scholarly journals An Exploratory Study of Soot Sample Integrity and Probe Perturbation in a Swirl-Stabilized Combustor

1981 ◽  
Vol 103 (4) ◽  
pp. 759-771 ◽  
Author(s):  
R. L. Hack ◽  
G. S. Samuelsen ◽  
C. C. Poon ◽  
W. D. Bachalo

In-flame measurements of soot particulate using conventional extractive and nonintrusive optical probes are compared for a swirl-stabilized combustor. Except for large (∼5μm) particulate present in the extracted samples, the soot particle size compares favorably with optically measured values, and the soot particle morphology reflects that formed in gas turbine combustors. Two, nonflame sources for the large particulate are suggested by the optical data: particles formed or elongated during transport subsequent to extraction, and particles attrited from upstream carbon deposits on a solid surface. The extractive probe produces a change in the local particle number density which varies from little change to a 70-fold suppression in reacting flow and a 200-fold increase in cold seeded flow depending on the location within the combustor of the optical sampling volume, the location of the extractive probe relative to the optical sampling volume, and the combustor operating conditions.

2021 ◽  
Author(s):  
Nick A. Eaves ◽  
Seth B. Dworkin ◽  
Murray J. Thomson

Given the recent EURO 6 regulations, which include limits on particle number density (and hence size) for soot emissions from land vehicles, soot models must be capable of accurately predicting soot particle sizes. Previous modeling work has demonstrated the importance of the relative strengths of nucleation and condensation in predicting soot primary particle size. Due to this importance, a fundamental reversible model for nucleation and condensation, called the reversible PAH clustering (RPC) model, was developed in previous work through the use of statistical mechanics and the results from several recent works. In the present work, the RPC model is enhanced to include multiple nucleation (or dimerization) events from 6 different PAH size groups, resulting in 21 unique dimer pairs. In addition, a soot PAH tracking model is developed to track the amount of each PAH size group within soot particles. The addition of this model resulted in reduced computation times and the ability to investigate PAH-PAH reactions within soot particles. The results of the enhanced RPC model demonstrate that smaller PAHs are most important for the nucleation process, while small and large PAHs are important for the condensation process. These results are shown to be due to the relatively lower reversibility of condensation versus the nucleation process. These findings are discussed in light of recent experimental results in the literature and are shown to be well supported. Keywords: reversibility, PAH nucleation, PAH condensation, laminar diffusion flame, soot model


2021 ◽  
Author(s):  
Nick A. Eaves ◽  
Seth B. Dworkin ◽  
Murray J. Thomson

Given the recent EURO 6 regulations, which include limits on particle number density (and hence size) for soot emissions from land vehicles, soot models must be capable of accurately predicting soot particle sizes. Previous modeling work has demonstrated the importance of the relative strengths of nucleation and condensation in predicting soot primary particle size. Due to this importance, a fundamental reversible model for nucleation and condensation, called the reversible PAH clustering (RPC) model, was developed in previous work through the use of statistical mechanics and the results from several recent works. In the present work, the RPC model is enhanced to include multiple nucleation (or dimerization) events from 6 different PAH size groups, resulting in 21 unique dimer pairs. In addition, a soot PAH tracking model is developed to track the amount of each PAH size group within soot particles. The addition of this model resulted in reduced computation times and the ability to investigate PAH-PAH reactions within soot particles. The results of the enhanced RPC model demonstrate that smaller PAHs are most important for the nucleation process, while small and large PAHs are important for the condensation process. These results are shown to be due to the relatively lower reversibility of condensation versus the nucleation process. These findings are discussed in light of recent experimental results in the literature and are shown to be well supported. Keywords: reversibility, PAH nucleation, PAH condensation, laminar diffusion flame, soot model


1993 ◽  
Vol 7 (6) ◽  
pp. 842-851 ◽  
Author(s):  
M. Queiroz ◽  
M. P. Bonin ◽  
J. S. Shirolkar ◽  
R. W. Dawson

2016 ◽  
Vol 7 (32) ◽  
pp. 5123-5131 ◽  
Author(s):  
O. L. J. Virtanen ◽  
M. Brugnoni ◽  
M. Kather ◽  
A. Pich ◽  
W. Richtering

Many applications of poly(N-isopropylacrylamide) microgels necessitate robust control over particle size.


Author(s):  
I. V. Novosselov ◽  
P. C. Malte ◽  
S. Yuan ◽  
R. Srinivasan ◽  
J. C. Y. Lee

A chemical reactor network (CRN) is developed and applied to a dry low emissions (DLE) industrial gas turbine combustor with the purpose of predicting exhaust emissions. The development of the CRN model is guided by reacting flow computational fluid dynamics (CFD) using the University of Washington (UW) eight-step global mechanism. The network consists of 31 chemical reactor elements representing the different flow and reaction zones of the combustor. The CRN is exercised for full load operating conditions with variable pilot flows ranging from 35% to 200% of the neutral pilot. The NOpilot. The NOx and the CO emissions are predicted using the full GRI 3.0 chemical kinetic mechanism in the CRN. The CRN results closely match the actual engine test rig emissions output. Additional work is ongoing and the results from this ongoing research will be presented in future publications.


2020 ◽  
Author(s):  
Γεώργιος Πατεράκης

The current work describes an experimental investigation of isothermal and turbulent reacting flow field characteristics downstream of axisymmetric bluff body stabilizers under a variety of inlet mixture conditions. Fully premixed and stratified flames established downstream of this double cavity premixer/burner configuration were measured and assessed under lean and ultra-lean operating conditions. The aim of this thesis was to further comprehend the impact of stratifying the inlet fuelair mixture on the reacting wake characteristics for a range of practical stabilizers under a variety of inlet fuel-air settings. In the first part of this thesis, the isothermal mean and turbulent flow features downstream of a variety of axisymmetric baffles was initially examined. The effect of different shapes, (cone or disk), blockage ratios, (0.23 and 0.48), and rim thicknesses of these baffles was assessed. The variations of the recirculation zones, back flow velocity magnitude, annular jet ejection angles, wake development, entrainment efficiency, as well as several turbulent flow features were obtained, evaluated and appraised. Next, a comparative examination of the counterpart turbulent cold fuel-air mixing performance and characteristics of stratified against fully-premixed operation was performed for a wide range of baffle geometries and inlet mixture conditions. Scalar mixing and entrainment properties were investigated at the exit plane, at the bluff body annular shear layer, at the reattachment region and along the developing wake were investigated. These isothermal studies provided the necessary background information for clarifying the combustion properties and interpreting the trends in the counterpart turbulent reacting fields. Subsequently, for selected bluff bodies, flame structures and behavior for operation with a variety of reacting conditions were demonstrated. The effect of inlet fuel-air mixture settings, fuel type and bluff body geometry on wake development, flame shape, anchoring and structure, temperatures and combustion efficiencies, over lean and close to blow-off conditions, was presented and analyzed. For the obtained measurements infrared radiation, particle image velocimetry, laser doppler velocimetry, chemiluminescence imaging set-ups, together with Fouriertransform infrared spectroscopy, thermocouples and global emission analyzer instrumentation was employed. This helped to delineate a number of factors that affectcold flow fuel-air mixing, flame anchoring topologies, wake structure development and overall burner performance. The presented data will also significantly assist the validation of computational methodologies for combusting flows and the development of turbulence-chemistry interaction models.


2017 ◽  
Vol 34 (7) ◽  
pp. 075203
Author(s):  
Rang-Yue Zhang ◽  
Yan-Hong Liu ◽  
Feng Huang ◽  
Zhao-Yang Chen ◽  
Chun-Yan Li

2001 ◽  
Author(s):  
S. L. Chang ◽  
C. Q. Zhou ◽  
B. Golchert ◽  
M. Petrick

Abstract A typical glass furnace consists of a combustion space and a melter. The intense heat, generated from the combustion of fuel and air/oxygen in the combustion space, is transferred mainly by radiation to the melter where the melt sand and cullet (scrap glass) are melted, creating molten glass. The melter flow is a complex multi-phase flow including solid batches of sand/cullet and molten glass. Proper modeling of the flow patterns of the solid batch and liquid glass is a key to determining the glass quality and furnace efficiency. A multi-phase CFD code has been developed to simulate glass melter flow. It uses an Eulerian approach for both the solid batch and the liquid glass-melt flows. The mass, momentum, and energy conservation equations of the batch flow are used to solve for local batch particle number density, velocity, and temperature. In a similar manner, the conservation equations of mass, momentum, and energy of the glass-melt flow are used to solve for local liquid molten glass pressure, velocity, and temperature. The solid batch is melted on the top by the heat from the combustion space and from below by heat from the glass-melt flow. The heat transfer rate from the combustion space is calculated from a radiation model calculation while the heat transfer rate from the glass-melt flow to the solid batch is calculated from a model based on local particle number density and glass-melt temperature. Energy and mass are balanced between the batch and the glass-melt. Batch coverage is determined from local particle number density and velocity. A commercial-scale glass melter has been simulated at different operating/design conditions.


1991 ◽  
Vol 130 ◽  
pp. 71-74
Author(s):  
A.Z. Dolginov ◽  
N.A. Silant’ev

AbstractA new method for the calculation of kinetic coefficients is presented. This method allows us to obtain the distribution of scalar and vector fields (such as the temperature, the admixture particle number density and the magnetic field) in turbulent cosmic media with any value of S = u0т0/R0. The explicit expression for the “turbulent” diffusivity DT is obtained. In some cases DT becomes negative, implying the clustering of the admixture particles in patches (a local increase of the temperature and magnetic fields). The magnetic α-effect is considered for the case S ~ 1.


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