Atmospheric deposition fluxes of 137Cs associated with dust fallout in the northeastern Arabian Gulf

2018 ◽  
Vol 192 ◽  
pp. 565-572 ◽  
Author(s):  
A. Aba ◽  
A.M. Al-Dousari ◽  
A. Ismaeel
Author(s):  
Viša Tasić ◽  
Aleksandar Simonovski ◽  
Tatjana Apostolovski-Trijić ◽  
Tamara Urošević ◽  
Aleksandra Ivanović

In this paper the analysis of atmospheric deposition fluxes of Pb, Cd, Ni, and As in the Bor town (Serbia) is presented for the period 2011-2020. The results of measurements from the period of operation of the old smelter (2011-2015) were compared with the results of measurements during the period of operation of the new smelter (2016-2020). As a result of changes in the copper smelting technology and the better treatment of waste gases in the smelter, the average level of the total atmospheric depositon (TAD) was reduced by 63% in the period 2016-2020. The reduction of atmospheric deposition fluxes of Pb (59%), Cd (34%), and As (65%) are detected at all sampling points in the period 2016-2020. In contrast, the fluxes of Ni were increased (211%). Also, pH values of TAD have been changed at all sampling points from acidic (5.7 pH), during the period of operation of the old smelter, to alkaline (7.7 pH) in the period of operation of the new smelter.The presence of a very strong (r>0.8) and strong (0.8>r>0.6) Pearson correlation between the atmospheric deposition fluxes of cancerogenic elements were determined at all sampling points during the period 2016-2020, as opposed to the period 2011-2015 where these correlations were weak (r<0.4).


1997 ◽  
Vol 31 (5) ◽  
pp. 1390-1398 ◽  
Author(s):  
Laura L. McConnell ◽  
Eric Nelson ◽  
Clifford P. Rice ◽  
Joel E. Baker ◽  
W. Edward Johnson ◽  
...  

2014 ◽  
Vol 2014 ◽  
pp. 1-27 ◽  
Author(s):  
M. Amodio ◽  
S. Catino ◽  
P. R. Dambruoso ◽  
G. de Gennaro ◽  
A. Di Gilio ◽  
...  

The atmosphere is a carrier on which some natural and anthropogenic organic and inorganic chemicals are transported, and the wet and dry deposition events are the most important processes that remove those chemicals, depositing it on soil and water. A wide variety of different collectors were tested to evaluate site-specificity, seasonality and daily variability of settleable particle concentrations. Deposition fluxes of POPs showed spatial and seasonal variations, diagnostic ratios of PAHs on deposited particles, allowed the discrimination between pyrolytic or petrogenic sources. Congener pattern analysis and bulk deposition fluxes in rural sites confirmed long-range atmospheric transport of PCDDs/Fs. More and more sophisticated and newly designed deposition samplers have being used for characterization of deposited mercury, demonstrating the importance of rain scavenging and the relatively higher magnitude of Hg deposition from Chinese anthropogenic sources. Recently biological monitors demonstrated that PAH concentrations in lichens were comparable with concentrations measured in a conventional active sampler in an outdoor environment. In this review the authors explore the methodological approaches used for the assessment of atmospheric deposition, from the analysis of the sampling methods, the analytical procedures for chemical characterization of pollutants and the main results from the scientific literature.


2013 ◽  
Vol 27 (2) ◽  
pp. 440-449 ◽  
Author(s):  
Alexie Heimburger ◽  
Rémi Losno ◽  
Sylvain Triquet ◽  
Elisabeth Bon Nguyen

2021 ◽  
Vol 2 (1) ◽  
Author(s):  
Aryeh Feinberg ◽  
Andrea Stenke ◽  
Thomas Peter ◽  
Eve-Lyn S. Hinckley ◽  
Charles T. Driscoll ◽  
...  

AbstractAtmospheric deposition is a major source of the nutrients sulfur and selenium to agricultural soils. Air pollution control and cleaner energy production have reduced anthropogenic emissions of sulfur and selenium, which has led to lower atmospheric deposition fluxes of these elements. Here, we use a global aerosol-chemistry-climate model to map recent (2005–2009) sulfur and selenium deposition, and project future (2095–2099) changes under two socioeconomic scenarios. Across the Northern Hemisphere, we find substantially decreased deposition to agricultural soils, by 70 to 90% for sulfur and by 55 to 80% for selenium. Recent trends in sulfur and selenium concentrations in USA streams suggest that catchment mass balances of these elements are already changing due to the declining atmospheric supply. Sustainable fertilizer management strategies will need to be developed to offset the decrease in atmospheric nutrient supply and ensure future food security and nutrition, while avoiding consequences for downstream aquatic ecosystems.


2021 ◽  
Vol 1 (1) ◽  
Author(s):  
Jozef HANČUĽÁK ◽  
Tomislav ŠPALDON ◽  
Oľga ŠESTINOVÁ

The contribution deals with the evaluation of atmospheric deposition monitoring in 2009–2017 which was realised in the vicinity of the copper smeltery in Krompachy (Slovakia). The samples were collected from the seven sites, which are located from 1.2 to 10 km from the main pollution source. The atmospheric deposition fluxes of solid particles and elements (Fe, Al, Mn, Zn, Pb, Cu, Cr, Cd, As) were determined separately for “water soluble” and “insoluble” fraction. The detailed analysis of deposition fluxes showed a significant effect of the copper smeltery. In addition to the expected high levels of deposition of copper (21–140), the above-average high deposition of lead (11–124), zinc (86–464) and cadmium (0.6–3.4 μg.m–2.day–1) were measured in comparison with different areas. The highest values of deposition fluxes of these elements were detected at sites near the copper smeltery. The level of zinc deposition disagrees with its registered emissions.


2021 ◽  
Author(s):  
JOSÉ A. SOLÍS CANUL ◽  
ROSA M. CERÓN BRETÓN ◽  
JULIA G. CERÓN BRETÓN ◽  
SIMÓN CARRANCO LOZADA ◽  
EVANGELINA RAMÍREZ LARA ◽  
...  

2020 ◽  
Author(s):  
Sanja Frka ◽  
Andrea Milinković ◽  
Abra Penezić ◽  
Saranda Bakija Alempijević ◽  
Blaženka Gašparović ◽  
...  

&lt;p&gt;&lt;strong&gt;Biochemical responses of oligotrophic Adriatic Sea surface layers to atmospheric deposition inputs&lt;/strong&gt;&lt;/p&gt;&lt;p&gt;&lt;strong&gt;&amp;#160;&lt;/strong&gt;&lt;/p&gt;&lt;p&gt;Frka&lt;sup&gt;1&lt;/sup&gt;, A. Milikovi&amp;#263;&lt;sup&gt;1&lt;/sup&gt;, A. Penezi&amp;#263;&lt;sup&gt;1&lt;/sup&gt;, S. Bakija Alempijevi&amp;#263;&lt;sup&gt;1&lt;/sup&gt;, B. Ga&amp;#353;parovi&amp;#263;&lt;sup&gt;1&lt;/sup&gt;, S. Skeji&amp;#263;&lt;sup&gt;2&lt;/sup&gt;, D. &amp;#352;anti&amp;#263;&lt;sup&gt;2&lt;/sup&gt;, S. Brzaj&lt;sup&gt;3&lt;/sup&gt;, V. D&amp;#382;aja Grgi&amp;#269;in&lt;sup&gt;3&lt;/sup&gt;, S. Vidi&amp;#269;&lt;sup&gt;3&lt;/sup&gt;, I. &amp;#352;imi&amp;#263;&lt;sup&gt;4&lt;/sup&gt;, I. Be&amp;#353;li&amp;#263;&lt;sup&gt;4&lt;/sup&gt;, S. &amp;#381;u&amp;#382;ul&lt;sup&gt;4&lt;/sup&gt;, R. Godec&lt;sup&gt;4&lt;/sup&gt;, G. Pehnec&lt;sup&gt;4&lt;/sup&gt;&lt;/p&gt;&lt;p&gt;&lt;sup&gt;1&lt;/sup&gt;Division for marine and environmental research, Ru&amp;#273;er Bo&amp;#353;kovi&amp;#263; Institute, Zagreb, Croatia&lt;/p&gt;&lt;p&gt;&lt;sup&gt;2&lt;/sup&gt;Institute of Oceanography and Fisheries, Split, Croatia&lt;/p&gt;&lt;p&gt;&lt;sup&gt;3&lt;/sup&gt;Croatian Meteorological and Hydrological Service, Zagreb, Croatia&lt;/p&gt;&lt;p&gt;&lt;sup&gt;4&lt;/sup&gt;Institute for Medical Research and Occupational Health, Zagreb, Croatia&lt;/p&gt;&lt;p&gt;&amp;#160;&lt;/p&gt;&lt;p&gt;The atmosphere is a significant pathway by which both natural and anthropogenic material is transported from continents to both coastal and open seas. Once deposited through atmospheric deposition (AD) processing, atmospheric particulate matter (PM) provides the aqueous ecosystems with an external source of nutrients and pollutants. This, in turn, influences the organic matter (OM) production by the phytoplankton, changes CO&lt;sub&gt;2&lt;/sub&gt; uptake and indirectly affects the climate. The input of AD is especially important in oligotrophic environments and it is expected to increase in the future scenarios of a warmer atmosphere with increased PM emissions and deposition rates. While the majority of the data related to the AD impacts generated so far in the Mediterranean have been conducted on its western and eastern regions, the effects of the AD inputs to oligotrophic surface waters of the Adriatic Sea sub-basin are unknown. This work is designed to assess the impact of AD on complex biochemical responses of Adriatic oligotrophic systems, considering the sea surface microlayer (SML) at the air-water interface.&lt;/p&gt;&lt;p&gt;Field campaign was conducted during the period of retrieval of sea surface oligotrophic conditions (February-July 2019) at the Martinska, Central Adriatic, Croatia. On-line black carbon (BC) concentrations were measured while the PM&lt;sub&gt;10&lt;/sub&gt;, wet and total deposition samples as well as the SML and underlying water (ULW; 0.5 m depth) samples were collected simultaneously. The temporal dynamics of the SML biology as well as concentrations of&amp;#160; inorganic and organic constituents enabled the assessment of their sources and the nature of the enrichments taking place within the SML. The first comprehensive insight into concentration levels of macro nutrients (N, P), trace metals (eg. Cu, Pb, Cd, Ni, Zn, Co) and OM (including aromatic pollutants) in atmospheric samples, their transport history, source apportionment and deposition fluxes to the oligotrophic Adriatic area will be presented. Daily and seasonal variations of PM&lt;sub&gt;10&lt;/sub&gt; composition were affected by local traffic and open-fire events as well as by local meteorological conditions and long-range transport. The BC contribution of biomass burning versus fossil fuel combustion changed seasonally. Source apportionment module of LOTOS-EUROS chemical transport model enabled identification and quantification of main source areas contributing to deposition of PM. The main PM contributor is a public power sector outside Croatia while other contributing sectors are energy production, traffic, residential combustion as well as shipping. First deposition fluxes estimates show reasonable agreement between model calculations and measured data, and could be used for more general assessments of atmospheric inputs.&lt;/p&gt;&lt;p&gt;&amp;#160;&lt;/p&gt;&lt;p&gt;&lt;strong&gt;Acknowledgment&lt;/strong&gt;: This work has been supported by Croatian Science Foundation under the IP-2018-01-3105 project: Biochemical responses of oligotrophic Adriatic surface ecosystems to atmospheric deposition inputs.&lt;/p&gt;


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