo (SSA) of black carbon (BC) with different coating materials are numerically investigated. BC with different coating materials can provide explanations for the small AAE, small EAE, and large AAE observed in the atmosphere, which is difficult to be explained by bare BC aggregate models. The addition of organic carbon (OC) does not necessarily increase AAE due to the transformation of BC morphologies and the existence of non-absorbing OC. The addition of coating materials does also not necessarily decrease EAE. While the addition of coating materials can increase the total size of BC-containing particles, the effective refractive index can be modified by introducing the coating materials, so increases the EAE. We found that it is not possible to differentiate between thinly- and heavily-coated BC based on EAE or AAE alone. On the other hand, SSA is much less sensitive to the size and can provide much more information for distinguishing heavily-coated BC from thinly-coated BC. For BC with different coating materials and mixing states, AAE, EAE, and SSA show rather different sensitivities to particle size and composition ratios, and their spectral-dependences also exhibit distinct differences. Different AAE and EAE trends with BC/OC ratio were also found for BC with different coating materials and mixing states. Furthermore, we also found empirical fittings for AAE, EAE, SSA, and optical cross-sections, which may be useful for retrieving the size information based on the optical measurements.


Atmosphere ◽  
2019 ◽  
Vol 10 (9) ◽  
pp. 482 ◽  
Author(s):  
Victor Nicolae ◽  
Camelia Talianu ◽  
Simona Andrei ◽  
Bogdan Antonescu ◽  
Dragoș Ene ◽  
...  

In this study, AERONET (Aerosol Robotic Network) and EARLINET (European Aerosol Research Lidar Network) data from 17 collocated lidar and sun photometer stations were used to characterize the optical properties of aerosol and their types for the 2008–2018 period in various regions of Europe. The analysis was done on six cluster domains defined using circulation types around each station and their common circulation features. As concluded from the lidar photometer measurements, the typical aerosol particles observed during 2008–2018 over Europe were medium-sized, medium absorbing particles with low spectral dependence. The highest mean values for the lidar ratio at 532 nm were recorded over Northeastern Europe and were associated with Smoke particles, while the lowest mean values for the Angstrom exponent were identified over the Southwest cluster and were associated with Dust and Marine particles. Smoke (37%) and Continental (25%) aerosol types were the predominant aerosol types in Europe, followed by Continental Polluted (17%), Dust (10%), and Marine/Cloud (10%) types. The seasonal variability was insignificant at the continental scale, showing a small increase in the percentage of Smoke during spring and a small increase of Dust during autumn. The aerosol optical depth (AOD) slightly decreased with time, while the Angstrom exponent oscillated between “hot and smoky” years (2011–2015) on the one hand and “dusty” years (2008–2010) and “wet” years (2017–2018) on the other hand. The high variability from year to year showed that aerosol transport in the troposphere became more and more important in the overall balance of the columnar aerosol load.


2013 ◽  
Vol 2013 ◽  
pp. 1-17 ◽  
Author(s):  
Boris B. Chen ◽  
Leonid G. Sverdlik ◽  
Sanjar A. Imashev ◽  
Paul A. Solomon ◽  
Jeffrey Lantz ◽  
...  

The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM2.5 and PM10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regional sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the Ångström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the Ångström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.


2017 ◽  
Vol 9 (7) ◽  
pp. 693 ◽  
Author(s):  
Yidan Si ◽  
Shenshen Li ◽  
Liangfu Chen ◽  
Huazhe Shang ◽  
Lei Wang ◽  
...  

2006 ◽  
Vol 6 (10) ◽  
pp. 2981-2990 ◽  
Author(s):  
M. Schnaiter ◽  
M. Gimmler ◽  
I. Llamas ◽  
C. Linke ◽  
C. Jäger ◽  
...  

Abstract. We have measured the extinction and absorption cross sections of carbon particles emitted by a propane diffusion flame both in an aerosol chamber and on size-segregated samples deposited on optical windows. The absorption cross section, the single scattering albedo, and the Ångström exponent show drastic dependencies both on the C/O ratio and on the particle size. This is interpretated as being due to the appearance of nucleation modes of smaller organic particles at higher C/O ratios, which were detected by SMPS measurements and partially by TEM analysis. The spectral range of the validity of the absorption power-law (Ångström exponent) model is investigated by vacuum ultraviolet extinction measurements. These measurements give also indications for a preferentially aromatic nature of the OC component of the flame products.


2010 ◽  
Vol 3 (3) ◽  
pp. 569-578 ◽  
Author(s):  
E. Giannakaki ◽  
D. S. Balis ◽  
V. Amiridis ◽  
C. Zerefos

Abstract. We present our combined Raman/elastic backscatter lidar observations which were carried out at the EARLINET station of Thessaloniki, Greece, during the period 2001–2007. The largest optical depths are observed for Saharan dust and smoke aerosol particles. For local and continental polluted aerosols the measurements indicate high aerosol loads. However, measurements associated with the local path indicate enhanced aerosol load within the Planetary Boundary Layer. The lowest value of aerosol optical depth is observed for continental aerosols, from West directions with less free tropospheric contribution. The largest lidar ratios, of the order of 70 sr, are found for biomass burning aerosols. A significant and distinct correlation between lidar ratio and backscatter related Ångström exponent values were estimated for different aerosol categories. Scatter plot between lidar ratio values and Ångström exponent values for local and continental polluted aerosols does not show a significant correlation, with a large variation in both parameters possibly due to variable absorption characteristics of these aerosols. Finally for continental aerosols with west and northwest directions that follow downward movement when arriving at our site constantly low lidar ratios almost independent of size are found.


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