Time-resolved and quasi-continuous wave three-dimensional tomographic imaging of objects in tissue-like turbid media

2004 ◽  
Author(s):  
Mohammad Alrubaiee ◽  
Min Xu ◽  
S. K. Gayen ◽  
Wei Cai ◽  
R. R. Alfano
Keyword(s):  
Continuous Wave ◽  
Three Dimensional ◽  
Tomographic Imaging ◽  
Turbid Media ◽  
Time Resolved

scholarly journals Three-Dimensional High Spatial Localization of Efficient Resonant Energy Transfer from Laser-Assisted Precipitated Silver Clusters to Trivalent Europium Ions

Crystals ◽  
2021 ◽  
Vol 11 (2) ◽  
pp. 148
Author(s):  
Yannick Petit ◽  
Gustavo Galleani ◽  
Guillaume Raffy ◽  
Jean-Charles Desmoulin ◽  
Véronique Jubéra ◽  
...  
Keyword(s):  
Energy Transfer ◽  
Continuous Wave ◽  
Three Dimensional ◽  
Fluorescence Emission ◽  
Rare Earth Ions ◽  
Radiative Energy ◽  
Silver Clusters ◽  
Time Resolved ◽  
Zinc Phosphate Glass ◽  
Direct Laser

We report on the 3D precipitation, using a direct laser writing approach, of highly fluorescent silver clusters in a Eu3+-doped silver-containing zinc phosphate glass. Micro-spectroscopy of fluorescence emission shows the ability to continuously adjust the local tri-chromatic coordinates in the CIE (Commission Internationale de l’Éclairage) chromaticity diagram between red and white colors, thanks to the laser-deposited dose and resulting tunable combination of emissions from Eu3+ and silver clusters. Moreover, continuous-wave and time-resolved FAST-FLIM spectroscopies showed a significant enhancement of the fluorescence emission of Eu3+ ions while being co-located with UV-excited laser-inscribed silver clusters. These results demonstrate the ability to perform efficient resonant non-radiative energy transfer from excited silver clusters to Eu3+, allowing such energy transfer to be highly localized on demand thanks to laser inscription. Such results open the route to 3D printing of the rare earth ions emission in glass.

Pump-Probe Measurements Using Silicon Nanocrystal Waveguides

2003 ◽  
Vol 770 ◽  
Author(s):  
Nathanael Smith ◽  
Max J. Lederer ◽  
Marek Samoc ◽  
Barry Luther-Davies ◽  
Robert G. Elliman
Keyword(s):  
Probe Beam ◽  
Time Resolution ◽  
Pump Beam ◽  
Silicon Nanocrystals ◽  
Continuous Wave ◽  
Optical Gain ◽  
Optical Pump ◽  
Time Resolved ◽  
Pump Probe ◽  
Probe Measurements

AbstractOptical pump-probe measurements were performed on planar slab waveguides containing silicon nanocrystals in an attempt to measure optical gain from photo-excited silicon nanocrystals. Two experiments were performed, one with a continuous-wave probe beam and a pulsed pump beam, giving a time resolution of approximately 25 ns, and the other with a pulsed pump and probe beam, giving a time resolution of approximately 10 ps. In both cases the intensity of the probe beam was found to be attenuated by the pump beam, with the attenuation increasing monotonically with increasing pump power. Time-resolved measurements using the first experimental arrangement showed that the probe signal recovered its initial intensity on a time scale of 45-70 μs, a value comparable to the exciton lifetime in Si nanocrystals. These data are shown to be consistent with an induced absorption process such as confined carrier absorption. No evidence for optical gain was observed.

scholarly journals Picosecond time-resolved photon antibunching measures nanoscale exciton motion and the true number of chromophores

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Gordon J. Hedley ◽  
Tim Schröder ◽  
Florian Steiner ◽  
Theresa Eder ◽  
Felix J. Hofmann ◽  
...  
Keyword(s):  
Rational Design ◽  
Three Dimensional ◽  
Dna Origami ◽  
Fluorescent Nanoparticles ◽  
Time Resolved ◽  
Exciton Diffusion ◽  
Polymer Aggregates ◽  
True Number ◽  
Particle Level ◽  
Photon Antibunching

AbstractThe particle-like nature of light becomes evident in the photon statistics of fluorescence from single quantum systems as photon antibunching. In multichromophoric systems, exciton diffusion and subsequent annihilation occurs. These processes also yield photon antibunching but cannot be interpreted reliably. Here we develop picosecond time-resolved antibunching to identify and decode such processes. We use this method to measure the true number of chromophores on well-defined multichromophoric DNA-origami structures, and precisely determine the distance-dependent rates of annihilation between excitons. Further, this allows us to measure exciton diffusion in mesoscopic H- and J-type conjugated-polymer aggregates. We distinguish between one-dimensional intra-chain and three-dimensional inter-chain exciton diffusion at different times after excitation and determine the disorder-dependent diffusion lengths. Our method provides a powerful lens through which excitons can be studied at the single-particle level, enabling the rational design of improved excitonic probes such as ultra-bright fluorescent nanoparticles and materials for optoelectronic devices.

Impact of an Aortic Nitinol Stent Graft on Flow Measurements by Time-resolved Three-dimensional Velocity-encoded MRI

2012 ◽  
Vol 19 (3) ◽  
pp. 274-280 ◽  
Author(s):  
Fabian Rengier ◽  
Michael Delles ◽  
Roland Unterhinninghofen ◽  
Sebastian Ley ◽  
Sasan Partovi ◽  
...  
Keyword(s):  
Stent Graft ◽  
Three Dimensional ◽  
Flow Measurements ◽  
Time Resolved ◽  
Nitinol Stent

scholarly journals Time-Resolved Quadrupole Mass Spectrometric Studies on Pulsed Laser Ablation of TiO2

1999 ◽  
Vol 18 (3) ◽  
pp. 99-109 ◽  
Author(s):  
Yongxin Tang ◽  
Zhenhui Han ◽  
Qizong Qin
Keyword(s):  
Laser Ablation ◽  
Continuous Wave ◽  
Center Of Mass ◽  
Pulsed Laser ◽  
Pulsed Laser Ablation ◽  
Ionic Species ◽  
Mass Spectrometric ◽  
Quadrupole Mass ◽  
Time Resolved ◽  
Ambient Oxygen

Pulsed laser ablation of TiO2 at 355 nm and 532 nm has been investigated using an angleand time-resolved quadrupole mass spectrometric technique. The major ablated species include O (m/e = 16), O2 (m/e = 32), Ti (m/e = 48), TiO (m/e = 64) and TiO2 (m/e = 80). The time-of-flight (TOF) spectra of ablated species are measured for the ionic and neutral ablated species, and they can be fitted by a Maxwell – Boltzmann (M – B) distribution with a center-of-mass velocity. The measured angular distributions of the ionic species (O+ and Ti+) and the neutral species (O and Ti) can be fitted with cos⁡nθ and a cos⁡θ + (1−a)cos⁡nθ, respectively. In addition, a continuous wave oxygen molecular beam is introduced into the ablated plume, and the enhancement of the signal intensities of TiO is observed. It implies that the ablated Ti atoms/ions species can react with ambient oxygen molecules in the gas phase. In the meanwhile, the physicochemical mechanism of pulsed laser ablation of TiO2 is discussed.

Effects of Downstream Vane Bowing and Asymmetry on Unsteadiness in a Transonic Turbine

2018 ◽  
Author(s):  
John P. Clark ◽  
Richard J. Anthony ◽  
Michael K. Ooten ◽  
John M. Finnegan ◽  
P. Dean Johnson ◽  
...  
Keyword(s):  
Turbine Blades ◽  
Three Dimensional ◽  
Navier Stokes ◽  
Time Resolved ◽  
Turbine Engine ◽  
Shock Interactions ◽  
Design Changes ◽  
Post Test ◽  
Measured Time ◽  
Transonic Turbine

Accurate predictions of unsteady forcing on turbine blades are essential for the avoidance of high-cycle-fatigue issues during turbine engine development. Further, if one can demonstrate that predictions of unsteady interaction in a turbine are accurate, then it becomes possible to anticipate resonant-stress problems and mitigate them through aerodynamic design changes during the development cycle. A successful reduction in unsteady forcing for a transonic turbine with significant shock interactions due to downstream components is presented here. A pair of methods to reduce the unsteadiness was considered and rigorously analyzed using a three-dimensional, time resolved Reynolds-Averaged Navier Stokes (RANS) solver. The first method relied on the physics of shock reflections itself and involved altering the stacking of downstream components to achieve a bowed airfoil. The second method considered was circumferentially-asymmetric vane spacing which is well known to spread the unsteadiness due to vane-blade interaction over a range of frequencies. Both methods of forcing reduction were analyzed separately and predicted to reduce unsteady pressures on the blade as intended. Then, both design changes were implemented together in a transonic turbine experiment and successfully shown to manipulate the blade unsteadiness in keeping with the design-level predictions. This demonstration was accomplished through comparisons of measured time-resolved pressures on the turbine blade to others obtained in a baseline experiment that included neither asymmetric spacing nor bowing of the downstream vane. The measured data were further compared to rigorous post-test simulations of the complete turbine annulus including a bowed downstream vane of non-uniform pitch.

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