In-cloud scavenging scheme for sectional aerosol modules – implementation in the framework of the Sectional Aerosol module for Large Scale Applications version 2.0 (SALSA2.0) global aerosol module

2021 ◽  
Author(s):  
Eemeli Holopainen ◽  
Harri Kokkola ◽  
Anton Laakso ◽  
Thomas Kühn
Keyword(s):  
Wet Deposition ◽  
Large Scale ◽  
Climate Model ◽  
Radiation Budget ◽  
Cloud Formation ◽  
The Arctic ◽  
Vertical Profiles ◽  
Size Classes ◽  
Aerosol Emission ◽  
Aerosol Module

<p><span>Black carbon (BC) affects the radiation budget of the Earth by absorbing solar radiation, darkening snow and ice covers, and influencing cloud formation and life cycle. Modelling BC in remote regions, such as the Arctic, has large inter-model variability which causes variation in the modelled aerosol effect over the Arctic. This variability can be due to differences in the transport of aerosol species which is affected by how wet deposition is modelled. </span></p><p><span> In this study we developed an aerosol size-resolved in-cloud wet deposition scheme for liquid and ice clouds for models which use a size-segregated aerosol description. This scheme was tested in the ECHAM-HAMMOZ global aerosol-climate model. The scheme was compared to the original wet deposition scheme which uses fixed scavenging coefficients for different sized particles. The comparison included vertical profiles and mass and number wet deposition fluxes, and it showed that the current scheme produced spuriously long BC lifetimes when compared to the estimates made in other studies. Thus, to find a better setup for simulating aerosol lifetimes and vertical profiles we conducted simulations where we altered the aerosol emission distribution and hygroscopicity.</span></p><p><span> We compared the modelled BC vertical profiles to the ATom aircraft campaign measurements. In addition, we compared the aerosol lifetimes against those from AEROCOM model means. We found that, without further tuning, the current scheme overestimates the BC concentrations and lifetimes more than the fixed scavenging scheme when compared to the measurements. Sensitivity studies showed that the model skill of reproducing the measured vertical BC mass concentrations improved when BC emissions were directed to larger size classes, they were mixed with soluble compounds during emission, or BC-containing particles were transferred to soluble size classes after aging. These changes also produced atmospheric BC lifetimes which were closer to AEROCOM model means. The best comparison with the measured vertical profiles and estimated BC lifetimes was when BC was mixed with soluble aerosol compounds during emission.</span></p>

scholarly journals In-cloud scavenging scheme for sectional aerosol modules – implementation in the framework of the Sectional Aerosol module for Large Scale Applications version 2.0 (SALSA2.0) global aerosol module

2020 ◽  
Vol 13 (12) ◽  
pp. 6215-6235
Author(s):  
Eemeli Holopainen ◽  
Harri Kokkola ◽  
Anton Laakso ◽  
Thomas Kühn
Keyword(s):  
Black Carbon ◽  
Wet Deposition ◽  
Large Scale ◽  
Cloud Droplet ◽  
Number Concentration ◽  
The Arctic ◽  
Vertical Profiles ◽  
Version 2.0 ◽  
Nucleation Scavenging ◽  
Aerosol Module

Abstract. In this study we introduce an in-cloud wet deposition scheme for liquid and ice phase clouds for global aerosol–climate models which use a size-segregated aerosol description. For in-cloud nucleation scavenging, the scheme uses cloud droplet activation and ice nucleation rates obtained from the host model. For in-cloud impaction scavenging, we used a method where the removal rate depends on the wet aerosol size and cloud droplet radii. We used the latest release version of ECHAM-HAMMOZ (ECHAM6.3-HAM2.3-MOZ1.0) with the Sectional Aerosol module for Large Scale Applications version 2.0 (SALSA) microphysics package to test and compare our scheme. The scheme was compared to a scheme that uses fixed scavenging coefficients. The comparison included vertical profiles and mass and number distributions of wet deposition fluxes of different aerosol compounds and for different latitude bands. Using the scheme presented here, mass concentrations for black carbon, organic carbon, sulfate, and the number concentration of particles with diameters larger than 100 nm are higher than using fixed scavenging coefficients, with the largest differences in the vertical profiles in the Arctic. On the other hand, the number concentrations of particles smaller than 100 nm in diameter show a decrease, especially in the Arctic region. These results could indicate that, compared to fixed scavenging coefficients, nucleation scavenging is less efficient, resulting in an increase in the number concentration of particles larger than 100 nm. In addition, changes in rates of impaction scavenging and new particle formation (NPF) can be the main cause of reduction in the number concentrations of particles smaller than 100 nm. Without further adjustments in the host model, our wet deposition scheme produced unrealistically high aerosol concentrations, especially at high altitudes. This also leads to a spuriously long lifetime of black carbon aerosol. To find a better setup for simulating aerosol vertical profiles and transport, sensitivity simulations were conducted where aerosol emission distribution and hygroscopicity were altered. Vertical profiles of aerosol species simulated with the scheme which uses fixed scavenging rates and the abovementioned sensitivity simulations were evaluated against vertical profiles from aircraft observations. The lifetimes of different aerosol compounds were also evaluated against the ensemble mean of models involved in the Aerosol Comparisons between Observations and Models (AEROCOM) project. The best comparison between the observations and the model was achieved with our wet deposition scheme when black carbon was emitted internally mixed with soluble compounds instead of keeping it externally mixed. This also produced atmospheric lifetimes for the other species which were comparable to the AEROCOM model means.

scholarly journals In-cloud scavenging scheme for aerosol modules

2020 ◽  
Author(s):  
Eemeli Holopainen ◽  
Harri Kokkola ◽  
Anton Laakso ◽  
Thomas Kühn
Keyword(s):  
Black Carbon ◽  
Wet Deposition ◽  
Climate Models ◽  
Removal Rate ◽  
Cloud Droplet ◽  
The Other ◽  
The Arctic ◽  
Vertical Profiles ◽  
Aerosol Emission ◽  
Nucleation Scavenging

Abstract. In this study we introduce an in-cloud wet deposition scheme for liquid and ice phase clouds for global aerosol-climate models which use a size-segregated aerosol description. For in-cloud nucleation scavenging, the scheme uses cloud droplet activation and ice nucleation rates obtained from the host model. For in-cloud impaction scavenging, we used a method where the removal rate depends on the aerosol size and cloud droplet radii. The scheme was compared to a scheme that uses fixed scavenging coefficients. The comparison included vertical profiles and mass and number distributions of wet deposition fluxes of different aerosol compounds and for different latitude bands. Using the scheme presented here, mass concentrations for black carbon, organic carbon, sulfate, and the number concentration of particles with diameters larger than 100 nm are higher than using fixed scavenging coefficients, with the largest differences in the vertical profiles in the Arctic. On the other hand, the number concentrations of small particles show a decrease, especially in the Arctic region. These results indicate that, compared to using fixed scavenging coefficients, nucleation scavenging is less efficient and impaction scavenging is increased in the scheme introduced here. Without further adjustments in the host model, our wet deposition scheme produced unrealistically high aerosol concentrations, especially at high altitudes. This also leads to a spuriously long lifetime of black carbon aerosol. To find a better setup for simulating aerosol vertical profiles and transport, sensitivity simulations were conducted where aerosol emission distribution and hygroscopicity were altered. The simulated vertical profiles of aerosol in these sensitivity studies were evaluated against aircraft observations. The lifetimes of different aerosol compounds were also evaluated against the ensemble mean of models involved in the Aerosol Comparisons between Observations and Models (AEROCOM) project. The best comparison between the observations and the model was achieved with the new wet deposition scheme when black carbon was emitted internally mixed with soluble compounds instead of keeping it externally mixed. This also produced atmospheric lifetimes for the other species which were comparable to the AEROCOM model means.

scholarly journals A simplified empirical method for determination of aerosol hygroscopicity and composition

2010 ◽  
Vol 10 (10) ◽  
pp. 23627-23656
Author(s):  
C. H. Chan ◽  
A. Y. S. Cheng ◽  
A. Viseu
Keyword(s):  
Atmospheric Aerosols ◽  
Climate Model ◽  
Empirical Method ◽  
Radiation Budget ◽  
Cloud Formation ◽  
Monthly Variation ◽  
Aerosol Composition ◽  
Remote System ◽  
Aerosol Hygroscopicity

Abstract. Atmospheric aerosols have substantial influence on the Earth's radiation budget, visibility, cloud formation and precipitation. The aerosol hygroscopicity and the composition of aerosols are of vital importance for solar radiation budget calculation, cloud formation mechanism, and measurement of aerosol spatiotemporal distribution through remote sensing, such as Lidar, MODIS and sun/star photometer. In this paper, hourly averaged records of humidity, visibility and aerosol concentration, conducted in Macao, P.R.C. from 1 February 2006 to 31 December 2008 (LT), are used to estimate aerosol hygroscopicity and composition with a simplified empirical method. The result of monthly variation of aerosol hygroscopicity indicates the important role of aerosol composition on optical properties, which is in agreement with the previous study. This aerosol composition pattern is also consistent with the Asiatic Monsoon pattern and vicinity, such as Hong Kong. The monthly variation of aerosol hygroscopicity and composition also shows the necessity to consider such a factor for the aerosols monitoring by remote system and aerosols forcing simulated by climate model.

scholarly journals The advective Brewer-Dobson circulation in the ERA5 reanalysis: variability and trends

2020 ◽  
Author(s):  
Mohamadou Diallo ◽  
Manfred Ern ◽  
Felix Ploeger
Keyword(s):  
Gravity Wave ◽  
Large Scale ◽  
Climate Model ◽  
Southern Oscillation ◽  
Natural Variability ◽  
Radiation Budget ◽  
Residual Circulation ◽  
Quasi Biennial Oscillation ◽  
Acceleration Rate ◽  
Good Agreement

Abstract. The stratospheric Brewer-Dobson circulation (BDC) is an important element of climate as it determines the transport and distributions of key radiatively active atmospheric trace gases, which affect the Earth’s radiation budget and surface climate. Here, we evaluate the inter-annual variability and trends of the BDC in the ERA5 reanalysis and inter-compare with the ERA-Interim reanalysis for the 1979–2018 period. We also assess the modulation of the circulation by the Quasi-Biennial Oscillation (QBO) and the El Niño-Southern Oscillation (ENSO), and the forcings of the circulation by the planetary and gravity wave drag. A comparison of ERA5 and ERA-Interim reanalyses shows a very good agreement in the morphology of the BDC and in its structural modulations by the natural variability related to QBO and ENSO. Despite the good agreement in the spatial structure, there are substantial differences in the strength of the BDC and of the natural variability impacts on the BDC between the two reanalyses, particularly in the upper troposphere and lower stratosphere (UTLS), and in the upper stratosphere. Throughout most regions of the stratosphere, the variability and trends of the advective BDC are stronger in the ERA5 reanalysis due to stronger planetary and gravity wave forcings, except in the UTLS below 20 km where the tropical upwelling is about 40 % weaker due to a weaker gravity wave forcings at the equatorial flank of the subtropical jet. In the extra-tropics, the large-scale downwelling is stronger in ERA5 than in ERA-Interim linked to significant differences in planetary and gravity wave forcings. Analysis of the BDC trend shows a global acceleration of the annual mean residual circulation with an acceleration rate of about 1.5 % per decade at 70 hPa due to the long-term intensification in gravity and planetary wave breaking, consistent with observed and future climate model predicted BDC changes.

Arctic Sea Ice Reemergence: The Role of Large-Scale Oceanic and Atmospheric Variability*

2015 ◽  
Vol 28 (14) ◽  
pp. 5477-5509 ◽  
Author(s):  
Mitchell Bushuk ◽  
Dimitrios Giannakis ◽  
Andrew J. Majda
Keyword(s):  
Sea Ice ◽  
Large Scale ◽  
Climate Model ◽  
Surface Air Temperature ◽  
Arctic Sea Ice ◽  
The Arctic ◽  
Sea Ice Concentration ◽  
Arctic Sea ◽  
Spring Sea Ice ◽  
Phase Relationships

Abstract Arctic sea ice reemergence is a phenomenon in which spring sea ice anomalies are positively correlated with fall anomalies, despite a loss of correlation over the intervening summer months. This work employs a novel data analysis algorithm for high-dimensional multivariate datasets, coupled nonlinear Laplacian spectral analysis (NLSA), to investigate the regional and temporal aspects of this reemergence phenomenon. Coupled NLSA modes of variability of sea ice concentration (SIC), sea surface temperature (SST), and sea level pressure (SLP) are studied in the Arctic sector of a comprehensive climate model and in observations. It is found that low-dimensional families of NLSA modes are able to efficiently reproduce the prominent lagged correlation features of the raw sea ice data. In both the model and observations, these families provide an SST–sea ice reemergence mechanism, in which melt season (spring) sea ice anomalies are imprinted as SST anomalies and stored over the summer months, allowing for sea ice anomalies of the same sign to reappear in the growth season (fall). The ice anomalies of each family exhibit clear phase relationships between the Barents–Kara Seas, the Labrador Sea, and the Bering Sea, three regions that compose the majority of Arctic sea ice variability. These regional phase relationships in sea ice have a natural explanation via the SLP patterns of each family, which closely resemble the Arctic Oscillation and the Arctic dipole anomaly. These SLP patterns, along with their associated geostrophic winds and surface air temperature advection, provide a large-scale teleconnection between different regions of sea ice variability. Moreover, the SLP patterns suggest another plausible ice reemergence mechanism, via their winter-to-winter regime persistence.

scholarly journals The GFDL CM3 Coupled Climate Model: Characteristics of the Ocean and Sea Ice Simulations

2011 ◽  
Vol 24 (13) ◽  
pp. 3520-3544 ◽  
Author(s):  
Stephen M. Griffies ◽  
Michael Winton ◽  
Leo J. Donner ◽  
Larry W. Horowitz ◽  
Stephanie M. Downes ◽  
...  
Keyword(s):  
Sea Ice ◽  
Large Scale ◽  
Climate Model ◽  
Atmospheric Model ◽  
Arctic Sea Ice ◽  
The Arctic ◽  
Climate Simulation ◽  
Climate Indices ◽  
Geophysical Fluid Dynamics Laboratory ◽  
Coupled Climate Model

Abstract This paper documents time mean simulation characteristics from the ocean and sea ice components in a new coupled climate model developed at the NOAA Geophysical Fluid Dynamics Laboratory (GFDL). The GFDL Climate Model version 3 (CM3) is formulated with effectively the same ocean and sea ice components as the earlier CM2.1 yet with extensive developments made to the atmosphere and land model components. Both CM2.1 and CM3 show stable mean climate indices, such as large-scale circulation and sea surface temperatures (SSTs). There are notable improvements in the CM3 climate simulation relative to CM2.1, including a modified SST bias pattern and reduced biases in the Arctic sea ice cover. The authors anticipate SST differences between CM2.1 and CM3 in lower latitudes through analysis of the atmospheric fluxes at the ocean surface in corresponding Atmospheric Model Intercomparison Project (AMIP) simulations. In contrast, SST changes in the high latitudes are dominated by ocean and sea ice effects absent in AMIP simulations. The ocean interior simulation in CM3 is generally warmer than in CM2.1, which adversely impacts the interior biases.

scholarly journals Cloud, precipitation and radiation responses to large perturbations in global dimethyl sulfide

2018 ◽  
Vol 18 (14) ◽  
pp. 10177-10198 ◽  
Author(s):  
Sonya L. Fiddes ◽  
Matthew T. Woodhouse ◽  
Zebedee Nicholls ◽  
Todd P. Lane ◽  
Robyn Schofield
Keyword(s):  
Large Scale ◽  
Climate Models ◽  
Dimethyl Sulfide ◽  
Cloud Fraction ◽  
Global Climate Models ◽  
Radiation Budget ◽  
Shortwave Radiation ◽  
Stratiform Cloud ◽  
Aerosol Emission ◽  
Low Cloud

Abstract. Natural aerosol emission represents one of the largest uncertainties in our understanding of the radiation budget. Sulfur emitted by marine organisms, as dimethyl sulfide (DMS), constitutes one-fifth of the global sulfur budget and yet the distribution, fluxes and fate of DMS remain poorly constrained. This study evaluates the Australian Community Climate and Earth System Simulator (ACCESS) United Kingdom Chemistry and Aerosol (UKCA) model in terms of cloud fraction, radiation and precipitation, and then quantifies the role of DMS in the chemistry–climate system. We find that ACCESS-UKCA has similar cloud and radiation biases to other global climate models. By removing all DMS, or alternatively significantly enhancing marine DMS, we find a top of the atmosphere radiative effect of 1.7 and −1.4 W m−2 respectively. The largest responses to these DMS perturbations (removal/enhancement) are in stratiform cloud decks in the Southern Hemisphere's eastern ocean basins. These regions show significant differences in low cloud (-9/+6 %), surface incoming shortwave radiation (+7/-5 W m−2) and large-scale rainfall (+15/-10 %). We demonstrate a precipitation suppression effect of DMS-derived aerosol in stratiform cloud deck regions due to DMS, coupled with an increase in low cloud fraction. The difference in low cloud fraction is an example of the aerosol lifetime effect. Globally, we find a sensitivity of temperature to annual DMS flux of 0.027 and 0.019 K per Tg yr−1 of sulfur, respectively. Other areas of low cloud formation, such as the Southern Ocean and stratiform cloud decks in the Northern Hemisphere, have a relatively weak response to DMS perturbations. We highlight the need for greater understanding of the DMS–climate cycle within the context of uncertainties and biases of climate models as well as those of DMS–climate observations.

scholarly journals Large-scale transport into the Arctic: the roles of the midlatitude jet and the Hadley Cell

2019 ◽  
Vol 19 (8) ◽  
pp. 5511-5528 ◽  
Author(s):  
Huang Yang ◽  
Darryn W. Waugh ◽  
Clara Orbe ◽  
Guang Zeng ◽  
Olaf Morgenstern ◽  
...  
Keyword(s):  
Large Scale ◽  
Climate Model ◽  
Source Region ◽  
Meridional Flow ◽  
Hadley Cell ◽  
The Arctic ◽  
Boreal Summer ◽  
Boreal Winter ◽  
Meridional Transport ◽  
Fixed Lifetime

Abstract. Transport from the Northern Hemisphere (NH) midlatitudes to the Arctic plays a crucial role in determining the abundance of trace gases and aerosols that are important to Arctic climate via impacts on radiation and chemistry. Here we examine this transport using an idealized tracer with a fixed lifetime and predominantly midlatitude land-based sources in models participating in the Chemistry Climate Model Initiative (CCMI). We show that there is a 25 %–45 % difference in the Arctic concentrations of this tracer among the models. This spread is correlated with the spread in the location of the Pacific jet, as well as the spread in the location of the Hadley Cell (HC) edge, which varies consistently with jet latitude. Our results suggest that it is likely that the HC-related zonal-mean meridional transport rather than the jet-related eddy mixing is the major contributor to the inter-model spread in the transport of land-based tracers into the Arctic. Specifically, in models with a more northern jet, the HC generally extends further north and the tracer source region is mostly covered by surface southward flow associated with the lower branch of the HC, resulting in less efficient transport poleward to the Arctic. During boreal summer, there are poleward biases in jet location in free-running models, and these models likely underestimate the rate of transport into the Arctic. Models using specified dynamics do not have biases in the jet location, but do have biases in the surface meridional flow, which may result in differences in transport into the Arctic. In addition to the land-based tracer, the midlatitude-to-Arctic transport is further examined by another idealized tracer with zonally uniform sources. With equal sources from both land and ocean, the inter-model spread of this zonally uniform tracer is more related to variations in parameterized convection over oceans rather than variations in HC extent, particularly during boreal winter. This suggests that transport of land-based and oceanic tracers or aerosols towards the Arctic differs in pathways and therefore their corresponding inter-model variabilities result from different physical processes.

The advective Brewer-Dobson circulation in the ERA5 reanalysis: climatology, variability, and trends

2021 ◽  
Author(s):  
Mohamadou Diallo ◽  
Manfred Ern ◽  
Felix Ploeger
Keyword(s):  
Gravity Wave ◽  
Large Scale ◽  
Climate Model ◽  
Southern Oscillation ◽  
Natural Variability ◽  
Radiation Budget ◽  
Residual Circulation ◽  
Quasi Biennial Oscillation ◽  
Acceleration Rate ◽  
Good Agreement

<p>The stratospheric Brewer-Dobson circulation (BDC) is an important element of climate as it determines the transport and distributions of key radiatively active atmospheric trace gases, which affect the Earth’s radiation budget and surface climate.<br>Here, we evaluate the inter-annual variability and trends of the BDC in the ERA5 reanalysis and inter-compare with the ERA-Interim reanalysis for the 1979–2018 period. We also assess the modulation of the circulation by the Quasi-Biennial Oscillation (QBO) and the El Niño-Southern Oscillation (ENSO), and the forcings of the circulation by the planetary and gravity wave drag. A comparison of ERA5 and ERA-Interim reanalyses shows a very good agreement in the morphology of the BDC and in its structural modulations by the natural variability related to QBO and ENSO. Despite the good agreement in the spatial structure, there are substantial differences in the strength of the BDC and of the natural variability impacts on the BDC between the two reanalyses, particularly in the upper troposphere and lower stratosphere (UTLS), and in the upper stratosphere. Throughout most regions of the stratosphere, the variability and trends of the advective BDC are stronger in the ERA5 reanalysis due to stronger planetary and gravity wave forcings, except in the UTLS below 20 km where the tropical upwelling is about 40 % weaker due to a weaker gravity wave forcings at the equatorial flank of the subtropical jet. In the extra-tropics, the large-scale downwelling is stronger in ERA5 than in ERA-Interim linked to significant differences in planetary and gravity wave forcings. Analysis of the BDC trend shows a global acceleration of the annual mean residual circulation with an acceleration rate of about 1.5 % per decade at 70 hPa due to the long-term intensification in gravity and planetary wave breaking, consistent with observed and future climate model predicted BDC changes.</p>

The ocean response to changes of the Greenland Ice sheet in a warming climate

2020 ◽  
Author(s):  
Marianne S. Madsen ◽  
Shuting Yang ◽  
Christian Rodehacke ◽  
Guðfinna Aðalgeirsdóttir ◽  
Synne H. Svendsen ◽  
...  
Keyword(s):  
Mass Loss ◽  
Ocean Circulation ◽  
Large Scale ◽  
Climate Model ◽  
Variable Mass ◽  
Ice Sheet ◽  
Greenland Ice Sheet ◽  
Model System ◽  
Meridional Overturning Circulation ◽  
The Arctic

<p>During recent decades, increased and highly variable mass loss from the Greenland ice sheet has been observed, implying that the ice sheet can respond to changes in ocean and atmospheric conditions on annual to decadal time scales. Changes in ice sheet topography and increased mass loss into the ocean may impact large scale atmosphere and ocean circulation. Therefore, coupling of ice sheet and climate models, to explicitly include the processes and feedbacks of ice sheet changes, is needed to improve the understanding of ice sheet-climate interactions.</p><p>Here, we present results from the coupled ice sheet-climate model system, EC-Earth-PISM. The model consists of the atmosphere, ocean and sea-ice model system EC-Earth, two-way coupled to the Parallel Ice Sheet Model, PISM. The surface mass balance (SMB) is calculated within EC-Earth, from the precipitation, evaporation and surface melt of snow and ice, to ensure conservation of mass and energy. The ice sheet model, PISM, calculates ice dynamical changes in ice discharge and basal melt as well as changes in ice extent and thickness. Idealized climate change experiments have been performed starting from pre-industrial conditions for a) constant forcing (pre-industrial control); b) abruptly quadrupling the CO<sub>2</sub> concentration; and c) gradually increasing the CO<sub>2</sub> concentration by 1% per year until 4xCO<sub>2</sub> is reached.  All three experiments are run for 350 years.</p><p>Our results show a significant impact of the interactive ice sheet component on heat and fresh water fluxes into the Arctic and North Atlantic Oceans. The interactive ice sheet causes freshening of the Arctic Ocean and affects deep water formation, resulting in a significant delay of the recovery of the Atlantic Meridional Overturning Circulation (AMOC) in the coupled 4xCO<sub>2</sub> experiments, when compared with uncoupled experiments.</p>

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