scholarly journals A weather regime characterisation of winter biomass aerosol transport in southern Africa

Author(s):  
Marco Gaetani ◽  
Maria del Carmen Alvarez Castro ◽  
Cyrille Flamant ◽  
Benjamin Pohl ◽  
Paola Formenti

<p>Atmospheric dynamics over southern Africa and South Atlantic is dominated by complex aerosol-radiation-cloud interactions, and the characterisation of the tropospheric distribution of aerosols is essential for the full understanding of these interactions.</p><p>During austral winter, a compact low cloud deck over South Atlantic contrasts clear sky over southern Africa, where forest fires triggered by dry conditions emit large amount of biomass burning aerosols in the free troposphere. Most of the aerosol burden crosses the Tropical Atlantic embedded in the tropical easterly flow. However, mid-latitude synoptic disturbances can deflect part of the aerosols from the main transport path towards southern extra-tropics.</p><p>In this study, a characterisation of the synoptic variability controlling biomass burning aerosols in southern Africa and South Atlantic during austral winter is presented. By analysing ECMWF reanalysis data, a weather regime classification of the region is constructed and used to characterise the aerosol distribution in the period 2003-2017. Results show three southward transport paths, each associated with a specific circulation regime.</p><p> </p>

2021 ◽  
Author(s):  
Marco Gaetani ◽  
Benjamin Pohl ◽  
Maria del Carmen Alvarez Castro ◽  
Cyrille Flamant ◽  
Paola Formenti

Abstract. During austral winter, a compact low cloud deck over South Atlantic contrasts with clear sky over southern Africa, where forest fires triggered by dry conditions emit large amount of biomass burning aerosols (BBA) in the free troposphere. Most of the BBA burden crosses South Atlantic embedded in the tropical easterly flow. However, midlatitude synoptic disturbances can deflect part of the aerosol from the main transport path towards southern extratropics. In this study, a characterisation of the synoptic variability controlling the spatial distribution of BBA in southern Africa and South Atlantic during austral winter (August to October) is presented. By analysing atmospheric circulation data from reanalysis products, a 6-class weather regime (WR) classification of the region is constructed. The classification reveals that the synoptic variability is composed by four WRs representing disturbances travelling at midlatitudes, and two WRs accounting for pressure anomalies in the South Atlantic. The WR classification is then successfully used to characterise the aerosol spatial distribution in the region in the period 2003–2017, in both reanalysis products and station data. Results show that the BBA transport towards southern extratropics is controlled by weather regimes associated with midlatitude synoptic disturbances. In particular, depending on the relative position of the pressure anomalies along the midlatitude westerly flow, the BBA transport is deflected from the main tropical route towards southern Africa or the South Atlantic. This paper presents the first objective classification of the winter synoptic circulation over South Atlantic and southern Africa. The classification shows skills in characterising the BBA transport, indicating the potential for using it as a diagnostic/predictive tool for aerosol dynamics, which is a key component for the full understanding and modelling of the complex radiation-aerosol-cloud interactions controlling the atmospheric radiative budget in the region.


2021 ◽  
Vol 21 (21) ◽  
pp. 16575-16591
Author(s):  
Marco Gaetani ◽  
Benjamin Pohl ◽  
Maria del Carmen Alvarez Castro ◽  
Cyrille Flamant ◽  
Paola Formenti

Abstract. During austral winter, a compact low cloud deck over the South Atlantic contrasts with clear sky over southern Africa, where forest fires triggered by dry conditions emit large amounts of biomass burning aerosols (BBAs) in the free troposphere. Most of the BBA burden crosses the South Atlantic embedded in the tropical easterly flow. However, midlatitude synoptic disturbances can deflect part of the aerosol from the main transport path towards southern extratropics. In this study, the first objective classification of the synoptic variability controlling the spatial distribution of BBA in southern Africa and the South Atlantic during austral winter (August to October) is presented. By analysing atmospheric circulation data from reanalysis products, a six-class weather regime (WR) classification of the region is constructed. The classification reveals that the synoptic variability is composed of four WRs, representing disturbances travelling at midlatitudes, and two WRs accounting for pressure anomalies in the South Atlantic. The WR classification is then successfully used to characterise the aerosol spatial distribution in the region in the period 2003–2017, in both reanalysis products and station data. Results show that the BBA transport towards southern extratropics is controlled by weather regimes associated with midlatitude synoptic disturbances. In particular, depending on the relative position of the pressure anomalies along the midlatitude westerly flow, the BBA transport is deflected from the main tropical route towards southern Africa or the South Atlantic. Moreover, the WRs accounting for midlatitude disturbances show organised transition sequences, which allow one to illustrate the evolution of the BBA northerly transport across the region in the context of a wave pattern. The skill in characterising the BBA transport shown by the WR classification indicates the potential for using it as a diagnostic/predictive tool for the aerosol dynamics, which is a key component for the full understanding and modelling of the complex radiation–aerosol–cloud interactions controlling the atmospheric radiative budget in the region.


2011 ◽  
Vol 11 (21) ◽  
pp. 11253-11266 ◽  
Author(s):  
Y. H. Mao ◽  
Q. B. Li ◽  
L. Zhang ◽  
Y. Chen ◽  
J. T. Randerson ◽  
...  

Abstract. Forest fires are an important source to carbonaceous aerosols in the Western United States (WUS). We quantify the relative contribution of biomass burning to black carbon (BC) in the WUS mountain ranges by analyzing surface BC observations for 2006 from the Interagency Monitoring of PROtected Visual Environment (IMPROVE) network using the GEOS-Chem global chemical transport model. Observed surface BC concentrations show broad maxima during late June to early November. Enhanced potassium concentrations and potassium/sulfur ratios observed during the high-BC events indicate a dominant biomass burning influence during the peak fire season. Model surface BC reproduces the observed day-to day and synoptic variabilities in regions downwind of but near urban centers. Major discrepancies are found at elevated mountainous sites during the July-October fire season when simulated BC concentrations are biased low by a factor of two. We attribute these low biases largely to the underestimated (by more than a factor of two) and temporally misplaced biomass burning emissions of BC in the model. Additionally, we find that the biomass burning contribution to surface BC concentrations in the USA likely was underestimated in a previous study using GEOS-Chem (Park et al., 2003), because of the unusually low planetary boundary layer (PBL) heights in the GEOS-3 meteorological reanalysis data used to drive the model. PBL heights from GEOS-4 and GEOS-5 reanalysis data are comparable to those from the North American Regional Reanalysis (NARR). Model simulations show slightly improved agreements with the observations when driven by GEOS-5 reanalysis data, but model results are still biased low. The use of biomass burning emissions with diurnal cycle, synoptic variability, and plume injection has relatively small impact on the simulated surface BC concentrations in the WUS.


2011 ◽  
Vol 11 (5) ◽  
pp. 13425-13467 ◽  
Author(s):  
Y. Mao ◽  
Q. Li ◽  
L. Zhang ◽  
Y. Chen ◽  
J. T. Randerson ◽  
...  

Abstract. Forest fires are an important source to carbonaceous aerosols in the western United States (WUS). We quantify the relative contribution of biomass burning to black carbon (BC) in the WUS mountain ranges by analyzing surface BC observations for 2006 from the Interagency Monitoring of PROtected Visual Environment (IMPROVE) network using the GEOS-Chem global chemical transport model. Observed surface BC concentrations show broad maxima during late June to early November. Enhanced potassium concentrations and potassium/sulfur ratios observed during the high-BC events indicate a dominant biomass burning influence during the peak fire season. Model surface BC reproduces the observed day-to-day and synoptic variabilities in regions downwind of and near urban centers. Major discrepancies are found at elevated mountainous sites during the July–October when simulated BC concentrations are biased low by a factor of two. We attribute these biases largely to the underestimated and temporally misplaced biomass burning emissions of BC in the model. Additionally, we find that the biomass burning contribution to surface BC concentrations in the US likely was underestimated in a previous study using GEOS-Chem (Park et al., 2003), because of the unusually low planetary boundary layer (PBL) heights and weak precipitation in the GEOS-3 meteorological reanalysis data used to drive the model. PBL heights from GEOS-4 and GEOS-5 reanalysis data are comparable to those from the North American Regional Reanalysis (NARR). Model simulations show improved agreements with the observations when driven by GEOS-5 reanalysis data, but model results are still biased low. The use of biomass burning emissions with diurnal cycle, synoptic variability, and plume injection has relatively small impact on the simulated surface BC concentrations in the WUS.


2019 ◽  
Vol 19 (6) ◽  
pp. 3557-3578 ◽  
Author(s):  
Martin Osborne ◽  
Florent F. Malavelle ◽  
Mariana Adam ◽  
Joelle Buxmann ◽  
Jaqueline Sugier ◽  
...  

Abstract. On 15–16 October 2017, ex-hurricane Ophelia passed to the west of the British Isles, bringing dust from the Sahara and smoke from Portuguese forest fires that was observable to the naked eye and reported in the UK's national press. We report here detailed observations of this event using the UK operational lidar and sun-photometer network, established for the early detection of aviation hazards, including volcanic ash. We also use ECMWF ERA5 wind field data and MODIS imagery to examine the aerosol transport. The observations, taken continuously over a period of 30 h, show a complex picture, dominated by several different aerosol layers at different times and clearly correlated with the passage of different air masses associated with the intense cyclonic system. A similar evolution was observed at several sites, with a time delay between them explained by their different location with respect to the storm and associated meteorological features. The event commenced with a shallow dust layer at 1–2 km in altitude and culminated in a deep and complex structure that lasted ∼12 h at each site over the UK, correlated with the storm's warm sector. For most of the time, the aerosol detected was dominated by mineral dust mixtures, as highlighted by depolarisation measurements, but an intense biomass burning aerosol (BBA) layer was observed towards the end of the event, lasting around 3 h at each site. The aerosol optical depth at 355 nm (AOD355) during the whole event ranged from 0.2 to 2.9, with the larger AOD correlated to the intense BBA layer. Such a large AOD is unprecedented in the UK according to AERONET records for the last 20 years. The Raman lidars permitted the measurement of the aerosol extinction coefficient at 355 nm, the particle linear depolarisation ratio (PLDR), and the lidar ratio (LR) and made the separation of the dust (depolarising) aerosol from other aerosol types possible. A specific extinction has also been computed to provide an estimate of the atmospheric concentration of both aerosol types separately, which peaked at 420±200 µg m−3 for the dust and 558±232 µg m−3 for the biomass burning aerosols. Back trajectories computed using the Numerical Atmospheric-dispersion Modelling Environment (NAME) were used to identify the sources and strengthen the conclusions drawn from the observations. The UK network represents a significant expansion of the observing capability in northern Europe, with instruments evenly distributed across Great Britain, from Camborne in Cornwall to Lerwick in the Shetland Islands, and this study represents the first attempt to demonstrate its capability and validate the methods in use. Its ultimate purpose will be the detection and quantification of volcanic plumes, but the present study clearly demonstrates the advanced capabilities of the network.


1998 ◽  
Vol 103 (D7) ◽  
pp. 8401-8423 ◽  
Author(s):  
Denise L. Mauzerall ◽  
Jennifer A. Logan ◽  
Daniel J. Jacob ◽  
Bruce E. Anderson ◽  
Donald R. Blake ◽  
...  

2016 ◽  
Vol 16 (18) ◽  
pp. 12329-12345 ◽  
Author(s):  
Jessie M. Creamean ◽  
Paul J. Neiman ◽  
Timothy Coleman ◽  
Christoph J. Senff ◽  
Guillaume Kirgis ◽  
...  

Abstract. Biomass burning plumes containing aerosols from forest fires can be transported long distances, which can ultimately impact climate and air quality in regions far from the source. Interestingly, these fires can inject aerosols other than smoke into the atmosphere, which very few studies have evidenced. Here, we demonstrate a set of case studies of long-range transport of mineral dust aerosols in addition to smoke from numerous fires (including predominantly forest fires and a few grass/shrub fires) in the Pacific Northwest to Colorado, US. These aerosols were detected in Boulder, Colorado, along the Front Range using beta-ray attenuation and energy-dispersive X-ray fluorescence spectroscopy, and corroborated with satellite-borne lidar observations of smoke and dust. Further, we examined the transport pathways of these aerosols using air mass trajectory analysis and regional- and synoptic-scale meteorological dynamics. Three separate events with poor air quality and increased mass concentrations of metals from biomass burning (S and K) and minerals (Al, Si, Ca, Fe, and Ti) occurred due to the introduction of smoke and dust from regional- and synoptic-scale winds. Cleaner time periods with good air quality and lesser concentrations of biomass burning and mineral metals between the haze events were due to the advection of smoke and dust away from the region. Dust and smoke present in biomass burning haze can have diverse impacts on visibility, health, cloud formation, and surface radiation. Thus, it is important to understand how aerosol populations can be influenced by long-range-transported aerosols, particularly those emitted from large source contributors such as wildfires.


2020 ◽  
Author(s):  
Ke Ding ◽  
Xin Huang ◽  
Aijun Ding ◽  
Minghuai Wang ◽  
Hang Su ◽  
...  

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