scholarly journals Polycyclic Aromatic Hydrocarbons (PAHs) In The Upstream Rivers of Taihu Lake Basin, China: Spatial Distribution, Sources And Environmental Risk

2021 ◽  
Author(s):  
Lingling Wang ◽  
Xiaoming Ren ◽  
Xiaoping Wang ◽  
Perran Ye ◽  
Fei Wang ◽  
...  
Keyword(s):  
Molecular Weight ◽  
Spatial Distribution ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Cancer Risk ◽  
Ecological Risk ◽  
Aromatic Hydrocarbons ◽  
Taihu Lake ◽  
Lake Basin ◽  
Taihu Lake Basin ◽  
Polycyclic Aromatic

Abstract The polycyclic aromatic hydrocarbons (PAHs) pollution in Taihu Lake Basin has caused widespread concern. However, the spatial temporal distribution of PAHs in the upstream rivers of Taihu Lake Basin remains largely unknown. Thus, this study aims to investigate the level, spatial distribution, sources and environment risk caused by PAHs in upstream rivers of Taihu Lake Basin. The concentrations of total 16 PAHs (∑16PAHs) ranged from 188.64 to 1060.39 ng/g, with an average of 472.62 ng/g. Compared with low-molecular-weight (LMW) PAHs, high-molecular-weight (HMW) PAHs were more resistant to degradation and easier to accumulate in the sediment. The results of source analysis demonstrated that the PAH pollution was mainly sourced from mixture of fuel combustion and direct petroleum spillage. The ecological risk assessment showed that moderate ecological risk caused by the PAH contaminants might occur in most sample sites. The incremental lifetime cancer risk (ILCRs) ranged from 2.07 ×10-4 - 2.66 × 10-3 for children and 9.66 ×10-5 - 1.24 × 10-3 for adult, indicating moderate cancer risk of PAH-contaminated sediments.

scholarly journals Spatial Occurrence and Sources of Polycyclic Aromatic Hydrocarbons in Sediments Drive the Ecological Risk of Taihu Lake, China

2021 ◽  
Author(s):  
Xiulu Lang ◽  
Xinghua He ◽  
Yanhua Wang ◽  
Xi Chen ◽  
Mingli Zhang ◽  
...  
Keyword(s):  
Molecular Weight ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Ecological Risk ◽  
Aromatic Hydrocarbons ◽  
Surface Sediments ◽  
Taihu Lake ◽  
Central Area ◽  
Toxicity Assessment ◽  
Ecological Risks ◽  
Polycyclic Aromatic

Abstract To study the spatial occurrence, sources, and ecological risks of 16 PAHs, surface sediments had been collected from seven major areas of Taihu Lake, China in April 2021. Results showed that the concentrations of ∑16PAHs varied between 1381.48~4682.16 ng g-1, and the contents of BghiP in each sample were the highest. The PAHs concentrations in the sediments near the lakeshore were much higher than those in the central area of the lake. The sedimentary ∑16PAHs were mainly composed of molecular-weight monomers and 4-ring PAHs showed superiority (35.69%~45.02%). According to the ratio of PAH monomer, the sedimentary PAHs in Taihu Lake were dominantly derived from the combustion. Through the biological toxicity assessment and the BaP equivalent (BaPE), great biological risks of PAHs monomers i.e. DahA and IcdP were found. Both concentrations of ∑16PAHs and dominant 4~6-ring monomers accompanied by carcinogenic risks in many areas of Taihu Lake increased. It is necessary to strengthen monitoring and take measures to control the input of organic pollutants.

scholarly journals Distribusi Spasial, Sumber Pencemaran, dan Kajian Risiko Ekologi Polisiklik Aromatik Hidrokarbon (PAH) dalam Sedimen Pesisir di Pulau Bintan, Indonesia

2019 ◽  
Vol 20 (2) ◽  
pp. 271
Author(s):  
Deny Yogaswara ◽  
Ita Wulandari ◽  
Khozanah Khozanah ◽  
Edward Edward ◽  
Dede Falahudin
Keyword(s):  
Spatial Distribution ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Ecological Risk ◽  
Aromatic Hydrocarbons ◽  
Surface Sediments ◽  
Biological Effects ◽  
Sediment Quality ◽  
Diagnostic Methods ◽  
Small Island ◽  
Polycyclic Aromatic

ABSTRACTBintan Island is the small island in the Riau Archipelago which borders Singapore and Malaysia. Its water is crossed by international shipping lines. Therefore, water quality in this area is potentially polluted by marine activities. The present study aimed to evaluate the concentration, spatial distribution, and assessment of ecological risks of polycyclic aromatic hydrocarbons (PAHs) in surface sediments from selected coastal water of Bintan. Surface sediments in this study were extracted by using the ultrasonic system and determined with GCMS. The data were visualized with ArGIS software for spatial distribution mapping, applied ratio diagnostic methods for the source of PAH contamination, and assess their ecological risk based on sediment quality guidelines. The results showed PAHs concentrations ranged from below the method detection limit (<DL) to 13.492 ng.g−1(dry weight) with the highest concentration of PAHs were detected at TJU 1 station as much as 13.492 ng.g-1. As many as seven types of PAHs were identified in Bintan water, they were Naphthalene (two rings), Fluorene and Anthracene (three rings); fluoranthene, Pyrene, Benzo (a) Pyrene and Chrysene (five rings). Based on diagnostic ratios, the sources of PAHs in this coastal area were mainly from pyrogenic origins. Ecological risk assessment has shown that the average value of ∑10 PAH in Bintan waters (5.855 ng.g-1) is lower than the corresponding ERL, ERM, TEL, and PEL value indicating that the adverse biological effects of PAHs are generally low.Keywords: Polycyclic Aromatic Hydrocarbons (PAHs), Distribution, Pollution, Bintan WatersABSTRAKPulau Bintan merupakan pulau kecil di Kepulauan Riau yang berbatasan langsung dengan negara Singapura dan Malaysia serta perairannya dilintasi oleh jalur pelayaran internasional sehingga potensi pencemaran dari aktivitas di laut sangat tinggi. Penelitian ini bertujuan untuk mengukur konsentrasi, distribusi spasial, sumber asal pencemaran dan analisis resiko lingkungan senyawa PAH dalam sedimen permukaan di perairan pesisir Pulau Bintan. Sedimen permukaan diekstraksi dengan sistem ultrasonik dan dianalisa akhir dengan GCMS. Data senyawa PAH diolah dengan software ArGIS untuk membuat peta distribusi spasial, dianalisa dengan metode diagnosa rasio untuk mengetahui sumber pencemarnya dan dibandingkan dengan nilai baku mutu sedimen untuk mengkaji resiko ekologinya. Hasil analisis di setiap stasiun sampling di Muara Pengudang dan Tanjung Uban menunjukkan konsentrasi Total PAH (TPAH) berkisar antara < limit deteksi alat (1 ngg-1) sampai 13,492 ng.g-1 berat kering dengan konsentrasi tertinggi terdeteksi di stasiun TJU 1 yaitu sebesar 13,492 ng.g-1.  Sebanyak tujuh jenis senyawa PAH teridentifikasi di perairan Bintan ini diantaranya Naphthalene, (dua cincin benzene), Fluorene dan Anthracene (tiga cincin benzene); Fluoranthene, Pyrene, Benzo (a) Pyrene, dan Chrysene (empat cincin benzene). Berdasarkan analisa diagnosa rasio, sumber pencemaran PAH di perairan pesisir Bintan adalah berasal dari kombinasi antara sumber pirogenik. Analisis resiko lingkungan menunjukkan nilai rata-rata ∑10 PAH di perairan Bintan (5,855 ngg-1) masih rendah dibandingkan nilai ERL, ERM, TEL dan PEL, hal tersebut mengindikasikan bahwa efek biologis senyawa PAH secara umum rendah.Kata kunci: Polisiklik Aromatik Hidrokarbon (PAH), Sebaran, Pencemaran, Perairan Bintan

scholarly journals Polycyclic Aromatic Hydrocarbons in Sediments from Typical Algae, Macrophyte Lake Bay and Adjoining River of Taihu Lake, China: Distribution, Sources, and Risk Assessment

Water ◽  
2021 ◽  
Vol 13 (4) ◽  
pp. 470
Author(s):  
Yibo Dong ◽  
Zaisheng Yan ◽  
Huifang Wu ◽  
Guoqing Zhang ◽  
Haichen Zhang ◽  
...  
Keyword(s):  
Risk Assessment ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Ecological Risk ◽  
Aromatic Hydrocarbons ◽  
Taihu Lake ◽  
Cyanobacterial Bloom ◽  
Freshwater Ecosystems ◽  
Petroleum Contamination ◽  
Riverine Sediments ◽  
Polycyclic Aromatic

Polycyclic aromatic hydrocarbons (PAHs) are ubiquitous environmental pollutants in sediments and pose a serious risk for freshwater ecosystems. In this study, sediment samples from 24 sites were collected from the cyanobacterial bloom-occurring, macrophyte-growing lake bay and adjoining river of Taihu Lake. Here, the concentration levels, sources, and risk assessment of 16 priority PAHs in the surface sediments from typical algae, macrophyte lake bay and adjoining river of Taihu Lake, were investigated, and the results were compared with those of previous studies. The total PAH (ΣPAH) concentrations ranged from 4900 to 16,800 ng·g−1 in sediments of the Taihu Lake bay and from 5736.2 to 69,362.8 ng·g−1 in sediments of the adjoining river. The level of PAHs in riverine sediments was significantly higher than those of the Taihu Lake bay, and that of the Dongshan River was significantly higher than that of the Mashan River, while there was no significant difference in the concentrations of PAHs between the cyanobacterial bloom-occurring and macrophyte-growing lake zone. The results indicated petroleum contamination was dominated in the cyanobacterial bloom-occurring, macrophyte-growing lake bay, while PAHs of the riverine sediments derived from petroleum contamination and the combined combustion including wood, coal combustion, and petroleum combustion according to the identification by the molecular diagnostic ratio and principal component analysis (PCA). Sediment risk assessment based on sediment quality guidelines (SQGs) suggested that partial regions of the Taihu Lake bay were subjected to the potential ecological risk of the 3-ring and 5-ring PAHs, and there existed negative effects related to naphthalene pollutant in all survey regions. The adjoining riverine sediments showed a high ecological risk.

scholarly journals Ecological risk assessment of the levels of polycyclic aromatic hydrocarbons in soils of the abandoned sections of Orji Mechanic Village, Owerri, Imo State, Nigeria

2021 ◽  
Vol 45 (1) ◽  
Author(s):  
Francis Chizoruo Ibe ◽  
Chidi Edbert Duru ◽  
Benaiah Obinna Isiuku ◽  
Jacienta Ngozi Akalazu
Keyword(s):  
Risk Assessment ◽  
Molecular Weight ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Ecological Risk ◽  
Ecological Risk Assessment ◽  
Aromatic Hydrocarbons ◽  
Soil Samples ◽  
Imo State ◽  
Polycyclic Aromatic ◽  
Hydrocarbons In Soils

Abstract Background Ecological risk assessment of the levels of polycyclic aromatic hydrocarbons in soils of the abandoned sections of Orji Mechanic Village, Owerri, Imo State, Nigeria. The main objective of the study was to determine the levels of soil contamination from polycyclic aromatic compounds (PAHs) due to anthropogenic events in the mechanic village before reclamation. Results Analysis of soil samples revealed mean PAH levels ranging from 1.22E−02 ± 0.00 to 5.60E−02 ± 0.01 mg/kg, with higher PAH concentrations observed at 0–10 cm compared to other depths. The sum of PAHs (∑PAHs) ranged from 1.58E−01 to 6.71E−01 mg/kg, as the sum of low molecular weight PAHs (∑LPAHs) varied from 7.16E−03 to 1–1.60E−01 mg/kg, while the sum of high molecular weight PAHs (∑HPAHs) ranged from 1.81E−02 to 5.42E−01 mg/kg. The sum of carcinogenic PAHs (∑Carcino-PAHs) varied from 5.39E−01 to 9.74E−02 mg/kg, indicating elevated levels of carcinogens in the sampled soils. Diagnostic ratio, principal component, and correlation analysis of the results revealed that pyrogenic sources were primarily responsible for the observed PAHs owing to the activities of automobile mechanics in the Orji Mechanic Village. Benzo(a)pyrene equivalent (BePeq) of the PAHs indicated high carcinogenic potency for sample A. The total cancer risk was above 1 × 10–6, indicating a greater risk of cancer due to contact with the contaminated soil samples; hence, the result of this study is a serious ecological concern. Conclusion There may be accumulation of these contaminants in the investigated area, which will eventually contaminate the groundwater as well as surface water resources. Remedial measures to prevent possible health problems due to the PAHs which results from the activities of automobile mechanics are therefore recommended.

scholarly journals Dynamics and Mass Balance of Polycyclic Aromatic Hydrocarbons in and around the Seto Inland Sea, Japan

2021 ◽  
Author(s):  
Hiroaki Tsuji ◽  
Yuta Akiyoshi ◽  
Daichi Asakawa ◽  
Shinya Nakashita ◽  
Yoko Iwamoto ◽  
...  
Keyword(s):  
Molecular Weight ◽  
Polycyclic Aromatic Hydrocarbons ◽  
Mass Balance ◽  
Ecological Risk ◽  
Aromatic Hydrocarbons ◽  
Benthic Communities ◽  
The Yellow Sea ◽  
Seto Inland Sea ◽  
The Seto Inland Sea ◽  
Polycyclic Aromatic

Abstract Polycyclic aromatic hydrocarbons (PAHs) were analyzed to elucidate the distribution, ecological risk, pathways, and fluxes of these pollutants in and around the Seto Inland Sea, Japan. High molecular weight PAHs (5–6 rings) were primarily found in regions close to the bay estuaries, and their proportions decreased at distances further from the estuaries (offshore areas), where low molecular weight PAHs (2–4 rings) were more ubiquitous. Ecological risk assessments revealed that the PAHs found in the sediments should have no adverse effects on benthic communities, with the exception of fluorene, which was detected in high levels in the sediment from Beppu Bay. A mass balance for PAHs in the Seto Inland Sea, calculated based on data collected in the field and published literature findings, showed the PAH flux into the Seto Inland Sea from atmospheric deposition were ca. 5 times higher than that from riverine inflows. Comparison of the amount of the PAH flux between the Seto Inland Sea and other seas suggested that the Seto Inland Sea is less polluted than the Gulf of Lion and the Bohai Sea, and more polluted than the Yellow Sea.

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