Extent of Shallow/Deep Trap States beyond the Conduction Band Minimum in Defect-Tolerant CsPbBr3 Perovskite Quantum Dot: Control over the Degree of Charge Carrier Recombination

2020 ◽  
Vol 11 (5) ◽  
pp. 1702-1707 ◽  
Author(s):  
Saptarshi Mandal ◽  
Soumen Mukherjee ◽  
Chayan K. De ◽  
Debjit Roy ◽  
Swarnali Ghosh ◽  
...  
Keyword(s):  
Quantum Dot ◽  
Charge Carrier ◽  
Conduction Band ◽  
Deep Trap ◽  
Conduction Band Minimum ◽  
Trap States ◽  
Carrier Recombination ◽  
Charge Carrier Recombination

Efficient Defect Passivation with Niacin for High-Performance and Stable Perovskite Solar Cells

2021 ◽  
Author(s):  
Jing Ren ◽  
Shurong Wang ◽  
Jianxing Xia ◽  
Chengbo Li ◽  
Lisha Xie ◽  
...  
Keyword(s):  
Solar Cells ◽  
Charge Carrier ◽  
High Performance ◽  
Perovskite Solar Cells ◽  
Trap States ◽  
Carrier Recombination ◽  
Defect Passivation ◽  
Recombination Centers ◽  
Charge Carrier Recombination ◽  
Halide Perovskite

Defects, inevitably produced in the solution-processed halide perovskite films, can act as charge carrier recombination centers to induce severe energy loss in perovskite solar cells (PSCs). Suppressing these trap states...

Oxygen Deficient TiO2 Photoanode for Photoelectrochemical Water Oxidation

2016 ◽  
Vol 253 ◽  
pp. 11-40 ◽  
Author(s):  
Yi Yang ◽  
Ying Chih Pu ◽  
Yat Li ◽  
Jin Zhang
Keyword(s):  
Oxygen Vacancy ◽  
Charge Carrier ◽  
Water Oxidation ◽  
Chemical Reduction ◽  
Hydrogen Treatment ◽  
Trap States ◽  
Ultrafast Laser Spectroscopy ◽  
Charge Carrier Dynamics ◽  
Carrier Recombination ◽  
Charge Carrier Recombination

Titanium dioxide (TiO2) has been widely used as photoanodes in photoelectrochemical (PEC) water splitting. However, the typically high density of bandgap trap states results in fast charge carrier recombination and poor electrical conductivity, and thereby weak PEC performance. Rational creation of oxygen vacancy (Vo) in TiO2 has been demonstrated as an effective method to modify the electronic and optical properties, as well as improved PEC performance. Different strategies have been developed to fabricate oxygen deficient TiO2 photoanodes, such as hydrogen treatment, thermal annealing, electrochemical reduction, flame reduction, and chemical reduction. In conjunction with oxygen vacancy creation, doping of TiO2 with elements further enhances the PEC activity by introducing other bandgap states. Various techniques, including ultrafast laser spectroscopy, have been employed to probe the chemical nature and associated charge carrier dynamics of the bandgap states.

Time-dependent Langevin-type bimolecular charge carrier recombination in regiorandom poly(3-hexylthiophene)

2005 ◽  
Vol 155 (2) ◽  
pp. 242-245 ◽  
Author(s):  
A. Pivrikas ◽  
R. Österbacka ◽  
G. Juška ◽  
K. Arlauskas ◽  
H. Stubb
Keyword(s):  
Charge Carrier ◽  
Time Dependent ◽  
Carrier Recombination ◽  
Charge Carrier Recombination

Bi-doped Graphitic Carbon Nitride Nanotubes Boosts the Degradation Photocatalysis of Rhodamine B

2022 ◽  
Author(s):  
Qingqing Gao ◽  
Qian Lei ◽  
Ruoyan Miao ◽  
Manyi Gao ◽  
Fang Song ◽  
...  
Keyword(s):  
Charge Carrier ◽  
Rhodamine B ◽  
High Stability ◽  
Carbon Nitride ◽  
Graphitic Carbon Nitride ◽  
Photocatalytic Efficiency ◽  
Metal Free ◽  
Carrier Recombination ◽  
Charge Carrier Recombination ◽  
Polymeric Carbon

Polymeric carbon nitride (PCN) is an emerging metal-free photocatalysts with high stability but is plagued by low photocatalytic efficiency due to the rapid charge carrier recombination behavior. Herein, Bi doped...

Few-Layered MoS2 Nanoparticles Loaded TiO2 Nanosheets with Exposed {001} Facets for Enhanced Photocatalytic Activity

NANO ◽  
2018 ◽  
Vol 13 (11) ◽  
pp. 1850129 ◽  
Author(s):  
Chujun Chen ◽  
Xia Xin ◽  
Jinniu Zhang ◽  
Gang Li ◽  
Yafeng Zhang ◽  
...  
Keyword(s):  
Photocatalytic Activity ◽  
Charge Carrier ◽  
Visible Light ◽  
Recombination Rate ◽  
Active Species ◽  
Molar Ratio ◽  
Carrier Recombination ◽  
Tio2 Nanosheets ◽  
Photocatalytic Activities ◽  
Charge Carrier Recombination

To improve the high charge carrier recombination rate and low visible light absorption of {001} facets exposed TiO2 [TiO2(001)] nanosheets, few-layered MoS2 nanoparticles were loaded on the surfaces of TiO2(001) nanosheets by a simple photodeposition method. The photocatalytic activities towards Rhodamine B (RhB) were investigated. The results showed that the MoS2–TiO2(001) nanocomposites exhibited much enhanced photocatalytic activities compared with the pure TiO2(001) nanosheets. At an optimal Mo/Ti molar ratio of 25%, the MoS2–TiO2(001) nanocomposites displayed the highest photocatalytic activity, which took only 30[Formula: see text]min to degrade 50[Formula: see text]mL of RhB (50[Formula: see text]mg/L). The active species in the degradation reaction were determined to be h[Formula: see text] and [Formula: see text]OH according to the free radical trapping experiments. The reduced charge carrier recombination rate, enhanced visible light utilization and increased surface areas contributed to the enhanced photocatalytic performances of the 25% MoS2–TiO2(001) nanocomposites.

scholarly journals Impact of charge carrier recombination and energy disorder on the open-circuit voltage of polymer solar cells

2020 ◽  
Vol 69 (4) ◽  
pp. 046101
Author(s):  
Qing-Zhong Zhou ◽  
Feng Guo ◽  
Ming-Rui Zhang ◽  
Qing-Liang You ◽  
Biao Xiao ◽  
...  
Keyword(s):  
Solar Cells ◽  
Charge Carrier ◽  
Open Circuit Voltage ◽  
Polymer Solar Cells ◽  
Open Circuit ◽  
Carrier Recombination ◽  
Energy Disorder ◽  
Charge Carrier Recombination

Effect of dihydronaphthyl-based C60 bisadduct as third component materials on the photovoltaic performance and charge carrier recombination of binary PBDB-T : ITIC polymer solar cells

Nanoscale ◽  
2018 ◽  
Vol 10 (18) ◽  
pp. 8483-8495 ◽  
Author(s):  
Shengli Niu ◽  
Zhiyong Liu ◽  
Ning Wang
Keyword(s):  
Solar Cells ◽  
Charge Carrier ◽  
Polymer Solar Cells ◽  
Photovoltaic Performance ◽  
Carrier Recombination ◽  
Binary Polymer ◽  
Component Material ◽  
Charge Carrier Recombination

A dihydronaphthyl-based C60 bisadduct (NCBA) acceptor was introduced as a third component material to typical binary polymer solar cells (PSCs).

Partial oxidation of the absorber layer reduces charge carrier recombination in antimony sulfide solar cells

2017 ◽  
Vol 19 (2) ◽  
pp. 1425-1430 ◽  
Author(s):  
Karl C. Gödel ◽  
Bart Roose ◽  
Aditya Sadhanala ◽  
Yana Vaynzof ◽  
Sandeep K. Pathak ◽  
...  
Keyword(s):  
Heat Treatment ◽  
Solar Cells ◽  
Charge Carrier ◽  
Partial Oxidation ◽  
Absorber Layer ◽  
Antimony Sulfide ◽  
Carrier Recombination ◽  
Charge Carrier Recombination ◽  
Sensitized Solar Cells

A controlled heat treatment of the absorber layer in air leads to improved Sb2S3 sensitized solar cells. A reduction in charge carrier recombination is the reason for the enhancement.

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