scholarly journals Potential of Raman Lidar for Profiling of Methane Mixing Ratio in the Lower Troposphere

2020 ◽  
Vol 237 ◽  
pp. 03024
Author(s):  
Igor Veselovskii ◽  
Philippe Goloub ◽  
Qiaoyun Hu ◽  
Thierry Podvin ◽  
Mikhail Korenskiy

The results of methane profiling in the lower troposphere by Raman lidar from Lille University observatory platform (France), are presented. The use of powerful DPSS tripled Nd:YAG laser allowed profiling of methane background mixing ratio of 2 ppm in the night time up to 4000 m with 100 m height and 1 hour temporal resolution. Enhancement of CH4 mixing ratio inside the boundary layer comparing to the free troposphere values was observed.

2018 ◽  
Author(s):  
Igor Veselovskii ◽  
Philippe Goloub ◽  
Qiaoyun Hu ◽  
Thierry Podvin ◽  
David N. Whiteman ◽  
...  

Abstract. We present the results of methane profiling in the lower troposphere using LILAS Raman lidar from Lille University observatory platform (France). The lidar is based on a tripled Nd:YAG laser and nighttime profiling up to 4000 m with 100 m height resolution is possible for methane. Agreement between measured the photon counting rate in the CH4 Raman channel in the free troposphere and numerical simulations for a typical CH4 background mixing ratio (2 ppm) confirms that CH4 Raman scattering is observed. Within the planetary boundary layer, an increase of the CH4 mixing ratio, up to a factor of 2, is observed. Different possible interfering factors, such as leakage of the elastic signal and aerosol fluorescence have been taken into consideration. Tests using backscattering from clouds confirmed that the filters in the Raman channel provide sufficient rejection of elastic scattering. The measured methane profiles do not correlate with aerosol backscattering, which corroborates the hypothesis that, in the PBL, not aerosol fluorescence but CH4 is observed. However, the fluorescence contribution cannot be completely excluded and, for future measurements, we plan to install an additional control channel close to 393 nm where no strong Raman lines exist and only fluorescence can be observed.


2019 ◽  
Vol 12 (1) ◽  
pp. 119-128 ◽  
Author(s):  
Igor Veselovskii ◽  
Philippe Goloub ◽  
Qiaoyun Hu ◽  
Thierry Podvin ◽  
David N. Whiteman ◽  
...  

Abstract. We present the results of methane profiling in the lower troposphere using LILAS Raman lidar from the Lille University observatory platform (France). The lidar is based on a frequency-tripled Nd:YAG laser, and nighttime profiling up to 4000 with 100 m height resolution is possible for methane. Agreement between the measured photon-counting rate in the CH4 Raman channel in the free troposphere and numerical simulations for a typical CH4 background mixing ratio (2 ppm) confirms that CH4 Raman scattering is detected. The mixing ratio is calculated from the ratio of methane (395.7 nm) and nitrogen (386.7 nm) Raman backscatters, and within the planetary boundary layer, an increase of the CH4 mixing ratio, up to a factor of 2, is observed. Different possible interfering factors, such as leakage of the elastic signal and aerosol fluorescence, have been taken into consideration. Tests using backscattering from clouds confirmed that the filters in the Raman channel provide sufficient rejection of elastic scattering. The measured methane profiles do not correlate with aerosol backscattering, which corroborates the hypothesis that, in the planetary boundary layer, not aerosol fluorescence but CH4 is observed. However, the fluorescence contribution cannot be completely excluded and, for future measurements, we plan to install an additional control channel close to 393 nm, where no strong Raman lines exist and only fluorescence can be observed.


2021 ◽  
Author(s):  
Diego Lange ◽  
Andreas Behrendt ◽  
Volker Wulfmeyer

<p>We present the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS), a new tool for observations in the atmospheric boundary layer and lower free troposphere during daytime and nighttime with very high resolution up to the turbulence scale, high accuracy and precision, and very short latency and illustrate its performance with new measurements examples. ARTHUS measurements resolve the strength of the inversion layer at the planetary boundary layer top, elevated lids in the free troposphere, and turbulent fluctuations in water vapor and temperature, simultaneously (Lange et al., 2019). In addition to thermodynamic variables, ARTHUS provides also independent profiles of the particle backscatter coefficient and the particle extinction coefficient from the rotational Raman signals at 355 nm with much better resolution than a conventional vibrational Raman lidar.</p><p>The observation of atmospheric moisture and temperature profiles is essential for the understanding and prediction of earth system processes. These are fundamental components of the global and regional energy and water cycles, they determine the radiative transfer through the atmosphere, and are critical for the cloud formation and precipitation (Wulfmeyer, 2015). Also, as confirmed by case studies, the assimilation of high-quality, lower tropospheric WV and T profiles results in a considerable improvement of the skill of weather forecast models particularly with respect to extreme events.</p><p>Very stable and reliable performance was demonstrated during more than 3000 hours of operation experiencing a huge variety of weather conditions, including seaborne operation during the EUREC4A campaign (Bony et al., 2017, Stevens et al., 2020). ARTHUS provides temperature profiles with resolutions of 10-60 s and 7.5-100 m vertically in the lower free troposphere. During daytime, the statistical uncertainty of the WV mixing ratio is <2 % in the lower troposphere for resolutions of 5 minutes and 100 m. Temperature statistical uncertainty is <0.5 K even up to the middle troposphere. Consequently, ARTHUS fulfills the stringent WMO breakthrough requirements on nowcasting and very short-range forecasting (see www. wmo‐sat.info/oscar/observingrequirements).</p><p>This performance serves very well the next generation of very fast rapid-update-cycle data assimilation systems. Ground-based stations and networks can be set up or extended for climate monitoring, verification of weather, climate and earth system models, data assimilation for improving weather forecasts.</p><p><strong>References:</strong></p><p>Bony et al., 2017, https://doi.org/10.1007/s10712-017-9428-0</p><p>Lange et al., 2019, https://doi.org/10.1029/2019GL085774</p><p>Stevens et al. 2020, submitted to ESSD</p><p>Wulfmeyer et al., 2015, doi:10.1002/2014RG000476</p>


2016 ◽  
Author(s):  
Paolo Di Girolamo ◽  
Marco Cacciani ◽  
Donato Summa ◽  
Andrea Scoccione ◽  
Benedetto De Rosa ◽  
...  

Abstract. Measurements carried out by the University of BASILicata Raman lidar system (BASIL) are reported to demonstrate the capability of this instrument to characterize turbulent processes within the convective boundary layer (CBL). In order to resolve the vertical profiles of turbulent variables, high resolution water vapour and temperature measurements, with a temporal resolution of 10 s and a vertical resolution of 90 m and 30 m, respectively, are considered. Measurements of higher-order moments of the turbulent fluctuations of water vapour mixing ratio and temperature are obtained based on the application of auto-covariance analyses to the water vapour mixing ratio and temperature time series. The algorithms are applied to a case study (11:30–13:30 UTC, 20 April 2013) from the High Definition Clouds and Precipitation for Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE), held in Western Germany in the spring 2013. A new correction scheme for the elastic-signal leakage in the low-quantum number rotational Raman signal is applied. The noise errors are small enough to derive up to fourth-order moments for both water vapour mixing ratio and temperature fluctuations. To the best of our knowledge, BASIL is the first Raman lidar with a demonstrated capability to simultaneously retrieve daytime profiles of water vapour turbulent fluctuations up to the fourth order throughout the atmospheric CBL, this capability being combined with the one to also measure daytime profiles of temperature fluctuations up to the fourth order. For the considered case study, which represents a well-mixed and quasi-stationary CBL, the mean boundary layer height is found to be 1290 ± 77 m a.g.l. Values of the integral scale for water vapour and temperature fluctuations at the top of the CBL are in the range of 70–125 s and 75–225 s, respectively; these values are much larger than the temporal resolution of the measurements (10 s), which testifies that the temporal resolution considered for the measurements is sufficiently high to resolve turbulence processes down to the inertial sub-range and consequently resolve the major part of the turbulent fluctuations. Peak values of all moments are found in the interfacial layer in the proximity of the top of the CBL. Specifically, water vapour and temperature second-order moment (variance) has a maximum value of 0.29 g2 kg−2 and 0.26 K2, respectively, water vapour and temperature third-order moment has a peak value of 0.156 g3 kg−3 and −0.067 K3, respectively, while water vapour and temperature fourth-order moment has a maximum value of 0.28 g4 kg−4 and 0.24 K4, respectively. Water vapour and temperature kurtosis have values of ~ 3 in the entrainment zone, which indicate normally distributed humidity and temperature fluctuations. Reported values of the higher-order moments result to be in good agreement with previous measurements at different locations, thus providing confidence on the possibility to use them for turbulence parameterization in weather and climate models. In the determination of the temperature profiles, particular care was dedicated to minimize potential effects associated with elastic signal leakage in the rotational Raman signals. For this purpose, a specific algorithm was defined and tested to identify and remove signal leakages and to assess the residual systematic uncertainty affecting temperature measurements after correction. The application of this approach confirms that for the present Raman lidar system the leakage factor keeps constant with time, and consequently an appropriate assessment of its constant value allows for a complete removal of the leaking elastic signal from the rotational Raman lidar signals at any time (with a residual error on temperature measurements after correction not exceeding 0.16 K).


2017 ◽  
Vol 17 (1) ◽  
pp. 745-767 ◽  
Author(s):  
Paolo Di Girolamo ◽  
Marco Cacciani ◽  
Donato Summa ◽  
Andrea Scoccione ◽  
Benedetto De Rosa ◽  
...  

Abstract. Measurements carried out by the University of Basilicata Raman lidar system (BASIL) are reported to demonstrate the capability of this instrument to characterise turbulent processes within the convective boundary layer (CBL). In order to resolve the vertical profiles of turbulent variables, high-resolution water vapour and temperature measurements, with a temporal resolution of 10 s and vertical resolutions of 90 and 30 m, respectively, are considered. Measurements of higher-order moments of the turbulent fluctuations of water vapour mixing ratio and temperature are obtained based on the application of autocovariance analyses to the water vapour mixing ratio and temperature time series. The algorithms are applied to a case study (11:30–13:30 UTC, 20 April 2013) from the High Definition Clouds and Precipitation for Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE), held in western Germany in the spring 2013. A new correction scheme for the removal of the elastic signal crosstalk into the low quantum number rotational Raman signal is applied. The noise errors are small enough to derive up to fourth-order moments for both water vapour mixing ratio and temperature fluctuations.To the best of our knowledge, BASIL is the first Raman lidar with a demonstrated capability to simultaneously retrieve daytime profiles of water vapour turbulent fluctuations up to the fourth order throughout the atmospheric CBL. This is combined with the capability of measuring daytime profiles of temperature fluctuations up to the fourth order. These measurements, in combination with measurements from other lidar and in situ systems, are important for verifying and possibly improving turbulence and convection parameterisation in weather and climate models at different scales down to the grey zone (grid increment  ∼  1 km; Wulfmeyer et al., 2016).For the considered case study, which represents a well-mixed and quasi-stationary CBL, the mean boundary layer height is found to be 1290 ± 75 m above ground level (a.g.l.). Values of the integral scale for water vapour and temperature fluctuations at the top of the CBL are in the range of 70–125 and 75–225 s, respectively; these values are much larger than the temporal resolution of the measurements (10 s), which testifies that the temporal resolution considered for the measurements is sufficiently high to resolve turbulent processes down to the inertial subrange and, consequently, to resolve the major part of the turbulent fluctuations. Peak values of all moments are found in the interfacial layer in the proximity of the top of the CBL. Specifically, water vapour and temperature second-order moments (variance) have maximum values of 0.29 g2 kg−2 and 0.26 K2; water vapour and temperature third-order moments have peak values of 0.156 g3 kg−3 and −0.067 K3, while water vapour and temperature fourth-order moments have maximum values of 0.28 g4 kg−4 and 0.24 K4. Water vapour and temperature kurtosis have values of  ∼  3 in the upper portion of the CBL, which indicate normally distributed humidity and temperature fluctuations. Reported values of the higher-order moments are in good agreement with previous measurements at different locations, thus providing confidence in the possibility of using these measurements for turbulence parameterisation in weather and climate models.In the determination of the temperature profiles, particular care was dedicated to minimise potential effects associated with elastic signal crosstalk on the rotational Raman signals. For this purpose, a specific algorithm was defined and tested to identify and remove the elastic signal crosstalk and to assess the residual systematic uncertainty affecting temperature measurements after correction. The application of this approach confirms that, for the present Raman lidar system, the crosstalk factor remains constant with time; consequently an appropriate assessment of its constant value allows for a complete removal of the leaking elastic signal from the rotational Raman lidar signals at any time (with a residual error on temperature measurements after correction not exceeding 0.18 K).


2014 ◽  
Vol 7 (5) ◽  
pp. 1201-1211 ◽  
Author(s):  
F. Navas-Guzmán ◽  
J. Fernández-Gálvez ◽  
M. J. Granados-Muñoz ◽  
J. L. Guerrero-Rascado ◽  
J. A. Bravo-Aranda ◽  
...  

Abstract. In this paper, we outline an iterative method to calibrate the water vapour mixing ratio profiles retrieved from Raman lidar measurements. Simultaneous and co-located radiosonde data are used for this purpose and the calibration results obtained during a radiosonde campaign in summer and autumn 2011 are presented. The water vapour profiles measured during night-time by the Raman lidar and radiosondes are compared and the differences between the methodologies are discussed. Then, a new approach to obtain relative humidity profiles by combination of simultaneous profiles of temperature (retrieved from a microwave radiometer) and water vapour mixing ratio (from a Raman lidar) is addressed. In the last part of this work, a statistical analysis of water vapour mixing ratio and relative humidity profiles obtained during 1 year of simultaneous measurements is presented.


2021 ◽  
Author(s):  
Diego Lange Vega ◽  
Andreas Behrendt ◽  
Volker Wulfmeyer

<p>Between 15 July 2020 and 19 September 2021, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS) collected data at the Lindenberg Observatory of the Deutscher Wetterdienst (DWD), including temperature and water vapor mixing ratio with a high temporal and range resolution.</p> <p>During the operation period, very stable 24/7 operation was achieved, and ARTHUS demonstrated that is capable to observe the atmospheric boundary layer and lower free troposphere during both daytime and nighttime up to the turbulence scale, with high accuracy and precision, and very short latency. During nighttime, the measurement range increases even up to the tropopause and lower stratosphere.</p> <p>ARTHUS measurements resolve the strength of the inversion layer at the planetary boundary layer top, elevated lids in the free troposphere, and turbulent fluctuations in water vapor and temperature, simultaneously (Lange et al., 2019, Wulfmeyer et al., 2015). In addition to thermodynamic variables, ARTHUS provides also independent profiles of the particle backscatter coefficient and the particle extinction coefficient from the rotational Raman signals at 355 nm with much better resolution than a conventional vibrational Raman lidar.</p> <p>At the conference, highlights of the measurements will be presented. Furthermore, the statistics of more than 150 comparisons with local radiosondes will be presented which confirm the high accuracy of the temperature and moisture measurements of ARTHUS.</p> <p><strong><em>Acknowledgements</em></strong></p> <p>The development of ARTHUS was supported by the Helmholtz Association of German Research Centers within the project Modular Observation Solutions for Earth Systems (MOSES). The measurements in Lindenberg were funded by DWD.</p> <p><strong><em>References </em></strong></p> <p>Lange, D., Behrendt, A., and Wulfmeyer, V. (2019). Compact operational tropospheric water vapor and temperature Raman lidar with turbulence resolution. <em>Geophysical Research Letters</em>, 46. https://doi.org/10.1029/2019GL085774</p> <p>Wulfmeyer, V., R. M. Hardesty, D. D. Turner, A. Behrendt, M. P. Cadeddu, P. Di Girolamo, P. Schlüssel, J. Van Baelen, and F. Zus (2015), A review of the remote sensing of lower tropospheric thermodynamic profiles and its indispensable role for the understanding and the simulation of water and energy cycles, <em>Rev. Geophys.</em>, 53,819–895, doi:10.1002/2014RG000476</p>


2014 ◽  
Vol 7 (9) ◽  
pp. 3127-3138 ◽  
Author(s):  
R. L. Herman ◽  
J. E. Cherry ◽  
J. Young ◽  
J. M. Welker ◽  
D. Noone ◽  
...  

Abstract. The EOS (Earth Observing System) Aura Tropospheric Emission Spectrometer (TES) retrieves the atmospheric HDO / H2O ratio in the mid-to-lower troposphere as well as the planetary boundary layer. TES observations of water vapor and the HDO isotopologue have been compared with nearly coincident in situ airborne measurements for direct validation of the TES products. The field measurements were made with a commercially available Picarro L1115-i isotopic water analyzer on aircraft over the Alaskan interior boreal forest during the three summers of 2011 to 2013. TES special observations were utilized in these comparisons. The TES averaging kernels and a priori constraints have been applied to the in situ data, using version 5 (V005) of the TES data. TES calculated errors are compared with the standard deviation (1σ) of scan-to-scan variability to check consistency with the TES observation error. Spatial and temporal variations are assessed from the in situ aircraft measurements. It is found that the standard deviation of scan-to-scan variability of TES δD is ±34.1‰ in the boundary layer and ± 26.5‰ in the free troposphere. This scan-to-scan variability is consistent with the TES estimated error (observation error) of 10–18‰ after accounting for the atmospheric variations along the TES track of ±16‰ in the boundary layer, increasing to ±30‰ in the free troposphere observed by the aircraft in situ measurements. We estimate that TES V005 δD is biased high by an amount that decreases with pressure: approximately +123‰ at 1000 hPa, +98‰ in the boundary layer and +37‰ in the free troposphere. The uncertainty in this bias estimate is ±20‰. A correction for this bias has been applied to the TES HDO Lite Product data set. After bias correction, we show that TES has accurate sensitivity to water vapor isotopologues in the boundary layer.


2015 ◽  
Vol 15 (5) ◽  
pp. 2867-2881 ◽  
Author(s):  
E. Hammann ◽  
A. Behrendt ◽  
F. Le Mounier ◽  
V. Wulfmeyer

Abstract. The temperature measurements of the rotational Raman lidar of the University of Hohenheim (UHOH RRL) during the High Definition of Clouds and Precipitation for advancing Climate Prediction (HD(CP)2) Observation Prototype Experiment (HOPE) in April and May 2013 are discussed. The lidar consists of a frequency-tripled Nd:YAG laser at 355 nm with 10 W average power at 50 Hz, a two-mirror scanner, a 40 cm receiving telescope, and a highly efficient polychromator with cascading interference filters for separating four signals: the elastic backscatter signal, two rotational Raman signals with different temperature dependence, and the vibrational Raman signal of water vapor. The main measurement variable of the UHOH RRL is temperature. For the HOPE campaign, the lidar receiver was optimized for high and low background levels, with a novel switch for the passband of the second rotational Raman channel. The instrument delivers atmospheric profiles of water vapor mixing ratio as well as particle backscatter coefficient and particle extinction coefficient as further products. As examples for the measurement performance, measurements of the temperature gradient and water vapor mixing ratio revealing the development of the atmospheric boundary layer within 25 h are presented. As expected from simulations, a reduction of the measurement uncertainty of 70% during nighttime was achieved with the new low-background setting. A two-mirror scanner allows for measurements in different directions. When pointing the scanner to low elevation, measurements close to the ground become possible which are otherwise impossible due to the non-total overlap of laser beam and receiving telescope field of view in the near range. An example of a low-level temperature measurement is presented which resolves the temperature gradient at the top of the stable nighttime boundary layer 100 m above the ground.


2010 ◽  
Vol 10 (6) ◽  
pp. 2847-2866 ◽  
Author(s):  
A. Lampert ◽  
C. Ritter ◽  
A. Hoffmann ◽  
J.-F. Gayet ◽  
G. Mioche ◽  
...  

Abstract. During the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR), which was conducted in Svalbard in March and April 2007, tropospheric Arctic clouds were observed with two ground-based backscatter lidar systems (micro pulse lidar and Raman lidar) and with an airborne elastic lidar. In the time period of the ASTAR 2007 campaign, an increase in low-level cloud cover (cloud tops below 2.5 km) from 51% to 65% was observed above Ny-Ålesund. Four different case studies of lidar cloud observations are analyzed: With the ground-based Raman lidar, a layer of spherical particles was observed at an altitude of 2 km after the dissolution of a cloud. The layer probably consisted of small hydrated aerosol (radius of 280 nm) with a high number concentration (around 300 cm−3) at low temperatures (−30 °C). Observations of a boundary layer mixed-phase cloud by airborne lidar and concurrent airborne in situ and spectral solar radiation sensors revealed the localized process of total glaciation at the boundary of different air masses. In the free troposphere, a cloud composed of various ice layers with very different optical properties was detected by the Raman lidar, suggesting large differences of ice crystal size, shape and habit. Further, a mixed-phase double layer cloud was observed by airborne lidar in the free troposphere. Local orography influenced the evolution of this cloud. The four case studies revealed relations of cloud properties and specific atmospheric conditions, which we plan to use as the base for numerical simulations of these clouds.


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