scholarly journals AerChemMIP: Quantifying the effects of chemistry and aerosols in CMIP6

Author(s):  
William J. Collins ◽  
Jean-François Lamarque ◽  
Michael Schulz ◽  
Olivier Boucher ◽  
Veronika Eyring ◽  
...  

Abstract. The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) is endorsed by the Coupled-Model Intercomparison Project 6 (CMIP6) and is designed to quantify the climate and air quality impacts of aerosols and chemically-reactive gases. These are specifically near-term climate forcers (NTCFs: tropospheric ozone and aerosols, and their precursors), methane, nitrous oxide and ozone-depleting halocarbons. The aim of AerChemMIP is to answer four scientific questions: 1. How have anthropogenic emissions contributed to global radiative forcing and affected regional climate over the historical period? 2. How will future policies (on climate, air quality and land use) affect these species and their climate impacts? 3. Can the uncertainties associated with anthropogenic emissions be quantified? 4. Can climate feedbacks occurring through changes in natural emissions be quantified? These questions will be addressed through targeted simulations with CMIP6 climate models that include an interactive representation of tropospheric aerosols and atmospheric chemistry. These simulations build on the CMIP6 Diagnostic, Evaluation and Characterization of Klima (DECK) experiments, the CMIP6 historical simulations, and future projections performed elsewhere in CMIP6, allowing the contributions from aerosols and chemistry to be quantified. Specific diagnostics are requested as part of the CMIP6 data request to evaluate the performance of the models, and to understand any differences in behaviour between them.

2017 ◽  
Vol 10 (2) ◽  
pp. 585-607 ◽  
Author(s):  
William J. Collins ◽  
Jean-François Lamarque ◽  
Michael Schulz ◽  
Olivier Boucher ◽  
Veronika Eyring ◽  
...  

Abstract. The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) is endorsed by the Coupled-Model Intercomparison Project 6 (CMIP6) and is designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases. These are specifically near-term climate forcers (NTCFs: methane, tropospheric ozone and aerosols, and their precursors), nitrous oxide and ozone-depleting halocarbons. The aim of AerChemMIP is to answer four scientific questions. 1. How have anthropogenic emissions contributed to global radiative forcing and affected regional climate over the historical period? 2. How might future policies (on climate, air quality and land use) affect the abundances of NTCFs and their climate impacts? 3.How do uncertainties in historical NTCF emissions affect radiative forcing estimates? 4. How important are climate feedbacks to natural NTCF emissions, atmospheric composition, and radiative effects? These questions will be addressed through targeted simulations with CMIP6 climate models that include an interactive representation of tropospheric aerosols and atmospheric chemistry. These simulations build on the CMIP6 Diagnostic, Evaluation and Characterization of Klima (DECK) experiments, the CMIP6 historical simulations, and future projections performed elsewhere in CMIP6, allowing the contributions from aerosols and/or chemistry to be quantified. Specific diagnostics are requested as part of the CMIP6 data request to highlight the chemical composition of the atmosphere, to evaluate the performance of the models, and to understand differences in behaviour between them.


2020 ◽  
Author(s):  
Zebedee R. J. Nicholls ◽  
Malte Meinshausen ◽  
Jared Lewis ◽  
Robert Gieseke ◽  
Dietmar Dommenget ◽  
...  

Abstract. Here we present results from the first phase of the Reduced Complexity Model Intercomparison Project (RCMIP). RCMIP is a systematic examination of reduced complexity climate models (RCMs), which are used to complement and extend the insights from more complex Earth System Models (ESMs), in particular those participating in the Sixth Coupled Model Intercomparison Project (CMIP6). In Phase 1 of RCMIP, with 14 participating models namely ACC2, AR5IR (2 and 3 box versions), CICERO-SCM, ESCIMO, FaIR, GIR, GREB, Hector, Held et al. two layer model, MAGICC, MCE, OSCAR and WASP, we highlight the structural differences across various RCMs and show that RCMs are capable of reproducing global-mean surface air temperature (GSAT) changes of ESMs and historical observations. We find that some RCMs are capable of emulating the GSAT response of CMIP6 models to within a root-mean square error of 0.2 °C (of the same order of magnitude as ESM internal variability) over a range of scenarios. Running the same model configurations for both RCP and SSP scenarios, we see that the SSPs exhibit higher effective radiative forcing throughout the second half of the 21st Century. Comparing our results to the difference between CMIP5 and CMIP6 output, we find that the change in scenario explains approximately 46 % of the increase in higher end projected warming between CMIP5 and CMIP6. This suggests that changes in ESMs from CMIP5 to CMIP6 explain the rest of the increase, hence the higher climate sensitivities of available CMIP6 models may not be having as large an impact on GSAT projections as first anticipated. A second phase of RCMIP will complement RCMIP Phase 1 by exploring probabilistic results and emulation in more depth to provide results available for the IPCC's Sixth Assessment Report author teams.


2020 ◽  
Vol 20 (16) ◽  
pp. 9591-9618 ◽  
Author(s):  
Christopher J. Smith ◽  
Ryan J. Kramer ◽  
Gunnar Myhre ◽  
Kari Alterskjær ◽  
William Collins ◽  
...  

Abstract. The effective radiative forcing, which includes the instantaneous forcing plus adjustments from the atmosphere and surface, has emerged as the key metric of evaluating human and natural influence on the climate. We evaluate effective radiative forcing and adjustments in 17 contemporary climate models that are participating in the Coupled Model Intercomparison Project (CMIP6) and have contributed to the Radiative Forcing Model Intercomparison Project (RFMIP). Present-day (2014) global-mean anthropogenic forcing relative to pre-industrial (1850) levels from climate models stands at 2.00 (±0.23) W m−2, comprised of 1.81 (±0.09) W m−2 from CO2, 1.08 (± 0.21) W m−2 from other well-mixed greenhouse gases, −1.01 (± 0.23) W m−2 from aerosols and −0.09 (±0.13) W m−2 from land use change. Quoted uncertainties are 1 standard deviation across model best estimates, and 90 % confidence in the reported forcings, due to internal variability, is typically within 0.1 W m−2. The majority of the remaining 0.21 W m−2 is likely to be from ozone. In most cases, the largest contributors to the spread in effective radiative forcing (ERF) is from the instantaneous radiative forcing (IRF) and from cloud responses, particularly aerosol–cloud interactions to aerosol forcing. As determined in previous studies, cancellation of tropospheric and surface adjustments means that the stratospherically adjusted radiative forcing is approximately equal to ERF for greenhouse gas forcing but not for aerosols, and consequentially, not for the anthropogenic total. The spread of aerosol forcing ranges from −0.63 to −1.37 W m−2, exhibiting a less negative mean and narrower range compared to 10 CMIP5 models. The spread in 4×CO2 forcing has also narrowed in CMIP6 compared to 13 CMIP5 models. Aerosol forcing is uncorrelated with climate sensitivity. Therefore, there is no evidence to suggest that the increasing spread in climate sensitivity in CMIP6 models, particularly related to high-sensitivity models, is a consequence of a stronger negative present-day aerosol forcing and little evidence that modelling groups are systematically tuning climate sensitivity or aerosol forcing to recreate observed historical warming.


2012 ◽  
Vol 12 (9) ◽  
pp. 23603-23644 ◽  
Author(s):  
K. Bowman ◽  
D. Shindell ◽  
H. Worden ◽  
J. F. Lamarque ◽  
P. J. Young ◽  
...  

Abstract. We use simultaneous observations of ozone and outgoing longwave radiation (OLR) from the Tropospheric Emission Spectrometer (TES) to evaluate ozone distributions and radiative forcing simulated by a suite of chemistry-climate models that participated in the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP). The ensemble mean of ACCMIP models show a persistent but modest tropospheric ozone low bias (5–20 ppb) in the Southern Hemisphere (SH) and modest high bias (5–10 ppb) in the Northern Hemisphere (NH) relative to TES for 2005–2010. These biases lead to substantial differences in ozone instantaneous radiative forcing between TES and the ACCMIP simulations. Using TES instantaneous radiative kernels (IRK), we show that the ACCMIP ensemble mean has a low bias in the SH tropics of up to 100 m W m−2 locally and a global low bias of 35 ± 44 m W m−2 relative to TES. Combining ACCMIP preindustrial ozone and the TES present-day ozone, we calculate an observationally constrained estimate of tropospheric ozone radiative forcing (RF) of 399 ± 70 m W m−2, which is about 7% higher than using the ACCMIP models alone but with the same standard deviation (Stevenson et al., 2012). In addition, we explore an alternate approach to constraining radiative forcing estimates by choosing a subset of models that best match TES ozone, which leads to an ozone RF of 369 ± 42 m W m−2. This estimate is closer to the ACCMIP ensemble mean RF but about a 40% reduction in standard deviation. These results point towards a profitable direction of combining observations and chemistry-climate model simulations to reduce uncertainty in ozone radiative forcing.


2016 ◽  
Vol 29 (4) ◽  
pp. 1417-1428 ◽  
Author(s):  
Petr Chylek ◽  
Timothy J. Vogelsang ◽  
James D. Klett ◽  
Nicholas Hengartner ◽  
Dave Higdon ◽  
...  

Abstract Phase 5 of the Coupled Model Intercomparison Project (CMIP5) climate models’ projections of the 2014–2100 Arctic warming under radiative forcing from representative concentration pathway 4.5 (RCP4.5) vary from 0.9° to 6.7°C. Climate models with or without a full indirect aerosol effect are both equally successful in reproducing the observed (1900–2014) Arctic warming and its trends. However, the 2014–2100 Arctic warming and the warming trends projected by models that include a full indirect aerosol effect (denoted here as AA models) are significantly higher (mean projected Arctic warming is about 1.5°C higher) than those projected by models without a full indirect aerosol effect (denoted here as NAA models). The suggestion is that, within models including full indirect aerosol effects, those projecting stronger future changes are not necessarily distinguishable historically because any stronger past warming may have been partially offset by stronger historical aerosol cooling. The CMIP5 models that include a full indirect aerosol effect follow an inverse radiative forcing to equilibrium climate sensitivity relationship, while models without it do not.


2013 ◽  
Vol 13 (6) ◽  
pp. 2939-2974 ◽  
Author(s):  
D. T. Shindell ◽  
J.-F. Lamarque ◽  
M. Schulz ◽  
M. Flanner ◽  
C. Jiao ◽  
...  

Abstract. The Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) examined the short-lived drivers of climate change in current climate models. Here we evaluate the 10 ACCMIP models that included aerosols, 8 of which also participated in the Coupled Model Intercomparison Project phase 5 (CMIP5). The models reproduce present-day total aerosol optical depth (AOD) relatively well, though many are biased low. Contributions from individual aerosol components are quite different, however, and most models underestimate east Asian AOD. The models capture most 1980–2000 AOD trends well, but underpredict increases over the Yellow/Eastern Sea. They strongly underestimate absorbing AOD in many regions. We examine both the direct radiative forcing (RF) and the forcing including rapid adjustments (effective radiative forcing; ERF, including direct and indirect effects). The models' all-sky 1850 to 2000 global mean annual average total aerosol RF is (mean; range) −0.26 W m−2; −0.06 to −0.49 W m−2. Screening based on model skill in capturing observed AOD yields a best estimate of −0.42 W m−2; −0.33 to −0.50 W m−2, including adjustment for missing aerosol components in some models. Many ACCMIP and CMIP5 models appear to produce substantially smaller aerosol RF than this best estimate. Climate feedbacks contribute substantially (35 to −58%) to modeled historical aerosol RF. The 1850 to 2000 aerosol ERF is −1.17 W m−2; −0.71 to −1.44 W m−2. Thus adjustments, including clouds, typically cause greater forcing than direct RF. Despite this, the multi-model spread relative to the mean is typically the same for ERF as it is for RF, or even smaller, over areas with substantial forcing. The largest 1850 to 2000 negative aerosol RF and ERF values are over and near Europe, south and east Asia and North America. ERF, however, is positive over the Sahara, the Karakoram, high Southern latitudes and especially the Arctic. Global aerosol RF peaks in most models around 1980, declining thereafter with only weak sensitivity to the Representative Concentration Pathway (RCP). One model, however, projects approximately stable RF levels, while two show increasingly negative RF due to nitrate (not included in most models). Aerosol ERF, in contrast, becomes more negative during 1980 to 2000. During this period, increased Asian emissions appear to have a larger impact on aerosol ERF than European and North American decreases due to their being upwind of the large, relatively pristine Pacific Ocean. There is no clear relationship between historical aerosol ERF and climate sensitivity in the CMIP5 subset of ACCMIP models. In the ACCMIP/CMIP5 models, historical aerosol ERF of about −0.8 to −1.5 W m−2 is most consistent with observed historical warming. Aerosol ERF masks a large portion of greenhouse forcing during the late 20th and early 21st century at the global scale. Regionally, aerosol ERF is so large that net forcing is negative over most industrialized and biomass burning regions through 1980, but remains strongly negative only over east and southeast Asia by 2000. Net forcing is strongly positive by 1980 over most deserts, the Arctic, Australia, and most tropical oceans. Both the magnitude of and area covered by positive forcing expand steadily thereafter.


2020 ◽  
Author(s):  
Sophie Nowicki ◽  
Antony J. Payne ◽  
Heiko Goelzer ◽  
Helene Seroussi ◽  
William H. Lipscomb ◽  
...  

Abstract. Projection of the contribution of ice sheets to sea-level change as part of the Coupled Model Intercomparison Project – phase 6 (CMIP6) takes the form of simulations from coupled ice-sheet-climate models and standalone ice sheet models, overseen by the Ice Sheet Model Intercomparison Project for CMIP6 (ISMIP6). This paper describes the experimental setup for process-based sea-level change projections to be performed with standalone Greenland and Antarctic ice sheet models in the context of ISMIP6. The ISMIP6 protocol relies on a suite of polar atmospheric and oceanic CMIP-based forcing for ice sheet models, in order to explore the uncertainty in projected sea-level change due to future emissions scenarios, CMIP models, ice sheet models, and parameterizations for ice-ocean interactions. We describe here the approach taken for defining the suite of ISMIP6 standalone ice sheet simulations, document the experimental framework and implementation, as well as present an overview of the ISMIP6 forcing to be used by participating ice sheet modeling groups.


2021 ◽  
Author(s):  
Paul Griffiths ◽  
Zeng Guang ◽  
Sungbo Shim ◽  
Jane Mulcahy ◽  
Lee Murray ◽  
...  

<p>A grand challenge in the field of chemistry-climate modelling is to understand the connection between anthropogenic emissions, atmospheric composition and the radiative forcing of trace gases and aerosols.   The AerChemMIP model intercomparison project, part of CMIP6, focuses on calculating the radiative forcing of gases and aerosol particles over the period 1850 to 2100.  We present an analysis of the trends in tropospheric ozone budget in the UKESM1 and other models from CMIP6 experiments. We discuss these trends in terms of chemical production and loss of ozone as well as physical processes such as transport and deposition.  Where possible, AerChemMIP attribution experiments such as histSST-piCH4, will be used to quantify the effect of individual emissions and forcing changes on the historical ozone burden and budget.  For future experiments, we focus on analogous experiments from the SSP3-70 scenario, a ‘regional rivalry’ shared socioeconomic pathway involving significant emissions changes.</p>


Author(s):  
Shuwen Zhao ◽  
Yongqiang Yu ◽  
Pengfei Lin ◽  
Hailong Liu ◽  
Bian He ◽  
...  

AbstractThe datasets for the tier-1 Scenario Model Intercomparison Project (ScenarioMIP) experiments from the Chinese Academy of Sciences (CAS) Flexible Global Ocean-Atmosphere-Land System model, finite-volume version 3 (CAS FGOALS-f3-L) are described in this study. ScenarioMIP is one of the core MIP experiments in phase 6 of the Coupled Model Intercomparison Project (CMIP6). Considering future CO2, CH4, N2O and other gases’ concentrations, as well as land use, the design of ScenarioMIP involves eight pathways, including two tiers (tier-1 and tier-2) of priority. Tier-1 includes four combined Shared Socioeconomic Pathways (SSPs) with radiative forcing, i.e., SSP1-2.6, SSP2-4.5, SSP3-7.0 and SSP5-8.5, in which the globally averaged radiative forcing at the top of the atmosphere around the year 2100 is approximately 2.6, 4.5, 7.0 and 8.5 W m−2, respectively. This study provides an introduction to the ScenarioMIP datasets of this model, such as their storage location, sizes, variables, etc. Preliminary analysis indicates that surface air temperatures will increase by about 1.89°C, 3.07°C, 4.06°C and 5.17°C by around 2100 under these four scenarios, respectively. Meanwhile, some other key climate variables, such as sea-ice extension, precipitation, heat content, and sea level rise, also show significant long-term trends associated with the radiative forcing increases. These datasets will help us understand how the climate will change under different anthropogenic and radiative forcings.


2018 ◽  
Vol 18 (3) ◽  
pp. 2287-2305 ◽  
Author(s):  
Rick D. Russotto ◽  
Thomas P. Ackerman

Abstract. The polar amplification of warming and the ability of the Intertropical Convergence Zone (ITCZ) to shift to the north or south are two very important problems in climate science. Examining these behaviors in global climate models (GCMs) running solar geoengineering experiments is helpful not only for predicting the effects of solar geoengineering but also for understanding how these processes work under increased carbon dioxide (CO2). Both polar amplification and ITCZ shifts are closely related to the meridional transport of moist static energy (MSE) by the atmosphere. This study examines changes in MSE transport in 10 fully coupled GCMs in experiment G1 of the Geoengineering Model Intercomparison Project (GeoMIP), in which the solar constant is reduced to compensate for the radiative forcing from abruptly quadrupled CO2 concentrations. In G1, poleward MSE transport decreases relative to preindustrial conditions in all models, in contrast to the Coupled Model Intercomparison Project phase 5 (CMIP5) abrupt4xCO2 experiment, in which poleward MSE transport increases. We show that since poleward energy transport decreases rather than increases, and local feedbacks cannot change the sign of an initial temperature change, the residual polar amplification in the G1 experiment must be due to the net positive forcing in the polar regions and net negative forcing in the tropics, which arise from the different spatial patterns of the simultaneously imposed solar and CO2 forcings. However, the reduction in poleward energy transport likely plays a role in limiting the polar warming in G1. An attribution study with a moist energy balance model shows that cloud feedbacks are the largest source of uncertainty regarding changes in poleward energy transport in midlatitudes in G1, as well as for changes in cross-equatorial energy transport, which are anticorrelated with ITCZ shifts.


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