scholarly journals Tropical tropospheric ozone columns from nadir retrievals of GOME-1/ERS-2, SCIAMACHY/Envisat, and GOME-2/MetOp-A (1996–2012)

2016 ◽  
Vol 9 (7) ◽  
pp. 3407-3427 ◽  
Author(s):  
Elpida Leventidou ◽  
Kai-Uwe Eichmann ◽  
Mark Weber ◽  
John P. Burrows
Keyword(s):  
Tropospheric Ozone ◽  
Convective Cloud ◽  
Uncertainty Estimation ◽  
Interannual Variations ◽  
Verification Algorithm ◽  
Cloud Parameters ◽  
Ozone Column ◽  
Total Column ◽  
Good Agreement

Abstract. Tropical tropospheric ozone columns are retrieved with the convective cloud differential (CCD) technique using total ozone columns and cloud parameters from different European satellite instruments. Monthly-mean tropospheric column amounts [DU] are calculated by subtracting the above-cloud ozone column from the total column. A CCD algorithm (CCD_IUP) has been developed as part of the verification algorithm developed for TROPOspheric Monitoring Instrument (TROPOMI) on Sentinel 5-precursor (S5p) mission, which was applied to GOME/ERS-2 (1995–2003), SCIAMACHY/Envisat (2002–2012), and GOME-2/MetOp-A (2007–2012) measurements. Thus a unique long-term record of monthly-mean tropical tropospheric ozone columns (20° S–20° N) from 1996 to 2012 is now available. An uncertainty estimation has been performed, resulting in a tropospheric ozone column uncertainty less than 2 DU ( < 10 %) for all instruments. The dataset has not been yet harmonised into one consistent; however, comparison between the three separate datasets (GOME/SCIAMACHY/GOME-2) shows that GOME-2 overestimates the tropical tropospheric ozone columns by about 8 DU, while SCIAMACHY and GOME are in good agreement. Validation with Southern Hemisphere ADditional OZonesondes (SHADOZ) data shows that tropospheric ozone columns from the CCD_IUP technique and collocated integrated ozonesonde profiles from the surface up to 200 hPa are in good agreement with respect to range, interannual variations, and variances. Biases within ±5 DU and root-mean-square (RMS) deviation of less than 10 DU are found for all instruments. CCD comparisons using SCIAMACHY data with tropospheric ozone columns derived from limb/nadir matching have shown that the bias and RMS deviation are within the range of the CCD_IUP comparison with the ozonesondes. The 17-year dataset can be helpful for evaluating chemistry models and performing climate change studies.

scholarly journals Tropical tropospheric ozone columns from nadir retrievals of GOME-1/ERS-2, SCIAMACHY/Envisat, and GOME-2/MetOp-A (1996-2012)

2016 ◽  
Author(s):  
Elpida Leventidou ◽  
Kai-Uwe Eichmann ◽  
Mark Weber ◽  
John P. Burrows
Keyword(s):  
Tropospheric Ozone ◽  
Annual Variations ◽  
Convective Clouds ◽  
Verification Algorithm ◽  
Cloud Parameters ◽  
Ozone Column ◽  
Total Column ◽  
Good Agreement ◽  
Rms Errors

Abstract. Tropical tropospheric ozone columns are retrieved with the Convective Clouds Differential (CCD) technique using total ozone columns and cloud parameters from different European satellite instruments. Monthly mean tropospheric column amounts [DU] are calculated by subtracting the above cloud ozone column from the total column. A CCD algorithm (CCD_IUP) has been developed (as part of the verification algorithm development for TROPOMI on Sentinel 5-precursor mission) which was applied to GOME/ ERS-2 (1995-2003), SCIAMACHY/ Envisat (2002-2012), and GOME-2/ MetOpA (2007-2012) measurements. Thus a unique long-term record of monthly mean tropical tropospheric ozone columns (20°S–20°N) from 1996 to 2012 is now available. An extensive error analysis has been performed, estimating the tropospheric ozone column uncertainties being between 5 and 7 DU (25–36%). Validation with SHADOZ ozonesonde data show that tropospheric ozone columns from CCD and collocated integrated ozonesonde profiles from the surface up to 200 hPa are in good agreement with respect to range, inter-annual variations, and variances. Biases within ±5 DU and RMS errors of less than 10 DU are found. CCD comparisons using SCIAMACHY data with tropospheric ozone columns derived from Limb Nadir Matching have shown that CCD results are less noisy and correlate better with ozonesondes. The 17-year dataset can be helpful for evaluating chemistry models and performing climate change studies.

scholarly journals Evaluation of tropospheric ozone columns derived from assimilated GOME ozone profile observations

2009 ◽  
Vol 9 (20) ◽  
pp. 8105-8120 ◽  
Author(s):  
A. T. J. de Laat ◽  
R. J. van der A ◽  
M. van Weele
Keyword(s):  
Tropospheric Ozone ◽  
Transport Model ◽  
Added Value ◽  
Chemistry Transport Model ◽  
Ozone Profile ◽  
Free Running ◽  
Tropospheric O3 ◽  
Total Column ◽  
Good Agreement

Abstract. Tropospheric O3 column estimates are produced and evaluated from spaceborne O3 observations by the subtraction of assimilated O3 profile observations from total column observations, the so-called Tropospheric O3 ReAnalysis or TORA method. Here we apply the TORA method to six years (1996–2001) of ERS-2 GOME/TOMS total O3 and ERS-2 GOME O3 profile observations using the TM5 global chemistry-transport model with a linearized O3 photochemistry parameterization scheme. Free running TM5 simulations show good agreement with O3 sonde observations in the upper-tropospheric and lower stratospheric region (UTLS), both for short day-to-day variability as well as for monthly means. The assimilation of GOME O3 profile observations counteracts the mid-latitude stratospheric O3 drift caused by the overstrong stratospheric meridional circulation in TM5. Assimilation of GOME O3 profile observations also improves the bias and correlations in the tropical UTLS region but slightly degrades the model-to-sonde correlations and bias of extra-tropical UTLS. We suggest that this degradation is related to the large ground pixel size of the GOME O3 measurements (960×100 km) in combination with retrieval and calibration errors. The added value of the assimilation of GOME O3 profiles compared to stand-alone model simulations lays in the long term variations of stratospheric O3, not in short term synoptic variations. The evaluation of daily and monthly tropospheric O3 columns obtained from total column observations and using the TORA methodology shows that the use of GOME UV-VIS nadir O3 profiles in combination with the spatial resolution of the model does not result in satisfactory residual tropospheric ozone columns.

scholarly journals Estimation of Antarctic ozone loss from ground-based total column measurements

2010 ◽  
Vol 10 (14) ◽  
pp. 6569-6581 ◽  
Author(s):  
J. Kuttippurath ◽  
F. Goutail ◽  
J.-P. Pommereau ◽  
F. Lefèvre ◽  
H. K. Roscoe ◽  
...  
Keyword(s):  
Ozone Depletion ◽  
Sensitivity Study ◽  
Satellite Measurements ◽  
Macquarie Island ◽  
Ozone Loss ◽  
Antarctic Ozone ◽  
The Antarctic ◽  
Ozone Column ◽  
Total Column ◽  
Good Agreement

Abstract. The passive tracer method is used to estimate ozone loss from ground-based measurements in the Antarctic. A sensitivity study shows that the ozone depletion can be estimated within an accuracy of ~4%. The method is then applied to the ground-based observations from Arrival Heights, Belgrano, Concordia, Dumont d'Urville, Faraday, Halley, Marambio, Neumayer, Rothera, South Pole, Syowa, and Zhongshan for the diagnosis of ozone loss in the Antarctic. On average, the ten-day boxcar average of the vortex mean ozone column loss deduced from the ground-based stations was about 55±5% in 2005–2009. The ozone loss computed from the ground-based measurements is in very good agreement with those derived from satellite measurements (OMI and SCIAMACHY) and model simulations (REPROBUS and SLIMCAT), where the differences are within ±3–5%. The historical ground-based total ozone observations in October show that the depletion started in the late 1970s, reached a maximum in the early 1990s and stabilised afterwards due to saturation. There is no indication of ozone recovery yet. At southern mid-latitudes, a reduction of 20–50% is observed for a few days in October–November at the newly installed Rio Gallegos station. Similar depletion of ozone is also observed episodically during the vortex overpasses at Kerguelen in October–November and at Macquarie Island in July–August of the recent winters. This illustrates the significance of measurements at the edges of Antarctica.

scholarly journals Uncertainty analysis of total ozone derived from direct solar irradiance spectra in the presence of unknown spectral deviations

2018 ◽  
Vol 11 (6) ◽  
pp. 3595-3610 ◽  
Author(s):  
Anna Vaskuri ◽  
Petri Kärhä ◽  
Luca Egli ◽  
Julian Gröbner ◽  
Erkki Ikonen
Keyword(s):  
Solar Irradiance ◽  
Total Ozone ◽  
Monte Carlo Model ◽  
Spectral Irradiance ◽  
Total Column Ozone ◽  
Column Ozone ◽  
Ozone Column ◽  
Total Column ◽  
Local Noon ◽  
Good Agreement

Abstract. We demonstrate the use of a Monte Carlo model to estimate the uncertainties in total ozone column (TOC) derived from ground-based direct solar spectral irradiance measurements. The model estimates the effects of possible systematic spectral deviations in the solar irradiance spectra on the uncertainties in retrieved TOC. The model is tested with spectral data measured with three different spectroradiometers at an intercomparison campaign of the research project “Traceability for atmospheric total column ozone” at Izaña, Tenerife on 17 September 2016. The TOC values derived at local noon have expanded uncertainties of 1.3 % (3.6 DU) for a high-end scanning spectroradiometer, 1.5 % (4.4 DU) for a high-end array spectroradiometer, and 4.7 % (13.3 DU) for a roughly adopted instrument based on commercially available components and an array spectroradiometer when correlations are taken into account. When neglecting the effects of systematic spectral deviations, the uncertainties reduce by a factor of 3. The TOC results of all devices have good agreement with each other, within the uncertainties, and with the reference values of the order of 282 DU during the analysed day, measured with Brewer spectrophotometer #183.

scholarly journals Validation of the GRAPE single view aerosol retrieval for ATSR-2 and insights into the long term global AOD trend over the ocean

2010 ◽  
Vol 10 (10) ◽  
pp. 4849-4866 ◽  
Author(s):  
G. E. Thomas ◽  
C. A. Poulsen ◽  
R. Siddans ◽  
A. M. Sayer ◽  
E. Carboni ◽  
...  
Keyword(s):  
Data Set ◽  
Single View ◽  
Cloud Parameters ◽  
Aerosol Retrieval ◽  
Time Period ◽  
Orbital Drift ◽  
Along Track ◽  
Best Fit ◽  
Good Agreement

Abstract. The Global Retrieval of ATSR Cloud Parameters and Evaluation (GRAPE) project has produced a global data-set of cloud and aerosol properties from the Along Track Scanning Radiometer-2 (ATSR-2) instrument, covering the time period 1995–2001. This paper presents the validation of aerosol optical depths (AODs) over the ocean from this product against AERONET sun-photometer measurements, as well as a comparison to the Advanced Very High Resolution Radiometer (AVHRR) optical depth product produced by the Global Aerosol Climatology Project (GACP). The GRAPE AOD over ocean is found to be in good agreement with AERONET measurements, with a Pearson's correlation coefficient of 0.79 and a best-fit slope of 1.0±0.1, but with a positive bias of 0.08±0.04. Although the GRAPE and GACP datasets show reasonable agreement, there are significant differences. These discrepancies are explored, and suggest that the downward trend in AOD reported by GACP may arise from changes in sampling due to the orbital drift of the AVHRR instruments.

scholarly journals Synergy of Using Nadir and Limb Instruments for Tropospheric Ozone Monitoring

2021 ◽  
Author(s):  
Viktoria F. Sofieva ◽  
Risto Hänninen ◽  
Mikhail Sofiev ◽  
Monika Szelag ◽  
Hei Shing Lee ◽  
...  
Keyword(s):  
Satellite Data ◽  
Tropospheric Ozone ◽  
Total Ozone ◽  
Stratospheric Ozone ◽  
Intermediate Step ◽  
Residual Method ◽  
Total Ozone Column ◽  
Clear Sky ◽  
Ozone Column ◽  
Good Agreement

Abstract. The satellite measurements in nadir and limb viewing geometry provide a complementary view of the atmosphere. An effective combination of the limb and nadir measurements can provide a new information about atmospheric composition. In this work, we present tropospheric ozone column datasets that have been created using combination of total ozone column from OMI and TROPOMI with stratospheric ozone column dataset from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). We have developed further the methodological aspects of assessment of tropospheric ozone using the residual method using simulations with the chemistry-transport model SILAM. It has been shown that the accurate assessment of ozone in the upper troposphere and the lower stratosphere (UTLS) is of high importance for detecting the ground-level ozone patterns. The stratospheric ozone column is derived from a combination of ozone profiles from several satellite instruments in limb-viewing geometry. We developed a method for the data homogenization, which includes the removal of biases and a-posteriori estimation (validation) of random uncertainties, thus making the data from different instruments compatible with each other. The high horizontal and vertical resolution dataset of ozone profiles is created via interpolation of the limb profiles from each day to 1° × 1° horizonal grid. A new kriging-type interpolation method, which takes into account data uncertainties and the information about natural ozone variations from the SILAM-adjusted ozone field, has been developed. To mitigate the limited accuracy and coverage of the limb profile data in the UTLS, a smooth transition to the model data is applied below the tropopause. This allows estimation of stratospheric ozone column with full coverage of the UTLS. The derived ozone profiles are in very good agreement with collocated ozonesonde measurements. The residual method was successfully applied to OMI and TROPOMI clear-sky total ozone data in combination with the stratospheric ozone column from the high-resolution limb profile dataset. The resulting tropospheric ozone column is in very good agreement with other satellite data. The global distributions of tropospheric ozone exhibit enhancements associated with the regions of high tropospheric ozone production. The main created datasets are (i) monthly 1° × 1° global tropospheric ozone column dataset using OMI and limb instruments, (ii) monthly 1° × 1° global tropospheric ozone column dataset using TROPOMI and limb instruments and (iii) daily 1° × 1° interpolated stratospheric ozone column from limb instruments. Other datasets, which are created as an intermediate step of creating the tropospheric ozone column data, are: (i) daily 1° × 1° clear sky and total ozone column from OMI and TROPOMI (ii) Daily 1° × 1° homogenized and interpolated dataset of ozone profiles and (iii) daily 1° × 1° dataset of ozone profiles from SILAM simulations with adjustment to satellite data. These datasets can be used in various studies related to ozone distributions, variability and trends, both in the troposphere and the stratosphere.

scholarly journals Analysis of Long Term Variation of the Total Column and Tropospheric Ozone over the Indian Region

2021 ◽  
Vol 11 (01) ◽  
pp. 194-213
Author(s):  
C. T. Resmi ◽  
T. Nishanth ◽  
P. S. Vijoy ◽  
M. K. Satheesh Kumar ◽  
M. Balachandramohan
Keyword(s):  
Tropospheric Ozone ◽  
Indian Region ◽  
Term Variation ◽  
Total Column

scholarly journals TROPOMI tropospheric ozone column data: Geophysical assessment and comparison to ozonesondes, GOME-2B and OMI

2020 ◽  
Author(s):  
Daan Hubert ◽  
Klaus-Peter Heue ◽  
Jean-Christopher Lambert ◽  
Tijl Verhoelst ◽  
Marc Allaart ◽  
...  
Keyword(s):  
Tropospheric Ozone ◽  
Convective Cloud ◽  
Horizontal Resolution ◽  
Measurement Systems ◽  
Clear Sky ◽  
International Regulations ◽  
Spatio Temporal ◽  
Sky Conditions ◽  
Ozone Column

Abstract. Ozone in the troposphere affects humans and ecosystems as a pollutant and as a greenhouse gas. Observing, understanding and modelling this dual role, as well as monitoring effects of international regulations on air quality and climate change, however, challenge measurement systems to operate at opposite ends of the spatio-temporal scale ladder. On board of the ESA/EU Copernicus Sentinel-5 Precursor (S5P) satellite launched in October 2017, TROPOspheric Monitoring Instrument (TROPOMI) aspires to take the next leap forward by measuring ozone and its precursors at unprecedented horizontal resolution until at least the mid 2020s. In this work, we assess the quality of TROPOMI's first release (V01.01.05–08) of tropical tropospheric ozone column data (TrOC). Derived with the Convective Cloud Differential (CCD) method, TROPOMI daily TrOC data represent the three-day moving mean ozone column between surface and 270 hpa under clear sky conditions gridded at 0.5° latitude by 1° longitude resolution. Comparisons to almost two years of co-located SHADOZ ozonesonde and satellite data (Aura OMI and MetOp-B GOME-2) conclude to TROPOMI biases between −0.1 and +2.3 DU (

scholarly journals Are there urban signatures in the tropospheric ozone column products derived from satellite measurements?

2010 ◽  
Vol 10 (2) ◽  
pp. 3807-3826
Author(s):  
J. Kar ◽  
J. Fishman ◽  
J. K. Creilson ◽  
A. Richter ◽  
J. Ziemke ◽  
...  
Keyword(s):  
Tropospheric Ozone ◽  
Lower Troposphere ◽  
Data Sets ◽  
Mixing Ratio ◽  
Satellite Measurements ◽  
Ratio Distribution ◽  
Total Column Ozone ◽  
Column Ozone ◽  
Ozone Column ◽  
Total Column

Abstract. In view of the proposed geostationary satellite missions to monitor air quality from space, it is important to first assess the capability of the current suite of satellite instruments to provide information on the urban scale pollution. We explore the possibility of detecting urban signatures in the tropospheric column ozone data derived from TOMS/SBUV and OMI/MLS satellite data. We find that distinct isolated plumes of tropospheric ozone near several large and polluted cities around the world may be detected in these data sets. The ozone plumes generally correspond with the tropospheric column NO2 plumes around these cities as observed by the SCIAMACHY instrument. Similar plumes are also seen in tropospheric mean ozone mixing ratio distribution after accounting for the surface and tropopause pressure variations. The total column ozone retrievals indicate fairly significant sensitivity to the lower troposphere over the polluted land areas, which might help explain these detections. These results indicate that UV measurements may, in principle, be able to capture the urban signatures and may have implications for future missions using geostationary satellites.

scholarly journals Estimation of Antarctic ozone loss from Ground-based total column measurements

2010 ◽  
Vol 10 (3) ◽  
pp. 7641-7674
Author(s):  
J. Kuttippurath ◽  
F. Goutail ◽  
J.-P. Pommereau ◽  
F. Lefèvre ◽  
H. K. Roscoe ◽  
...  
Keyword(s):  
Total Ozone ◽  
Sensitivity Study ◽  
Ozone Monitoring Instrument ◽  
Macquarie Island ◽  
Ozone Loss ◽  
Antarctic Ozone ◽  
The Antarctic ◽  
Ozone Column ◽  
Total Column ◽  
Good Agreement

Abstract. The passive ozone method is used to estimate ozone loss from ground-based measurements in the Antarctic. A sensitivity study shows that the O3 loss can be estimated within an accuracy of ~4%. The method is then applied to the observations from Amundsen-Scott/South Pole, Arrival Heights, Belgrano, Concordia, Dumont d'Urville, Faraday, Halley, Marambio, Neumayer, Rothera, Syowa and Zhongshan for the diagnosis of ozone loss in the Antarctic. On average, the five-day running mean of the vortex averaged ozone column loss deduced from the ground-based stations shows about 53% in 2009, 59% in 2008, 55% in 2007, 56% in 2006 and 61% in 2005. The observed O3 loss and loss rates are in very good agreement with the satellite observations (Ozone Monitoring Instrument and Sciamachy) and are well reproduced by the model (Reprobus and SLIMCAT) calculations. The historical ground-based total ozone measurements show that the depletion started in the late 1970s, reached a maximum in the early 1990s, stabilising afterwards at this level until present, with the exception of 2002, the year of an early vortex break-up. There is no indication of significant recovery yet. At southern mid-latitudes, a total ozone reduction of 40–50% is observed at the newly installed station Rio Gallegos and 25–35% at Kerguelen in October–November of 2008–2009 and 2005–2009 (except 2008) respectively, and of 10–20% at Macquarie Island in July–August of 2006–2009. This illustrates the significance of measurements at the edges of Antarctica.

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