Abstract. A prescribed burning of a boreal forest was conducted on 26 June 2009 in Hyytiälä, Finland, to study aerosol and trace gas emissions from wildfires and the effects of fire on soil properties in a controlled environment. A 0.8 ha forest near the SMEAR II was cut clear; some tree trunks, all tree tops and branches were left on the ground and burned. The amount of burned organic material was ~46.8 t (i.e., ~60 t ha−1). The flaming phase lasted 2 h 15 min, the smoldering phase 3 h. Measurements were conducted on the ground with both fixed and mobile instrumentation, and from a research aircraft. In the middle of the burning area, CO2 concentration peaks were around 2000–3000 ppm above the baseline and peak vertical flow velocities were 6 ± 3 m s−1, as measured a 10-Hz 3-D sonic anemometer placed within the burn area. Peak particle number concentrations were approximately 1–2 × 106 cm−3 in the plume at a distance of 100–200 m from the burn area. The geometric mean diameter of the mode with the highest concentration was at 80 ± 1 nm during the flaming phase and in the middle of the smoldering phase but at the end of the smoldering phase the largest mode was at 122 nm. In the volume size distributions geometric mean diameter of the largest volume mode was at 153 nm during the flaming phase and at 300 nm during the smoldering phase. The lowest single-scattering albedo of the ground-level measurents was 0.7 in the flaming-phase plume and ~0.9 in the smoldering phase. The radiative forcing efficiency was negative above dark surfaces, in other words, the particles cool the atmosphere. Elevated concentrations of several VOCs (including acetonitrile which is a biomass burning marker) were observed in the smoke plume at ground level. The forest floor (i.e., richly organic layer of soil and debris, characteristic of forested land) measurements showed that VOC fluxes were generally low and consisted mainly of monoterpenes, but a clear peak of VOC flux was observed after the burning. After one year, the fluxes were nearly stabilised close to the level before the burning. The clearcutting and burning of slash increased the total long-term CO2 release from the soil, altered the soil's physical, chemical and biological properties such as increased the available nitrogen contents of the soil, which in turn, affected the level of the long-term fluxes of greenhouse gases.
Supplementary material to "Diurnal evolution of negative atmospheric ions above the boreal forest: From ground level to the free troposphere"
