scholarly journals Above-cloud aerosol optical depth from airborne observations in the southeast Atlantic

2020 ◽  
Vol 20 (3) ◽  
pp. 1565-1590 ◽  
Author(s):  
Samuel E. LeBlanc ◽  
Jens Redemann ◽  
Connor Flynn ◽  
Kristina Pistone ◽  
Meloë Kacenelenbogen ◽  
...  

Abstract. The southeast Atlantic (SEA) region is host to a climatologically significant biomass burning aerosol layer overlying marine stratocumulus. We present the first results of the directly measured above-cloud aerosol optical depth (ACAOD) from the recent ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) airborne field campaign during August and September 2016. In our analysis, we use data from the Spectrometers for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR) instrument and found an average ACAOD of 0.32 at 501 nm (range of 0.02 to 1.04), with an average Ångström exponent (AE) above clouds of 1.71. The AE is much lower at 1.25 for the full column (including below-cloud-level aerosol, with an average of 0.36 at 501 nm and a range of 0.02 to 0.74), indicating the presence of large aerosol particles, likely marine aerosol, in the lower atmospheric column. The ACAOD is observed from 4STAR to be highest near the coast at about 12∘ S, whereas its variability is largest at the southern edge of the average aerosol plume, as indicated by 12 years of MODIS observations. In comparison to MODIS-derived ACAOD and long-term fine-mode plume-average AOD along a diagonal routine track extending out from the coast of Namibia, the directly measured ACAOD from 4STAR is slightly lower than the ACAOD product from MODIS. The peak ACAOD expected from MODIS AOD retrievals averaged over a long term along the routine diagonal flight track (peak of 0.5) was measured to be closer to coast in 2016 at about 1.5–4∘ E, with 4STAR ACAOD averages showing a peak of 0.42. When considering the full observation set over the SEA, by spatially binning each sampled AOD, we obtain a geographically representative mean ACAOD of 0.37. Vertical profiles of AOD showcase the variability in the altitude of the aerosol plume and its separation from the cloud top. We measured larger AOD at a high altitude near the coast than farther from the coast, while generally observing a larger vertical gap farther from the coast. Changes in AOD with altitude are correlated with carbon monoxide, a gas tracer of the biomass burning aerosol plume. Vertical extent of gaps between aerosol and cloud show a wide distribution, with a near-zero gap being most frequent. The gap distribution with longitude is observed to be largest at about 7∘ E, farther from coast than expected from previous studies.

2019 ◽  
Author(s):  
Samuel E. LeBlanc ◽  
Jens Redemann ◽  
Connor Flynn ◽  
Kristina Pistone ◽  
Meloë Kacenelenbogen ◽  
...  

Abstract. The South-East Atlantic (SEA) is host to a climatologically significant biomass burning aerosol layer overlying marine stratocumulus. We present directly measured Above Cloud Aerosol Optical Depth (ACAOD) from the recent ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) airborne field campaign during August and September 2016. In our analysis, we use data from the Spectrometers for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR) instrument and found an average ACAOD of 0.32 at 501 nm, with an average Ångström exponent (AE) of 1.71. The AE is much lower at 1.25 for the full column (including below cloud level aerosol), indicating the presence of large aerosol particles, likely marine aerosol, embedded within the vertical column. ACAOD is observed to be highest near coast at about 12° S, whereas its variability is largest at the southern edge of the average aerosol plume, as indicated by 12 years of MODIS observations. In comparison to MODIS derived ACAOD and long term fine-mode plume-average AOD, the directly-measured ACAOD from 4STAR is slightly lower than the ACAOD product from MODIS. The peak ACAOD expected from long term retrievals is measured to be closer to coast in 2016 at about 1.5°–4° W. By spatially binning the sampled AOD, we obtain a mean ACAOD of 0.37 for the SEA region. Vertical profiles of AOD showcase the variability of the altitude of the aerosol plume and its separation from cloud top. We measured larger AOD at high altitude near coast than farther from coast, while generally observing a larger vertical gap further from coast. Changes of AOD with altitude are correlated with a gas tracer of the biomass burning aerosol plume. Vertical extent of gaps between aerosol and cloud show a large distribution of extent, dominated by near zero gap. The gap distribution with longitude is observed to be largest at about 7° W, farther from coast than expected.


2014 ◽  
Vol 14 (23) ◽  
pp. 32177-32231 ◽  
Author(s):  
V. Buchard ◽  
A. M. da Silva ◽  
P. R. Colarco ◽  
A. Darmenov ◽  
C. A. Randles ◽  
...  

Abstract. A radiative transfer interface has been developed to simulate the UV Aerosol Index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and Aerosol Absorption Optical Depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the Aerosol Robotic Network (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the South African and South American biomass burning regions indicates that revising the spectrally-dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons. Finally, during a period where the Asian region was mainly dominated by anthropogenic aerosols, we have performed a qualitative analysis in which the specification of anthropogenic emissions in GEOS-5 is adjusted to provide insight into discrepancies observed in AI comparisons.


2015 ◽  
Vol 15 (10) ◽  
pp. 5743-5760 ◽  
Author(s):  
V. Buchard ◽  
A. M. da Silva ◽  
P. R. Colarco ◽  
A. Darmenov ◽  
C. A. Randles ◽  
...  

Abstract. A radiative transfer interface has been developed to simulate the UV aerosol index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and aerosol absorption optical depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the AErosol RObotic NETwork (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model-produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the southern African and South American biomass burning regions indicates that revising the spectrally dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons. Finally, during a period where the Asian region was mainly dominated by anthropogenic aerosols, we have performed a qualitative analysis in which the specification of anthropogenic emissions in GEOS-5 is adjusted to provide insight into discrepancies observed in AI comparisons.


2020 ◽  
Author(s):  
Allison B. Marquardt Collow ◽  
Mark A. Miller ◽  
Lynne C. Trabachino ◽  
Michael P. Jensen ◽  
Meng Wang

Abstract. Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. Further uncertainties in the cloud structure arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean where biomass burning aerosol is transported from the African continent. As the aerosol plume progresses across the southeast Atlantic Ocean, radiative heating within the aerosol layer has the potential to alter the thermodynamic environment and therefore the cloud structure; however, this has yet to be quantified. The deployment of the First Atmospheric Radiation Measurement Mobile Facility (AMF1) in support of the Layered Atlantic Smoke Interactions with Clouds (LASIC) field campaign provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Using observed profiles of temperature, humidity, and clouds from the LASIC field campaign, alongside aerosol optical properties from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) as input for the Rapid Radiation Transfer Model (RRTM), profiles of the radiative heating rate due to aerosols and clouds were computed. Radiative heating is also assessed across the southeast Atlantic Ocean using an ensemble of back trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory Model (HYSPLIT). Idealized experiments using RRTM with and without aerosols and a range of values for the single scattering albedo demonstrate that shortwave (SW) heating within the aerosol layer above Ascension Island can locally range between 2 and 8 K per day, though impacts of the aerosol can be felt elsewhere in the atmospheric column. SW radiative heating due to biomass burning aerosol is not balanced by additional longwave cooling, and the net radiative impact results in a stabilization of the lower troposphere. However, these results are extremely sensitive to the single scatter albedo and the height of the aerosol plume with respect to the inversion layer.


2020 ◽  
Author(s):  
Yohei Shinozuka ◽  
Meloë S. Kacenelenbogen ◽  
Sharon P. Burton ◽  
Steven G. Howell ◽  
Paquita Zuidema ◽  
...  

Abstract. To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime 532 nm aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights in recent airborne lidar and sunphotometer observations above the southeast Atlantic. The mean AOD difference is between 0 and −0.01, when comparing the two sides, each up to 20 km wide, of cloud edges. The difference is not statistically significant according to a paired t-test. Systematic differences in the wavelength dependence of AOD and in situ single scattering albedo are also minute. These results hold regardless of the vertical distance between cloud top and aerosol layer bottom. AOD aggregated over ~ 2° grid boxes for each of September 2016, August 2017 and October 2018 also shows little correlation with the presence of low-level clouds. We posit that a satellite retrieval artifact is entirely responsible for a previous finding of generally smaller AOD over clouds (Chung et al., 2016), at least for the region and season of our study. Our results also suggest that the same values can be assumed for the intensive properties of free-tropospheric biomass-burning aerosol regardless of whether clouds exist below.


2020 ◽  
Vol 12 (14) ◽  
pp. 2330
Author(s):  
Yan Tong ◽  
Lian Feng ◽  
Kun Sun ◽  
Jing Tang

Assessments of long-term changes of air quality and global radiative forcing at a large scale heavily rely on satellite aerosol optical depth (AOD) datasets, particularly their temporal binning products. Although some attempts focusing on the validation of long-term satellite AOD have been conducted, there is still a lack of comprehensive quantification and understanding of the representativeness of satellite AOD at different temporal binning scales. Here, we evaluated the performances of the Moderate Resolution Imaging Spectroradiometer (MODIS) AOD products at various temporal scales by comparing the MODIS AOD datasets from both the Terra and Aqua satellites with the entire global AErosol RObotic NETwork (AERONET) observation archive between 2000 and 2017. The uncertainty levels of the MODIS hourly and daily AOD products were similarly high, indicating that MODIS AOD retrievals could be used to represent daily aerosol conditions. The MODIS data showed the reduced quality when integrated from the daily to monthly scale, where the relative mean bias (RMB) changed from 1.09 to 1.21 for MODIS Terra and from 1.04 to 1.17 for MODIS Aqua, respectively. The limitation of valid data availability within a month appeared to be the primary reason for the increased uncertainties in the monthly binning products, and the monthly data associated uncertainties could be reduced when the number of valid AOD retrievals reached 15 times in one month. At all three temporal scales, the uncertainty levels of satellite AOD products decreased with increasing AOD values. The results of this study could provide crucial information for satellite AOD users to better understand the reliability of different temporal AOD binning products and associated uncertainties in their derived long-term trends.


2011 ◽  
Vol 4 (2) ◽  
pp. 131-141 ◽  
Author(s):  
C. Kittaka ◽  
D. M. Winker ◽  
M. A. Vaughan ◽  
A. Omar ◽  
L. A. Remer

Abstract. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) is carried on the CALIPSO satellite and has acquired global aerosol profiles since June 2006. CALIPSO is flown in formation with the Aqua satellite as part of the A-train satellite constellation, so that a large number of coincident aerosol observations are available from CALIOP and the MODIS-Aqua instrument. This study compares column aerosol optical depth at 0.532 μm derived from CALIOP aerosol profiles with MODIS-Aqua 0.55 μm aerosol optical depth over the period June 2006 through August 2008. The study is based on the CALIOP Version 2 Aerosol Layer Product and MODIS Collection 5. While CALIOP is first and foremost a profiling instrument, this comparison of column aerosol optical depth provides insight into quality of CALIOP aerosol data. It is found that daytime aerosol optical depth from the CALIOP Version 2 product has only a small global mean bias relative to MODIS Collection 5. Regional biases, of both signs, are larger and biases are seen to vary somewhat with season. Good agreement between the two sensors in ocean regions with low cloudiness suggests that the selection of lidar ratios used in the CALIOP aerosol retrieval is sufficient to provide a regional mean AOD consistent with that retrieved from MODIS. Although differences over land are observed to be larger than over ocean, the bias between CALIOP and MODIS AOD on a regional-seasonal basis is found to be roughly within the envelope of the MODIS expected uncertainty over land and ocean. This work forms a basis for further comparisons using the recently released CALIOP Version 3 data.


2012 ◽  
Vol 12 (4) ◽  
pp. 10461-10492 ◽  
Author(s):  
Y. Xue ◽  
H. Xu ◽  
L. Mei ◽  
J. Guang ◽  
J. Guo ◽  
...  

Abstract. Agricultural biomass burning (ABB) in Central and East China occurs every year from May to October and peaks in June. The biomass burning event in June 2007 was very strong. During the period from 26 May to 16 June 2007, ABB occurred mainly in Anhui, Henan, Jiangsu and Shandong provinces. A comprehensive set of aerosol optical depth (AOD) data, produced by a merger of AOD product data from the Moderate Resolution Imaging Spectroradiometer (MODIS) and the Multiangle Imaging Spectroradiometer (MIRS), is used to study the spatial and temporal distribution of agricultural biomass aerosols in Central and East China combining with ground observations from both AErosol RObotic NETwork (AERONET) and China Aerosol Remote Sensing NETwork (CARSNET) measurements. We compared merged AOD data with single-sensor single-algorithm AOD data (MODIS Dark Target AOD data, MODIS Deep Blue AOD data, SRAP-MODIS AOD data and MISR AOD data). In this comparison, we found merged AOD products can improve the quality of AOD products from single-sensor single-algorithm data sets by expanding the spatial coverage of the study area and keeping the statistical confidence in AOD parameters. There existed high correlation (0.8479) between the merged AOD data and AERONET measurements. Our merged AOD data make use of synergetic information conveyed in all of the available satellite data. The merged AOD data were used for the analysis of the biomass burning event from 26 May to 16 June 2007 together with meteorological data. The merged AOD products and the ground observations from China suggest that biomass burning in Central and East China has had great impact on AOD over China. Influenced by this ABB, the highest AOD value in Beijing on 12 June 2007 reached 5.71.


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