Investigation of weather conditions and tropospheric BrO transport during Bromine Explosion Events in the Arctic and ozone depletion in Ny-Ålesund observed by satellite and ground-based remote sensing

2021 ◽  
Author(s):  
Bianca Zilker ◽  
Anne-Marlene Blechschmidt ◽  
Sora Seo ◽  
Ilias Bougoudis ◽  
Tim Bösch ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Detection Limit ◽  
Wind Speed ◽  
Ozone Depletion ◽  
Weather Conditions ◽  
Tropospheric Chemistry ◽  
The Arctic ◽  
Blowing Snow ◽  
High Wind ◽  
Wind Speeds

<p align="justify">Bromine Explosion Events (BEEs) have been observed since the late 1990s in the Arctic and Antarctic during polar spring and play an important role in tropospheric chemistry. In a heterogeneous, autocatalytic, chemical chain reaction cycle, inorganic bromine is released from the cryosphere into the troposphere and depletes ozone often to below detection limit. Ozone is a source of the most important tropospheric oxidizing agent OH and the oxidizing capacity and radiative forcing of the troposphere are thus being impacted. Bromine also reacts with gaseous mercury, thereby facilitating the deposition of toxic mercury, which has adverse environmental impacts. C<span lang="en-US">old saline surfaces, such as young sea ice, frost flowers, and snow are likely bromine sources </span><span lang="en-US">during BEEs. </span><span lang="en-US">D</span>ifferent meteorological conditions seem to favor the development of these events: on the one hand, low wind speeds and a stable boundary layer, where bromine can accumulate and deplete ozone, and on the other hand, high wind speeds above approximately 10 m/s with blowing snow and a higher unstable boundary layer. In high wind speed conditions – occurring for example along fronts of polar cyclones – recycling of bromine on snow and aerosol surfaces may take place aloft.</p> <p align="justify">To improve the understanding of weather conditions and bromine sources leading to the development of BEEs, case studies using high resolution S5P TROPOMI retrievals of tropospheric BrO together with meteorological simulations by the WRF model and Lagrangian transport simulations of BrO by FLEXPART-WRF are carried out. WRF simulations show, that high tropospheric BrO columns observed by TROPOMI often coincide with areas of high wind speeds. This probably points to release of bromine from blowing snow with cold temperatures favoring the bromine explosion reactions. However, some BrO plumes are observed over areas with very low wind speed and a stable low boundary layer. To monitor the amount of ozone depleted during a BEE, ozone sonde measurements from Ny-Ålesund are compared with MAX-DOAS BrO profiles. First evaluations show a drastic decrease in ozone, partly below the detection limit, while measuring enhanced BrO values at the same time. <span lang="en-US">In order to analyze </span><span lang="en-US">the possible origin</span><span lang="en-US"> of the BrO </span><span lang="en-US">plume </span><span lang="en-US">arriving in </span><span lang="en-US">Ny-</span><span lang="en-US">Å</span><span lang="en-US">lesund</span><span lang="en-US">, </span><span lang="en-US">and to investigate its transportation route, </span><span lang="en-US">FLEXPART-WRF runs are </span><span lang="en-US">executed </span><span lang="en-US">for the times of observed ozone depletion.</span></p> <p align="justify"> </p> <p align="justify"><em>This work was supported by the</em><em> DFG funded Transregio-project TR 172 “Arctic Amplification </em>(AC)<sup>3</sup><em>“.</em></p>

scholarly journals BrO, blizzards, and drivers of polar tropospheric ozone depletion events

2009 ◽  
Vol 9 (2) ◽  
pp. 8903-8941
Author(s):  
A. E. Jones ◽  
P. S. Anderson ◽  
M. Begoin ◽  
N. Brough ◽  
M. A. Hutterli ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Ozone Depletion ◽  
Stable Boundary Layer ◽  
Weddell Sea ◽  
Blowing Snow ◽  
High Wind ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Global Impacts ◽  
Boundary Layer Ozone

Abstract. The source of bromine that drives polar boundary layer ozone depletion events (ODEs) is still open to some debate. While ODEs are generally noted to form under conditions of a shallow stable boundary layer, observations of depleted air under high wind conditions are taken as being transport-related. Here we report observations from Antarctica in which an unusually large cloud of BrO formed over the Weddell Sea. The enhanced BrO was observed over Halley station in coastal Antarctica, providing an opportunity to probe the conditions within an active "bromine explosion" event. On this occasion, enhanced BrO and depleted boundary layer ozone coincided with high wind speeds and saline blowing snow. We derive a simple model to consider the environmental conditions that favour ODEs and find two maxima, one at low wind/stable boundary layer and one at high wind speeds with blowing snow. Modelling calculations aiming to reproduce the wider regional or global impacts of ODEs, either via radiative effects or as a halogen source, will also need to account for high wind speed mechanisms.

scholarly journals BrO, blizzards, and drivers of polar tropospheric ozone depletion events

2009 ◽  
Vol 9 (14) ◽  
pp. 4639-4652 ◽  
Author(s):  
A. E. Jones ◽  
P. S. Anderson ◽  
M. Begoin ◽  
N. Brough ◽  
M. A. Hutterli ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Ozone Depletion ◽  
Stable Boundary Layer ◽  
Weddell Sea ◽  
Blowing Snow ◽  
High Wind ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Global Impacts ◽  
Boundary Layer Ozone

Abstract. The source of bromine that drives polar boundary layer ozone depletion events (ODEs) is still open to some debate. While ODEs are generally noted to form under conditions of a shallow stable boundary layer, observations of depleted air under high wind conditions are taken as being transport-related. Here we report observations from Antarctica in which an unusually large cloud of BrO formed over the Weddell Sea. The enhanced BrO was observed over Halley station in coastal Antarctica, providing an opportunity to probe the conditions within an active "bromine explosion" event. On this occasion, enhanced BrO and depleted boundary layer ozone coincided with high wind speeds and saline blowing snow. We derive a simple model to consider the environmental conditions that favour ODEs and find two maxima, one at low wind/stable boundary layer and one at high wind speeds with blowing snow. Modelling calculations aiming to reproduce the wider regional or global impacts of ODEs, either via radiative effects or as a halogen source, will also need to account for high wind speed mechanisms.

scholarly journals Catch Characteristics of Precipitation Gauges in High-Latitude Regions with High Winds

2006 ◽  
Vol 7 (5) ◽  
pp. 984-994 ◽  
Author(s):  
Konosuke Sugiura ◽  
Tetsuo Ohata ◽  
Daqing Yang
Keyword(s):  
Wind Speed ◽  
High Latitude ◽  
Cold Climate ◽  
Strong Wind ◽  
Blowing Snow ◽  
High Wind ◽  
Wind Speeds ◽  
Solid Precipitation ◽  
High Winds ◽  
Correction Equations

Abstract Intercomparison of solid precipitation measurement at Barrow, Alaska, has been carried out to examine the catch characteristics of various precipitation gauges in high-latitude regions with high winds and to evaluate the applicability of the WMO precipitation correction procedures. Five manual precipitation gauges (Canadian Nipher, Hellmann, Russian Tretyakov, U.S. 8-in., and Wyoming gauges) and a double fence intercomparison reference (DFIR) as an international reference standard have been installed. The data collected in the last three winters indicates that the amount of solid precipitation is characteristically low, and the zero-catch frequency of the nonshielded gauges is considerably high, 60%–80% of precipitation occurrences. The zero catch in high-latitude high-wind regions becomes a significant fraction of the total precipitation. At low wind speeds, the catch characteristics of the gauges are roughly similar to the DFIR, although it is noteworthy that the daily catch ratios decreased more rapidly with increasing wind speed compared to the WMO correction equations. The dependency of the daily catch ratios on air temperature was confirmed, and the rapid decrease in the daily catch ratios is due to small snow particles caused by the cold climate. The daily catch ratio of the Wyoming gauge clearly shows wind-induced losses. In addition, the daily catch ratios are considerably scattered under strong wind conditions due to the influence of blowing snow. This result suggests that it is not appropriate to extrapolate the WMO correction equations for the shielded gauges in high-latitude regions for high wind speed of over 6 m s−1.

scholarly journals The Effect of Blowing Snow on Katabatic Winds in Antarctica

1985 ◽  
Vol 6 ◽  
pp. 59-62 ◽  
Author(s):  
Yuji Kodama ◽  
Gerd Wendler ◽  
Joan Gosink
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Atmospheric Boundary Layer ◽  
Geostrophic Wind ◽  
Blowing Snow ◽  
Katabatic Winds ◽  
Wind Speeds ◽  
Weather Stations ◽  
The Difference ◽  
The Relationship

An acceleration of the katabatic winds during periods of blowing snow was observed in Adelie Land, Antarctica. Data collected by Automatic Weather Stations' (AWS) showed a change in the relationship between the katabatic term of the surface geostrophic wind (katabatic force) and the wind speed for periods of blowing snow. When measurements of the katabatic force were plotted against the cube of the wind speed, the slope was steeper for wind speeds at less than a threshold speed for blowing snow. The difference between these two slopes was partly explained by the effect of blowing snow entrained into the atmospheric boundary layer.

scholarly journals The Effect of Blowing Snow on Katabatic Winds in Antarctica

1985 ◽  
Vol 6 ◽  
pp. 59-62 ◽  
Author(s):  
Yuji Kodama ◽  
Gerd Wendler ◽  
Joan Gosink
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Atmospheric Boundary Layer ◽  
Geostrophic Wind ◽  
Blowing Snow ◽  
Katabatic Winds ◽  
Wind Speeds ◽  
Weather Stations ◽  
The Difference ◽  
The Relationship

An acceleration of the katabatic winds during periods of blowing snow was observed in Adelie Land, Antarctica. Data collected by Automatic Weather Stations' (AWS) showed a change in the relationship between the katabatic term of the surface geostrophic wind (katabatic force) and the wind speed for periods of blowing snow. When measurements of the katabatic force were plotted against the cube of the wind speed, the slope was steeper for wind speeds at less than a threshold speed for blowing snow. The difference between these two slopes was partly explained by the effect of blowing snow entrained into the atmospheric boundary layer.

scholarly journals A social Beaufort scale to detect high winds using language in social media posts

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Iain S. Weaver ◽  
Hywel T. P. Williams ◽  
Rudy Arthur
Keyword(s):  
Social Media ◽  
Wind Speed ◽  
Temporal Correlation ◽  
Weather Conditions ◽  
Local Area ◽  
High Wind ◽  
Wind Speeds ◽  
The Uk ◽  
The Relationship ◽  
High Winds

AbstractPeople often talk about the weather on social media, using different vocabulary to describe different conditions. Here we combine a large collection of wind-related Twitter posts (tweets) and UK Met Office wind speed observations to explore the relationship between tweet volume, tweet language and wind speeds in the UK. We find that wind speeds are experienced subjectively relative to the local baseline, so that the same absolute wind speed is reported as stronger or weaker depending on the typical weather conditions in the local area. Different linguistic tokens (words and emojis) are associated with different wind speeds. These associations can be used to create a simple text classifier to detect ‘high-wind’ tweets with reasonable accuracy; this can be used to detect high winds in a locality using only a single tweet. We also construct a ‘social Beaufort scale’ to infer wind speeds based only on the language used in tweets. Together with the classifier, this demonstrates that language alone is indicative of weather conditions, independent of tweet volume. However, the number of high-wind tweets shows a strong temporal correlation with local wind speeds, increasing the ability of a combined language-plus-volume system to successfully detect high winds. Our findings complement previous work in social sensing of weather hazards that has focused on the relationship between tweet volume and severity. These results show that impacts of wind and storms are found in how people communicate and use language, a novel dimension in understanding the social impacts of extreme weather.

scholarly journals An exemplary case of a bromine explosion event linked to cyclone development in the Arctic

2016 ◽  
Vol 16 (3) ◽  
pp. 1773-1788 ◽  
Author(s):  
A.-M. Blechschmidt ◽  
A. Richter ◽  
J. P. Burrows ◽  
L. Kaleschke ◽  
K. Strong ◽  
...  
Keyword(s):  
Numerical Models ◽  
Weather Conditions ◽  
Conveyor Belt ◽  
Arctic Sea Ice ◽  
The Arctic ◽  
Blowing Snow ◽  
Air Stream ◽  
Combined Use ◽  
Arctic Sea ◽  
Development Duration

Abstract. Intense, cyclone-like shaped plumes of tropospheric bromine monoxide (BrO) are regularly observed by GOME-2 on board the MetOp-A satellite over Arctic sea ice in polar spring. These plumes are often transported by high-latitude cyclones, sometimes over several days despite the short atmospheric lifetime of BrO. However, only few studies have focused on the role of polar weather systems in the development, duration and transport of tropospheric BrO plumes during bromine explosion events. The latter are caused by an autocatalytic chemical chain reaction associated with tropospheric ozone depletion and initiated by the release of bromine from cold brine-covered ice or snow to the atmosphere. In this manuscript, a case study investigating a comma-shaped BrO plume which developed over the Beaufort Sea and was observed by GOME-2 for several days is presented. By making combined use of satellite data and numerical models, it is shown that the occurrence of the plume was closely linked to frontal lifting in a polar cyclone and that it most likely resided in the lowest 3 km of the troposphere. In contrast to previous case studies, we demonstrate that the dry conveyor belt, a potentially bromine-rich stratospheric air stream which can complicate interpretation of satellite retrieved tropospheric BrO, is spatially separated from the observed BrO plume. It is concluded that weather conditions associated with the polar cyclone favoured the bromine activation cycle and blowing snow production, which may have acted as a bromine source during the bromine explosion event.

scholarly journals Evaluation of the AMPS Boundary Layer Simulations on the Ross Ice Shelf, Antarctica, with Unmanned Aircraft Observations

2017 ◽  
Vol 56 (8) ◽  
pp. 2239-2258 ◽  
Author(s):  
Jonathan D. Wille ◽  
David H. Bromwich ◽  
John J. Cassano ◽  
Melissa A. Nigro ◽  
Marian E. Mateling ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Relative Humidity ◽  
High Wind ◽  
Ice Shelf ◽  
High Wind Speed ◽  
Near Surface ◽  
Ross Ice Shelf ◽  
Low Cloud ◽  
The Antarctic

AbstractAccurately predicting moisture and stability in the Antarctic planetary boundary layer (PBL) is essential for low-cloud forecasts, especially when Antarctic forecasters often use relative humidity as a proxy for cloud cover. These forecasters typically rely on the Antarctic Mesoscale Prediction System (AMPS) Polar Weather Research and Forecasting (Polar WRF) Model for high-resolution forecasts. To complement the PBL observations from the 30-m Alexander Tall Tower! (ATT) on the Ross Ice Shelf as discussed in a recent paper by Wille and coworkers, a field campaign was conducted at the ATT site from 13 to 26 January 2014 using Small Unmanned Meteorological Observer (SUMO) aerial systems to collect PBL data. The 3-km-resolution AMPS forecast output is combined with the global European Centre for Medium-Range Weather Forecasts interim reanalysis (ERAI), SUMO flights, and ATT data to describe atmospheric conditions on the Ross Ice Shelf. The SUMO comparison showed that AMPS had an average 2–3 m s−1 high wind speed bias from the near surface to 600 m, which led to excessive mechanical mixing and reduced stability in the PBL. As discussed in previous Polar WRF studies, the Mellor–Yamada–Janjić PBL scheme is likely responsible for the high wind speed bias. The SUMO comparison also showed a near-surface 10–15-percentage-point dry relative humidity bias in AMPS that increased to a 25–30-percentage-point deficit from 200 to 400 m above the surface. A large dry bias at these critical heights for aircraft operations implies poor AMPS low-cloud forecasts. The ERAI showed that the katabatic flow from the Transantarctic Mountains is unrealistically dry in AMPS.

scholarly journals Atmospheric Circulation Effects on Wind Speed Variability at Turbine Height

2007 ◽  
Vol 46 (4) ◽  
pp. 445-456 ◽  
Author(s):  
Katherine Klink
Keyword(s):  
Wind Speed ◽  
Pressure Gradient ◽  
Large Scale ◽  
Ground Level ◽  
The Arctic ◽  
Circulation Index ◽  
Regression Equations ◽  
Change Models ◽  
Wind Speeds ◽  
The North

Abstract Mean monthly wind speed at 70 m above ground level is investigated for 11 sites in Minnesota for the period 1995–2003. Wind speeds at these sites show significant spatial and temporal coherence, with prolonged periods of above- and below-normal values that can persist for as long as 12 months. Monthly variation in wind speed primarily is determined by the north–south pressure gradient, which captures between 22% and 47% of the variability (depending on the site). Regression on wind speed residuals (pressure gradient effects removed) shows that an additional 6%–15% of the variation can be related to the Arctic Oscillation (AO) and Niño-3.4 sea surface temperature (SST) anomalies. Wind speeds showed little correspondence with variation in the Pacific–North American (PNA) circulation index. The effect of the strong El Niño of 1997/98 on the wind speed time series was investigated by recomputing the regression equations with this period excluded. The north–south pressure gradient remains the primary determinant of mean monthly 70-m wind speeds, but with 1997/98 removed the influence of the AO increases at nearly all stations while the importance of the Niño-3.4 SSTs generally decreases. Relationships with the PNA remain small. These results suggest that long-term patterns of low-frequency wind speed (and thus wind power) variability can be estimated using large-scale circulation features as represented by large-scale climatic datasets and by climate-change models.

scholarly journals Local Characteristics of the Nocturnal Boundary Layer in Response to External Pressure Forcing

2017 ◽  
Vol 56 (11) ◽  
pp. 3035-3047 ◽  
Author(s):  
Steven J. A. van der Linden ◽  
Peter Baas ◽  
J. Antoon van Hooft ◽  
Ivo G. S. van Hooijdonk ◽  
Fred C. Bosveld ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Stable Boundary Layer ◽  
Dynamical Behavior ◽  
Geostrophic Wind ◽  
External Pressure ◽  
Near Surface ◽  
Stable Boundary ◽  
Wind Speeds ◽  
Turbulent Characteristics

AbstractGeostrophic wind speed data, derived from pressure observations, are used in combination with tower measurements to investigate the nocturnal stable boundary layer at Cabauw, the Netherlands. Since the geostrophic wind speed is not directly influenced by local nocturnal stability, it may be regarded as an external forcing parameter of the nocturnal stable boundary layer. This is in contrast to local parameters such as in situ wind speed, the Monin–Obukhov stability parameter (z/L), or the local Richardson number. To characterize the stable boundary layer, ensemble averages of clear-sky nights with similar geostrophic wind speeds are formed. In this manner, the mean dynamical behavior of near-surface turbulent characteristics and composite profiles of wind and temperature are systematically investigated. The classification is found to result in a gradual ordering of the diagnosed variables in terms of the geostrophic wind speed. In an ensemble sense the transition from the weakly stable to very stable boundary layer is more gradual than expected. Interestingly, for very weak geostrophic winds, turbulent activity is found to be negligibly small while the resulting boundary cooling stays finite. Realistic numerical simulations for those cases should therefore have a comprehensive description of other thermodynamic processes such as soil heat conduction and radiative transfer.

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