Carbon dot-coupled BiVO4/reduced graphene hydrogel for significant enhancement of photocatalytic activity: antibiotic degradation and CO2 reduction

2021 ◽  
pp. 150564
Author(s):  
Changchang Ma ◽  
Zhuohong Xie ◽  
Won Cheol Seo ◽  
Syed Taj Ud Din ◽  
Jeongwoo Lee ◽  
...  
Author(s):  
Tingting Cai ◽  
Qing Chang ◽  
Bin Liu ◽  
Caihong Hao ◽  
Jinlong Yang ◽  
...  

The photocatalyst performance highly relies on the quantity of carrier transfer from the bulk to surface during the catalytic process. However, the polarization electric field induced by charge accumulation at...


2021 ◽  
pp. 138897
Author(s):  
Suresh Sagadevan ◽  
J. Anita Lett ◽  
Getu Kassegn Weldegebrieal ◽  
Md Rokon ud Dowla Biswas ◽  
Won Chun Oh ◽  
...  

2017 ◽  
Vol 198 ◽  
pp. 397-407 ◽  
Author(s):  
Tomoaki Takayama ◽  
Ko Sato ◽  
Takehiro Fujimura ◽  
Yuki Kojima ◽  
Akihide Iwase ◽  
...  

CuGaS2, (AgInS2)x–(ZnS)2−2x, Ag2ZnGeS4, Ni- or Pb-doped ZnS, (ZnS)0.9–(CuCl)0.1, and ZnGa0.5In1.5S4 showed activities for CO2 reduction to form CO and/or HCOOH in an aqueous solution containing K2SO3 and Na2S as electron donors under visible light irradiation. Among them, CuGaS2 and Ni-doped ZnS photocatalysts showed relatively high activities for CO and HCOOH formation, respectively. CuGaS2 was applied in a powdered Z-scheme system combining with reduced graphene oxide (RGO)-incorporated TiO2 as an O2-evolving photocatalyst. The powdered Z-scheme system produced CO from CO2 in addition to H2 and O2 due to water splitting. Oxygen evolution with an almost stoichiometric amount indicates that water was consumed as an electron donor in the Z-schematic CO2 reduction. Thus, we successfully demonstrated CO2 reduction of artificial photosynthesis using a simple Z-scheme system in which two kinds of photocatalyst powders (CuGaS2 and an RGO–TiO2 composite) were only dispersed in water under 1 atm of CO2.


Chemosphere ◽  
2021 ◽  
pp. 131731
Author(s):  
Alvin Lim Teik Zheng ◽  
Sarah Sabidi ◽  
Teruhisa Ohno ◽  
Maeda Toshinari ◽  
Yoshito Andou

RSC Advances ◽  
2016 ◽  
Vol 6 (18) ◽  
pp. 15080-15086 ◽  
Author(s):  
Zegao Wang ◽  
Yuanfu Chen ◽  
Pingjian Li ◽  
Jiarui He ◽  
Wanli Zhang ◽  
...  

The silicon-doped reduced graphene oxide was synthesized via annealing treatment of triphenylsilane and graphene oxide. It exhibits significant enhancement in electrocatalytic and electrochemical properties.


NANO ◽  
2017 ◽  
Vol 12 (03) ◽  
pp. 1750032 ◽  
Author(s):  
H.-Y. He

Reduced graphene oxide-SnSe (rGO-SnSe) nanohybrids were synthesized with a solution chemical reaction at room temperature. The nanohybrids were characterized by various techniques for their microstructural and photocatalytic activities in photodegradation of alkaline dye malachite green in the water. The effects of rGO/SnSe ratio, initial solution pH, and H2O2 concentration on the photodegradation efficiency were studied. The SnSe nanocrystallines with nanoscale size and narrow bandgap were formed and uniformly adhered on the rGO surface. Raman analysis confirmed the reduction of GO. The experimental results indicated that the nanohybrids showed excellent sunlight-excited photocatalytic activity in degrading malachite green in the water. Significantly, the nanohybrids showed remarkable photo-Fenton-like catalytic activity. The photodegradation rates of the hybrids were greater than that of SnSe nanoparticles, increased with increasing rGO/SnSe ratio, and related to operation parameters. High photocatalytic activities were ascribed to the efficiency interface effect that was confirmed by the calculations of band energy level and photoconductivity. The TOC measurement further verified the photodegradation results. The nanoparticles and nanohybrids also showed excellent reusability.


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