Carbon Dioxide Conversion to Synthesis Gas when Combined with Methane using a New Designed of Non-thermal Plasma Reactor

2014 ◽  
Vol 7 (4) ◽  
pp. 226-235 ◽  
Author(s):  
Widiatmini Sih Winant ◽  
Setijo Bismo ◽  
Widodo Wahyu Purwanto
Author(s):  
Onur Taylan ◽  
Halil Berberoglu

This paper reports a numerical study on the discharge of carbon dioxide using a non-thermal dielectric barrier discharge (DBD) plasma reactor at ambient conditions. DBD plasma reactors have been used for various applications due to their ease of production, process control, operation at different conditions. The applications of DBD plasma reactors include discharge of gases. Carbon dioxide is a greenhouse gas formed as a byproduct of fossil fuel combustion. Use of DBD non-thermal plasma reactor can be a promising technology for carbon dioxide mitigation due to its operation at low temperatures, lack of need for catalysts, and flexibility in controlling the products generated. In this study, a tubular DBD non-thermal plasma reactor was modeled with different electrode materials separated by different dielectric materials. The aim was to provide guidelines for the design and material selection for optimizing DBD plasma reactors for CO2 discharge. A parametric set of simulations was performed using a finite element solver to investigate how electrode and dielectric materials affect the discharge volume of CO2 and power requirement of the non-thermal plasma discharge of CO2. The results showed that electrode material did not affect the discharge or the power requirement. However, dielectric material with higher permittivity or lower conductivity increased the gas discharge and power requirement. Among the analyzed materials, aluminum electrode and mica tube were suggested based on the simulation results for the maximum gas discharge and low power requirement.


2014 ◽  
Vol 5 (1) ◽  
pp. 51 ◽  
Author(s):  
Widiatmini Sih Winanti ◽  
Widodo Wahyu Purwanto ◽  
Setijo Bismo

2019 ◽  
Vol 52 (25) ◽  
pp. 255201 ◽  
Author(s):  
T Xia ◽  
A Kleinheksel ◽  
E M Lee ◽  
Z Qiao ◽  
K R Wigginton ◽  
...  

Author(s):  
Daniel-Eusebiu Cretu ◽  
Radu Burlica ◽  
Oana Beniuga ◽  
Dragos Astanei ◽  
Catalin Rusu ◽  
...  

2021 ◽  
Vol 25 (12) ◽  
pp. 30-37
Author(s):  
L.G. Pinaeva ◽  
A.S. Noskov

Existing (production of urea, dimethyl carbonate, polypropylene carbonate) and promising (production of methanol, synthesis gas, monomers dedicated to synthesis of polyurethanes and polycarbonate) chemical technologies which any, time soon, may become CO2 based economy for producing motor fuels and basic chemicals have been overviewed. Based on estimates of CO2 removals in these processes, it has been concluded that there is a potential for developing technologies to produce methanol from CO2 to a competitive cost of the target product. It is expected that interest in this process will decrease if stable carbon dioxide conversion catalysts for methane are introduced into the market.


2014 ◽  
Vol 68 (3) ◽  
Author(s):  
Siti Musliha Aishah Musa ◽  
RK Raja Ibrahim ◽  
Asrul Izam Azmi

This paper presents early work on Fiber Bragg grating (FBG) as temperature sensor to monitor temperature variation inside a packed-bed non-thermal plasma reactor. FBG made from germania-doped fiber with center Bragg wavelength of 1552.5 nm was embedded inside non-thermal plasma reactor with sphere shape dielectric bead (barium titanate) and used to probe the temperature variation inside the reactor. The experimental works have proven that FBG is a suitable sensor to monitor temperature variation inside of reactor via LabVIEW program. Besides that, Optical Spectrum Analyzer (OSA) recorded Bragg wavelength shift as voltage of power supply increases, which indicate the non-uniform temperature variation occurring inside the reactor. However, it does not affect the chemical reaction inside the reactor because the temperature condition is in steady state.


Author(s):  
A. M. Vandenbroucke ◽  
R. Morent ◽  
N. De Geyter ◽  
C. Leys

AbstractThe aim of this paper is to give a review of the research on the decomposition of trichloroethylene (TCE), a common industrial solvent, with combined use of non-thermal plasma and heterogeneous catalysis, i.e. plasma-catalysis. This air purification technique has been investigated over the last decade in an effort to overcome the disadvantages of non-thermal plasma treatment of waste air containing volatile organic compounds (VOCs). Some examples of different plasma technologies used for plasma-catalysis are given. These include the dielectric barrier discharge, the pulsed corona discharge and the atmospheric pressure glow discharge. In a plasma-catalytic hybrid system the catalyst can either be located in the discharge region or downstream of the plasma reactor. The mechanisms that drive both configurations are briefly discussed, followed by an extended literature overview of the removal of TCE with plasma-catalysis.


2021 ◽  
pp. 131-135
Author(s):  
P.P. Platonov ◽  
S.V. Dudin ◽  
V.A. Lisovskiy

Numerical simulation of a bulk-type plasma reactor for carbon dioxide conversion with distributed gas injection and pumping has been performed in hydrodynamic approximation by solution of Navier-Stokes equation using the mathematical package COMSOL. It is shown that the geometry of gas injection and pumping, which determines the trajectories of the particles and their residence time in reactor, can significantly affect the energy efficiency of the conversion. Different particles on their way from inlet to pumping hole move along different trajectories and spend different times inside the reactor. If the residence time of the gas in the reactor is less than optimal, the gas conversion will be incomplete. If this time is more than optimal, then an excessive amount of energy will be applied to the already converted gas. It is shown that the reactor height affects significantly the energy efficiency of plasma conversion of carbon dioxide.


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