scholarly journals Dominant synoptic patterns associated with the decay process of PM<sub>2.5</sub> pollution episodes around Beijing

2020 ◽  
Author(s):  
Xiaoyan Wang ◽  
Renhe Zhang ◽  
Yanke Tan ◽  
Wei Yu
Keyword(s):  
Boundary Layer ◽  
Relative Humidity ◽  
Air Pollutants ◽  
Wet Deposition ◽  
Decay Process ◽  
Horizontal Wind ◽  
Synoptic Patterns ◽  
Circulation Patterns ◽  
Autumn And Winter ◽  
Pollution Episodes

Abstract. The variation in the concentrations of ambient PM2.5 (particles with an aerodynamic diameter less than 2.5 μm) generally forms a continuous sawtooth cycle with a recurring smooth increase followed by a sharp decrease. The abrupt decay of pollution episode is mostly meteorological in origin, and is controlled by the passage of synoptic systems. One affordable and effective measure for the quickly reducing PM2.5 concentrations in northern China is to wait for strong wind to arrive. However, it is still unclear how strong the wind needs to be and exactly what kind of synoptic system most effectively results in the rapid decay of air pollution episodes. PM2.5 variations over the 28 pollution channel cities of Beijing are investigated to determine the mechanisms by which synoptic patterns affect the decay processes of pollution episodes. This work shows more obvious day-to-day variations in PM2.5 concentration in winter than in summer, which implies that wintertime PM2.5 variations are more sensitive to meteorological factors. There were 365 decay processes from January 2014 to March 2020, and 97 of them were related to the effective wet deposition. 26 %~43 % of PM2.5 pollutant is removed by the wet deposition in different seasons. Two dominant circulation patterns are identified in summer, and the same three circulation types (CTs) are identified in the other three seasons based on the dry-day cases. The circulation patterns beneficial to the decay processes all exhibit a higher than normal surface wind speed, a negative relative humidity anomaly and positive divergence in the PM2.5 horizontal flux. In addition, CT1 in spring, autumn and winter is controlled by northeasterly wind and features the most significant horizontal net-outflow of air pollutants and effective upward spread of air pollutants to the free atmosphere, which promotes the abrupt reduction of local PM2.5 concentrations. CT2 is the most frequent synoptic pattern leading to decay processes in autumn and winter, and the domain region is located to the east of an anticyclone system. CT2 features a strong northwesterly wind of 2.98~3.88 m/s, the lowest relative humidity and the highest boundary layer height (BLH) among the three CTs, all of which are favorable for the reduction of PM2.5 concentrations. In CT3, a prevailing westerly wind anomaly occurs in the domain, with remarkable zonal divergence in the PM2.5 flux and strong horizontal wind shear in the near-surface under the boundary layer. PM2.5 concentrations show significant decreases of more than 37 %, 41 % and 27 % after the passage of CT1, CT2 and CT3, respectively. A dry air mass with a positive BLH anomaly and the effective horizontal outflow of air pollutants are the main reasons for the abrupt decay phase in summer. PM2.5 concentrations after the decay process show a significant decreasing trend from 2014 to 2020, reflecting successful emission mitigation. Emission reductions have led to a 4.3~5.7 μg/(m3.yr) decrease in PM2.5 concentrations in the 28 pollution channel cities of Beijing.

scholarly journals Dominant synoptic patterns associated with the decay process of PM<sub>2.5</sub> pollution episodes around Beijing

2021 ◽  
Vol 21 (4) ◽  
pp. 2491-2508
Author(s):  
Xiaoyan Wang ◽  
Renhe Zhang ◽  
Yanke Tan ◽  
Wei Yu
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Relative Humidity ◽  
Air Pollutants ◽  
Wet Deposition ◽  
Decay Process ◽  
Synoptic Patterns ◽  
Circulation Patterns ◽  
Autumn And Winter ◽  
Pollution Episodes

Abstract. The variation in the concentrations of ambient PM2.5 (particles with an aerodynamic diameter less than 2.5 µm) generally forms a continuous sawtooth cycle with a recurring smooth increase followed by a sharp decrease. The episode of abrupt decay of pollution is mostly meteorological in origin and is controlled by the passage of synoptic systems. One affordable and effective measure for quickly reducing PM2.5 concentrations in northern China is to wait for a strong wind to arrive. However, it is still unclear how strong the wind needs to be and exactly what kind of synoptic system most effectively results in the rapid decay of air pollution episodes. PM2.5 variations over the 28 pollution channel cities of the Beijing region are investigated to determine the mechanisms by which synoptic patterns affect the decay processes of pollution episodes. This work shows more obvious day-to-day variations in PM2.5 concentration in winter than in summer, which implies that wintertime PM2.5 variations are more sensitive to meteorological factors. There were 365 decay processes from January 2014 to March 2020, and 97 of them were related to the effective wet deposition. In total, 26 %–43 % of PM2.5 pollutant is removed by the wet deposition in different seasons. Two dominant circulation patterns are identified in summer. All the other three seasons have three circulation types (CTs), respectively. The three CTs in spring show the same patterns as those in autumn and winter. The circulation patterns beneficial to the decay processes all exhibit a higher-than-normal surface wind speed, a negative relative humidity anomaly and net outflow of PM2.5 from the domain. In addition, CT1 in spring, autumn and winter is controlled by northeasterly wind and features the most significant horizontal net outflow of air pollutants and effective upward spread of air pollutants to the free atmosphere. CT2 is the most frequent CT in autumn and winter, with the highest wind speed from the northwest, highest boundary layer height (BLH) and lowest relative humidity among the three CTs, all of which are favorable for the reduction of PM2.5 concentrations. In CT3, strong vertical wind shear within the boundary layer enhances the mixing of surface air pollutants, which is the extra cleaning mechanism besides dry and clean air mass inflow. PM2.5 concentrations show significant decreases of more than 37 %, 41 % and 27 % after the passage of CT1, CT2 and CT3, respectively. A dry airflow with a positive BLH anomaly and the effective horizontal outflow of air pollutants are the main reasons for the abrupt decay phase in summer. PM2.5 concentrations after the decay process show a significant decreasing trend from 2014 to 2020, reflecting successful emission mitigation. Emission reductions have led to a 4.3–5.7 µgm-3yr-1 decrease in PM2.5 concentrations in the 28 pollution channel cities of the Beijing region.

scholarly journals Feedback effects of boundary-layer meteorological factors on cumulative explosive growth of PM<sub>2.5</sub> during winter heavy pollution episodes in Beijing from 2013 to 2016

2018 ◽  
Vol 18 (1) ◽  
pp. 247-258 ◽  
Author(s):  
Junting Zhong ◽  
Xiaoye Zhang ◽  
Yunsheng Dong ◽  
Yaqiang Wang ◽  
Cheng Liu ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Relative Humidity ◽  
Meteorological Factors ◽  
Meteorological Data ◽  
Heterogeneous Reactions ◽  
Hygroscopic Growth ◽  
Surface Cooling ◽  
Boundary Layer Height ◽  
Aerosol Pollution ◽  
Pollution Episodes

Abstract. In January 2013, February 2014, December 2015 and December 2016 to 10 January 2017, 12 persistent heavy aerosol pollution episodes (HPEs) occurred in Beijing, which received special attention from the public. During the HPEs, the precise cause of PM2.5 explosive growth (mass concentration at least doubled in several hours to 10 h) is uncertain. Here, we analyzed and estimated relative contributions of boundary-layer meteorological factors to such growth, using ground and vertical meteorological data. Beijing HPEs are generally characterized by the transport stage (TS), whose aerosol pollution formation is primarily caused by pollutants transported from the south of Beijing, and the cumulative stage (CS), in which the cumulative explosive growth of PM2.5 mass is dominated by stable atmospheric stratification characteristics of southerly slight or calm winds, near-ground anomalous inversion, and moisture accumulation. During the CSs, observed southerly weak winds facilitate local pollutant accumulation by minimizing horizontal pollutant diffusion. Established by TSs, elevated PM2.5 levels scatter more solar radiation back to space to reduce near-ground temperature, which very likely causes anomalous inversion. This surface cooling by PM2.5 decreases near-ground saturation vapor pressure and increases relative humidity significantly; the inversion subsequently reduces vertical turbulent diffusion and boundary-layer height to trap pollutants and accumulate water vapor. Appreciable near-ground moisture accumulation (relative humidity> 80 %) would further enhance aerosol hygroscopic growth and accelerate liquid-phase and heterogeneous reactions, in which incompletely quantified chemical mechanisms need more investigation. The positive meteorological feedback noted on PM2.5 mass explains over 70 % of cumulative explosive growth.

scholarly journals Effects of atmospheric dynamics and aerosols on the fraction of supercooled water clouds

2017 ◽  
Vol 17 (3) ◽  
pp. 1847-1863 ◽  
Author(s):  
Jiming Li ◽  
Qiaoyi Lv ◽  
Min Zhang ◽  
Tianhe Wang ◽  
Kazuaki Kawamoto ◽  
...  
Keyword(s):  
Relative Humidity ◽  
Vertical Velocity ◽  
Meteorological Parameters ◽  
Temporal Correlation ◽  
Supercooled Liquid ◽  
Satellite Observation ◽  
Static Stability ◽  
Global Scale ◽  
Atmospheric Dynamics ◽  
Horizontal Wind

Abstract. Based on 8 years of (January 2008–December 2015) cloud phase information from the GCM-Oriented Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) Cloud Product (GOCCP), aerosol products from CALIPSO and meteorological parameters from the ERA-Interim products, the present study investigates the effects of atmospheric dynamics on the supercooled liquid cloud fraction (SCF) during nighttime under different aerosol loadings at global scale to better understand the conditions of supercooled liquid water gradually transforming to ice phase. Statistical results indicate that aerosols' effect on nucleation cannot fully explain all SCF changes, especially in those regions where aerosols' effect on nucleation is not a first-order influence (e.g., due to low ice nuclei aerosol frequency). By performing the temporal and spatial correlations between SCFs and different meteorological factors, this study presents specifically the relationship between SCF and different meteorological parameters under different aerosol loadings on a global scale. We find that the SCFs almost decrease with increasing of aerosol loading, and the SCF variation is closely related to the meteorological parameters but their temporal relationship is not stable and varies with the different regions, seasons and isotherm levels. Obviously negative temporal correlations between SCFs versus vertical velocity and relative humidity indicate that the higher vertical velocity and relative humidity the smaller SCFs. However, the patterns of temporal correlation for lower-tropospheric static stability, skin temperature and horizontal wind are relatively more complex than those of vertical velocity and humidity. For example, their close correlations are predominantly located in middle and high latitudes and vary with latitude or surface type. Although these statistical correlations have not been used to establish a certain causal relationship, our results may provide a unique point of view on the phase change of mixed-phase cloud and have potential implications for further improving the parameterization of the cloud phase and determining the climate feedbacks.

Observations of Small-Scale Turbulence and Energy Dissipation Rates in the Cloudy Boundary Layer

2006 ◽  
Vol 63 (5) ◽  
pp. 1451-1466 ◽  
Author(s):  
Holger Siebert ◽  
Katrin Lehmann ◽  
Manfred Wendisch
Keyword(s):  
Boundary Layer ◽  
Energy Dissipation ◽  
Wind Velocity ◽  
Turbulence Theory ◽  
Horizontal Wind ◽  
Inertial Subrange ◽  
Intermittent Flow ◽  
Small Scale ◽  
Dissipation Rates ◽  
Wide Range

Abstract Tethered balloon–borne measurements with a resolution in the order of 10 cm in a cloudy boundary layer are presented. Two examples sampled under different conditions concerning the clouds' stage of life are discussed. The hypothesis tested here is that basic ideas of classical turbulence theory in boundary layer clouds are valid even to the decimeter scale. Power spectral densities S( f ) of air temperature, liquid water content, and wind velocity components show an inertial subrange behavior down to ≈20 cm. The mean energy dissipation rates are ∼10−3 m2 s−3 for both datasets. Estimated Taylor Reynolds numbers (Reλ) are ∼104, which indicates the turbulence is fully developed. The ratios between longitudinal and transversal S( f ) converge to a value close to 4/3, which is predicted by classical turbulence theory for local isotropic conditions. Probability density functions (PDFs) of wind velocity increments Δu are derived. The PDFs show significant deviations from a Gaussian distribution with longer tails typical for an intermittent flow. Local energy dissipation rates ɛτ are derived from subsequences with a duration of τ = 1 s. With a mean horizontal wind velocity of 8 m s−1, τ corresponds to a spatial scale of 8 m. The PDFs of ɛτ can be well approximated with a lognormal distribution that agrees with classical theory. Maximum values of ɛτ ≈ 10−1 m2 s−3 are found in the analyzed clouds. The consequences of this wide range of ɛτ values for particle–turbulence interaction are discussed.

scholarly journals Evaluation of the AMPS Boundary Layer Simulations on the Ross Ice Shelf, Antarctica, with Unmanned Aircraft Observations

2017 ◽  
Vol 56 (8) ◽  
pp. 2239-2258 ◽  
Author(s):  
Jonathan D. Wille ◽  
David H. Bromwich ◽  
John J. Cassano ◽  
Melissa A. Nigro ◽  
Marian E. Mateling ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Relative Humidity ◽  
High Wind ◽  
Ice Shelf ◽  
High Wind Speed ◽  
Near Surface ◽  
Ross Ice Shelf ◽  
Low Cloud ◽  
The Antarctic

AbstractAccurately predicting moisture and stability in the Antarctic planetary boundary layer (PBL) is essential for low-cloud forecasts, especially when Antarctic forecasters often use relative humidity as a proxy for cloud cover. These forecasters typically rely on the Antarctic Mesoscale Prediction System (AMPS) Polar Weather Research and Forecasting (Polar WRF) Model for high-resolution forecasts. To complement the PBL observations from the 30-m Alexander Tall Tower! (ATT) on the Ross Ice Shelf as discussed in a recent paper by Wille and coworkers, a field campaign was conducted at the ATT site from 13 to 26 January 2014 using Small Unmanned Meteorological Observer (SUMO) aerial systems to collect PBL data. The 3-km-resolution AMPS forecast output is combined with the global European Centre for Medium-Range Weather Forecasts interim reanalysis (ERAI), SUMO flights, and ATT data to describe atmospheric conditions on the Ross Ice Shelf. The SUMO comparison showed that AMPS had an average 2–3 m s−1 high wind speed bias from the near surface to 600 m, which led to excessive mechanical mixing and reduced stability in the PBL. As discussed in previous Polar WRF studies, the Mellor–Yamada–Janjić PBL scheme is likely responsible for the high wind speed bias. The SUMO comparison also showed a near-surface 10–15-percentage-point dry relative humidity bias in AMPS that increased to a 25–30-percentage-point deficit from 200 to 400 m above the surface. A large dry bias at these critical heights for aircraft operations implies poor AMPS low-cloud forecasts. The ERAI showed that the katabatic flow from the Transantarctic Mountains is unrealistically dry in AMPS.

scholarly journals Atmospheric pollution over the eastern Mediterranean during summer – a review

2017 ◽  
Vol 17 (21) ◽  
pp. 13233-13263 ◽  
Author(s):  
Uri Dayan ◽  
Philippe Ricaud ◽  
Régina Zbinden ◽  
François Dulac
Keyword(s):  
Boundary Layer ◽  
Carbon Monoxide ◽  
Long Range ◽  
Mixed Layer ◽  
Air Pollutants ◽  
Asian Monsoon ◽  
Eastern Mediterranean ◽  
Long Range Transport ◽  
Range Transport ◽  
Ventilation Rates

Abstract. The eastern Mediterranean (EM) is one of the regions in the world where elevated concentrations of primary and secondary gaseous air pollutants have been reported frequently, mainly in summer. This review discusses published studies of the atmospheric dispersion and transport conditions characterizing this region during the summer, followed by a description of some essential studies dealing with the corresponding concentrations of air pollutants such as ozone, carbon monoxide, total reactive nitrogen, methane, and sulfate aerosols observed there. The interlaced relationship between the downward motion of the subsiding air aloft induced by global circulation systems affecting the EM and the depth of the Persian Trough, a low-pressure trough that extends from the Asian monsoon at the surface controlling the spatiotemporal distribution of the mixed boundary layer during summer, is discussed. The strength of the wind flow within the mixed layer and its depth affect much the amount of pollutants transported and determine the potential of the atmosphere to disperse contaminants off their origins in the EM. The reduced mixed layer and the accompanying weak westerlies, characterizing the summer in this region, led to reduced ventilation rates, preventing an effective dilution of the contaminants. Several studies pointing at specific local (e.g., ventilation rates) and regional peculiarities (long-range transport) enhancing the build-up of air pollutant concentrations are presented. Tropospheric ozone (O3) concentrations observed in the summer over the EM are among the highest over the Northern Hemisphere. The three essential processes controlling its formation (i.e., long-range transport of polluted air masses, dynamic subsidence at mid-tropospheric levels, and stratosphere-to-troposphere exchange) are reviewed. Airborne campaigns and satellite-borne initiatives have indicated that the concentration values of reactive nitrogen identified as precursors in the formation of O3 over the EM were found to be 2 to 10 times higher than in the hemispheric background troposphere. Several factors favor sulfate particulate abundance over the EM. Models, aircraft measurements, and satellite-derived data have clearly shown that sulfate has a maximum during spring and summer over the EM. The carbon monoxide (CO) seasonal cycle, as obtained from global background monitoring sites in the EM, is mostly controlled by the tropospheric concentration of the hydroxyl radical (OH) and therefore demonstrates high concentrations over winter months and the lowest concentrations during summer when photochemistry is active. Modeling studies have shown that the diurnal variations in CO concentration during the summer result from long-range CO transport from European anthropogenic sources, contributing 60 to 80 % of the boundary-layer CO over the EM. The values retrieved from satellite data enable us to derive the spatial distribution of methane (CH4), identifying August as the month with the highest levels over the EM. The outcomes of a recent extensive examination of the distribution of methane over the tropospheric Mediterranean Basin, as part of the Chemistry-Aerosol Mediterranean Experiment (ChArMEx) program, using model simulations and satellite measurements, are coherent with other previous studies. Moreover, this methane study provides some insight into the role of the Asian monsoon anticyclone in controlling the variability of CH4 pollutant within mid-to-upper tropospheric levels above the EM in summer.

Rising Planetary Boundary Layer Height over the Sahara Desert and Arabian Peninsula in a Warming Climate

2021 ◽  
Vol 34 (10) ◽  
pp. 4043-4068
Author(s):  
Liming Zhou ◽  
Yuhong Tian ◽  
Nan Wei ◽  
Shu-peng Ho ◽  
Jing Li
Keyword(s):  
Boundary Layer ◽  
Relative Humidity ◽  
Planetary Boundary Layer ◽  
Large Scale ◽  
Arabian Peninsula ◽  
Climate Model ◽  
Statistical Significance ◽  
Maximum Height ◽  
Sahara Desert ◽  
Sensible Heat

AbstractTurbulent mixing in the planetary boundary layer (PBL) governs the vertical exchange of heat, moisture, momentum, trace gases, and aerosols in the surface–atmosphere interface. The PBL height (PBLH) represents the maximum height of the free atmosphere that is directly influenced by Earth’s surface. This study uses a multidata synthesis approach from an ensemble of multiple global datasets of radiosonde observations, reanalysis products, and climate model simulations to examine the spatial patterns of long-term PBLH trends over land between 60°S and 60°N for the period 1979–2019. By considering both the sign and statistical significance of trends, we identify large-scale regions where the change signal is robust and consistent to increase our confidence in the obtained results. Despite differences in the magnitude and sign of PBLH trends over many areas, all datasets reveal a consensus on increasing PBLH over the enormous and very dry Sahara Desert and Arabian Peninsula (SDAP) and declining PBLH in India. At the global scale, the changes in PBLH are significantly correlated positively with the changes in surface heating and negatively with the changes in surface moisture, consistent with theory and previous findings in the literature. The rising PBLH is in good agreement with increasing sensible heat and surface temperature and decreasing relative humidity over the SDAP associated with desert amplification, while the declining PBLH resonates well with increasing relative humidity and latent heat and decreasing sensible heat and surface warming in India. The PBLH changes agree with radiosonde soundings over the SDAP but cannot be validated over India due to lack of good-quality radiosonde observations.

scholarly journals Temporal and Spatial variation of Contribution from Ship Emissions to the concentration and deposition of air pollutants in the Baltic Sea

2016 ◽  
Author(s):  
Karin Haglund ◽  
Björn Claremar ◽  
Anna Rutgersson
Keyword(s):  
Atmospheric Deposition ◽  
Baltic Sea ◽  
Dry Deposition ◽  
Air Pollutants ◽  
Wet Deposition ◽  
Sulphur Content ◽  
The Baltic Sea ◽  
Near Surface ◽  
Baltic Sea Region ◽  
The Baltic

Abstract. The shipping sector contributes significantly to increasing emissions of air pollutants. In order to achieve sustainable shipping, primarily through new regulations and techniques, greater knowledge of dispersion and deposition of air pollutants is required. Regional model calculations of the dispersion and deposition of sulphur, nitrogen and particulate matter from the international maritime sector in the Baltic Sea and the North Sea have been made for the years 2009 to 2013. In some areas in the Baltic Sea region the contribution of sulphur dioxide, nitrogen oxide and nitrogen dioxide from international shipping represented up to 80 % of the total near surface concentration of the pollutants. Contributions from shipping of PM2,5 and PM10 were calculated to a maximum of 21 % and 13 % respectively. The contribution of wet deposition of sulphur from shipping was maximum 29 % of the total wet deposition, and for dry deposition the contribution from shipping was maximum 84 %. The highest percentage contribution of wet deposition of nitrogen from shipping reached 28 % and for dry deposition 47 %. The highest concentrations and deposition of the pollutants in the study were found near large ports and shipping lanes. High concentrations were also found over larger areas at sea and over land where many people are exposed. With enhanced regulations for sulphur content in maritime fuel, the cleaning of exhausts through scrubbers has become a possible economic solution. Wet scrubbers meet the air quality criteria but their consequences for the marine environment are largely unknown. The resulting potential of future acidification in the Baltic Sea, both from atmospheric deposition and from open-loop scrubber water along the shipping lanes, based on different assumptions about sulphur content in fuel and scrubber usage has been assessed. Shipping is expected to increase globally and in the Baltic Sea region, deposition of sulphur due to shipping will depend on traffic density, emission regulations and technology choices for the emission controls. To evaluate future changes scenarios are developed considering the amount of scrubber technology used. The increase in deposition for the different scenarios differs slightly for the basins in the Baltic Sea. The proportion of ocean acidifying sulphur from ships increases when taking scrubber water into account and the major reason to increasing acidifying nitrogen from ships are due to increasing ship traffic. This study also generates a database of scenarios for atmospheric deposition and scrubber exhaust from the period 2011 to 2050.

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