Flame Characteristics and Turbulent Flame Speeds of Turbulent, High-Pressure, Lean Premixed Methane/Air Flames

Author(s):  
P. Griebel ◽  
R. Bombach ◽  
A. Inauen ◽  
R. Scha¨ren ◽  
S. Schenker ◽  
...  

The present experimental study focuses on flame characteristics and turbulent flame speeds of lean premixed flames typical for stationary gas turbines. Measurements were performed in a generic combustor at a preheating temperature of 673 K, pressures up to 14.4 bars (absolute), a bulk velocity of 40 m/s, and an equivalence ratio in the range of 0.43–0.56. Turbulence intensities and integral length scales were measured in an isothermal flow field with Particle Image Velocimetry (PIV). The turbulence intensity (u′) and the integral length scale (LT) at the combustor inlet were varied using turbulence grids with different blockage ratios and different hole diameters. The position, shape, and fluctuation of the flame front were characterized by a statistical analysis of Planar Laser Induced Fluorescence images of the OH radical (OH-PLIF). Turbulent flame speeds were calculated and their dependence on operating conditions (p, φ) and turbulence quantities (u′, LT) are discussed and compared to correlations from literature. No influence of pressure on the most probable flame front position or on the turbulent flame speed was observed. As expected, the equivalence ratio had a strong influence on the most probable flame front position, the spatial flame front fluctuation, and the turbulent flame speed. Decreasing the equivalence ratio results in a shift of the flame front position farther downstream due to the lower fuel concentration and the lower adiabatic flame temperature and subsequently lower turbulent flame speed. Flames operated at leaner equivalence ratios show a broader spatial fluctuation as the lean blow-out limit is approached and therefore are more susceptible to flow disturbances. In addition, because of a lower turbulent flame speed these flames stabilize farther downstream in a region with higher velocity fluctuations. This increases the fluctuation of the flame front. Flames with higher turbulence quantities (u′, LT) in the vicinity of the combustor inlet exhibited a shorter length and a higher calculated flame speed. An enhanced turbulent heat and mass transport from the recirculation zone to the flame root location due to an intensified mixing which might increase the preheating temperature or the radical concentration is believed to be the reason for that.

Author(s):  
Pradeep Parajuli ◽  
Tyler Paschal ◽  
Mattias A. Turner ◽  
Eric L. Petersen ◽  
Waruna D. Kulatilaka

Abstract Natural gas is a major fuel source for many industrial and power-generation applications. The primary constituent of natural gas is methane (CH4), while smaller quantities of higher order hydrocarbons such as ethane (C2H6) and propane (C3H8) can also be present. Detailed understanding of natural gas combustion is important to obtain the highest possible combustion efficiency with minimal environmental impact in devices such as gas turbines and industrial furnaces. For a better understanding the combustion performance of natural gas, several important parameters to study are the flame temperature, heat release zone, flame front evolution, and laminar flame speed as a function of flame equivalence ratio. Spectrally and temporally resolved, high-speed chemiluminescence imaging can provide direct measurements of some of these parameters under controlled laboratory conditions. A series of experiments were performed on premixed methane/ethane-air flames at different equivalence ratios inside a closed flame speed vessel that allows the direct observation of the spherically expanding flame front. The vessel was filled with the mixtures of CH4 and C2H6 along with respective partial pressures of O2 and N2, to obtain the desired equivalence ratios at 1 atm initial pressure. A high-speed camera coupled with an image intensifier system was used to capture the chemiluminescence emitted by the excited hydroxyl (OH*) and methylidyne (CH*) radicals, which are two of the most important species present in the natural gas flames. The calculated laminar flame speeds for an 80/20 methane/ethane blend based on high-speed chemiluminescence images agreed well with the previously conducted Z-type schlieren imaging-based measurements. A high-pressure test, conducted at 5 atm initial pressure, produced wrinkles in the flame and decreased flame propagation rate. In comparison to the spherically expanding laminar flames, subsequent turbulent flame studies showed the sporadic nature of the flame resulting from multiple flame fronts that were evolved discontinuously and independently with the time. This paper documents some of the first results of quantitative spherical flame speed experiments using high-speed chemiluminescence imaging.


Author(s):  
Alireza Kalantari ◽  
Nicolas Auwaijan ◽  
Vincent McDonell

Abstract Lean-premixed combustion is commonly used in gas turbines to achieve low pollutant emissions, in particular nitrogen oxides. But use of hydrogen-rich fuels in premixed systems can potentially lead to flashback. Adding significant amounts of hydrogen to fuel mixtures substantially impacts the operating range of the combustor. Hence, to incorporate high hydrogen content fuels into gas turbine power generation systems, flashback limits need to be determined at relevant conditions. The present work compares two boundary layer flashback prediction methods developed for turbulent premixed jet flames. The Damköhler model was developed at University of California Irvine (UCI) and evaluated against flashback data from literature including actual engines. The second model was developed at Paul Scherrer Institut (PSI) using data obtained at gas turbine premixer conditions and is based on turbulent flame speed. Despite different overall approaches used, both models characterize flashback in terms of similar parameters. The Damköhler model takes into account the effect of thermal coupling and predicts flashback limits within a reasonable range. But the turbulent flame speed model provides a good agreement for a cooled burner, but shows less agreement for uncooled burner conditions. The impact of hydrogen addition (0 to 100% by volume) to methane or carbon monoxide is also investigated at different operating conditions and flashback prediction trends are consistent with the existing data at atmospheric pressure.


Author(s):  
Thoralf G. Reichel ◽  
Katharina Goeckeler ◽  
Oliver Paschereit

In the context of lean premixed combustion, the prevention of upstream flame propagation in the premixing zone, referred to as flashback (FB), is a crucial challenge related to the application of hydrogen as a fuel for gas turbines. The location of flame anchoring and its impact on FB tendencies in a technically premixed, swirl-stabilized hydrogen burner are investigated experimentally at atmospheric pressure conditions using planar laser-induced fluorescence of hydroxyl radicals (OH-PLIF). The inlet conditions are systematically varied with respect to equivalence ratio (ϕ=0.2−1.0), bulk air velocity u0 = 30–90 m/s, and burner preheat temperature ranging from 300 K to 700 K. The burner is mounted in an atmospheric combustion test rig, firing at a power of up to 220 kW into a 105 mm diameter quartz cylinder, which provides optical access to the flame region. The experiments were performed using an in-house burner design that previously proved to be highly resistant against FB occurrence by applying the axial air injection strategy. Axial air injection constitutes a nonswirling air jet on the central axis of the radial swirl generator. While a high rate of axial air injection yields excellent FB resistance, reduced rates of air injection are utilized to trigger FB, which allowed to investigate the near FB flame behavior. Results show that both, fuel momentum of hydrogen and axial air injection, alter the isothermal flow field as they cause a downstream shift of vortex breakdown and, thus, the axial flame front location. Such a shift is proven beneficial for FB resistance from the recorded FB limits. This effect was quantified by applying an edge detection algorithm to the OH-PLIF images, in order to extract the location of maximum flame front probability xF. By these means, it was revealed that for hydrogen xF is shifted downstream with increasing equivalence ratio due to the added momentum of the fuel flow, superseding any parallel augmentation in the turbulent flame speed. The parameter xF is identified to be governed by J, the momentum ratio between fuel and air flow, over a wide range of inlet conditions. These results contribute to the understanding of the sensitivity of FB to changes in the flow field, stemming from geometry changes or specific fuel properties.


Fluids ◽  
2019 ◽  
Vol 4 (3) ◽  
pp. 146 ◽  
Author(s):  
Aaron Endres ◽  
Thomas Sattelmayer

Boundary layer flashback from the combustion chamber into the premixing section is a threat associated with the premixed combustion of hydrogen-containing fuels in gas turbines. In this study, the effect of pressure on the confined flashback behaviour of hydrogen-air flames was investigated numerically. This was done by means of large eddy simulations with finite rate chemistry as well as detailed chemical kinetics and diffusion models at pressures between 0 . 5 and 3 . It was found that the flashback propensity increases with increasing pressure. The separation zone size and the turbulent flame speed at flashback conditions decrease with increasing pressure, which decreases flashback propensity. At the same time the quenching distance decreases with increasing pressure, which increases flashback propensity. It is not possible to predict the occurrence of boundary layer flashback based on the turbulent flame speed or the ratio of separation zone size to quenching distance alone. Instead the interaction of all effects has to be accounted for when modelling boundary layer flashback. It was further found that the pressure rise ahead of the flame cannot be approximated by one-dimensional analyses and that the assumptions of the boundary layer theory are not satisfied during confined boundary layer flashback.


Author(s):  
Thoralf G. Reichel ◽  
Katharina Goeckeler ◽  
Oliver Paschereit

In the context of lean premixed combustion, the prevention of upstream flame propagation in the premixing zone, referred to as flashback, is a crucial challenge related to the application of hydrogen as a fuel for gas turbines. The location of flame anchoring and its impact on flashback tendencies in a technically premixed, swirl-stabilized hydrogen burner are investigated experimentally at atmospheric pressure conditions using planar laser-induced fluorescence of hydroxyl radicals (OH-PLIF). The inlet conditions are systematically varied with respect to equivalence ratio (ϕ = 0.2–1.0), bulk air velocity u0 = 30–90m/s and burner preheat temperature ranging from 300K to 700K. The burner is mounted in the atmospheric combustion test rig at the HFI, firing at a power of up to 220 kW into a 105 mm diameter quartz cylinder, which provides optical access to the flame region. The experiments were performed using an in-house burner design that previously proved to be highly resistant against flashback occurrence by applying the axial air injection strategy. Axial air injection constitutes a non-swirling air jet on the central axis of the radial swirl generator, thus, influencing the vortex breakdown position. High axial air injection yields excellent flashback resistance and is used to investigate the whole inlet parameter space. In order to trigger flashback, the amount of axially injected air is reduced, which allowed to investigate the near flashback flame behavior. Results show that both, fuel momentum of hydrogen and axial air injection alter the isothermal flow field and cause a downstream shift of the axial flame front location. Such a shift is proven beneficial for flashback resistance. This effect was quantified by applying an edge detection algorithm to the OH-PLIF images, in order to extract the location of maximum flame front likelihood xF. The temperature and equivalence ratio dependence of the parameters xF is identified to be governed by the momentum ratio between fuel and air flow J. These results contribute to the understanding of the superior flashback limits of configurations applying high amounts of axial air injection over medium or none air injection.


Author(s):  
Andrew Marshall ◽  
Julia Lundrigan ◽  
Prabhakar Venkateswaran ◽  
Jerry Seitzman ◽  
Tim Lieuwen

Fuel composition has a strong influence on the turbulent flame speed, even at very high turbulence intensities. An important implication of this result is that the turbulent flame speed cannot be extrapolated from one fuel to the next using only the laminar flame speed and turbulence intensity as scaling variables. This paper presents curvature and tangential strain rate statistics of premixed turbulent flames for high hydrogen content fuels. Global (unconditioned) stretch statistics are presented as well as measurements conditioned on the leading points of the flame front. These measurements are motivated by previous experimental and theoretical work that suggests the turbulent flame speed is controlled by the flame front characteristics at these points. The data were acquired with high speed particle image velocimetry (PIV) in a low swirl burner (LSB). We attained measurements for several H2:CO mixtures over a range of mean flow velocities and turbulence intensities. The results show that fuel composition has a systematic, yet weak effect on curvatures and tangential strain rates at the leading points. Instead, stretch statistics at the leading points are more strongly influenced by mean flow velocity and turbulence level. It has been argued that the increased turbulent flame speeds seen with increasing hydrogen content are the result of increasing flame stretch rates, and therefore SL,max values, at the flame leading points. However, the differences observed with changing fuel compositions are not significant enough to support this hypothesis. Additional analysis is needed to understand the physical mechanisms through which the turbulent flame speed is altered by fuel composition effects.


Author(s):  
Alejandro M. Briones ◽  
Balu Sekar ◽  
Timothy Erdmann

The effect of centrifugal force on flame propagation velocity of stoichiometric propane-, kerosene-, and n-octane-air turbulent premixed flames was numerically examined. The quasi-turbulent numerical model was set in an unsteady two-dimensional geometry with finite length in the transverse and streamwise directions but with infinite length in the spanwise direction. There was relatively good comparison between literature-reported measurements and predictions of propane-air flame propagation velocity as a function of centrifugal force. It was found that for all mixtures the flame propagation velocity increases with centrifugal force. It reaches a maximum then falls off rapidly with further increases in centrifugal force. The results of this numerical study suggest there are no distinct differences among the three mixtures in terms of the effect of centrifugal force on the flame propagation velocity. There are, however, quantitative differences. The numerical models are set in a non-inertial, rotating reference frame. This rotation imposes a radially outward (centrifugal) force. The ignited mixture at one end of the tube raises the temperature and its heat release tends to laminarize the flow. The attained density difference combined with the direction of the centrifugal force promotes Rayleigh-Taylor instability. This instability with thermal expansion and turbulent flame speed constitute the flame propagation mechanism towards the other tube end. A wave is also originated but propagates faster than the flame. During propagation the flame interacts with eddies that wrinkle and/or corrugate the flame. The flame front wrinkles interact with streamtubes that enhance Landau-Darrieus (hydrodynamic) instability, giving rise to a corrugated flame. Under strong stretch conditions the stabilizing equidiffusive-curvature mechanism fails and the flame front breaks up, allowing inflow of unburned mixture into the flame. This phenomenon slows down the flame temporarily and then the flame speeds up faster than before. However, if corrugation is large and the inflow of unburned mixture into the flame is excessive, the latter locally quenches and slows down the flame. This occurs when the centrifugal force is large, tending to blowout the flame. The wave in the tube interacts continuously with the flame through baroclinic torques at the flame front that further enhances the above mentioned flame-eddies interactions. Only at low centrifugal forces the wave intermingles several times with the flame before the averaged flame propagation velocity is determined. The centrifugal force does not substantially increase the turbulent flame speed as commented by previous experimental investigations. The results also suggest that an ultra-compact combustor (UCC) with high-g cavity (HGC) will be limited to centrifugal force levels in the 2000–3000g range.


Author(s):  
S. Ravi ◽  
A. Morones ◽  
E. L. Petersen ◽  
F. Güthe

Natural gas is the primary fuel for stationary, powergeneration gas turbines, and it is necessary to understand its combustion characteristics under engine-relevant (turbulent) conditions. Since its composition varies depending on the fuel source, a natural gas surrogate (NG 18% C2+) and admixtures with H2 have been utilized recently by the authors to aid chemical kinetics modeling using ignition delay times and laminar flame speed experiments. The present study focused on measuring turbulent flame speeds (displacement speeds) of natural gas (NG2) and methane with H2 using a fan-stirred flame bomb. The apparatus is a closed, cylindrical chamber fitted with four radial impellers that generate a central spherical volume of homogeneous and isotropic turbulence with negligible mean flow. Schlieren imaging was used to visually track the growth of the spherically expanding turbulent kernels during the constant-pressure period. The turbulence levels were fixed at an average RMS intensity level of 1.5 m/s and at an integral length scale of 27 mm. Turbulent flame speeds (ST,0.1) of NG2 blends were measured over a wide range of equivalence ratios between 0.7 and 1.3. ST,0.1 for the natural gas surrogate closely matched with those of methane for near-stoichiometric mixtures. However, preferential-diffusion effects (fuel effects) were observed under turbulent conditions for off-stoichiometric cases. The effects of hydrogen addition on the turbulent flame speeds of NG2 (25/75 and 50/50 (by volume) blends of H2/NG2) were also investigated and were compared with the flame speeds reported in a recent paper by the authors (ASME GT2014-26742) on the effects of hydrogen addition to turbulent flame speeds of methane. The effect of the hydrogen addition was to increase the turbulent flame speed (by about a factor of two for 50% H2 addition), although this effect was much more pronounced for the lean and stoichiometric mixtures. Interestingly, the flame speeds (both laminar and turbulent) of the CH4 blends with H2 were slightly larger than those for the NG2 blend at equivalent conditions, or about 10–20% larger at 50% H2 addition. This behavior can be explained kinetically by the increased importance of the inhibiting reaction CH3 + H (+M) ↔ CH4 (+M), where ethane oxidation produces more CH3 radicals than methane at similar conditions.


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