scholarly journals Influence of the trajectory of air masses on the in situ measurements of aerosol properties in Valencia

2012 ◽  
Author(s):  
Esteve
Keyword(s):  
In Situ Measurements ◽  
Air Masses ◽  
Aerosol Properties

scholarly journals Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements

2021 ◽  
Vol 21 (19) ◽  
pp. 15023-15063
Author(s):  
Charles A. Brock ◽  
Karl D. Froyd ◽  
Maximilian Dollner ◽  
Christina J. Williamson ◽  
Gregory Schill ◽  
...  
Keyword(s):  
Optical Properties ◽  
Global Scale ◽  
In Situ Measurements ◽  
Sea Salt ◽  
Size Distributions ◽  
Global Models ◽  
Air Masses ◽  
Aerosol Types ◽  
Aerosol Properties

Abstract. In situ measurements of aerosol microphysical, chemical, and optical properties were made during global-scale flights from 2016–2018 as part of the Atmospheric Tomography Mission (ATom). The NASA DC-8 aircraft flew from ∼ 84∘ N to ∼ 86∘ S latitude over the Pacific, Atlantic, Arctic, and Southern oceans while profiling nearly continuously between altitudes of ∼ 160 m and ∼ 12 km. These global circuits were made once each season. Particle size distributions measured in the aircraft cabin at dry conditions and with an underwing probe at ambient conditions were combined with bulk and single-particle composition observations and measurements of water vapor, pressure, and temperature to estimate aerosol hygroscopicity and hygroscopic growth factors and calculate size distributions at ambient relative humidity. These reconstructed, composition-resolved ambient size distributions were used to estimate intensive and extensive aerosol properties, including single-scatter albedo, the asymmetry parameter, extinction, absorption, Ångström exponents, and aerosol optical depth (AOD) at several wavelengths, as well as cloud condensation nuclei (CCN) concentrations at fixed supersaturations and lognormal fits to four modes. Dry extinction and absorption were compared with direct in situ measurements, and AOD derived from the extinction profiles was compared with remotely sensed AOD measurements from the ground-based Aerosol Robotic Network (AERONET); this comparison showed no substantial bias. The purpose of this work is to describe the methodology by which ambient aerosol properties are estimated from the in situ measurements, provide statistical descriptions of the aerosol characteristics of different remote air mass types, examine the contributions to AOD from different aerosol types in different air masses, and provide an entry point to the ATom aerosol database. The contributions of different aerosol types (dust, sea salt, biomass burning, etc.) to AOD generally align with expectations based on location of the profiles relative to continental sources of aerosols, with sea salt and aerosol water dominating the column extinction in most remote environments and dust and biomass burning (BB) particles contributing substantially to AOD, especially downwind of the African continent. Contributions of dust and BB aerosols to AOD were also significant in the free troposphere over the North Pacific. Comparisons of lognormally fitted size distribution parameters to values in the Optical Properties of Aerosols and Clouds (OPAC) database commonly used in global models show significant differences in the mean diameters and standard deviations for accumulation-mode particles and coarse-mode dust. In contrast, comparisons of lognormal parameters derived from the ATom data with previously published shipborne measurements in the remote marine boundary layer show general agreement. The dataset resulting from this work can be used to improve global-scale representation of climate-relevant aerosol properties in remote air masses through comparison with output from global models and assumptions used in retrievals of aerosol properties from both ground-based and satellite remote sensing.

scholarly journals Ambient aerosol properties in the remote atmosphere from global-scale in-situ measurements

2021 ◽  
Author(s):  
Charles A. Brock ◽  
Karl D. Froyd ◽  
Maximilian Dollner ◽  
Christina J. Williamson ◽  
Gregory Schill ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Global Scale ◽  
In Situ Measurements ◽  
Sea Salt ◽  
Size Distributions ◽  
Global Models ◽  
Air Masses ◽  
Aerosol Types ◽  
Aerosol Properties

Abstract. In situ measurements of aerosol microphysical, chemical, and optical properties were made during global-scale flights from 2016–2018 as part of the Atmospheric Tomography Mission (ATom). A NASA DC-8 aircraft flew from ~84 °N to ~86 °S latitude over the Pacific, Atlantic, Arctic, and Southern oceans while profiling nearly continuously between altitudes of ~160 m and ~12 km. These global circuits were made once each season. Particle size distributions measured in the aircraft cabin at dry conditions and with an underwing probe at ambient conditions were combined with bulk and single-particle composition observations and measurements of water vapor, pressure and temperature to estimate aerosol hygroscopicity and hygroscopic growth factors and calculate size distributions at ambient relative humidity. These reconstructed, composition-resolved ambient size distributions were used to estimate intensive and extensive aerosol properties, including single scatter albedo, asymmetry parameter, extinction, absorption, Ångström exponents, and aerosol optical depth (AOD) at several wavelengths, as well as CCN concentrations at fixed supersaturations and lognormal fits to four modes. Dry extinction and absorption were compared with direct, in situ measurements, and AOD derived from the extinction profiles was compared with remotely sensed AOD measurements from the ground-based Aerosol Robotic Network (AERONET); these calculated parameters were in agreement with the direct observations within expected uncertainties. The purpose of this work is to describe the methodology by which ambient aerosol properties are estimated from the in situ measurements, provide statistical descriptions of the aerosol characteristics of different remote air mass types, examine the contributions to AOD from different aerosol types in different air masses, and provide an entry point to the ATom aerosol database. The contributions of different aerosol types (dust, sea salt, biomass burning, etc.) to AOD generally align with expectations based on location of the profiles relative to continental sources of aerosols, with sea salt and aerosol water dominating the column extinction in most remote environments and dust and biomass burning (BB) particles contributing substantially to AOD, especially downwind of the African continent. Contributions of dust and BB aerosols to AOD were also significant in the free troposphere over the North Pacific. Comparisons of lognormally fitted size distribution parameters to values in a database commonly used in global models show significant differences in the mean diameters and standard deviations for accumulation-mode particles and coarse-mode dust. In contrast, comparisons of lognormal parameters derived from the ATom data with previously published ship-borne measurements in the remote marine boundary layer show general agreement. The dataset resulting from this work can be used to improve global-scale representation of climate-relevant aerosol properties in remote air masses through comparison with output from global models and with assumptions used in retrievals of aerosol properties from both ground-based and satellite remote sensing.

scholarly journals Synergetic monitoring of Saharan dust plumes and potential impact on surface: a case study of dust transport from Canary Islands to Iberian Peninsula

2011 ◽  
Vol 11 (7) ◽  
pp. 3067-3091 ◽  
Author(s):  
C. Córdoba-Jabonero ◽  
M. Sorribas ◽  
J. L. Guerrero-Rascado ◽  
J. A. Adame ◽  
Y. Hernández ◽  
...  
Keyword(s):  
Iberian Peninsula ◽  
Particle Deposition ◽  
Ground Level ◽  
In Situ Measurements ◽  
Saharan Dust ◽  
Dust Transport ◽  
Air Masses ◽  
Potential Impact

Abstract. The synergetic use of meteorological information, remote sensing both ground-based active (lidar) and passive (sun-photometry) techniques together with backtrajectory analysis and in-situ measurements is devoted to the characterization of dust intrusions. A case study of air masses advected from the Saharan region to the Canary Islands and the Iberian Peninsula, located relatively close and far away from the dust sources, respectively, was considered for this purpose. The observations were performed over three Spanish geographically strategic stations within the dust-influenced area along a common dust plume pathway monitored from 11 to 19 of March 2008. A 4-day long dust event (13–16 March) over the Santa Cruz de Tenerife Observatory (SCO), and a linked short 1-day dust episode (14 March) in the Southern Iberian Peninsula over the Atmospheric Sounding Station "El Arenosillo" (ARN) and the Granada station (GRA) were detected. Meteorological conditions favoured the dust plume transport over the area under study. Backtrajectory analysis clearly revealed the Saharan region as the source of the dust intrusion. Under the Saharan air masses influence, AERONET Aerosol Optical Depth at 500 nm (AOD500) ranged from 0.3 to 0.6 and Ångström Exponent at 440/675 nm wavelength pair (AE440/675) was lower than 0.5, indicating a high loading and predominance of coarse particles during those dusty events. Lidar observations characterized their vertical layering structure, identifying different aerosol contributions depending on altitude. In particular, the 3-km height dust layer transported from the Saharan region and observed over SCO site was later on detected at ARN and GRA stations. No significant differences were found in the lidar (extinction-to-backscatter) ratio (LR) estimation for that dust plume over all stations when a suitable aerosol scenario for lidar data retrieval is selected. Lidar-retrieved LR values of 60–70 sr were obtained during the main dust episodes. These similar LR values found in all the stations suggest that dust properties were kept nearly unchanged in the course of its medium-range transport. In addition, the potential impact on surface of that Saharan dust intrusion over the Iberian Peninsula was evaluated by means of ground-level in-situ measurements for particle deposition assessment together with backtrajectory analysis. However, no connection between those dust plumes and the particle sedimentation registered at ground level is found. Differences on particle deposition processes observed in both Southern Iberian Peninsula sites are due to the particular dust transport pattern occurred over each station. Discrepancies between columnar-integrated and ground-level in-situ measurements show a clear dependence on height of the dust particle size distribution. Then, further vertical size-resolved observations are needed for evaluation of the impact on surface of the Saharan dust arrival to the Iberian Peninsula.

scholarly journals Different strategies to retrieve aerosol properties at night-time with the GRASP algorithm

2019 ◽  
Vol 19 (22) ◽  
pp. 14149-14171 ◽  
Author(s):  
Jose Antonio Benavent-Oltra ◽  
Roberto Román ◽  
Juan Andrés Casquero-Vera ◽  
Daniel Pérez-Ramírez ◽  
Hassan Lyamani ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Sierra Nevada ◽  
Volume Concentration ◽  
In Situ Measurements ◽  
Saharan Dust ◽  
Scattering Coefficient ◽  
Night Time ◽  
Aerosol Properties

Abstract. This study evaluates the potential of the GRASP algorithm (Generalized Retrieval of Aerosol and Surface Properties) to retrieve continuous day-to-night aerosol properties, both column-integrated and vertically resolved. The study is focused on the evaluation of GRASP retrievals during an intense Saharan dust event that occurred during the Sierra Nevada Lidar aerOsol Profiling Experiment I (SLOPE I) field campaign. For daytime aerosol retrievals, we combined the measurements of the ground-based lidar from EARLINET (European Aerosol Research Lidar Network) station and sun–sky photometer from AERONET (Aerosol Robotic Network), both instruments co-located in Granada (Spain). However, for night-time retrievals three different combinations of active and passive remote-sensing measurements are proposed. The first scheme (N0) uses lidar night-time measurements in combination with the interpolation of sun–sky daytime measurements. The other two schemes combine lidar night-time measurements with night-time aerosol optical depth obtained by lunar photometry either using intensive properties of the aerosol retrieved during sun–sky daytime measurements (N1) or using the Moon aureole radiance obtained by sky camera images (N2). Evaluations of the columnar aerosol properties retrieved by GRASP are done versus standard AERONET retrievals. The coherence of day-to-night evolutions of the different aerosol properties retrieved by GRASP is also studied. The extinction coefficient vertical profiles retrieved by GRASP are compared with the profiles calculated by the Raman technique at night-time with differences below 30 % for all schemes at 355, 532 and 1064 nm. Finally, the volume concentration and scattering coefficient retrieved by GRASP at 2500 m a.s.l. are evaluated by in situ measurements at this height at Sierra Nevada Station. The differences between GRASP and in situ measurements are similar for the different schemes, with differences below 30 % for both volume concentration and scattering coefficient. In general, for the scattering coefficient, the GRASP N0 and N1 show better results than the GRASP N2 schemes, while for volume concentration, GRASP N2 shows the lowest differences against in situ measurements (around 10 %) for high aerosol optical depth values.

Study of the vertical variability of aerosol properties based on cable cars in-situ measurements

2017 ◽  
Vol 8 (5) ◽  
pp. 968-978 ◽  
Author(s):  
O. Zawadzka ◽  
M. Posyniak ◽  
K. Nelken ◽  
P. Markuszewski ◽  
M.T. Chilinski ◽  
...  
Keyword(s):  
In Situ Measurements ◽  
Aerosol Properties ◽  
Vertical Variability

scholarly journals CCN concentration and INP-relevant aerosol profiles in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements

2019 ◽  
Author(s):  
Moritz Haarig ◽  
Adrian Walser ◽  
Albert Ansmann ◽  
Maximilian Dollner ◽  
Dietrich Althausen ◽  
...  
Keyword(s):  
Surface Area ◽  
Cloud Condensation Nuclei ◽  
Number Concentration ◽  
In Situ Measurements ◽  
Saharan Air Layer ◽  
Lidar Measurements ◽  
Research Aircraft ◽  
Lidar Observations ◽  
Aerosol Properties

Abstract. The present study aims to validate lidar retrievals of cloud-relevant aerosol properties by using polarization lidar and coincident airborne in situ measurements in the Saharan Air Layer over the Barbados region. Vertical profiles of the number concentration of cloud condensation nuclei (CCN), large particles (diameter d > 500 nm), surface area, and ice nucleating particles (INP) are estimated from the lidar measurements and compared with CCN concentrations and the INP-relevant aerosol properties in situ measured with aircraft in the framework of the Saharan Aerosol Long-range Transport and Aerosol–Cloudinteraction Experiment (SALTRACE) in summer 2013. The CCN number concentrations derived from lidar observations were up to a factor of two higher than the ones measured in situ on board the research aircraft Falcon. However, a reasonable agreement was obtained when taking the lidar uncertainty into account. The number concentration of particles with dry radius > 250 nm and the surface area concentration obtained from the lidar observations and used as input for the INP parameterizations agreed well (

scholarly journals Overview of the SLOPE I and II campaigns: aerosol properties retrieved with lidar and sun–sky photometer measurements

2021 ◽  
Vol 21 (12) ◽  
pp. 9269-9287
Author(s):  
Jose Antonio Benavent-Oltra ◽  
Juan Andrés Casquero-Vera ◽  
Roberto Román ◽  
Hassan Lyamani ◽  
Daniel Pérez-Ramírez ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Absorption Coefficient ◽  
Sierra Nevada ◽  
Volume Concentration ◽  
In Situ Measurements ◽  
Absorption Coefficients ◽  
Desert Dust ◽  
Particle Sizer ◽  
Aerosol Properties

Abstract. The Sierra Nevada Lidar aerOsol Profiling Experiment I and II (SLOPE I and II) campaigns were intended to determine the vertical structure of aerosols by remote sensing instruments and test the various retrieval schemes for obtaining aerosol microphysical and optical properties with in situ measurements. The SLOPE I and II campaigns were developed during the summers of 2016 and 2017, respectively, combining active and passive remote sensing with in situ measurements at stations belonging to the AGORA observatory (Andalusian Global ObseRvatory of the Atmosphere) in the Granada area (Spain). In this work, we use the in situ measurements of these campaigns to evaluate aerosol properties retrieved by the GRASP code (Generalized Retrieval of Atmosphere and Surface Properties) combining lidar and sun–sky photometer measurements. We show an overview of aerosol properties retrieved by GRASP during the SLOPE I and II campaigns. In addition, we evaluate the GRASP retrievals of total aerosol volume concentration (discerning between fine and coarse modes), extinction and scattering coefficients, and for the first time we present an evaluation of the absorption coefficient. The statistical analysis of aerosol optical and microphysical properties, both column-integrated and vertically resolved, from May to July 2016 and 2017 shows a large variability in aerosol load and types. The results show a strong predominance of desert dust particles due to North African intrusions. The vertically resolved analysis denotes a decay of the atmospheric aerosols with an altitude up to 5 km a.s.l. Finally, desert dust and biomass burning events were chosen to show the high potential of GRASP to retrieve vertical profiles of aerosol properties (e.g. absorption coefficient and single scattering albedo) for different aerosol types. The aerosol properties retrieved by GRASP show good agreement with simultaneous in situ measurements (nephelometer, aethalometer, scanning mobility particle sizer, and aerodynamic particle sizer) performed at the Sierra Nevada Station (SNS) in Granada. In general, GRASP overestimates the in situ data at the SNS with a mean difference lower than 6 µm3 cm−3 for volume concentration, and 11 and 2 Mm−1 for the scattering and absorption coefficients. On the other hand, the comparison of GRASP with airborne measurements also shows an overestimation with mean absolute differences of 14 ± 10 and 1.2 ± 1.2 Mm−1 for the scattering and absorption coefficients, showing a better agreement for the absorption (scattering) coefficient with higher (lower) aerosol optical depth. The potential of GRASP shown in this study will contribute to enhancing the representativeness of the aerosol vertical distribution and provide information for satellite and global model evaluation.

scholarly journals Detecting moisture transport pathways to the subtropical North Atlantic free troposphere using paired H<sub>2</sub>O-<i>δ</i>D in situ measurements

2016 ◽  
Vol 16 (7) ◽  
pp. 4251-4269 ◽  
Author(s):  
Yenny González ◽  
Matthias Schneider ◽  
Christoph Dyroff ◽  
Sergio Rodríguez ◽  
Emanuel Christner ◽  
...  
Keyword(s):  
North Atlantic ◽  
In Situ Measurements ◽  
Back Trajectory ◽  
Free Troposphere ◽  
Night Time ◽  
Humid Air ◽  
Transport Pathways ◽  
Air Masses ◽  
Dry Convection

Abstract. We present two years of in situ measurements of water vapour (H2O) and its isotopologue ratio (δD, the standardized ratio between H216O and HD16O), made at two remote mountain sites on Tenerife in the subtropical North Atlantic. We show that the data – if measured during night-time – are well representative for the lower/middle free troposphere. We use the measured H2O-δD pairs, together with dust measurements and back trajectory modelling for analysing the moisture pathways to this region. We can identify four principally different transport pathways. The air mass transport from high altitudes and high latitudes shows two different scenarios. The first scenario brings dry air masses to the stations, as the result of condensation events occurring at low temperatures. The second scenario brings humid air masses to the stations, due to cross-isentropic mixing with lower-level and more humid air during transport since last condensation (LC). The third pathway is transportation from lower latitudes and lower altitudes, whereby we can identify rain re-evaporation as an occasional source of moisture. The fourth pathway is linked to the African continent, where during summer, dry convection processes over the Sahara very effectively inject humidity from the boundary layer to higher altitudes. This so-called Saharan Air Layer (SAL) is then advected westward over the Atlantic and contributes to moisten the free troposphere. We demonstrate that the different pathways leave distinct fingerprints on the measured H2O-δD pairs.

scholarly journals Supplementary material to "Ambient aerosol properties in the remote atmosphere from global-scale in-situ measurements"

2021 ◽  
Author(s):  
Charles A. Brock ◽  
Karl D. Froyd ◽  
Maximilian Dollner ◽  
Christina J. Williamson ◽  
Gregory Schill ◽  
...  
Keyword(s):  
Global Scale ◽  
In Situ Measurements ◽  
Ambient Aerosol ◽  
Supplementary Material ◽  
Aerosol Properties
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