scholarly journals Investigations to Hygroscopic Aerosol Growth Within the Convective Boundary Layer

2020 ◽  
Vol 237 ◽  
pp. 02016
Author(s):  
Dietrich Althausen ◽  
Andrew Reigert ◽  
Ulla Wandinger ◽  
Jens Reichardt

We present a new method to determine the hygroscopic growth of atmospheric particles. This method combines lidar measurements with high temporal resolution of the particle backscatter coefficient and water vapor mixing ratio with temperature measurements from radiosondes and a microwave radiometer. The hygroscopic growth is described by an equation that represents the two observed branches of the growth curve with different dependencies on the relative humidity. An example is presented to illustrate a first result from a continental air mass case.

2014 ◽  
Vol 7 (5) ◽  
pp. 1201-1211 ◽  
Author(s):  
F. Navas-Guzmán ◽  
J. Fernández-Gálvez ◽  
M. J. Granados-Muñoz ◽  
J. L. Guerrero-Rascado ◽  
J. A. Bravo-Aranda ◽  
...  

Abstract. In this paper, we outline an iterative method to calibrate the water vapour mixing ratio profiles retrieved from Raman lidar measurements. Simultaneous and co-located radiosonde data are used for this purpose and the calibration results obtained during a radiosonde campaign in summer and autumn 2011 are presented. The water vapour profiles measured during night-time by the Raman lidar and radiosondes are compared and the differences between the methodologies are discussed. Then, a new approach to obtain relative humidity profiles by combination of simultaneous profiles of temperature (retrieved from a microwave radiometer) and water vapour mixing ratio (from a Raman lidar) is addressed. In the last part of this work, a statistical analysis of water vapour mixing ratio and relative humidity profiles obtained during 1 year of simultaneous measurements is presented.


2019 ◽  
Vol 77 (3) ◽  
pp. 1081-1100 ◽  
Author(s):  
Neil P. Lareau

Abstract Doppler and Raman lidar observations of vertical velocity and water vapor mixing ratio are used to probe the physics and statistics of subcloud and cloud-base latent heat fluxes during cumulus convection at the ARM Southern Great Plains (SGP) site in Oklahoma, United States. The statistical results show that latent heat fluxes increase with height from the surface up to ~0.8Zi (where Zi is the convective boundary layer depth) and then decrease to ~0 at Zi. Peak fluxes aloft exceeding 500 W m−2 are associated with periods of increased cumulus cloud cover and stronger jumps in the mean humidity profile. These entrainment fluxes are much larger than the surface fluxes, indicating substantial drying over the 0–0.8Zi layer accompanied by moistening aloft as the CBL deepens over the diurnal cycle. We also show that the boundary layer humidity budget is approximately closed by computing the flux divergence across the 0–0.8Zi layer. Composite subcloud velocity and water vapor anomalies show that clouds are linked to coherent updraft and moisture plumes. The moisture anomaly is Gaussian, most pronounced above 0.8Zi and systematically wider than the velocity anomaly, which has a narrow central updraft flanked by downdrafts. This size and shape disparity results in downdrafts characterized by a high water vapor mixing ratio and thus a broad joint probability density function (JPDF) of velocity and mixing ratio in the upper CBL. We also show that cloud-base latent heat fluxes can be both positive and negative and that the instantaneous positive fluxes can be very large (~10 000 W m−2). However, since cloud fraction tends to be small, the net impact of these fluxes remains modest.


2018 ◽  
Vol 18 (10) ◽  
pp. 7001-7017 ◽  
Author(s):  
Andrés Esteban Bedoya-Velásquez ◽  
Francisco Navas-Guzmán ◽  
María José Granados-Muñoz ◽  
Gloria Titos ◽  
Roberto Román ◽  
...  

Abstract. This study focuses on the analysis of aerosol hygroscopic growth during the Sierra Nevada Lidar AerOsol Profiling Experiment (SLOPE I) campaign by using the synergy of active and passive remote sensors at the ACTRIS Granada station and in situ instrumentation at a mountain station (Sierra Nevada, SNS). To this end, a methodology based on simultaneous measurements of aerosol profiles from an EARLINET multi-wavelength Raman lidar (RL) and relative humidity (RH) profiles obtained from a multi-instrumental approach is used. This approach is based on the combination of calibrated water vapor mixing ratio (r) profiles from RL and continuous temperature profiles from a microwave radiometer (MWR) for obtaining RH profiles with a reasonable vertical and temporal resolution. This methodology is validated against the traditional one that uses RH from co-located radiosounding (RS) measurements, obtaining differences in the hygroscopic growth parameter (γ) lower than 5 % between the methodology based on RS and the one presented here. Additionally, during the SLOPE I campaign the remote sensing methodology used for aerosol hygroscopic growth studies has been checked against Mie calculations of aerosol hygroscopic growth using in situ measurements of particle number size distribution and submicron chemical composition measured at SNS. The hygroscopic case observed during SLOPE I showed an increase in the particle backscatter coefficient at 355 and 532 nm with relative humidity (RH ranged between 78 and 98 %), but also a decrease in the backscatter-related Ångström exponent (AE) and particle linear depolarization ratio (PLDR), indicating that the particles became larger and more spherical due to hygroscopic processes. Vertical and horizontal wind analysis is performed by means of a co-located Doppler lidar system, in order to evaluate the horizontal and vertical dynamics of the air masses. Finally, the Hänel parameterization is applied to experimental data for both stations, and we found good agreement on γ measured with remote sensing (γ532=0.48±0.01 and γ355=0.40±0.01) with respect to the values calculated using Mie theory (γ532=0.53±0.02 and γ355=0.45±0.02), with relative differences between measurements and simulations lower than 9 % at 532 nm and 11 % at 355 nm.


2013 ◽  
Vol 6 (6) ◽  
pp. 10481-10510
Author(s):  
F. Navas-Guzmán ◽  
J. Fernández-Gálvez ◽  
M. J. Granados-Muñoz ◽  
J. L. Guerrero-Rascado ◽  
J. A. Bravo-Aranda ◽  
...  

Abstract. In this paper, we outline an iterative method to calibrate the water vapour mixing ratio profiles retrieved from Raman lidar measurements. Simultaneous and co-located radiosonde data are used for this purpose and the calibration results obtained during a radiosonde campaign performed in Summer and Autumn 2011 are presented. The water vapour profiles measured during nighttime by the Raman lidar and radiosondes are compared and the differences between the methodologies are discussed. Moreover, a new approach to obtain relative humidity profiles by combination of simultaneous profiles of temperature (retrieved from a microwave radiometer) and water vapour mixing ratio (from a Raman lidar) is addressed. In the last part of this work, a statistical analysis of water vapour mixing ratio and relative humidity profiles obtained during one year of simultaneous measurements is presented.


2016 ◽  
Author(s):  
Darren R. Clabo

Abstract. This study presents an analysis of the water vapor mixing ratio contained within multiple mid-tropospheric smoke plumes as diagnosed by a ground-based passive microwave radiometer. Measurements from the radiometer were compared to smoke opacity as diagnosed from visible satellite imagery on three different days: 12, 16, and 20 August 2013. It was found that the water vapor mixing ratio within the smoke plume could be as much as 20–250 % higher than the mixing ratio within the ambient, non-smoke environmental air. Significant intra-smoke plume variability also existed and the mixing ratio was found to be higher (lower) in more optically thick (thin) areas of the plume. This study demonstrates that a radiometer is valuable tool that can be used to remotely measure the water vapor content within smoke plumes.


2009 ◽  
Vol 26 (6) ◽  
pp. 1021-1039 ◽  
Author(s):  
Mariana Adam

Abstract The temperature dependence of molecular backscatter coefficients must be taken into account when narrowband interference filters are used in lidar measurements. Thus, the spectral backscatter differential cross section of the molecules involved in the backscattering of the radiation has to be calculated or measured and the interference filter transmission efficiency must be known. The present paper is intended to describe in an easily reproducible manner the procedure involved in calculating the temperature-dependent functions introduced in the lidar equations, including the computation of the differential cross sections for air, nitrogen, and water vapor. The temperature-dependent functions are computed for the Howard University Raman lidar (HURL). The interference filter efficiencies are given by the manufacturer. Error estimates in water vapor mixing ratio and aerosol backscatter ratio involved when temperature-dependent functions are omitted are given for measurements taken with HURL. For the data analyzed, it is found that errors in estimating the water vapor mixing ratio are up to ∼6% while in estimating the aerosol backscattering ratio the errors are up to ∼1.3% in the planetary boundary layer and ∼2.2% in cirrus clouds. Theoretical computations are performed to determine temperature-dependent functions for nitrogen, water vapor, and their ratio, using simulated Gaussian-shaped filters. The goal is to find the optimum combination of different filters that will determine the ratio profiles of the temperature-dependent functions that are either the closest to unity or the least variable. The analyses reveal that quite constant profiles can be obtained for several combinations of the filters.


2017 ◽  
Author(s):  
Holger Baars ◽  
Patric Seifert ◽  
Ronny Engelmann ◽  
Ulla Wandinger

Abstract. Absolute calibrated signals at 532 and 1064 nm and the depolarization ratio from a multiwavelength lidar are used to categorize primary aerosol but also clouds in high temporal and spatial resolution. Automatically derived particle backscatter coefficient profiles in low temporal resolution (30 min) are applied to calibrate the lidar signals. From these calibrated lidar signals, new atmospheric parameters in temporally high resolution (quasi particle backscatter coefficient) are derived. By using thresholds obtained from multi-year, multi-site EARLINET measurements, four aerosol classes (small; large, spherical; large, non-spherical; mixed, partly non-spherical) and several cloud classes (liquid, ice) are defined. Thus, particles are classified by their physical feature (shape and size) instead of a classification by source. The methodology is applied to two months of continuous observations (24 hours, 7 days a week) with the multiwavelength-Raman-polarization lidar PollyXT during the HOPE campaign in spring 2013. Cloudnet equipment was operated continuously directly next to the lidar and is used for comparison. By discussing three 24-h case studies, it is shown that the aerosol discrimination is very feasible and informative and gives a good complement to the Cloudnet target categorization. By analyzing the entire HOPE campaign, almost 1 million pixel (5 min times 30 m) could be successfully classified from the two months data set with the newly developed tool. We find that the majority of the aerosol, trapped in the planetary boundary layer (PBL), were small particles as expected for a heavily populated and industrialized area. Large, spherical aerosol was observed mostly at the top of the PBL and close to the identified cloud bases indicating the importance of hygroscopic growth of the particles at high relative humidity. Interestingly, it is found that on several days non-spherical particles were dispersed into the atmosphere from ground.


Atmosphere ◽  
2018 ◽  
Vol 9 (7) ◽  
pp. 258 ◽  
Author(s):  
Jessica Kleiss ◽  
Erin Riley ◽  
Charles Long ◽  
Laura Riihimaki ◽  
Larry Berg ◽  
...  

We develop a new approach that resolves cloud area distributions of single-layer shallow cumuli from ground-based observations. Our simple and computationally inexpensive approach uses images obtained from a Total Sky Imager (TSI) and complementary information on cloud base height provided by lidar measurements to estimate cloud equivalent diameter (CED) over a wide range of cloud sizes (about 0.01–3.5 km) with high temporal resolution (30 s). We illustrate the feasibility of our approach by comparing the estimated CEDs with those derived from collocated and coincident high-resolution (0.03 km) Landsat cloud masks with different spatial and temporal patterns of cloud cover collected over the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site. We demonstrate that (1) good (~7%) agreement between TSI and Landsat characteristic cloud size can be obtained for clouds that fall within the region of the sky observable by the TSI and (2) large clouds that extend beyond this region are responsible for noticeable (~16%) underestimation of the TSI characteristic cloud size. Our approach provides a previously unavailable dataset for process studies in the convective boundary layer and evaluation of shallow cumuli in cloud-resolving models.


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