QUANTUM WELL LUMINESCENCE FROM METALLIC MONOLAYERS

2002 ◽  
Vol 01 (01) ◽  
pp. 53-62 ◽  
Author(s):  
GERMAR HOFFMANN ◽  
RICHARD BERNDT

The emission of visible light is observed from the metallic quantum well system Na on Cu(111) when electrons tunnel from the tip of a scanning tunnelling microscope to an unoccupied state of the sample. Spectral analysis of the emission along with tunnelling spectroscopy is used to show that the emission is comprised of two components. A sharp spectral feature is found to be due to an interband transition between quantum well states of the Na layer. The other component is similar to plasmon-mediated emission observed previously from clean metal surfaces. The results suggest that light emission is a unique local probe of the electronic structure of quantum well systems.

2016 ◽  
Vol 27 (46) ◽  
pp. 465201 ◽  
Author(s):  
B Rogez ◽  
S Cao ◽  
G Dujardin ◽  
G Comtet ◽  
E Le Moal ◽  
...  

2001 ◽  
Vol 482-485 ◽  
pp. 1159-1162 ◽  
Author(s):  
G. Hoffmann ◽  
J. Aizpurua ◽  
P. Apell ◽  
R. Berndt

Author(s):  
W.K. Lo ◽  
J.C.H. Spence

An improved design for a combination Scanning Tunnelling Microscope/TEM specimen holder is presented. It is based on earlier versions which have been used to test the usefulness of such a device. As with the earlier versions, this holder is meant to replace the standard double-tilt specimen holder of an unmodified Philips 400T TEM. It allows the sample to be imaged simultaneously by both the STM and the TEM when the TEM is operated in the reflection mode (see figure 1).The resolution of a STM is determined by its tip radii as well as its stability. This places strict limitations on the mechanical stability of the tip with respect to the sample. In this STM the piezoelectric tube scanner is rigidly mounted inside the endcap of the STM holder. The tip coarse approach to the sample (z-direction) is provided by an Inchworm which is located outside the TEM vacuum.


1996 ◽  
Vol 6 (11) ◽  
pp. 1461-1467 ◽  
Author(s):  
C. Sommers ◽  
P. M. Levy

2018 ◽  
Author(s):  
Gaolei Zhan ◽  
Younes Makoudi ◽  
Judicael Jeannoutot ◽  
Simon Lamare ◽  
Michel Féron ◽  
...  

Over the past decade, on-surface fabrication of organic nanostructures has been widely investigated for the development of molecular electronic devices, nanomachines, and new materials. Here, we introduce a new strategy to obtain alkyl oligomers in a controlled manner using on-surface radical oligomerisations that are triggered by the electrons/holes between the sample surface and the tip of a scanning tunnelling microscope. The resulting radical-mediated mechanism is substantiated by a detailed theoretical study. This electron transfer event only occurs when <i>V</i><sub>s</sub> < -3 V or <i>V</i><sub>s</sub> > + 3 V and allows access to reactive radical species under exceptionally mild conditions. This transfer can effectively ‘switch on’ a sequence leading to formation of oligomers of defined size distribution due to the on-surface confinement of reactive species. Our approach enables new ways to initiate and control radical oligomerisations with tunnelling electrons, leading to molecularly precise nanofabrication.


2014 ◽  
Vol 5 (1) ◽  
Author(s):  
Nasser Alidoust ◽  
Guang Bian ◽  
Su-Yang Xu ◽  
Raman Sankar ◽  
Madhab Neupane ◽  
...  

Nanoscale ◽  
2021 ◽  
Author(s):  
Tuhin Shuvra Basu ◽  
Simon Diesch ◽  
Ryoma Hayakawa ◽  
Yutaka Wakayama ◽  
Elke Scheer

We examined the modified electronic structure and single-carrier transport of individual hybrid core–shell metal–semiconductor Au-ZnS quantum dots using a scanning tunnelling microscope.


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