scholarly journals Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia

2015 ◽  
Vol 15 (24) ◽  
pp. 35591-35643 ◽  
Author(s):  
X. Dong ◽  
J. S. Fu ◽  
K. Huang ◽  
D. Tong
Keyword(s):  
Soil Moisture ◽  
Air Quality ◽  
East Asia ◽  
Model Development ◽  
Dust Emission ◽  
Temporal Variations ◽  
Heterogeneous Chemistry ◽  
Dust Aerosols ◽  
Meteorological Simulation ◽  
The Impact

Abstract. The Community Multiscale Air Quality (CMAQ) model has been further developed in terms of simulating natural wind-blown dust in this study, with a series of modifications aimed at improving the model's capability to predict the emission, transport, and chemical reactions of dust aerosols. The default parameterization of threshold friction velocity constants in the CMAQ are revised to avoid double counting of the impact of soil moisture based on the re-analysis of field experiment data; source-dependent speciation profiles for dust emission are derived based on local measurements for the Gobi and Taklamakan deserts in East Asia; and dust heterogeneous chemistry is implemented to simulate the reactions involving dust aerosol. The improved dust module in the CMAQ was applied over East Asia for March and April from 2006 to 2010. Evaluation against observations has demonstrated that simulation bias of PM10 and aerosol optical depth (AOD) is reduced from −55.42 and −31.97 % in the original CMAQ to −16.05 and −22.1 % in the revised CMAQ, respectively. Comparison with observations at the nearby Gobi stations of Duolun and Yulin indicates that applying a source-dependent profile helps reduce simulation bias for trace metals. Implementing heterogeneous chemistry is also found to result in better agreement with observations for sulfur dioxide (SO2), sulfate (SO42-), nitric acid (HNO3), nitrous oxides (NOx), and nitrate (NO3-). Investigation of a severe dust storm episode from 19 to 21 March 2010 suggests that the revised CMAQ is capable of capturing the spatial distribution and temporal variations of dust aerosols. Model evaluation indicates potential uncertainties within the excessive soil moisture fraction used by meteorological simulation. The mass contribution of fine mode aerosol in dust emission may be underestimated by 50 %. The revised revised CMAQ provides a useful tool for future studies to investigate the emission, transport, and impact of wind-blown dust over East Asia and elsewhere.

scholarly journals Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia

2016 ◽  
Vol 16 (13) ◽  
pp. 8157-8180 ◽  
Author(s):  
Xinyi Dong ◽  
Joshua S. Fu ◽  
Kan Huang ◽  
Daniel Tong ◽  
Guoshun Zhuang
Keyword(s):  
Soil Moisture ◽  
Air Quality ◽  
East Asia ◽  
Model Evaluation ◽  
Model Development ◽  
Dust Emission ◽  
Heterogeneous Chemistry ◽  
Fine Mode ◽  
Meteorological Simulation ◽  
The Impact

Abstract. The Community Multiscale Air Quality (CMAQ) model has been further developed in terms of simulating natural wind-blown dust in this study, with a series of modifications aimed at improving the model's capability to predict the emission, transport, and chemical reactions of dust. The default parameterization of initial threshold friction velocity constants are revised to correct the double counting of the impact of soil moisture in CMAQ by the reanalysis of field experiment data; source-dependent speciation profiles for dust emission are derived based on local measurements for the Gobi and Taklamakan deserts in East Asia; and dust heterogeneous chemistry is also implemented. The improved dust module in the CMAQ is applied over East Asia for March and April from 2006 to 2010. The model evaluation result shows that the simulation bias of PM10 and aerosol optical depth (AOD) is reduced, respectively, from −55.42 and −31.97 % by the original CMAQ to −16.05 and −22.1 % by the revised CMAQ. Comparison with observations at the nearby Gobi stations of Duolun and Yulin indicates that applying a source-dependent profile helps reduce simulation bias for trace metals. Implementing heterogeneous chemistry also results in better agreement with observations for sulfur dioxide (SO2), sulfate (SO42−), nitric acid (HNO3), nitrous oxides (NOx), and nitrate (NO3−). The investigation of a severe dust storm episode from 19 to 21 March 2010 suggests that the revised CMAQ is capable of capturing the spatial distribution and temporal variation of dust. The model evaluation also indicates potential uncertainty within the excessive soil moisture used by meteorological simulation. The mass contribution of fine-mode particles in dust emission may be underestimated by 50 %. The revised CMAQ model provides a useful tool for future studies to investigate the emission, transport, and impact of wind-blown dust over East Asia and elsewhere.

scholarly journals The impact of measures to reduce ambient air PM<sub>10</sub> concentrations originating from road dust, evaluated for a street canyon in Helsinki

2019 ◽  
Vol 19 (17) ◽  
pp. 11199-11212 ◽  
Author(s):  
Ana Stojiljkovic ◽  
Mari Kauhaniemi ◽  
Jaakko Kukkonen ◽  
Kaarle Kupiainen ◽  
Ari Karppinen ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
Street Canyon ◽  
Dust Emission ◽  
Road Dust ◽  
Ambient Air ◽  
Air Quality Measurements ◽  
Emission Models ◽  
The Impact ◽  
Quality Measurements

Abstract. We have numerically evaluated how effective selected potential measures would be for reducing the impact of road dust on ambient air particulate matter (PM10). The selected measures included a reduction of the use of studded tyres on light-duty vehicles and a reduction of the use of salt or sand for traction control. We have evaluated these measures for a street canyon located in central Helsinki for four years (2007–2009 and 2014). Air quality measurements were conducted in the street canyon for two years, 2009 and 2014. Two road dust emission models, NORTRIP (NOn-exhaust Road TRaffic Induced Particle emissions) and FORE (Forecasting Of Road dust Emissions), were applied in combination with the Operational Street Pollution Model (OSPM), a street canyon dispersion model, to compute the street increments of PM10 (i.e. the fraction of PM10 concentration originating from traffic emissions at the street level) within the street canyon. The predicted concentrations were compared with the air quality measurements. Both road dust emission models reproduced the seasonal variability of the PM10 concentrations fairly well but under-predicted the annual mean values. It was found that the largest reductions of concentrations could potentially be achieved by reducing the fraction of vehicles that use studded tyres. For instance, a 30 % decrease in the number of vehicles using studded tyres would result in an average decrease in the non-exhaust street increment of PM10 from 10 % to 22 %, depending on the model used and the year considered. Modelled contributions of traction sand and salt to the annual mean non-exhaust street increment of PM10 ranged from 4 % to 20 % for the traction sand and from 0.1 % to 4 % for the traction salt. The results presented here can be used to support the development of optimal strategies for reducing high springtime particulate matter concentrations originating from road dust.

scholarly journals Why do models perform differently on particulate matter over East Asia? A multi-model intercomparison study for MICS-Asia III

2020 ◽  
Vol 20 (12) ◽  
pp. 7393-7410 ◽  
Author(s):  
Jiani Tan ◽  
Joshua S. Fu ◽  
Gregory R. Carmichael ◽  
Syuichi Itahashi ◽  
Zhining Tao ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Air Quality ◽  
East Asia ◽  
Dust Emission ◽  
Sulfur Oxidation ◽  
Atmospheric Modeling ◽  
Weather Research And Forecasting ◽  
Forecasting Model ◽  
Air Quality Prediction ◽  
Weather Research

Abstract. This study compares the performance of 12 regional chemical transport models (CTMs) from the third phase of the Model Inter-Comparison Study for Asia (MICS-Asia III) on simulating the particulate matter (PM) over East Asia (EA) in 2010. The participating models include the Weather Research and Forecasting model coupled with Community Multiscale Air Quality (WRF-CMAQ; v4.7.1 and v5.0.2), the Regional Atmospheric Modeling System coupled with CMAQ (RAMS-CMAQ; v4.7.1 and v5.0.2), the Weather Research and Forecasting model coupled with chemistry (WRF-Chem; v3.6.1 and v3.7.1), Goddard Earth Observing System coupled with chemistry (GEOS-Chem), a non-hydrostatic model coupled with chemistry (NHM-Chem), the Nested Air Quality Prediction Modeling System (NAQPMS) and the NASA-Unified WRF (NU-WRF). This study investigates three model processes as the possible reasons for different model performances on PM. (1) Models perform very differently in the gas–particle conversion of sulfur (S) and oxidized nitrogen (N). The model differences in sulfur oxidation ratio (50 %) are of the same magnitude as that in SO42- concentrations. The gas–particle conversion is one of the main reasons for different model performances on fine mode PM. (2) Models without dust emission modules can perform well on PM10 at non-dust-affected sites but largely underestimate (up to 50 %) the PM10 concentrations at dust sites. The implementation of dust emission modules in the models has largely improved the model accuracies at dust sites (reduce model bias to −20 %). However, both the magnitude and distribution of dust pollution are not fully captured. (3) The amounts of modeled depositions vary among models by 75 %, 39 %, 21 % and 38 % for S wet, S dry, N wet and N dry depositions, respectively. Large inter-model differences are found in the washout ratios of wet deposition (at most 170 % in India) and dry deposition velocities (generally 0.3–2 cm s−1 differences over inland regions).

scholarly journals Emission, transport, and radiative effects of mineral dust from the Taklimakan and Gobi deserts: comparison of measurements and model results

2017 ◽  
Vol 17 (3) ◽  
pp. 2401-2421 ◽  
Author(s):  
Siyu Chen ◽  
Jianping Huang ◽  
Litai Kang ◽  
Hao Wang ◽  
Xiaojun Ma ◽  
...  
Keyword(s):  
East Asia ◽  
Dust Emission ◽  
Dust Concentration ◽  
Dust Particles ◽  
Storm Event ◽  
Gobi Desert ◽  
Radiative Effects ◽  
Dust Aerosols ◽  
Budget Analysis ◽  
Westerly Jets

Abstract. The Weather Research and Forecasting Model with chemistry (WRF-Chem model) was used to investigate a typical dust storm event that occurred from 18 to 23 March 2010 and swept across almost all of China, Japan, and Korea. The spatial and temporal variations in dust aerosols and the meteorological conditions over East Asia were well reproduced by the WRF-Chem model. The simulation results were used to further investigate the details of processes related to dust emission, long-range transport, and radiative effects of dust aerosols over the Taklimakan Desert (TD) and Gobi Desert (GD). The results indicated that weather conditions, topography, and surface types in dust source regions may influence dust emission, uplift height, and transport at the regional scale. The GD was located in the warm zone in advance of the cold front in this case. Rapidly warming surface temperatures and cold air advection at high levels caused strong instability in the atmosphere, which strengthened the downward momentum transported from the middle and low troposphere and caused strong surface winds. Moreover, the GD is located in a relatively flat, high-altitude region influenced by the confluence of the northern and southern westerly jets. Therefore, the GD dust particles were easily lofted to 4 km and were the primary contributor to the dust concentration over East Asia. In the dust budget analysis, the dust emission flux over the TD was 27.2 ± 4.1 µg m−2 s−1, which was similar to that over the GD (29 ± 3.6 µg m−2 s−1). However, the transport contribution of the TD dust (up to 0.8 ton d−1) to the dust sink was much smaller than that of the GD dust (up to 3.7 ton d−1) because of the complex terrain and the prevailing wind in the TD. Notably, a small amount of the TD dust (PM2.5 dust concentration of approximately 8.7 µg m−3) was lofted to above 5 km and transported over greater distances under the influence of the westerly jets. Moreover, the direct radiative forcing induced by dust was estimated to be −3 and −7 W m−2 at the top of the atmosphere, −8 and −10 W m−2 at the surface, and +5 and +3 W m−2 in the atmosphere over the TD and GD, respectively. This study provides confidence for further understanding the climate effects of the GD dust.

scholarly journals Impacts of Late-Spring North Eurasian Soil Moisture Variation on Summer Rainfall Anomalies in Northern East Asia

2021 ◽  
Author(s):  
Yinghan Sang ◽  
Hong-Li Ren ◽  
Yi Deng ◽  
Xiaofeng Xu ◽  
Xueli Shi ◽  
...  
Keyword(s):  
Soil Moisture ◽  
Temperature Gradient ◽  
East Asia ◽  
Summer Rainfall ◽  
Low Pressure ◽  
Late Spring ◽  
Boreal Summer ◽  
Pressure Center ◽  
North Eurasia ◽  
The Impact

Abstract This paper reports findings from a diagnostic and modeling analysis that investigates the impact of the late-spring soil moisture anomaly over North Eurasia on the boreal summer rainfall over northern East Asia (NEA). Soil moisture in May in the region from the Kara-Laptev Sea coasts to Central Siberian Plateau is found to be negatively correlated with the summer rainfall from Mongolia to Northeast China. The atmospheric circulation anomalies associated with the anomalously dry soil are characterized by a pressure dipole with the high-pressure center located over North Eurasia and the low-pressure center over NEA, where an anomalous lower-level moisture convergence occurs, favoring rainfall formation. Diagnoses and Modeling experiments demonstrate that the effect of the spring low soil moisture over North Eurasia may persist into the following summer through modulating local surface latent and sensible heat fluxes, increasing low-level air temperature at higher latitudes, and effectively reducing the meridional temperature gradient. The weakened temperature gradient could induce the decreased zonal wind and the generation of a low-pressure center over NEA, associated with a favorable condition of local synoptic activity. The above relationships and mechanisms are vice versa for the prior wetter soil and decreased NEA rainfall. These findings suggest that soil moisture anomalies over North Eurasia may act as a new precursor providing an additional predictability source for better predicting the summer rainfall in NEA.

Irrigation in JULES Land-Only Simulations over South and East Asia

2021 ◽  
Author(s):  
Markus Todt ◽  
Pier Luigi Vidale ◽  
Patrick C. McGuire ◽  
Omar V. Müller
Keyword(s):  
Soil Moisture ◽  
East Asia ◽  
Land Surface ◽  
River Flow ◽  
Heat Fluxes ◽  
Global Climate Models ◽  
Irrigated Agriculture ◽  
Irrigation Season ◽  
Irrigation Scheme ◽  
The Impact

&lt;p&gt;Capturing soil moisture-atmosphere feedbacks in a weather or climate model requires realistic simulation of various land surface processes. However, irrigation and other water management methods are still missing in most global climate models today, despite irrigated agriculture being the dominant land use in parts of Asia. In this study, we test the irrigation scheme available in the land model JULES (Joint UK Land Environment Simulator) by running land-only simulations over South and East Asia driven by WFDEI (WATCH Forcing Data ERA-Interim) forcing data. Irrigation in JULES is applied on a daily basis by replenishing soil moisture in the upper soil layers to field capacity, and we use a version of the irrigation scheme that extracts water for irrigation from groundwater and rivers, which physically limits the amount of irrigation that can be applied. We prescribe irrigation for C3 grasses in order to simulate the effects of agriculture, albeit retaining the simpler, widely used 5-PFT (plant functional type) configuration in JULES. Irrigation generally increases soil moisture and evapotranspiration, which results in increasing latent heat fluxes and decreasing sensible heat fluxes. Comparison with combined observational/machine-learning products for turbulent fluxes shows that while irrigation can reduce biases, other biases in JULES, unrelated to irrigation, are larger than improvements due to the inclusion of irrigation. Irrigation also affects water fluxes within the soil, e.g. runoff and drainage into the groundwater level, as well as soil moisture outside of the irrigation season. We find that the irrigation scheme, at least in the uncoupled land-atmosphere setting, can rapidly deplete groundwater to the point that river flow becomes the main source of irrigation (over the North China Plain and the Indus region) and can have the counterintuitive effect of decreasing annual average soil moisture (over the Ganges plain). Subsequently, we will explore the impact of irrigation on regional climate by conducting coupled land-atmosphere simulations.&lt;/p&gt;

scholarly journals The impact of measures to reduce road dust, evaluated for a street canyon in Helsinki

2018 ◽  
Author(s):  
Ana Stojiljkovic ◽  
Mari Kauhaniemi ◽  
Jaakko Kukkonen ◽  
Kaarle Kupiainen ◽  
Ari Karppinen ◽  
...  
Keyword(s):  
Air Quality ◽  
Street Canyon ◽  
Dispersion Model ◽  
Dust Emission ◽  
Optimal Strategies ◽  
Road Dust ◽  
Mean Values ◽  
Air Quality Measurements ◽  
The Impact ◽  
Quality Measurements

Abstract. We have evaluated numerically how effective a few selected measures would be for reducing road dust. The selected measures included the reduction of the use of studded tyres in light-duty vehicles and phasing-out of salt or sand in traction control. We have evaluated these measures for a street canyon location in central Helsinki, for four years (2007–2009 and 2014). Air quality measurements were conducted in the street canyon for two years, 2009 and 2014. Two road dust emission models, NORTRIP and FORE, were applied in combination with the street canyon dispersion model OSPM to compute the street increments of PM10 within the street canyon. The predicted concentrations were compared with the air quality measurements. Both models reproduced the seasonal variability of the PM10 concentrations but under-predicted the yearly mean values. It was found that the largest reductions of concentrations could potentially be achieved by reducing the fraction of vehicles that use studded tyres. For instance, a 30 % percent decrease in the number of vehicles using studded tyres would result in an average decrease of the non-exhaust increment of PM10 from 10 to 22 %, depending on the model used and the year considered. The corresponding decrease after removal of sanding and salting would be from 4 % and 20 % and from 0.1 % to 4 %, respectively. The results can be used for finding optimal strategies for reducing the high springtime particulate matter concentrations originated from road dust.

scholarly journals Implementation of dust emission and chemistry into the Community Multiscale Air Quality modeling system and initial application to an Asian dust storm episode

2012 ◽  
Vol 12 (21) ◽  
pp. 10209-10237 ◽  
Author(s):  
K. Wang ◽  
Y. Zhang ◽  
A. Nenes ◽  
C. Fountoukis
Keyword(s):  
Air Quality ◽  
Dust Storm ◽  
Dust Emission ◽  
Forecast Model ◽  
Heterogeneous Reactions ◽  
Dust Particles ◽  
Aerodynamic Diameter ◽  
Dust Emissions ◽  
New Model ◽  
The Impact

Abstract. The US Environmental Protection Agency's (EPA) Community Multiscale Air Quality (CMAQ) modeling system version 4.7 is further developed to enhance its capability in simulating the photochemical cycles in the presence of dust particles. The new model treatments implemented in CMAQ v4.7 in this work include two online dust emission schemes (i.e., the Zender and Westphal schemes), nine dust-related heterogeneous reactions, an updated aerosol inorganic thermodynamic module ISORROPIA II with an explicit treatment of crustal species, and the interface between ISORROPIA II and the new dust treatments. The resulting improved CMAQ (referred to as CMAQ-Dust), offline-coupled with the Weather Research and Forecast model (WRF), is applied to the April 2001 dust storm episode over the trans-Pacific domain to examine the impact of new model treatments and understand associated uncertainties. WRF/CMAQ-Dust produces reasonable spatial distribution of dust emissions and captures the dust outbreak events, with the total dust emissions of ~111 and 223 Tg when using the Zender scheme with an erodible fraction of 0.5 and 1.0, respectively. The model system can reproduce well observed meteorological and chemical concentrations, with significant improvements for suspended particulate matter (PM), PM with aerodynamic diameter of 10 μm, and aerosol optical depth than the default CMAQ v4.7. The sensitivity studies show that the inclusion of crustal species reduces the concentration of PM with aerodynamic diameter of 2.5 μm (PM2.5) over polluted areas. The heterogeneous chemistry occurring on dust particles acts as a sink for some species (e.g., as a lower limit estimate, reducing O3 by up to 3.8 ppb (~9%) and SO2 by up to 0.3 ppb (~27%)) and as a source for some others (e.g., increasing fine-mode SO42− by up to 1.1 μg m−3 (~12%) and PM2.5 by up to 1.4 μg m−3 (~3%)) over the domain. The long-range transport of Asian pollutants can enhance the surface concentrations of gases by up to 3% and aerosol species by up to 20% in the Western US.

Spatial and Temporal Model Development for Analysis the Impact of Concentration of Pollutants and Emissions to the Air Quality

2016 ◽  
Vol 22 (12) ◽  
pp. 4069-4072 ◽  
Author(s):  
Yayat Ruhiat ◽  
Firmanul C Wibowo ◽  
Aceng Hasani ◽  
. Kuswantoro ◽  
Rian Fahrizal ◽  
...  
Keyword(s):  
Air Quality ◽  
Model Development ◽  
Temporal Model ◽  
The Impact

scholarly journals Implementation of dust emission and chemistry into the Community Multiscale Air Quality modeling system and initial application to an Asian dust storm episode

2012 ◽  
Vol 12 (5) ◽  
pp. 13457-13514 ◽  
Author(s):  
K. Wang ◽  
Y. Zhang ◽  
A. Nenes ◽  
C. Fountoukis
Keyword(s):  
Air Quality ◽  
Dust Storm ◽  
Dust Emission ◽  
Heterogeneous Reactions ◽  
Dust Particles ◽  
Aerodynamic Diameter ◽  
Dust Emissions ◽  
New Model ◽  
The Us ◽  
The Impact

Abstract. The US Environmental Protection Agency (EPA)'s Community Multiscale Air Quality (CMAQ) modeling system version 4.7 is further developed to enhance its capability in simulating the photochemical cycles in the presence of dust particles. The new model treatments implemented in CMAQ v4.7 in this work include two online-dust emission schemes, nine dust-related heterogeneous reactions, an updated aerosol inorganic thermodynamic module ISORROPIA II with an explicit treatment of crustal species, and the interface between ISORROPIA II and the new dust treatments. The resulting improved CMAQ (referred to as CMAQ-Dust), offline-coupled with the Weather Research and Forecast model (WRF), are applied to the April 2001 dust storm episode over the trans-Pacific domain to examine the impact of new model treatments and understand associated uncertainties. WRF/CMAQ-Dust produces reasonable spatial distribution of dust emissions and captures the dust outbreak events, with the total dust emissions of ∼111 and 223 Tg when the erodible fraction is assumed to be 0.5 and 1.0, respectively, for the April 2001 episode. The model system can reproduce well observed meteorological and chemical concentrations, with significant improvements for suspended particulate matter (PM), PM with aerodynamic diameter of 10 μm and aerosol optical depth than default CMAQ v4.7. The sensitivity studies show that the inclusion of crustal species reduces the concentration of PM with aerodynamic diameter of 2.5 μm (PM2.5) over polluted areas. The heterogeneous chemistry occurring on dust particles acts as a sink for some species (e.g., as a lower limit estimate, O3 by up to 3.8 ppb (∼9%) and SO2 by up to 0.3 ppb (∼27%)) and as a source for some others (e.g., fine-mode SO42− by up to 1.1 μg m−3 (∼12%) and PM2.5 by up to 1.4 μg m−3 (∼3%) over the domain. The long-range transport of Asian pollutants can enhance the background concentrations of gases by up to 3% and aerosol species by up to 20% in the US.

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