scholarly journals A novel methodology for large-scale daily assessment of the direct radiative forcing of smoke aerosols

2015 ◽  
Vol 15 (10) ◽  
pp. 5471-5483 ◽  
Author(s):  
E. T. Sena ◽  
P. Artaxo

Abstract. A new methodology was developed for obtaining daily retrievals of the direct radiative forcing of aerosols (24h-DARF) at the top of the atmosphere (TOA) using satellite remote sensing. Simultaneous CERES (Clouds and Earth's Radiant Energy System) shortwave flux at the top of the atmosphere and MODIS (Moderate Resolution Spectroradiometer) aerosol optical depth (AOD) retrievals were used. To analyse the impact of forest smoke on the radiation balance, this methodology was applied over the Amazonia during the peak of the biomass burning season from 2000 to 2009. To assess the spatial distribution of the DARF, background smoke-free scenes were selected. The fluxes at the TOA under clean conditions (Fcl) were estimated as a function of the illumination geometry (θ0) for each 0.5° × 0.5° grid cell. The instantaneous DARF was obtained as the difference between the clean (Fcl (θ0)) and the polluted flux at the TOA measured by CERES in each cell (Fpol (θ0)). The radiative transfer code SBDART (Santa Barbara DISORT Radiative Transfer model) was used to expand instantaneous DARFs to 24 h averages. This new methodology was applied to assess the DARF both at high temporal resolution and over a large area in Amazonia. The spatial distribution shows that the mean 24h-DARF can be as high as −30 W m−2 over some regions. The temporal variability of the 24h-DARF along the biomass burning season was also studied and showed large intraseasonal and interannual variability. We showed that our methodology considerably reduces statistical sources of uncertainties in the estimate of the DARF, when compared to previous approaches. DARF assessments using the new methodology agree well with ground-based measurements and radiative transfer models. This demonstrates the robustness of the new proposed methodology for assessing the radiative forcing for biomass burning aerosols. To our knowledge, this is the first time that satellite remote sensing assessments of the DARF have been compared with ground-based DARF estimates.

2014 ◽  
Vol 14 (22) ◽  
pp. 31515-31550
Author(s):  
E. T. Sena ◽  
P. Artaxo

Abstract. A new methodology was developed for obtaining daily retrievals of the direct radiative forcing of aerosols (24h-DARF) at the top of the atmosphere (TOA) using satellite remote sensing. For that, simultaneous CERES (Clouds and Earth's Radiant Energy System) shortwave flux at the top of the atmosphere (TOA) and MODIS (Moderate Resolution Spectroradiometer) aerosol optical depth (AOD) retrievals were used. This methodology is applied over a large region of Brazilian Amazonia. We focused our studies on the peak of the biomass burning season (August to September) from 2000 to 2009 to analyse the impact of forest smoke on the radiation balance. To assess the spatial distribution of the DARF, background scenes without biomass burning impacts, were defined as scenes with MODIS AOD < 0.1. The fluxes at the TOA retrieved by CERES for those clean conditions (Fcl) were estimated as a function of the illumination geometry (θ0) for each 0.5° × 0.5° grid cell. The instantaneous DARF was obtained as the difference between clean Fcl (θ0) and the polluted mean flux at the TOA measured by CERES in each cell (Fpol (θ0)). The radiative transfer code SBDART (Santa Barbara DISORT Radiative Transfer model) was used to expand instantaneous DARFs to 24 h averages. With this methodology it is possible to assess the DARF both at large scale and at high temporal resolution. This new methodology also showed to be more robust, because it considerably reduces statistical sources of uncertainties in the estimates of the DARF, when compared to previous assessments of the DARF using satellite remote sensing. The spatial distribution of the 24h-DARF shows that, for some cases, the mean 24h-DARF presents local values as high as −30 W m−2. The temporal variability of the 24h-DARF along the biomass burning season was also studied and showed large intraseasonal and interannual variability. In an attempt to validate the radiative forcing obtained in this work using CERES and MODIS, those results were compared to coincident AERONET ground based estimates of the DARF. This analysis showed that CERES-MODIS and AERONET 24h-DARF are related as DARFCERES-MODIS24 h = (1.07 ± 0.04)DARFAERONET24 h −(0.0 ± 0.6). This is a significant result, considering that the 24h-DARF retrievals were obtained by applying completely different methodologies, and using different instruments. The instantaneous CERES-MODIS DARF was also compared with radiative transfer evaluations of the forcing. To validate the aerosol and surface models used in the simulations, downward shortwave fluxes at the surface evaluated using SBDART and measured by pyranometers were compared. The simulated and measured downward fluxes are related through FBOAPYRANOMETER = (1.00 ± 0.04)FBOASBDART −(20 ± 27), indicating that the models and parameters used in the simulations were consistent. The relationship between CERES-MODIS instantaneous DARF and calculated SBDART forcing was satisfactory, with DARFCERES-MODIS = (0.86 ± 0.06)DARFSBDART −(6 ± 2). Those analysis showed a good agreement between satellite remote sensing, ground-based and radiative transfer evaluated DARF, demonstrating the robustness of the new proposed methodology for calculated radiative forcing for biomass burning aerosols. To our knowledge, this was the first time satellite remote sensing assessments of the DARF were compared with ground based DARF estimates.


2018 ◽  
Vol 18 (12) ◽  
pp. 8829-8848 ◽  
Author(s):  
Justyna Lisok ◽  
Anna Rozwadowska ◽  
Jesper G. Pedersen ◽  
Krzysztof M. Markowicz ◽  
Christoph Ritter ◽  
...  

Abstract. The aim of the presented study was to investigate the impact on the radiation budget of a biomass-burning plume, transported from Alaska to the High Arctic region of Ny-Ålesund, Svalbard, in early July 2015. Since the mean aerosol optical depth increased by the factor of 10 above the average summer background values, this large aerosol load event is considered particularly exceptional in the last 25 years. In situ data with hygroscopic growth equations, as well as remote sensing measurements as inputs to radiative transfer models, were used, in order to estimate biases associated with (i) hygroscopicity, (ii) variability of single-scattering albedo profiles, and (iii) plane-parallel closure of the modelled atmosphere. A chemical weather model with satellite-derived biomass-burning emissions was applied to interpret the transport and transformation pathways. The provided MODTRAN radiative transfer model (RTM) simulations for the smoke event (14:00 9 July–11:30 11 July) resulted in a mean aerosol direct radiative forcing at the levels of −78.9 and −47.0 W m−2 at the surface and at the top of the atmosphere, respectively, for the mean value of aerosol optical depth equal to 0.64 at 550 nm. This corresponded to the average clear-sky direct radiative forcing of −43.3 W m−2, estimated by radiometer and model simulations at the surface. Ultimately, uncertainty associated with the plane-parallel atmosphere approximation altered results by about 2 W m−2. Furthermore, model-derived aerosol direct radiative forcing efficiency reached on average −126 W m-2/τ550 and −71 W m-2/τ550 at the surface and at the top of the atmosphere, respectively. The heating rate, estimated at up to 1.8 K day−1 inside the biomass-burning plume, implied vertical mixing with turbulent kinetic energy of 0.3 m2 s−2.


2012 ◽  
Vol 12 (6) ◽  
pp. 14837-14874 ◽  
Author(s):  
E. T. Sena ◽  
P. Artaxo ◽  
A. L. Correia

Abstract. This paper addresses the Amazonian radiative budget after considering three aspects of deforestation: (i) the emission of aerosols from biomass burning due to forest fires; (ii) changes in surface albedo after deforestation and (iii) modifications in the column water vapour amount over deforested areas. Simultaneous Clouds and the Earth's Radiant Energy System (CERES) shortwave fluxes and aerosol optical depth (AOD) retrievals from the Moderate Resolution Imaging SpectroRadiometer (MODIS) were analysed during the peak of the biomass burning seasons (August and September) from 2000 to 2009. A discrete-ordinate radiative transfer (DISORT) code was used to extend instantaneous remote sensing radiative forcing assessments into 24-h averages. The mean direct radiative forcing of aerosols at the top of the atmosphere (TOA) during the biomass burning season for the 10-yr studied period was −5.6 ± 1.7 W m−2. Furthermore, the spatial distribution of the direct radiative forcing of aerosols over Amazon was obtained for the biomass burning season of each year. It was observed that for high AOD (larger than 1 at 550 nm) the imbalance in the radiative forcing at the TOA may be as high as −20 W m−2 locally. The surface reflectance plays a major role in the aerosol direct radiative effect. The study of the effects of biomass burning aerosols over different surface types shows that the direct radiative forcing is systematically more negative over forest than over savannah-like covered areas. Values of −15.7 ± 2.4 W m−2/τ550 nm and −9.3 ± 1.7 W m−2/τ550 nm were calculated for the mean daily aerosol forcing efficiencies over forest and savannah-like vegetation respectively. The overall mean annual albedo-change radiative forcing due to deforestation over the state of Rondônia, Brazil, was determined as −7.3 ± 0.9 W m−2. Biomass burning aerosols impact the radiative budget for approximately two months per year, whereas the surface albedo impact is observed throughout the year. Because of this difference, the estimated impact in the Amazonian annual radiative budget due to surface albedo-change is approximately 6 times higher than the impact due to aerosol emissions. The influence of atmospheric water vapour content in the radiative budget was also studied using AERONET column water vapour. It was observed that column water vapour is in average smaller by about 0.35 cm over deforested areas compared to forested areas. Our results indicate that this drying impact contributes to an increase in the shortwave radiative effect that varies from 0.4 W m−2 to 1.2 W m−2, depending on the column water vapour content before deforestation. The large radiative forcing values presented in this study point out that deforestation has strong implications in convection, cloud development and photosynthesis rate over the Amazon region.


2013 ◽  
Vol 13 (3) ◽  
pp. 1261-1275 ◽  
Author(s):  
E. T. Sena ◽  
P. Artaxo ◽  
A. L. Correia

Abstract. This paper addresses the Amazonian shortwave radiative budget over cloud-free conditions after considering three aspects of deforestation: (i) the emission of aerosols from biomass burning due to forest fires; (ii) changes in surface albedo after deforestation; and (iii) modifications in the column water vapour amount over deforested areas. Simultaneous Clouds and the Earth's Radiant Energy System (CERES) shortwave fluxes and aerosol optical depth (AOD) retrievals from the Moderate Resolution Imaging SpectroRadiometer (MODIS) were analysed during the peak of the biomass burning seasons (August and September) from 2000 to 2009. A discrete-ordinate radiative transfer (DISORT) code was used to extend instantaneous remote sensing radiative forcing assessments into 24-h averages. The mean direct radiative forcing of aerosols at the top of the atmosphere (TOA) during the biomass burning season for the 10-yr studied period was −5.6 ± 1.7 W m−2. Furthermore, the spatial distribution of the direct radiative forcing of aerosols over Amazonia was obtained for the biomass burning season of each year. It was observed that for high AOD (larger than 1 at 550 nm) the maximum daily direct aerosol radiative forcing at the TOA may be as high as −20 W m−2 locally. The surface reflectance plays a major role in the aerosol direct radiative effect. The study of the effects of biomass burning aerosols over different surface types shows that the direct radiative forcing is systematically more negative over forest than over savannah-like covered areas. Values of −15.7 ± 2.4 W m−2τ550 nm and −9.3 ± 1.7 W m−2τ550 nm were calculated for the mean daily aerosol forcing efficiencies over forest and savannah-like vegetation respectively. The overall mean annual land use change radiative forcing due to deforestation over the state of Rondônia, Brazil, was determined as −7.3 ± 0.9 W m−2. Biomass burning aerosols impact the radiative budget for approximately two months per year, whereas the surface albedo impact is observed throughout the year. Because of this difference, the estimated impact in the Amazonian annual radiative budget due to surface albedo-change is approximately 6 times higher than the impact due to aerosol emissions. The influence of atmospheric water vapour content in the radiative budget was also studied using AERONET column water vapour. It was observed that column water vapour is on average smaller by about 0.35 cm (around 10% of the total column water vapour) over deforested areas compared to forested areas. Our results indicate that this drying contributes to an increase in the shortwave radiative forcing, which varies from 0.4 W m−2 to 1.2 W m−2 depending on the column water vapour content before deforestation. The large radiative forcing values presented in this study point out that deforestation could have strong implications in convection, cloud development and the ratio of direct to diffuse radiation, which impacts carbon uptake by the forest.


2017 ◽  
Author(s):  
Justyna Lisok ◽  
Anna Rozwadowska ◽  
Jesper G. Pedersen ◽  
Krzysztof M. Markowicz ◽  
Christoph Ritter ◽  
...  

Abstract. The aim of the presented study was to investigate the impact on the radiation budget of biomass burning smoke plume transported from Alaska to high Arctic region (Ny-Alesund, Svalbard) in early July 2015. This high aerosol load event is considered exceptional in the last 25 years with mean aerosol optical depth increased by the factor of 10 in comparison to the average summer background values. We utilised in-situ data with hygroscopic growth equations as well as remote sensing measurements as inputs to radiative transfer models with an objective to estimate biases associated with (i) hygroscopicity, (ii) variability of ω profiles and (iii) plane-parallel closure of the modelled atmosphere. A chemical weather model with satellite-derived biomass burning emissions was used to interpret the transport and transformations pathways. Provided MODTRAN simulations resulted in the mean aerosol direct radiative forcing on the level of −78.9 W m−2 and −47.0 W m−2 at the surface and the top of the atmosphere respectively for the mean value of aerosol optical depth equal to 0.64 at 550 nm. It corresponded to the average clear-sky direct radiative forcing of −43.3 W m−2 estimated by radiometers and model simulations. Furthermore, model-derived aerosol direct radiative forcing efficiency reached on average −126 W m−2 / τ550 and −71 W m−2 / τ550 at the surface and at the top of the atmosphere. Estimated heating rate up to 1.8 K day−1 inside the BB plume implied vertical mixing with the turbulent kinetic energy of 0.3 m2 s−2. Ultimately, uncertainty connected with the plane-parallel atmosphere approximation altered results by about 2 W m−2.


2021 ◽  
Author(s):  
Ilaria Clemenzi ◽  
David Gustafsson ◽  
Jie Zhang ◽  
Björn Norell ◽  
Wolf Marchand ◽  
...  

&lt;p&gt;Snow in the mountains is the result of the interplay between meteorological conditions, e.g., precipitation, wind and solar radiation, and landscape features, e.g., vegetation and topography. For this reason, it is highly variable in time and space. It represents an important water storage for several sectors of the society including tourism, ecology and hydropower. The estimation of the amount of snow stored in winter and available in the form of snowmelt runoff can be strategic for their sustainability. In the hydropower sector, for example, the occurrence of higher snow and snowmelt runoff volumes at the end of the spring and in the early summer compared to the estimated one can substantially impact reservoir regulation with energy and economical losses. An accurate estimation of the snow volumes and their spatial and temporal distribution is thus essential for spring flood runoff prediction. Despite the increasing effort in the development of new acquisition techniques, the availability of extensive and representative snow and density measurements for snow water equivalent estimations is still limited. Hydrological models in combination with data assimilation of ground or remote sensing observations is a way to overcome these limitations. However, the impact of using different types of snow observations on snowmelt runoff predictions is, little understood. In this study we investigated the potential of assimilating in situ and remote sensing snow observations to improve snow water equivalent estimates and snowmelt runoff predictions. We modelled the seasonal snow water equivalent distribution in the Lake &amp;#214;veruman catchment, Northern Sweden, which is used for hydropower production. Simulations were performed using the semi-distributed hydrological model HYPE for the snow seasons 2017-2020. For this purpose, a snowfall distribution model based on wind-shelter factors was included to represent snow spatial distribution within model units. The units consist of 2.5x2.5 km&lt;sup&gt;2&lt;/sup&gt; grid cells, which were further divided into hydrological response units based on elevation, vegetation and aspect. The impact on the estimation of the total catchment mean snow water equivalent and snowmelt runoff volume were evaluated using for data assimilation, gpr-based snow water equivalent data acquired along survey lines in the catchment in the early spring of the four years, snow water equivalent data obtained by a machine learning algorithm and satellite-based fractional snow cover data. Results show that the wind-shelter based snow distribution model was able to represent a similar spatial distribution as the gpr survey lines, when assessed on the catchment level. Deviations in the model performance within and between specific gpr survey lines indicate issues with the spatial distribution of input precipitation, and/or need to include explicit representation of snow drift between model units. The explicit snow distribution model also improved runoff simulations, and the ability of the model to improve forecast through data assimilation.&lt;/p&gt;


2013 ◽  
Vol 13 (5) ◽  
pp. 2423-2434 ◽  
Author(s):  
B. H. Samset ◽  
G. Myhre ◽  
M. Schulz ◽  
Y. Balkanski ◽  
S. Bauer ◽  
...  

Abstract. The impact of black carbon (BC) aerosols on the global radiation balance is not well constrained. Here twelve global aerosol models are used to show that at least 20% of the present uncertainty in modeled BC direct radiative forcing (RF) is due to diversity in the simulated vertical profile of BC mass. Results are from phases 1 and 2 of the global aerosol model intercomparison project (AeroCom). Additionally, a significant fraction of the variability is shown to come from high altitudes, as, globally, more than 40% of the total BC RF is exerted above 5 km. BC emission regions and areas with transported BC are found to have differing characteristics. These insights into the importance of the vertical profile of BC lead us to suggest that observational studies are needed to better characterize the global distribution of BC, including in the upper troposphere.


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