Spontaneous decay-induced quantum dynamics in Rydberg-blockaded Λ-type atoms

Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, spontaneous decay from the Rydberg state to an additional pooling state renders the ensemble no longer a closed superatom. Herein we present a computationally efficient model to characterize the interaction between a fully Rydberg-blockaded ensemble of N Λ-type three-level atoms and a strong probe light field in a coherent state. The model enables us to achieve a decomposition of the coupled dynamics in the strong field limit, which significantly reduces the complexity of computing the N-body system evolution and paves the way for practical analysis in experiments. A quasi-steady-state power spectrum with multiple sidebands is found in the scattered field. The relative heights of the sidebands show a time-dependence determined by the atomic relaxation, which illuminates potential applications of using the system in information transfer of quantum networks. With negligible dissipative flipping to the unsymmetrical states, the atomic relaxation time, indicating a linearly increasing pooling state fraction, is derived analytically as a function of the number of atoms.

Direct insight into the structure-property relation of interfaces from constrained crystal structure prediction

A major issue that prevents a full understanding of heterogeneous materials is the lack of systematic first-principles methods to consistently predict energetics and electronic properties of reconstructed interfaces. In this work we address this problem with an efficient and accurate computational scheme. We extend the minima-hopping method implementing constraints crafted for two-dimensional atomic relaxation and enabling variations of the atomic density close to the interface. A combination of density-functional and accurate density-functional tight-binding calculations supply energy and forces to structure prediction. We demonstrate the power of this method by applying it to extract structure-property relations for a large and varied family of symmetric and asymmetric tilt boundaries in polycrystalline silicon. We find a rich polymorphism in the interface reconstructions, with recurring bonding patterns that we classify in increasing energetic order. Finally, a clear relation between bonding patterns and electrically active grain boundary states is unveiled and discussed.

Development of a new database for Auger electron and X-ray spectra

An energy correction method is described to account for the Breit and QED effects on Auger electrons and X-ray energies in the recently developed atomic relaxation model BrIccEmis. The results are compared with literature and new experimental data for Z = 52. Overall this improves the agreement of the calculated energies with the literature values. A new atomic radiation database NS_Radlist, will contain atomic transition energies from the BrIccEmis program with these energy corrections.

Study of the spatial resolution of low-material GEM tracking detectors

The spatial resolution of GEM based tracking detectors has been simulated and measured. The simulation includes the GEANT4 based transport of high energy electrons with careful accounting for atomic relaxation processes including emission of fluorescent photons and Auger electrons and custom post-processing, including accounting for diffusion, gas amplification fluctuations, the distribution of signals on readout electrodes, electronics noise and a particular algorithm of the final coordinate calculation (center of gravity). The simulation demonstrates that a minimum of the spatial resolution of about 10 μm can be achieved with strip pitches from 250 μm to 300 μm. For larger pitches the resolution is quickly degrading reaching 80-100 μm at a pitch of 500 μm. The spatial resolution of low-material triple-GEM detectors for the DEUTRON facility at the VEPP-3 storage ring is measured at the extracted beam facility of the VEPP-4M collider. The amount of material in these detectors is reduced by etching the copper of the GEMs electrodes and using a readout structure on a thin kapton foil rather than on a glass fibre plate. The exact amount of material in one DEUTRON detector is measured by studying multiple scattering of 100 MeV electrons in it. The result of these measurements is X/X0 = 2.4×10−3 corresponding to a thickness of the copper layers of the GEM foils of 3 μm. The spatial resolution of one DEUTRON detector is measured with 500 MeV electrons and the measured value is equal to 35 ± 1 μm for orthogonal tracks.