scholarly journals BrO, blizzards, and drivers of polar tropospheric ozone depletion events

2009 ◽  
Vol 9 (14) ◽  
pp. 4639-4652 ◽  
Author(s):  
A. E. Jones ◽  
P. S. Anderson ◽  
M. Begoin ◽  
N. Brough ◽  
M. A. Hutterli ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Ozone Depletion ◽  
Stable Boundary Layer ◽  
Weddell Sea ◽  
Blowing Snow ◽  
High Wind ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Global Impacts ◽  
Boundary Layer Ozone

Abstract. The source of bromine that drives polar boundary layer ozone depletion events (ODEs) is still open to some debate. While ODEs are generally noted to form under conditions of a shallow stable boundary layer, observations of depleted air under high wind conditions are taken as being transport-related. Here we report observations from Antarctica in which an unusually large cloud of BrO formed over the Weddell Sea. The enhanced BrO was observed over Halley station in coastal Antarctica, providing an opportunity to probe the conditions within an active "bromine explosion" event. On this occasion, enhanced BrO and depleted boundary layer ozone coincided with high wind speeds and saline blowing snow. We derive a simple model to consider the environmental conditions that favour ODEs and find two maxima, one at low wind/stable boundary layer and one at high wind speeds with blowing snow. Modelling calculations aiming to reproduce the wider regional or global impacts of ODEs, either via radiative effects or as a halogen source, will also need to account for high wind speed mechanisms.

scholarly journals BrO, blizzards, and drivers of polar tropospheric ozone depletion events

2009 ◽  
Vol 9 (2) ◽  
pp. 8903-8941
Author(s):  
A. E. Jones ◽  
P. S. Anderson ◽  
M. Begoin ◽  
N. Brough ◽  
M. A. Hutterli ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Ozone Depletion ◽  
Stable Boundary Layer ◽  
Weddell Sea ◽  
Blowing Snow ◽  
High Wind ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Global Impacts ◽  
Boundary Layer Ozone

Abstract. The source of bromine that drives polar boundary layer ozone depletion events (ODEs) is still open to some debate. While ODEs are generally noted to form under conditions of a shallow stable boundary layer, observations of depleted air under high wind conditions are taken as being transport-related. Here we report observations from Antarctica in which an unusually large cloud of BrO formed over the Weddell Sea. The enhanced BrO was observed over Halley station in coastal Antarctica, providing an opportunity to probe the conditions within an active "bromine explosion" event. On this occasion, enhanced BrO and depleted boundary layer ozone coincided with high wind speeds and saline blowing snow. We derive a simple model to consider the environmental conditions that favour ODEs and find two maxima, one at low wind/stable boundary layer and one at high wind speeds with blowing snow. Modelling calculations aiming to reproduce the wider regional or global impacts of ODEs, either via radiative effects or as a halogen source, will also need to account for high wind speed mechanisms.

Investigation of weather conditions and tropospheric BrO transport during Bromine Explosion Events in the Arctic and ozone depletion in Ny-Ålesund observed by satellite and ground-based remote sensing

2021 ◽  
Author(s):  
Bianca Zilker ◽  
Anne-Marlene Blechschmidt ◽  
Sora Seo ◽  
Ilias Bougoudis ◽  
Tim Bösch ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Detection Limit ◽  
Wind Speed ◽  
Ozone Depletion ◽  
Weather Conditions ◽  
Tropospheric Chemistry ◽  
The Arctic ◽  
Blowing Snow ◽  
High Wind ◽  
Wind Speeds

<p align="justify">Bromine Explosion Events (BEEs) have been observed since the late 1990s in the Arctic and Antarctic during polar spring and play an important role in tropospheric chemistry. In a heterogeneous, autocatalytic, chemical chain reaction cycle, inorganic bromine is released from the cryosphere into the troposphere and depletes ozone often to below detection limit. Ozone is a source of the most important tropospheric oxidizing agent OH and the oxidizing capacity and radiative forcing of the troposphere are thus being impacted. Bromine also reacts with gaseous mercury, thereby facilitating the deposition of toxic mercury, which has adverse environmental impacts. C<span lang="en-US">old saline surfaces, such as young sea ice, frost flowers, and snow are likely bromine sources </span><span lang="en-US">during BEEs. </span><span lang="en-US">D</span>ifferent meteorological conditions seem to favor the development of these events: on the one hand, low wind speeds and a stable boundary layer, where bromine can accumulate and deplete ozone, and on the other hand, high wind speeds above approximately 10 m/s with blowing snow and a higher unstable boundary layer. In high wind speed conditions – occurring for example along fronts of polar cyclones – recycling of bromine on snow and aerosol surfaces may take place aloft.</p> <p align="justify">To improve the understanding of weather conditions and bromine sources leading to the development of BEEs, case studies using high resolution S5P TROPOMI retrievals of tropospheric BrO together with meteorological simulations by the WRF model and Lagrangian transport simulations of BrO by FLEXPART-WRF are carried out. WRF simulations show, that high tropospheric BrO columns observed by TROPOMI often coincide with areas of high wind speeds. This probably points to release of bromine from blowing snow with cold temperatures favoring the bromine explosion reactions. However, some BrO plumes are observed over areas with very low wind speed and a stable low boundary layer. To monitor the amount of ozone depleted during a BEE, ozone sonde measurements from Ny-Ålesund are compared with MAX-DOAS BrO profiles. First evaluations show a drastic decrease in ozone, partly below the detection limit, while measuring enhanced BrO values at the same time. <span lang="en-US">In order to analyze </span><span lang="en-US">the possible origin</span><span lang="en-US"> of the BrO </span><span lang="en-US">plume </span><span lang="en-US">arriving in </span><span lang="en-US">Ny-</span><span lang="en-US">Å</span><span lang="en-US">lesund</span><span lang="en-US">, </span><span lang="en-US">and to investigate its transportation route, </span><span lang="en-US">FLEXPART-WRF runs are </span><span lang="en-US">executed </span><span lang="en-US">for the times of observed ozone depletion.</span></p> <p align="justify"> </p> <p align="justify"><em>This work was supported by the</em><em> DFG funded Transregio-project TR 172 “Arctic Amplification </em>(AC)<sup>3</sup><em>“.</em></p>

scholarly journals Local Characteristics of the Nocturnal Boundary Layer in Response to External Pressure Forcing

2017 ◽  
Vol 56 (11) ◽  
pp. 3035-3047 ◽  
Author(s):  
Steven J. A. van der Linden ◽  
Peter Baas ◽  
J. Antoon van Hooft ◽  
Ivo G. S. van Hooijdonk ◽  
Fred C. Bosveld ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Stable Boundary Layer ◽  
Dynamical Behavior ◽  
Geostrophic Wind ◽  
External Pressure ◽  
Near Surface ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Turbulent Characteristics

AbstractGeostrophic wind speed data, derived from pressure observations, are used in combination with tower measurements to investigate the nocturnal stable boundary layer at Cabauw, the Netherlands. Since the geostrophic wind speed is not directly influenced by local nocturnal stability, it may be regarded as an external forcing parameter of the nocturnal stable boundary layer. This is in contrast to local parameters such as in situ wind speed, the Monin–Obukhov stability parameter (z/L), or the local Richardson number. To characterize the stable boundary layer, ensemble averages of clear-sky nights with similar geostrophic wind speeds are formed. In this manner, the mean dynamical behavior of near-surface turbulent characteristics and composite profiles of wind and temperature are systematically investigated. The classification is found to result in a gradual ordering of the diagnosed variables in terms of the geostrophic wind speed. In an ensemble sense the transition from the weakly stable to very stable boundary layer is more gradual than expected. Interestingly, for very weak geostrophic winds, turbulent activity is found to be negligibly small while the resulting boundary cooling stays finite. Realistic numerical simulations for those cases should therefore have a comprehensive description of other thermodynamic processes such as soil heat conduction and radiative transfer.

Impact of wind speeds on turbulent transport of carbon dioxide (CO2) fluxes at a tropical location in Ile - Ife, southwest Nigeria

2020 ◽  
Author(s):  
Theodora Bello ◽  
Adewale Ajao ◽  
Oluwagbemiga Jegede
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Land Surface ◽  
Stable Boundary Layer ◽  
Turbulent Transport ◽  
Strong Wind ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Low Wind Speed ◽  
Tropical Area

<p>The study investigates impact of wind speeds on the turbulent transport of CO<sub>2 </sub>fluxes for a land-surface atmosphere interface in a low-wind tropical area between May 28<sup>th</sup> and June 14<sup>th</sup>, 2010; and May 24<sup>th</sup> and June 15<sup>th</sup>, 2015. Eddy covariance technique was used to acquire turbulent mass fluxes of CO<sub>2</sub> and wind speed at the study site located inside the main campus of Obafemi Awolowo University, Ile – Ife, Nigeria. The results showed high levels of CO<sub>2 </sub>fluxes at nighttime attributed to stable boundary layer conditions and low wind speed. Large transport and distribution of CO<sub>2 </sub>fluxes were observed in the early mornings due to strong wind speeds recorded at the study location. In addition, negative CO<sub>2 </sub>fluxes were observed during the daytime attributed to prominent convective and photosynthetic activities. The study concludes there was an inverse relationship between turbulent transport of CO<sub>2 </sub>fluxes and wind speed for daytime period while nighttime CO<sub>2</sub> fluxes showed no significant correlation.</p><p><strong>Keywords</strong>: CO<sub>2 </sub>fluxes, Wind speed, Turbulent transport, Low-wind tropical area, Stable boundary layer</p>

scholarly journals Horizontal-Velocity and Variance Measurements in the Stable Boundary Layer Using Doppler Lidar: Sensitivity to Averaging Procedures

2008 ◽  
Vol 25 (8) ◽  
pp. 1307-1327 ◽  
Author(s):  
Yelena L. Pichugina ◽  
Sara C. Tucker ◽  
Robert M. Banta ◽  
W. Alan Brewer ◽  
Neil D. Kelley ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Sonic Anemometer ◽  
Correlation Coefficients ◽  
Doppler Lidar ◽  
High Wind ◽  
Stable Boundary ◽  
Mean Wind Speed ◽  
The Mean ◽  
Low Level Jet

Abstract Quantitative data on turbulence variables aloft—above the region of the atmosphere conveniently measured from towers—have been an important but difficult measurement need for advancing understanding and modeling of the stable boundary layer (SBL). Vertical profiles of streamwise velocity variances obtained from NOAA’s high-resolution Doppler lidar (HRDL), which have been shown to be approximately equal to turbulence kinetic energy (TKE) for stable conditions, are a measure of the turbulence in the SBL. In the present study, the mean horizontal wind component U and variance σ2u were computed from HRDL measurements of the line-of-sight (LOS) velocity using a method described by Banta et al., which uses an elevation (vertical slice) scanning technique. The method was tested on datasets obtained during the Lamar Low-Level Jet Project (LLLJP) carried out in early September 2003, near the town of Lamar in southeastern Colorado. This paper compares U with mean wind speed obtained from sodar and sonic anemometer measurements. The results for the mean U and mean wind speed measured by sodar and in situ instruments for all nights of LLLJP show high correlation (0.71–0.97), independent of sampling strategies and averaging procedures, and correlation coefficients consistently >0.9 for four high-wind nights, when the low-level jet speeds exceeded 15 m s−1 at some time during the night. Comparison of estimates of variance, on the other hand, proved sensitive to both the spatial and temporal averaging parameters. Several series of averaging tests are described, to find the best correlation between TKE calculated from sonic anemometer data at several tower levels and lidar measurements of horizontal-velocity variance σ2u. Because of the nonstationarity of the SBL data, the best results were obtained when the velocity data were first averaged over intervals of 1 min, and then further averaged over 3–15 consecutive 1-min intervals, with best results for the 10- and 15-min averaging periods. For these cases, correlation coefficients exceeded 0.9. As a part of the analysis, Eulerian integral time scales (τ) were estimated for the four high-wind nights. Time series of τ through each night indicated erratic behavior consistent with the nonstationarity. Histograms of τ showed a mode at 4–5 s, but frequent occurrences of larger τ values, mostly between 10 and 100 s.

scholarly journals Mechanisms for Wind Direction Changes in the Very Stable Boundary Layer

2018 ◽  
Vol 57 (11) ◽  
pp. 2623-2637 ◽  
Author(s):  
D. Finn ◽  
R. M. Eckman ◽  
Z. Gao ◽  
H. Liu
Keyword(s):  
Boundary Layer ◽  
Wind Direction ◽  
Stable Boundary Layer ◽  
Meteorological Factors ◽  
Heat Fluxes ◽  
Tracer Study ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Low Wind Speed ◽  
Low Wind Speeds

AbstractLarge, rapid, and intermittent changes in wind direction were commonly observed in low–wind speed conditions in the very stable boundary layer during the phase 2 of the Project Sagebrush field tracer study. This paper investigates the occurrence and magnitude of these wind direction changes in the very stable boundary layer and explores their associated meteorological factors. The evidence indicates that these wind direction changes occur mainly at wind speeds of less than 1.5 m s−1 and are associated with momentum and sensible heat fluxes approaching zero in low–wind shear conditions. This results in complete vertical decoupling. They are only weakly dependent on the magnitude of turbulence. The magnitude of the wind direction changes is generally greatest near the surface, because of the greater prevalence of low wind speeds there, and decreases upward.

scholarly journals Ventilation of a Mid-Size City under Stable Boundary Layer Conditions: A Simulation Using the LES Model PALM

Atmosphere ◽  
2021 ◽  
Vol 12 (3) ◽  
pp. 401
Author(s):  
Jonathan Biehl ◽  
Bastian Paas ◽  
Otto Klemm
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Passive Scalar ◽  
City Center ◽  
Street Canyons ◽  
Stable Boundary ◽  
Northwest Germany ◽  
Stable Conditions ◽  
Les Model ◽  
The City

City centers have to cope with an increasing amount of air pollution. The supply of fresh air is crucial yet difficult to ensure, especially under stable conditions of the atmospheric boundary layer. This case study used the PArallelized Large eddy simulation (LES) Model PALM to investigate the wind field over an urban lake that had once been built as a designated fresh air corridor for the city center of Münster, northwest, Germany. The model initialization was performed using the main wind direction and stable boundary layer conditions as input. The initial wind and temperature profiles included a weak nocturnal low-level jet. By emitting a passive scalar at one point on top of a bridge, the dispersion of fresh air could be traced over the lake’s surface, within street canyons leading to the city center and within the urban boundary layer above. The concept of city ventilation was confirmed in principle, but the air took a direct route from the shore of the lake to the city center above a former river bed and its adjoining streets rather than through the street canyons. According to the dispersion of the passive scalar, half of the city center was supplied with fresh air originating from the lake. PALM proved to be a useful tool to study fresh air corridors under stable boundary layer conditions.

scholarly journals Thermal Submeso Motions in the Nocturnal Stable Boundary Layer. Part 2: Generating Mechanisms and Implications

2021 ◽  
Author(s):  
Lena Pfister ◽  
Karl Lapo ◽  
Larry Mahrt ◽  
Christoph K. Thomas
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Side Wall ◽  
Cold Pool ◽  
Continuous Data ◽  
Valley Bottom ◽  
Near Surface ◽  
Cold Air ◽  
Stable Boundary ◽  
Surface Temperatures

AbstractIn the stable boundary layer, thermal submesofronts (TSFs) are detected during the Shallow Cold Pool experiment in the Colorado plains, Colorado, USA in 2012. The topography induces TSFs by forming two different air layers converging on the valley-side wall while being stacked vertically above the valley bottom. The warm-air layer is mechanically generated by lee turbulence that consistently elevates near-surface temperatures, while the cold-air layer is thermodynamically driven by radiative cooling and the corresponding cold-air drainage decreases near-surface temperatures. The semi-stationary TSFs can only be detected, tracked, and investigated in detail when using fibre-optic distributed sensing (FODS), as point observations miss TSFs most of the time. Neither the occurrence of TSFs nor the characteristics of each air layer are connected to a specific wind or thermal regime. However, each air layer is characterized by a specific relationship between the wind speed and the friction velocity. Accordingly, a single threshold separating different flow regimes within the boundary layer is an oversimplification, especially during the occurrence of TSFs. No local forcings or their combination could predict the occurrence of TSFs except that they are less likely to occur during stronger near-surface or synoptic-scale flow. While classical conceptualizations and techniques of the boundary layer fail in describing the formation of TSFs, the use of spatially continuous data obtained from FODS provide new insights. Future studies need to incorporate spatially continuous data in the horizontal and vertical planes, in addition to classic sensor networks of sonic anemometry and thermohygrometers to fully characterize and describe boundary-layer phenomena.

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