Strong Coupling: Polariton Bose Condensation

Author(s):  
Alexey V. Kavokin ◽  
Jeremy J. Baumberg ◽  
Guillaume Malpuech ◽  
Fabrice P. Laussy

In this Chapter we address the physics of Bose-Einstein condensation and its implications to a driven-dissipative system such as the polariton laser. We discuss the dynamics of exciton-polaritons non-resonantly pumped within a microcavity in the strong coupling regime. It is shown how the stimulated scattering of exciton-polaritons leads to formation of bosonic condensates that may be stable at elevated temperatures, including room temperature.

Author(s):  
Alexey V. Kavokin ◽  
Jeremy J. Baumberg ◽  
Guillaume Malpuech ◽  
Fabrice P. Laussy

This chapter presents experimental studies performed on planar semiconductor microcavities in the strong-coupling regime. The first section reviews linear experiments performed in the 1990s that evidence the linear optical properties of cavity exciton-polaritons. The chapter is then focused on experimental and theoretical studies of resonantly excited microcavity emission. We mainly describe experimental configuations in which stimulated scattering was observed due to formation of a dynamical condensate of polaritons. Pump-probe and cw experiments are described in addition. Dressing of the polariton dispersion and bistability of the polariton system due to inter-condensate interactions are discussed. The semiclassical and the quantum theories of these effects are presented and their results analysed. The potential for realization of devices is also discussed.


2020 ◽  
Vol 71 (1) ◽  
pp. 435-459 ◽  
Author(s):  
Jonathan Keeling ◽  
Stéphane Kéna-Cohen

Bose–Einstein condensation describes the macroscopic occupation of a single-particle mode: the condensate. This state can in principle be realized for any particles obeying Bose–Einstein statistics; this includes hybrid light-matter excitations known as polaritons. Some of the unique optoelectronic properties of organic molecules make them especially well suited for the realization of polariton condensates. Exciton-polaritons form in optical cavities when electronic excitations couple collectively to the optical mode supported by the cavity. These polaritons obey bosonic statistics at moderate densities, are stable at room temperature, and have been observed to form a condensed or lasing state. Understanding the optimal conditions for polariton condensation requires careful modeling of the complex photophysics of organic molecules. In this article, we introduce the basic physics of exciton-polaritons and condensation and review experiments demonstrating polariton condensation in molecular materials.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Raj Pandya ◽  
Richard Y. S. Chen ◽  
Qifei Gu ◽  
Jooyoung Sung ◽  
Christoph Schnedermann ◽  
...  

AbstractStrong-coupling between excitons and confined photonic modes can lead to the formation of new quasi-particles termed exciton-polaritons which can display a range of interesting properties such as super-fluidity, ultrafast transport and Bose-Einstein condensation. Strong-coupling typically occurs when an excitonic material is confided in a dielectric or plasmonic microcavity. Here, we show polaritons can form at room temperature in a range of chemically diverse, organic semiconductor thin films, despite the absence of an external cavity. We find evidence of strong light-matter coupling via angle-dependent peak splittings in the reflectivity spectra of the materials and emission from collective polariton states. We additionally show exciton-polaritons are the primary photoexcitation in these organic materials by directly imaging their ultrafast (5 × 106 m s−1), ultralong (~270 nm) transport. These results open-up new fundamental physics and could enable a new generation of organic optoelectronic and light harvesting devices based on cavity-free exciton-polaritons


2013 ◽  
Vol 13 (3) ◽  
pp. 247-252 ◽  
Author(s):  
Johannes D. Plumhof ◽  
Thilo Stöferle ◽  
Lijian Mai ◽  
Ullrich Scherf ◽  
Rainer F. Mahrt

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
B. Divinskiy ◽  
H. Merbouche ◽  
V. E. Demidov ◽  
K. O. Nikolaev ◽  
L. Soumah ◽  
...  

AbstractThe quanta of magnetic excitations – magnons – are known for their unique ability to undergo Bose-Einstein condensation at room temperature. This fascinating phenomenon reveals itself as a spontaneous formation of a coherent state under the influence of incoherent stimuli. Spin currents have been predicted to offer electronic control of Bose-Einstein condensates, but this phenomenon has not been experimentally evidenced up to now. Here we show that current-driven Bose-Einstein condensation can be achieved in nanometer-thick films of magnetic insulators with tailored nonlinearities and minimized magnon interactions. We demonstrate that, above a certain threshold, magnons injected by the spin current overpopulate the lowest-energy level forming a highly coherent spatially extended state. We quantify the chemical potential of the driven magnon gas and show that, at the critical current, it reaches the energy of the lowest magnon level. Our results pave the way for implementation of integrated microscopic quantum magnonic and spintronic devices.


2019 ◽  
Vol 2019 ◽  
pp. 1-8 ◽  
Author(s):  
A. A. Isaev

The paper presents experimental results of the interaction of a focused optical beam with a suspension of CdSe/ZnS quantum dots in toluene. Two autographs characteristic only of the behavior of a superfluid quantum liquid were experimentally observed. The first was the fountain effect from the region of local heating of the suspension with an optical beam; the second was the complete “creeping out” of the QDs suspension in the form of a thin film along the walls of the cuvette in which the suspension was located. The results of the work suggest that superfluid quantum liquid may arise at room temperature as a result of the functioning of many-particle quantum superposition. Bose-Einstein condensation of entangled quantum states is proposed as a physical mechanism for producing a superfluid liquid, regardless of temperature.


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