scholarly journals Theoretical basis for convective invigoration due to increased aerosol concentration

2011 ◽  
Vol 11 (1) ◽  
pp. 2773-2842 ◽  
Author(s):  
Z. J. Lebo ◽  
J. H. Seinfeld
Keyword(s):  
Cloud Microphysics ◽  
Number Concentration ◽  
Latent Heating ◽  
Microphysics Scheme ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Significant Difference ◽  
Deep Convective Clouds ◽  
Bin Microphysics ◽  
Cumulative Precipitation

Abstract. The potential effects of increased aerosol loading on the development of deep convective clouds and resulting precipitation amounts are studied by employing the Weather Research and Forecasting (WRF) model as a detailed high-resolution cloud resolving model (CRM) with both detailed bulk and bin microphysics schemes. The bulk microphysics scheme incorporates a physically based parameterization of cloud droplet activation as well as homogeneous and heterogeneous freezing in order to explicitly resolve the possible aerosol-induced effects on the cloud microphysics. These parameterizations allow one to segregate the effects of an increase in the aerosol number concentration into enhanced cloud condensation nuclei (CCN) and/or ice nuclei (IN) concentrations using bulk microphysics. The bin microphysics scheme, with its explicit calculations of cloud particle collisions, is shown to better predict cumulative precipitation. Increases in the CCN number concentration may not have a monotonic influence on the cumulative precipitation resulting from deep convective clouds. We demonstrate that the aerosol-induced effect is controlled by the balance between latent heating and the increase in condensed water aloft, each having opposing effects on buoyancy. It is also shown that under polluted conditions and in relatively dry environments, increases in the CCN number concentration reduce the cumulative precipitation due to the competition between the sedimentation and evaporation/sublimation timescales. The effect of an increase in the IN number concentration on the dynamics of deep convective clouds is small, but may act to suppress precipitation. A comparison of the predictions using the bin and bulk microphysics schemes demonstrate a significant difference between the predicted precipitation and the influence of aerosol perturbations on updraft velocity within the convective core. The bulk microphysics scheme is shown to be unable to capture the changes in latent heating that occur as a result of changes in the CCN number concentration, while the bin microphysics scheme demonstrates significant increases in the latent heating aloft with increasing CCN number concentration. This suggests that a detailed two-bulk microphysics scheme, which is more computationally efficient than bin microphysics schemes, may not be sufficient, even when coupled to a detailed activation scheme, to predict small changes that result from perturbations in aerosol loading.

scholarly journals Theoretical basis for convective invigoration due to increased aerosol concentration

2011 ◽  
Vol 11 (11) ◽  
pp. 5407-5429 ◽  
Author(s):  
Z. J. Lebo ◽  
J. H. Seinfeld
Keyword(s):  
Number Concentration ◽  
Latent Heating ◽  
Heating Rates ◽  
Microphysics Scheme ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Significant Difference ◽  
Deep Convective Clouds ◽  
Bin Microphysics ◽  
Cumulative Precipitation

Abstract. The potential effects of increased aerosol loading on the development of deep convective clouds and resulting precipitation amounts are studied by employing the Weather Research and Forecasting (WRF) model as a detailed high-resolution cloud resolving model (CRM) with both detailed bulk and bin microphysics schemes. Both models include a physically-based activation scheme that incorporates a size-resolved aerosol population. We demonstrate that the aerosol-induced effect is controlled by the balance between latent heating and the increase in condensed water aloft, each having opposing effects on buoyancy. It is also shown that under polluted conditions, increases in the CCN number concentration reduce the cumulative precipitation due to the competition between the sedimentation and evaporation/sublimation timescales. The effect of an increase in the IN number concentration on the dynamics of deep convective clouds is small and the resulting decrease in domain-averaged cumulative precipitation is shown not to be statistically significant, but may act to suppress precipitation. It is also shown that even in the presence of a decrease in the domain-averaged cumulative precipitation, an increase in the precipitation variance, or in other words, andincrease in rainfall intensity, may be expected in more polluted environments, especially in moist environments. A significant difference exists between the predictions based on the bin and bulk microphysics schemes of precipitation and the influence of aerosol perturbations on updraft velocity within the convective core. The bulk microphysics scheme shows little change in the latent heating rates due to an increase in the CCN number concentration, while the bin microphysics scheme demonstrates significant increases in the latent heating aloft with increasing CCN number concentration. This suggests that even a detailed two-bulk microphysics scheme, coupled to a detailed activation scheme, may not be sufficient to predict small changes that result from perturbations in aerosol loading.

scholarly journals Are simulated aerosol-induced effects on deep convective clouds strongly dependent on saturation adjustment?

2012 ◽  
Vol 12 (4) ◽  
pp. 10059-10114 ◽  
Author(s):  
Z. J. Lebo ◽  
H. Morrison ◽  
J. H. Seinfeld
Keyword(s):  
Mass Flux ◽  
Cold Pool ◽  
Latent Heating ◽  
Time Step ◽  
Microphysics Scheme ◽  
Surface Precipitation ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Deep Convective Clouds ◽  
Bulk Model

Abstract. Three configurations of a bulk microphysics scheme in conjunction with a detailed bin scheme are implemented in the Weather Research and Forecasting (WRF) model to specifically address the role of the saturation adjustment assumption (i.e., condensing/evaporating the surplus/deficit water vapor relative to saturation in one time step) on aerosol-induced invigoration of deep convective clouds. The bulk model configurations are designed to treat cloud droplet condensation/evaporation using either saturation adjustment, as employed in most bulk models, or an explicit representation of supersaturation over a time step, as used in bin models. Results demonstrate that the use of saturation adjustment artificially enhances condensation and latent heating at low levels and limits the potential for an increase in aerosol concentration to increase buoyancy at mid to upper levels. This leads to a small weakening of the time- and domain-averaged convective mass flux (~ -3%) in polluted compared to clean conditions. In contrast, the bin model and bulk scheme with explicit prediction of supersaturation simulate an increase in latent heating aloft and the convective updraft mass flux is weakly invigorated (~5%). The bin model also produces a large increase in domain-mean cumulative surface precipitation in polluted conditions (~18%), while all of the bulk model configurations simulate little change in precipitation. Finally, it is shown that the cold pool weakens substantially with increased aerosol loading when saturation adjustment is applied, which acts to reduce the low-level convergence and weaken the convective dynamics. With an explicit treatment of supersaturation in the bulk and bin models there is little change in cold pool strength, so that the convective response to polluted conditions is influenced more by changes in latent heating aloft. It is concluded that the use of saturation adjustment can explain differences in the response of cold pool evolution and convective dynamics with aerosol loading simulated by the bulk and bin models, but cannot explain large differences in the response of surface precipitation between these models.

scholarly journals Sensitivity study of the aerosol effects on a supercell storm throughout its lifetime

2014 ◽  
Vol 14 (17) ◽  
pp. 24087-24118 ◽  
Author(s):  
A. Takeishi ◽  
T. Storelvmo
Keyword(s):  
Droplet Size ◽  
Cloud Condensation Nuclei ◽  
Wrf Model ◽  
Convective Cloud ◽  
Sensitivity Study ◽  
Cloud Microphysics ◽  
Microphysics Scheme ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Deep Convective Clouds

Abstract. An increase in atmospheric aerosol loading could alter the microphysics, dynamics, and radiative characteristics of deep convective clouds. Earlier modeling studies have shown that the effects of increased aerosols on the amount of precipitation from deep convective clouds are model-dependent. This study aims to understand the effects of increased aerosol loading on a deep convective cloud throughout its lifetime with the use of the Weather Research and Forecasting (WRF) model as a cloud-resolving model (CRM). It simulates an idealized supercell thunderstorm with 8 different aerosol loadings, for three different cloud microphysics schemes. Variation in aerosol concentration is mimicked by varying either cloud droplet number concentration or the number of activated cloud condensation nuclei. We show that the sensitivity to aerosol loading is dependent on the choice of microphysics scheme. For the schemes that are sensitive to aerosols loading, the production of graupel via riming of snow is the key factor determining the precipitation response. The formulation of snow riming depends on the microphysics scheme and is usually a function of two competing effects, the size effect and the number effect. In many simulations, a decrease in riming is seen with increased aerosol loading, due to the decreased droplet size that lowers the riming efficiency drastically. This decrease in droplet size also results in a delay in the onset of precipitation, as well as so-called warm rain suppression. Although these characteristics of convective invigoration (Rosenfeld et al., 2008) are seen in the first few hours of the simulations, variation in the accumulated precipitation mainly stems from graupel production rather than convective invigoration. These results emphasize the importance of accurate representations of graupel formation in microphysics schemes.

scholarly journals Non-Monotonic Dependencies of Cloud Microphysics and Precipitation on Aerosol Loading in Deep Convective Clouds: A Case Study Using the WRF Model with Bin Microphysics

Atmosphere ◽  
2018 ◽  
Vol 9 (11) ◽  
pp. 434 ◽  
Author(s):  
Ye-Lim Jeon ◽  
Sungju Moon ◽  
Hyunho Lee ◽  
Jong-Jin Baik ◽  
Jambajamts Lkhamjav
Keyword(s):  
Precipitation Amount ◽  
Cloud Microphysics ◽  
Ice Crystals ◽  
Precipitation Event ◽  
Cold Pool ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Optimal Value ◽  
Deep Convective Clouds ◽  
Bin Microphysics

Aerosol-cloud-precipitation interactions in deep convective clouds are investigated through numerical simulations of a heavy precipitation event over South Korea on 15–16 July 2017. The Weather Research and Forecasting model with a bin microphysics scheme is used, and various aerosol number concentrations in the range N0 = 50–12,800 cm−3 are considered. Precipitation amount changes non-monotonically with increasing aerosol loading, with a maximum near a moderate aerosol loading (N0 = 800 cm−3). Up to this optimal value, an increase in aerosol number concentration results in a greater quantity of small droplets formed by nucleation, increasing the number of ice crystals. Ice crystals grow into snow particles through deposition and riming, leading to enhanced melting and precipitation. Beyond the optimal value, a greater aerosol loading enhances generation of ice crystals while the overall growth of ice hydrometeors through deposition stagnates. Subsequently, the riming rate decreases because of the smaller size of snow particles and supercooled drops, leading to a decrease in ice melting and a slight suppression of precipitation. As aerosol loading increases, cold pool and low-level convergence strengthen monotonically, but cloud development is more strongly affected by latent heating and convection within the system that is non-monotonically reinforced.

scholarly journals Are simulated aerosol-induced effects on deep convective clouds strongly dependent on saturation adjustment?

2012 ◽  
Vol 12 (20) ◽  
pp. 9941-9964 ◽  
Author(s):  
Z. J. Lebo ◽  
H. Morrison ◽  
J. H. Seinfeld
Keyword(s):  
Mass Flux ◽  
Cold Pool ◽  
Latent Heating ◽  
Time Step ◽  
Microphysics Scheme ◽  
Surface Precipitation ◽  
Convective Clouds ◽  
Aerosol Loading ◽  
Deep Convective Clouds ◽  
Bulk Model

Abstract. Three configurations of a bulk microphysics scheme in conjunction with a detailed bin scheme are implemented in the Weather Research and Forecasting (WRF) model to specifically address the role of the saturation adjustment assumption (i.e., condensing/evaporating the surplus/deficit water vapor relative to saturation in one time step) on aerosol-induced invigoration of deep convective clouds. The bulk model configurations are designed to treat cloud droplet condensation/evaporation using either saturation adjustment, as employed in most bulk models, or an explicit representation of supersaturation over a time step, as used in bin models. Results demonstrate that the use of saturation adjustment artificially enhances condensation and latent heating at low levels and limits the potential for an increase in aerosol concentration to increase buoyancy at mid to upper levels. This leads to a small weakening of the time- and domain-averaged convective mass flux (~-3%) in polluted compared to clean conditions. In contrast, the bin model and bulk scheme with explicit prediction of supersaturation simulate an increase in latent heating aloft and the convective updraft mass flux is weakly invigorated (~5%). The bin model also produces a large increase in domain-mean cumulative surface precipitation in polluted conditions (~18%), while all of the bulk model configurations simulate little change in precipitation. Finally, it is shown that the cold pool weakens substantially with increased aerosol loading when saturation adjustment is applied, which acts to reduce the low-level convergence and weaken the convective dynamics. With an explicit treatment of supersaturation in the bulk and bin models there is little change in cold pool strength, so that the convective response to polluted conditions is influenced more by changes in latent heating aloft. It is concluded that the use of saturation adjustment can explain differences in the response of cold pool evolution and convective dynamics with aerosol loading simulated by the bulk and bin models, but cannot explain large differences in the response of surface precipitation between these models.

scholarly journals Aerosol effects on deep convection: the propagation of aerosol perturbations through convective cloud microphysics

2019 ◽  
Vol 19 (4) ◽  
pp. 2601-2627 ◽  
Author(s):  
Max Heikenfeld ◽  
Bethan White ◽  
Laurent Labbouz ◽  
Philip Stier
Keyword(s):  
Latent Heat ◽  
Cloud Condensation Nuclei ◽  
Cloud Microphysics ◽  
Latent Heating ◽  
Microphysics Scheme ◽  
Convective Clouds ◽  
Wide Range ◽  
Microphysical Processes ◽  
Aerosol Effects ◽  
The Impact

Abstract. The impact of aerosols on ice- and mixed-phase processes in deep convective clouds remains highly uncertain, and the wide range of interacting microphysical processes is still poorly understood. To understand these processes, we analyse diagnostic output of all individual microphysical process rates for two bulk microphysics schemes in the Weather and Research Forecasting model (WRF). We investigate the response of individual processes to changes in aerosol conditions and the propagation of perturbations through the microphysics all the way to the macrophysical development of the convective clouds. We perform simulations for two different cases of idealised supercells using two double-moment bulk microphysics schemes and a bin microphysics scheme. The simulations cover a comprehensive range of values for cloud droplet number concentration (CDNC) and cloud condensation nuclei (CCN) concentration as a proxy for aerosol effects on convective clouds. We have developed a new cloud tracking algorithm to analyse the morphology and time evolution of individually tracked convective cells in the simulations and their response to the aerosol perturbations. This analysis confirms an expected decrease in warm rain formation processes due to autoconversion and accretion for more polluted conditions. There is no evidence of a significant increase in the total amount of latent heat, as changes to the individual components of the integrated latent heating in the cloud compensate each other. The latent heating from freezing and riming processes is shifted to a higher altitude in the cloud, but there is no significant change to the integrated latent heat from freezing. Different choices in the treatment of deposition and sublimation processes between the microphysics schemes lead to strong differences including feedbacks onto condensation and evaporation. These changes in the microphysical processes explain some of the response in cloud mass and the altitude of the cloud centre of gravity. However, there remain some contrasts in the development of the bulk cloud parameters between the microphysics schemes and the two simulated cases.

scholarly journals The propagation of aerosol perturbations in convective cloud microphysics

2018 ◽  
Author(s):  
Max Heikenfeld ◽  
Bethan White ◽  
Laurent Labbouz ◽  
Philip Stier
Keyword(s):  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
Convective Cloud ◽  
Cloud Microphysics ◽  
Number Concentration ◽  
Microphysics Scheme ◽  
Microphysical Process ◽  
Convective Clouds ◽  
Wide Range ◽  
The Impact

Abstract. The impact of aerosols on ice- and mixed-phase processes in deep convective clouds remains highly uncertain and the wide range of interacting microphysical processes are still poorly understood. To understand these processes, we analyse diagnostic output of all individual microphysical process rates for two cloud microphysics schemes in the Weather and Research Forecasting model (WRF). We investigate the response of individual processes to changes in aerosol conditions and the propagation of perturbations through the microphysics all the way to the macrophysical development of the convective clouds. We perform simulations for two different cases of idealised supercells using two double-moment bulk microphysics schemes and a bin microphysics scheme. We use simulations with a comprehensive range of values for cloud droplet number concentration (CDNC) and cloud condensation nuclei (CCN) concentration as a proxy for aerosol effects on convective clouds. We have developed a new cloud tracking algorithm to analyse the morphology and time evolution of individually tracked convective cells in the simulations and their response to the aerosol perturbations. This analysis confirms an expected decrease in warm rain formation processes due to autoconversion and accretion for polluted conditions. The height at which the freezing occurs increases with increasing CDNC. However, there is no evidence of a significant increase in the total amount of latent heat release from freezing and riming. The cloud mass and the altitude of the cloud centre of gravity show contrasting responses to changes in proxies for aerosol number concentration between the different microphysics schemes.

Microphysical Processes Evident in Aerosol Forcing of Tropical Deep Convective Clouds

2013 ◽  
Vol 70 (2) ◽  
pp. 430-446 ◽  
Author(s):  
Rachel L. Storer ◽  
Susan C. van den Heever
Keyword(s):  
Vertical Velocity ◽  
Large Scale ◽  
Extreme Values ◽  
Cloud Microphysics ◽  
Aerosol Concentration ◽  
Convective Precipitation ◽  
Latent Heating ◽  
Convective Clouds ◽  
Budget Analysis ◽  
Deep Convective Clouds

Abstract This study investigates the effects of aerosols on tropical deep convective clouds (DCCs). A series of large-scale, two-dimensional cloud-resolving model simulations was completed, differing only in the concentration of aerosols available to act as cloud condensation nuclei (CCN). Polluted simulations contained more DCCs, wider storms, higher cloud tops, and more convective precipitation domainwide. Differences in warm cloud microphysics were largely consistent with the first and second aerosol indirect effects. The average surface precipitation produced in each DCC column decreased with increasing aerosol concentration. A detailed microphysical budget analysis showed that the reduction in collision and coalescence largely dominated the trend in average precipitation. The production of rain from ice, though it also decreased, became a more important contribution to precipitation as the aerosol concentration increased. The DCCs in polluted simulations contained more frequent extreme values of vertical velocity, but the average updraft speed decreased with increasing aerosols in DCCs above 6 km. An examination of the buoyancy term of the vertical velocity equation demonstrates that the drag associated with condensate loading is an important factor in determining the average updraft strength. The largest contributions to latent heating in DCCs were cloud nucleation and vapor deposition onto water and ice, but changes in latent heating were, on average, an order of magnitude smaller than those in the condensate loading term. The average updraft speed was largely affected by increased drag from condensate loading in more mature updrafts, while early storm updrafts experienced convective invigoration from increased latent heating.

scholarly journals Tropical deep convective life cycle: Cb-anvil cloud microphysics from high-altitude aircraft observations

2014 ◽  
Vol 14 (23) ◽  
pp. 13223-13240 ◽  
Author(s):  
W. Frey ◽  
S. Borrmann ◽  
F. Fierli ◽  
R. Weigel ◽  
V. Mitev ◽  
...  
Keyword(s):  
Life Cycle ◽  
High Altitude ◽  
Potential Temperature ◽  
Cloud Microphysics ◽  
Mature Stage ◽  
Convective System ◽  
Ice Crystal ◽  
Convective Clouds ◽  
Tropical Tropopause ◽  
Deep Convective Clouds

Abstract. The case study presented here focuses on the life cycle of clouds in the anvil region of a tropical deep convective system. During the SCOUT-O3 campaign from Darwin, Northern Australia, the Hector storm system has been probed by the Geophysica high-altitude aircraft. Clouds were observed by in situ particle probes, a backscatter sonde, and a miniature lidar. Additionally, aerosol number concentrations have been measured. On 30 November 2005 a double flight took place and Hector was probed throughout its life cycle in its developing, mature, and dissipating stage. The two flights were four hours apart and focused on the anvil region of Hector in altitudes between 10.5 and 18.8 km (i.e. above 350 K potential temperature). Trajectory calculations, satellite imagery, and ozone measurements have been used to ensure that the same cloud air masses have been probed in both flights. The size distributions derived from the measurements show a change not only with increasing altitude but also with the evolution of Hector. Clearly different cloud to aerosol particle ratios as well as varying ice crystal morphology have been found for the different development stages of Hector, indicating different freezing mechanisms. The development phase exhibits the smallest ice particles (up to 300 μm) with a rather uniform morphology. This is indicative for rapid glaciation during Hector's development. Sizes of ice crystals are largest in the mature stage (larger than 1.6 mm) and even exceed those of some continental tropical deep convective clouds, also in their number concentrations. The backscatter properties and particle images show a change in ice crystal shape from the developing phase to rimed and aggregated particles in the mature and dissipating stages; the specific shape of particles in the developing phase cannot be distinguished from the measurements. Although optically thin, the clouds in the dissipating stage have a large vertical extent (roughly 6 km) and persist for at least 6 h. Thus, the anvils of these high-reaching deep convective clouds have a high potential for affecting the tropical tropopause layer by modifying the humidity and radiative budget, as well as for providing favourable conditions for subvisible cirrus formation. The involved processes may also influence the amount of water vapour that ultimately reaches the stratosphere in the tropics.

scholarly journals Quantifying the aerosol effect on droplet size distribution at cloud-top

2018 ◽  
Author(s):  
Lianet Hernández Pardo ◽  
Luiz Augusto Toledo Machado ◽  
Micael Amore Cecchini ◽  
Madeleine Sánchez Gácita
Keyword(s):  
Size Distribution ◽  
Initial Conditions ◽  
Droplet Size Distribution ◽  
Cloud Microphysics ◽  
Number Concentration ◽  
Population Characteristics ◽  
Aerosol Size Distribution ◽  
Effective Diameter ◽  
Bin Microphysics ◽  
Aerosol Properties

Abstract. This work uses the number concentration-effective diameter phase-space to test cloud sensitivity to variations in the aerosol population characteristics, such as the aerosol size distribution, number concentration and hygroscopicity. It is based on the information from the top of a cloud simulated by a bin-microphysics single-column model, for initial conditions typical of the Amazon. It is shown that the cloud-top evolution can be very sensitive to aerosol properties, but the relative importance of each parameter is variable. The sensitivity to each aerosol characteristic varies as a function of the tested parameter and is conditioned by the base values of the other parameters. The median radius of the aerosols showed the largest influence on this sensitivity. We show that all aerosol properties can have significant impacts on cloud microphysics, especially if the median radius of the aerosol size distribution is smaller than 0.05 μm.

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