Flame Front Characteristic and Turbulent Flame Speed of Lean Premixed Syngas Combustion at Gas Turbine Relevant Conditions

Author(s):  
S. Daniele ◽  
P. Jansohn ◽  
K. Boulouchos

This paper focuses on the description of the turbulent flame speed, at gas turbine like conditions, for different syngas mixtures, selected in order to simulate syngas compositions typically derived from gasification of coal, oil, biomass, and used for power generation in integrated gasification combined cycle (IGCC) processes. In this paper the turbulent flame speed is reported as global consumption rate and calculated based on a mass continuity approach applied to the combustor inlet area and the flame front surface, which was detected experimentally. Flame front detection was done by means of planar laser induced fluorescence technique taking OH radicals as seeding dyes. An in-house developed flame front detection software tool has been further improved and utilized in this work in order to better fit ultra-lean H2-rich flames. Experiments were carried out in a High Pressure Test Rig for operating pressures up to 15 bar. Data provided in this paper will focus on a pressure level of 5 bar, adiabatic flame temperatures up to 1900 K, inlet velocities from 40 to 80 m/s, and inlet temperature of 672 and 772 K. As expected, the results highlight the strongly elevated values of turbulent flame speed for high hydrogen containing fuel gas mixtures. Compared with flame speed data for pure CH4 the ratio (STSyn/STCH4) takes up values of 7 to 8. In absolute terms values go up even beyond 10 m/s. With increased H2 content in the mixture the burning velocity raises, due to the faster chemical kinetics characteristic of this compound and due to physical properties of H2 (Le<1) which enhance flame front corrugation (i.e. flame front surface). Inlet velocity and pressure variations showed to have weak effect on the average flame front position whereas this last parameter is strongly affected by the mixture composition, the equivalence ratio and inlet temperature.

Author(s):  
Andrew Marshall ◽  
Julia Lundrigan ◽  
Prabhakar Venkateswaran ◽  
Jerry Seitzman ◽  
Tim Lieuwen

Fuel composition has a strong influence on the turbulent flame speed, even at very high turbulence intensities. An important implication of this result is that the turbulent flame speed cannot be extrapolated from one fuel to the next using only the laminar flame speed and turbulence intensity as scaling variables. This paper presents curvature and tangential strain rate statistics of premixed turbulent flames for high hydrogen content fuels. Global (unconditioned) stretch statistics are presented as well as measurements conditioned on the leading points of the flame front. These measurements are motivated by previous experimental and theoretical work that suggests the turbulent flame speed is controlled by the flame front characteristics at these points. The data were acquired with high speed particle image velocimetry (PIV) in a low swirl burner (LSB). We attained measurements for several H2:CO mixtures over a range of mean flow velocities and turbulence intensities. The results show that fuel composition has a systematic, yet weak effect on curvatures and tangential strain rates at the leading points. Instead, stretch statistics at the leading points are more strongly influenced by mean flow velocity and turbulence level. It has been argued that the increased turbulent flame speeds seen with increasing hydrogen content are the result of increasing flame stretch rates, and therefore SL,max values, at the flame leading points. However, the differences observed with changing fuel compositions are not significant enough to support this hypothesis. Additional analysis is needed to understand the physical mechanisms through which the turbulent flame speed is altered by fuel composition effects.


Author(s):  
Andrew Marshall ◽  
Julia Lundrigan ◽  
Prabhakar Venkateswaran ◽  
Jerry Seitzman ◽  
Tim Lieuwen

Fuel composition has a strong influence on the turbulent flame speed, even at very high turbulence intensities. An important implication of this result is that the turbulent flame speed cannot be extrapolated from one fuel to the next using only the laminar flame speed and turbulence intensity as scaling variables. This paper presents curvature and tangential strain rate statistics of premixed turbulent flames for high hydrogen content (HHC) fuels. Global (unconditioned) stretch statistics are presented as well as measurements conditioned on the leading points of the flame front. These measurements are motivated by previous experimental and theoretical work that suggests the turbulent flame speed is controlled by the flame front characteristics at these points. The data were acquired with high-speed particle image velocimetry (PIV) in a low-swirl burner (LSB). We attained measurements for several H2:CO mixtures over a range of mean flow velocities and turbulence intensities. The results show that fuel composition has a systematic, yet weak effect on curvatures and tangential strain rates at the leading points. Instead, stretch statistics at the leading points are more strongly influenced by mean flow velocity and turbulence level. It has been argued that the increased turbulent flame speeds seen with increasing hydrogen content are the result of increasing flame stretch rates, and therefore, SL,max values, at the flame leading points. However, the differences observed with changing fuel compositions are not significant enough to support this hypothesis. Additional analysis is needed to understand the physical mechanisms through which the turbulent flame speed is altered by fuel composition effects.


Author(s):  
P. Griebel ◽  
R. Bombach ◽  
A. Inauen ◽  
R. Scha¨ren ◽  
S. Schenker ◽  
...  

The present experimental study focuses on flame characteristics and turbulent flame speeds of lean premixed flames typical for stationary gas turbines. Measurements were performed in a generic combustor at a preheating temperature of 673 K, pressures up to 14.4 bars (absolute), a bulk velocity of 40 m/s, and an equivalence ratio in the range of 0.43–0.56. Turbulence intensities and integral length scales were measured in an isothermal flow field with Particle Image Velocimetry (PIV). The turbulence intensity (u′) and the integral length scale (LT) at the combustor inlet were varied using turbulence grids with different blockage ratios and different hole diameters. The position, shape, and fluctuation of the flame front were characterized by a statistical analysis of Planar Laser Induced Fluorescence images of the OH radical (OH-PLIF). Turbulent flame speeds were calculated and their dependence on operating conditions (p, φ) and turbulence quantities (u′, LT) are discussed and compared to correlations from literature. No influence of pressure on the most probable flame front position or on the turbulent flame speed was observed. As expected, the equivalence ratio had a strong influence on the most probable flame front position, the spatial flame front fluctuation, and the turbulent flame speed. Decreasing the equivalence ratio results in a shift of the flame front position farther downstream due to the lower fuel concentration and the lower adiabatic flame temperature and subsequently lower turbulent flame speed. Flames operated at leaner equivalence ratios show a broader spatial fluctuation as the lean blow-out limit is approached and therefore are more susceptible to flow disturbances. In addition, because of a lower turbulent flame speed these flames stabilize farther downstream in a region with higher velocity fluctuations. This increases the fluctuation of the flame front. Flames with higher turbulence quantities (u′, LT) in the vicinity of the combustor inlet exhibited a shorter length and a higher calculated flame speed. An enhanced turbulent heat and mass transport from the recirculation zone to the flame root location due to an intensified mixing which might increase the preheating temperature or the radical concentration is believed to be the reason for that.


Author(s):  
George Mallouppas ◽  
Graham Goldin ◽  
Yongzhe Zhang ◽  
Piyush Thakre ◽  
Jim Rogerson

Abstract Three Flamelet Generated Manifold reaction source term closure options and two different reactor types are examined with Large Eddy Simulation of an industrial gas turbine combustor operating at 3 bar. This work presents the results for the SGT-100 Dry Low Emission (DLE) gas turbine provided by Siemens Industrial Turbomachinery Ltd. The related experimental study was performed at the German Aerospace Centre, DLR, Stuttgart, Germany. The FGM model approximates the thermo-chemistry in a turbulent flame as that in a simple 0D constant pressure ignition reactors and 1D strained opposed-flow premixed reactors, parametrized by mixture fraction, progress variable, enthalpy and pressure. The first objective of this work is to compare the flame shape and position predicted by these two FGM reactor types. The Kinetic Rate (KR) model, studied in this work, uses the chemical rate from the FGM with assumed shapes, which are a Beta function for mixture fraction and delta functions for reaction progress variable and enthalpy. Another model investigated is the Turbulent Flame-Speed Closure (TFC) model with Zimont turbulent flame speed, which propagates premixed flame fronts at specified turbulent flame speeds. The Thickened Flame Model (TFM), which artificially thickens the flame to sufficiently resolve the internal flame structure on the computational grid, is also explored. Therefore, a second objective of this paper is to compare KR, TFC and TFM with the available experimental data.


Author(s):  
David Beerer ◽  
Vincent McDonell ◽  
Peter Therkelsen ◽  
Robert K. Cheng

This paper reports flashback limits and turbulent flame local displacement speed measurements in flames stabilized by a low swirl injector operated at elevated pressures and inlet temperatures with hydrogen and methane blended fuels. The goal of this study is to understand the physics that relate turbulent flame speed to flashback events at conditions relevant to gas turbine engines. Testing was conducted in an optically accessible single nozzle combustor rig at pressures ranging from 1 to 8 atm, inlet temperatures from 290 to 600 K, and inlet bulk velocities between 20 and 60 m/s for natural gas and a 90%/10% (by volume) hydrogen/methane blend. The propensity of flashback is dependent upon the proximity of the lifted flame to the nozzle that is itself dependent upon pressure, inlet temperature, and bulk velocity. Flashback occurs when the leading edge of the flame in the core of the flow ingresses within the nozzle, even in cases when the flame is attached to the burner rim. In general the adiabatic flame temperature at flashback is proportional to the bulk velocity and inlet temperature and inversely proportional to the pressure. The unburned reactant velocity field approaching the flame was measured using a laser Doppler velocimeter with water seeding. Turbulent displacement flame speeds were found to be linearly proportional to the root mean square of the velocity fluctuations about the mean velocity. For identical inlet conditions, high-hydrogen flames had a turbulent flame local displacement speed roughly twice that of natural gas flames. Pressure, inlet temperature, and flame temperature had surprisingly little effect on the local displacement turbulent flame speed. However, the flow field is affected by changes in inlet conditions and is the link between turbulent flame speed, flame position, and flashback propensity.


Author(s):  
S. Daniele ◽  
P. Jansohn ◽  
K. Boulouchos

Nowadays, the establishment of IGCC (integrated gasification combined cycle) plants, prompts a growing interest in synthetic fuels for gas turbine based power generation. This interest has as direct consequence the need for understanding of flashback phenomena for premixed systems operated with H2-rich gases. This is due to the different properties of H2 (e.g. reactivity and diffusivity) with respect to CH4 which lead to higher flame speeds in the case of syngases (mixtures of H2-CO). This paper presents the results of experiments at gas turbine like conditions (pressure up to 15 bar, 0.2 < Φ < 0.7, 577K < T0 < 674K) aimed to determine flashback limits and their dependence on the combustion parameters (pressure, inlet temperature and inlet velocity). For the experimental facility used for this work the back propagation of the flame is believed to happen into the boundary layer of the fuel/air duct. Flashback propensity was found to have an appreciable dependence on pressure and inlet temperature while the effects of inlet velocity variations are weak. Explanations for the dependence on these three parameters, based on consideration on laminar and turbulent flame speed data (from modeling and experiments), are proposed. Within the frame of this work, in order to avoid major damages, the experimental facility was equipped with an automatic control system for flashback described in the paper. The control system is able to detect flame propagation into the fuel/air supply, arrest it and restore safe operating conditions by moving the flame out of the fuel/air section without blowing it out. This avoids destruction of components (burner/mixing) and time consuming shut downs of the test rig.


Author(s):  
Y.-C. Lin ◽  
S. Daniele ◽  
P. Jansohn ◽  
K. Boulouchos

In this paper, characteristics of turbulent combustion and NOx emission for high hydrogen-content fuel gases (H2 > 70 vol. %; “hydrogen-rich”) are addressed. An experimental investigation is performed in a perfectly-premixed axial-dump combustor under gas turbine relevant conditions. Fundamental features of turbulent combustion for these mixtures are evaluated based on OH-PLIF diagnostics. On the other hand, NOx emissions are measured with an exhaust gas sampling probe positioned downstream the combustor outlet. Compared to syngas mixtures (H2 + CO), the operational limits for hydrogen-rich fuel gases are found to occur at even leaner conditions concerning flashback phenomena. With respect to effects of operating pressure, a strongly reduced operational envelope is observed at elevated pressure. Only with decreasing the preheat temperature a viable approach to further extend the operational range is seen. Evaluation of the averaged turbulent flame shape shows that the profile of the flame front is generally approaching that of an ideal cone. Thus a simplified approach for estimating the turbulent flame speed via the location of the flame tip alone can be applied. The level of NOx emission for the hydrogen-rich fuel mixtures is generally above that of syngas mixtures, which exhibit already higher NOx emission values than natural gas. Distinct chemical kinetic features are found specifically at elevated pressure. While the pressure effects are weak for syngas, a non-monotonic behavior is observed for the hydrogen-rich fuels. Reaction path analysis is performed to complement and provide more insight to the findings from the measurements. From chemical kinetic calculations a distinct shift in NOx formation pathways (thermal NOx vs. NOx through N2O/NNH reaction channels) can be observed for the different fuel mixtures at different pressure levels.


Author(s):  
Alireza Kalantari ◽  
Nicolas Auwaijan ◽  
Vincent McDonell

Abstract Lean-premixed combustion is commonly used in gas turbines to achieve low pollutant emissions, in particular nitrogen oxides. But use of hydrogen-rich fuels in premixed systems can potentially lead to flashback. Adding significant amounts of hydrogen to fuel mixtures substantially impacts the operating range of the combustor. Hence, to incorporate high hydrogen content fuels into gas turbine power generation systems, flashback limits need to be determined at relevant conditions. The present work compares two boundary layer flashback prediction methods developed for turbulent premixed jet flames. The Damköhler model was developed at University of California Irvine (UCI) and evaluated against flashback data from literature including actual engines. The second model was developed at Paul Scherrer Institut (PSI) using data obtained at gas turbine premixer conditions and is based on turbulent flame speed. Despite different overall approaches used, both models characterize flashback in terms of similar parameters. The Damköhler model takes into account the effect of thermal coupling and predicts flashback limits within a reasonable range. But the turbulent flame speed model provides a good agreement for a cooled burner, but shows less agreement for uncooled burner conditions. The impact of hydrogen addition (0 to 100% by volume) to methane or carbon monoxide is also investigated at different operating conditions and flashback prediction trends are consistent with the existing data at atmospheric pressure.


Author(s):  
Xiaoxiang Zhang ◽  
Nur Farizan Munjat ◽  
Jeevan Jayasuriya ◽  
Reza Fakhrai ◽  
Torsten Fransson

It is essentially important to use appropriate chemical kinetic models in the simulation process of gas turbine combustion. To integrate the detailed kinetics into complex combustion simulations has proven to be a computationally expensive task with tens to thousands of elementary reaction steps. It has been suggested that an appropriate simplified kinetics which are computationally efficient could be used instead. Therefore reduced kinetics are often used in CFD simulation of gas turbine combustion. At the same time, simplified kinetics for specific fuels and operation conditions need to be carefully selected to fulfill the accuracy requirements. The applicability of several simplified kinetics for premixed Gasified Biomass Gas (GBG) and air combustion are evaluated in this paper. The current work is motivated by the growing demand of gasified biomass gas (GBG) fueled combustion. Even though simplified kinetic schemes developed for hydrocarbon combustions are published by various researchers, there is little research has been found in literature to evaluate the ability of the simplified chemical kinetics for the GBG combustion. The numerical Simulation tool “CANTERA” is used in the current study for the comparison of both detailed and simplified chemical kinetics. A simulated gas mixture of CO/H2/CH4/CO2/N2 is used for the current evaluation, since the fluctuation of GBG components may have an unpredictable influence on the simulation results. The laminar flame speed has an important influence with flame stability, extinction limits and turbulent flame speed, here it is chosen as an indicator for validation. The simulation results are compared with the experimental data from the previous study [1] which is done by our colleagues. Water vapour which has shown a dilution effect in the experimental study are also put into concern for further validation. As the results indicate, the reduced kinetics which are developed for hydrocarbon or hydrogen combustion need to be highly optimized before using them for GBG combustion. Further optimization of the reduced kinetics is done for GBG and moderate results are achieved using the optimized kinetics compared with the detailed combustion kinetics.


2014 ◽  
Vol 39 (35) ◽  
pp. 20242-20254 ◽  
Author(s):  
Yu-Chun Lin ◽  
Peter Jansohn ◽  
Konstantinos Boulouchos

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