scholarly journals Small Irregular Ice Crystals in Tropical Cirrus

2011 ◽  
Vol 68 (11) ◽  
pp. 2614-2627 ◽  
Author(s):  
Timo Nousiainen ◽  
Hannakaisa Lindqvist ◽  
Greg M. McFarquhar ◽  
Junshik Um

Abstract Images acquired by a Cloud Particle Imager (CPI) are analyzed to compile a statistical covariance function of radius for an ensemble of small, irregular, quasi-spherical ice crystals in tropical cirrus measured during the Department of Energy Atmospheric Radiation Measurement Program’s Tropical Warm Pool International Cloud Experiment. The infrequent occurrence of multiple particles in single CPI frames suggests that most crystals sampled were natural ice crystals rather than artifacts from large particles shattering on probe tips. The covariance function is used in conjunction with the Gaussian random sphere geometry to generate three-dimensional model ice particles for ray-optics simulations at 550-nm wavelength. The crystal shapes and single-scattering properties are compared with those obtained by the same methodology for midlatitude cirrus sampled over Oklahoma. The small tropical ice crystals are closer to spherical than their midlatitude counterparts and, consequently, their asymmetry parameters are larger, but the differences are not significant from the standpoint of climate studies. Because some quasi-spherical ice crystals seem partially faceted, a convex hull transformation is introduced that increases the asymmetry parameter from 0.785 to 0.808. Further modifying the covariance function to promote sixfold symmetry in the model crystals increases the asymmetry parameter to 0.818. The introduction of internal scatterers, such as air bubbles, has a larger impact, decreasing the asymmetry parameter by up to tens of percent, depending on their amount and characteristics. Unfortunately, no data are available to determine realistic values for the internal scatterers to assess their likely actual impact.

2002 ◽  
Vol 15 (4) ◽  
pp. 333-352 ◽  
Author(s):  
Toshihiko Takemura ◽  
Teruyuki Nakajima ◽  
Oleg Dubovik ◽  
Brent N. Holben ◽  
Stefan Kinne

1996 ◽  
Vol 14 (11) ◽  
pp. 1192-1197 ◽  
Author(s):  
C. Liu ◽  
P. R. Jonas ◽  
C. P. R. Saunders

Abstract. Phase functions have been calculated using the Monte Carlo/geometric ray tracing method for single hexagonal pyramidal ice crystals (such as solid and hollow bullets) randomly oriented in space and horizontal plane, in order to study the concentric halo formations. Results from three dimensional model calculations show that 9° halo can be as bright as the common 22° halo for pyramidal angle of 28°, and the 18°, 20°, 24° and 35° halos cannot be seen due to the strong 22° halo domination in the scattering phase function between 18° and 35°. For solid pyramidal ice crystals randomly oriented horizontally, the 35° arc can be produced and its intensity depends on the incident ray solar angle and the particle aspect ratio.


2012 ◽  
Vol 12 (12) ◽  
pp. 32063-32107
Author(s):  
B. van Diedenhoven ◽  
B. Cairns ◽  
A. M. Fridlind ◽  
A. S. Ackerman ◽  
T. J. Garrett

Abstract. A new method to retrieve ice cloud asymmetry parameters from multi-directional polarized reflectance measurements is applied to measurements of the airborne Research Scanning Polarimeter (RSP) obtained during the CRYSTAL-FACE campaign in 2002. The method assumes individual hexagonal ice columns and plates serve as proxies for more complex shapes and aggregates. The closest fit is searched in a look-up table of simulated polarized reflectances computed for cloud layers that contain individual, randomly oriented hexagonal columns and plates with a virtually continuous selection of aspect ratios and distortion. The asymmetry parameter, aspect ratio and distortion of the hexagonal particle that leads to the best fit with the measurements are considered the retrieved values. Two cases of thick convective clouds and two cases of thinner anvil cloud layers are analyzed. Median asymmetry parameters retrieved by the RSP range from 0.76 to 0.78, and are generally smaller that those currently assumed in most climate models and satellite retrievals. In all cases the measurements indicate roughened ice crystals, which is consistent with previous findings. Retrieved aspect ratios in three of the cases range from 0.9 to 1.6, indicating compact particles dominate the cloud-top shortwave radiation. Retrievals for the remaining case indicate plate-like ice crystals with aspect ratios around 0.3. The RSP retrievals are qualitatively consistent with the CPI images obtained in the same cloud layers. Retrieved asymmetry parameters are compared to those determined in situ by the Cloud Integrating Nephelometer (CIN). For two cases, the median values of asymmetry parameter retrieved by CIN and RSP agree within 0.01, while for the two other cases RSP asymmetry parameters are about 0.03–0.05 greater than those obtained by the CIN. Part of this bias might be explained by vertical variation of the asymmetry parameter.


2011 ◽  
Vol 50 (8) ◽  
pp. 1740-1755 ◽  
Author(s):  
Krzysztof M. Markowicz ◽  
Marcin L. Witek

AbstractThe aim of this study is to investigate the sensitivity of radiative-forcing computations to various contrail crystal shape models. Contrail optical properties in the shortwave and longwave ranges are derived using a ray-tracing geometric method and the discrete dipole approximation method, respectively. Both methods present good correspondence of the single-scattering albedo and the asymmetry parameter in a transition range (3–8 μm). There are substantial differences in single-scattering properties among 10 crystal models investigated here (e.g., hexagonal columns and plates with different aspect ratios, and spherical particles). The single-scattering albedo and the asymmetry parameter both vary by up to 0.1 among various crystal shapes. The computed single-scattering properties are incorporated in the moderate-resolution atmospheric radiance and transmittance model (MODTRAN) radiative transfer code to simulate solar and infrared fluxes at the top of the atmosphere. Particle shapes have a strong impact on the contrail radiative forcing in both the shortwave and longwave ranges. The differences in the net radiative forcing among optical models reach 50% with respect to the mean model value. The hexagonal-column and hexagonal-plate particles show the smallest net radiative forcing, and the largest forcing is obtained for the spheres. The balance between the shortwave forcing and longwave forcing is highly sensitive with respect to the assumed crystal shape and may even change the sign of the net forcing. The optical depth at which the mean diurnal radiative forcing changes sign from positive to negative varies from 4.5 to 10 for a surface albedo of 0.2 and from 2 to 6.5 for a surface albedo of 0.05. Contrails are probably never that optically thick (except for some aged contrail cirrus), however, and so will not have a cooling effect on climate.


2016 ◽  
Author(s):  
A. M. Fridlind ◽  
R. Atlas ◽  
B. van Diedenhoven ◽  
J. Um ◽  
G. M. McFarquhar ◽  
...  

Abstract. Single-crystal images collected in mid-latitude cirrus are analyzed to provide internally consistent ice physical and optical properties for a size-resolved cloud microphysics model, including single-particle mass, projected area, fall speed, capacitance, single-scattering albedo, and asymmetry parameter. Using measurements gathered during two flights through a widespread synoptic cirrus shield, bullet rosettes are found to be the dominant identifiable habit among ice crystals with maximum dimension (Dmax) greater than 100 μm. Properties are therefore first derived for bullet rosettes based on measurements of arm lengths and widths, then for aggregates of bullet rosettes and for unclassified (irregular) crystals. Derived bullet rosette masses are substantially greater than reported in existing literature, whereas measured projected areas are similar or lesser, resulting in factors of 1.5–2 greater fall speeds, and, in the limit of large Dmax, near-infrared single-scattering albedo and asymmetry parameter (g) greater by ~ 0.2 and 0.05, respectively. A model that includes commonly imaged side plane growth on bullet rosettes exhibits relatively little difference in microphysical and optical properties aside from ~ 0.05 increase in mid-visible g primarily attributable to plate aspect ratio. In parcel simulations, ice size distribution and g are sensitive to assumed ice properties.


2013 ◽  
Vol 13 (6) ◽  
pp. 3185-3203 ◽  
Author(s):  
B. van Diedenhoven ◽  
B. Cairns ◽  
A. M. Fridlind ◽  
A. S. Ackerman ◽  
T. J. Garrett

Abstract. A new method to retrieve ice cloud asymmetry parameters from multi-directional polarized reflectance measurements is applied to measurements of the airborne Research Scanning Polarimeter (RSP) obtained during the CRYSTAL-FACE campaign in 2002. The method assumes individual hexagonal ice columns and plates serve as proxies for more complex shapes and aggregates. The closest fit is searched in a look-up table of simulated polarized reflectances computed for cloud layers that contain individual, randomly oriented hexagonal columns and plates with a virtually continuous selection of aspect ratios and distortion. The asymmetry parameter, aspect ratio and distortion of the hexagonal particle that leads to the best fit with the measurements are considered the retrieved values. Two cases of thick convective clouds and two cases of thinner anvil cloud layers are analyzed. Median asymmetry parameters retrieved by the RSP range from 0.76 to 0.78, and are generally smaller than those currently assumed in most climate models and satellite retrievals. In all cases the measurements indicate roughened or distorted ice crystals, which is consistent with previous findings. Retrieved aspect ratios in three of the cases range from 0.9 to 1.6, indicating compact particles dominate the cloud-top shortwave radiation. Retrievals for the remaining case indicate plate-like ice crystals with aspect ratios around 0.3. The RSP retrievals are qualitatively consistent with the CPI images obtained in the same cloud layers. Retrieved asymmetry parameters are compared to those determined in situ by the Cloud Integrating Nephelometer (CIN). For two cases, the median values of asymmetry parameter retrieved by CIN and RSP agree within 0.01, while for the two other cases RSP asymmetry parameters are about 0.03–0.05 greater than those obtained by the CIN. Part of this bias might be explained by vertical variation of the asymmetry parameter or ice shattering on the CIN probe, or both.


2020 ◽  
Vol 77 (4) ◽  
pp. 1245-1260 ◽  
Author(s):  
Bastiaan van Diedenhoven ◽  
Brian Cairns

Abstract We provide a parameterization of the extinction efficiency, single-scattering albedo, and asymmetry parameter of single ice crystals with any combination of particle volume, projected area, component aspect ratio, and crystal distortion at any wavelength between 0.2 and 100 μm. The parameterization is an extension of the one previously published by van Diedenhoven et al. In addition, the parameterized optical properties are integrated over size distributions yielding bulk extinction efficiencies, single-scattering albedos, and asymmetry parameters for large ranges of effective radii, particle component aspect ratios, and crystal distortion values. The parameterization of single-particle optical properties is evaluated with a reference database. The bulk optical properties are evaluated against the ice model selected for the Moderate Resolution Imaging Spectroradiometer (MODIS) collection 6 products, for which accurate optical properties are available. Mean absolute errors in parameterized extinction efficiency, asymmetry parameter, and single-scattering albedo are shown to be 0.0272, 0.008 90, and 0.004 68, respectively, for shortwave wavelengths, while they are 0.0641, 0.0368, and 0.0200 in the longwave. Shortwave and longwave asymmetry parameters and single-scattering albedos are shown to vary strongly with particle component aspect ratio and distortion, resulting in substantial variation in shortwave fluxes, but relatively small variations in longwave cloud emissivity. The parameterization and bulk optical properties are made publicly available.


2013 ◽  
Vol 70 (1) ◽  
pp. 330-347 ◽  
Author(s):  
Ping Yang ◽  
Lei Bi ◽  
Bryan A. Baum ◽  
Kuo-Nan Liou ◽  
George W. Kattawar ◽  
...  

Abstract A data library is developed containing the scattering, absorption, and polarization properties of ice particles in the spectral range from 0.2 to 100 μm. The properties are computed based on a combination of the Amsterdam discrete dipole approximation (ADDA), the T-matrix method, and the improved geometric optics method (IGOM). The electromagnetic edge effect is incorporated into the extinction and absorption efficiencies computed from the IGOM. A full set of single-scattering properties is provided by considering three-dimensional random orientations for 11 ice crystal habits: droxtals, prolate spheroids, oblate spheroids, solid and hollow columns, compact aggregates composed of eight solid columns, hexagonal plates, small spatial aggregates composed of 5 plates, large spatial aggregates composed of 10 plates, and solid and hollow bullet rosettes. The maximum dimension of each habit ranges from 2 to 10 000 μm in 189 discrete sizes. For each ice crystal habit, three surface roughness conditions (i.e., smooth, moderately roughened, and severely roughened) are considered to account for the surface texture of large particles in the IGOM applicable domain. The data library contains the extinction efficiency, single-scattering albedo, asymmetry parameter, six independent nonzero elements of the phase matrix (P11, P12, P22, P33, P43, and P44), particle projected area, and particle volume to provide the basic single-scattering properties for remote sensing applications and radiative transfer simulations involving ice clouds. Furthermore, a comparison of satellite observations and theoretical simulations for the polarization characteristics of ice clouds demonstrates that ice cloud optical models assuming severely roughened ice crystals significantly outperform their counterparts assuming smooth ice crystals.


2011 ◽  
Vol 29 (6) ◽  
pp. 973-985 ◽  
Author(s):  
K. Niranjan ◽  
B. Spandana ◽  
T. Anjana Devi ◽  
V. Sreekanth ◽  
B. L. Madhavan

Abstract. Information on the aerosol intensive properties like Single Scattering Albedo (SSA) and asymmetry parameter are very limited, particularly over the peninsular India, though extensive reports are available on the aerosol bulk properties. In view of the importance of these parameters in evaluating the aerosol radiative forcing, we present for the first time the temporal variation in SSA with measurements on aerosol absorption and scattering coefficients over Visakhapatnam (17.72° N, 83.32° E; located on the east coast of India) for the year 2007. The inferred SSA was in the range of 0.65 and 0.9 with an annual mean of 0.76 ± 0.013 and with a probable value of 0.80, indicating a marginal atmospheric warming over the region. The mixed layer contribution to column Aerosol Optical depth is found to be 35 % in summer while it is well above 35 % in winter, indicating the confinement of aerosol within the boundary layer during winter. The asymmetry parameter which represents the angular scattering in radiative forcing estimation is found to be around 0.65 ± 0.1 for the location. The day to day variability in SSA is found to be well correlated with the variations in surface BC mass concentrations and/or the relative dominance of the fine/coarse mode aerosol. The results are discussed in light of the aerosol physical and optical properties and the asymmetry parameter.


2016 ◽  
Vol 16 (11) ◽  
pp. 7251-7283 ◽  
Author(s):  
Ann M. Fridlind ◽  
Rachel Atlas ◽  
Bastiaan van Diedenhoven ◽  
Junshik Um ◽  
Greg M. McFarquhar ◽  
...  

Abstract. Single-crystal images collected in mid-latitude cirrus are analyzed to provide internally consistent ice physical and optical properties for a size-resolved cloud microphysics model, including single-particle mass, projected area, fall speed, capacitance, single-scattering albedo, and asymmetry parameter. Using measurements gathered during two flights through a widespread synoptic cirrus shield, bullet rosettes are found to be the dominant identifiable habit among ice crystals with maximum dimension (Dmax) greater than 100 µm. Properties are therefore first derived for bullet rosettes based on measurements of arm lengths and widths, then for aggregates of bullet rosettes and for unclassified (irregular) crystals. Derived bullet rosette masses are substantially greater than reported in existing literature, whereas measured projected areas are similar or lesser, resulting in factors of 1.5–2 greater fall speeds, and, in the limit of large Dmax, near-infrared single-scattering albedo and asymmetry parameter (g) greater by  ∼  0.2 and 0.05, respectively. A model that includes commonly imaged side plane growth on bullet rosettes exhibits relatively little difference in microphysical and optical properties aside from  ∼ 0.05 increase in mid-visible g primarily attributable to plate aspect ratio. In parcel simulations, ice size distribution, and g are sensitive to assumed ice properties.


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