Confined Transducer Geometries to Enhance Sensitivity to Thermal Boundary Conductance in Frequency-Domain Thermoreflectance Measurements

2021 ◽  
Author(s):  
Ronald J. Warzoha ◽  
Adam A. Wilson ◽  
Brian F. Donovan ◽  
Andy Clark ◽  
Xuemei Cheng ◽  
...  

Abstract Quantifying the resistance to heat flow across well-bonded, planar interfaces is critical in modern electronics packaging architectures, particularly as device length scales are reduced and power demands continue to grow unabated. However, very few experimental techniques are capable of measuring the thermal resistance across such interfaces due to limitations in the required measurement resolution provided by the characterization technique (i.e., Rth < 0.1 mm2·K/W in steady-state configurations) and restrictions on the thermal penetration depth that can be achieved as a result of the heating event that is typically imposed on a sample’s surface (for optical pump-probe thermoreflectance techniques). A recent numerical fitting routine for Frequency-domain Thermoreflectance (FDTR) developed by the authors1 offers a potential avenue to rectify these issues if the transducer’s geometry can be confined. This work utilizes numerical simulations to evaluate the sensitivity of FDTR to a range of thermal boundary resistance (TBR) values as a function of the thermal resistance of adjacent material layers. Experimental measurements are performed across a handful of different material systems to validate our computational results and to demonstrate the the extent to which confined transducer geometries can improve our sensitivyt to the TBR across so-called “buried” interfaces when characterized with FDTR.

Author(s):  
Patrick E. Hopkins ◽  
Justin R. Serrano ◽  
Leslie M. Phinney

Pump-probe transient thermoreflectance (TTR) techniques are powerful tools for measuring thermophysical properties of thin films, such as thermal conductivity, Λ, or thermal boundary conductance, G. TTR experimental setups rely on lock-in techniques to detect the response of the probe signal relative to the pump heating event. The temporal decays of the lock-in signal are then compared to thermal models to deduce the Λ and G in and across various materials. There are currently two thermal models that are used to relate the measured signals from the lock-in to the Λ and G in the sample of interest. In this work, the thermal models, their assumptions, and their ranges of applicability are compared. The advantages and disadvantages of each technique are elucidated from the results of the thermophysical property measurements.


2003 ◽  
Vol 770 ◽  
Author(s):  
Nathanael Smith ◽  
Max J. Lederer ◽  
Marek Samoc ◽  
Barry Luther-Davies ◽  
Robert G. Elliman

AbstractOptical pump-probe measurements were performed on planar slab waveguides containing silicon nanocrystals in an attempt to measure optical gain from photo-excited silicon nanocrystals. Two experiments were performed, one with a continuous-wave probe beam and a pulsed pump beam, giving a time resolution of approximately 25 ns, and the other with a pulsed pump and probe beam, giving a time resolution of approximately 10 ps. In both cases the intensity of the probe beam was found to be attenuated by the pump beam, with the attenuation increasing monotonically with increasing pump power. Time-resolved measurements using the first experimental arrangement showed that the probe signal recovered its initial intensity on a time scale of 45-70 μs, a value comparable to the exciton lifetime in Si nanocrystals. These data are shown to be consistent with an induced absorption process such as confined carrier absorption. No evidence for optical gain was observed.


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Konrad Rolle ◽  
Dmytro Yaremkevich ◽  
Alexey V. Scherbakov ◽  
Manfred Bayer ◽  
George Fytas

AbstractHypersonic phononic bandgap structures confine acoustic vibrations whose wavelength is commensurate with that of light, and have been studied using either time- or frequency-domain optical spectroscopy. Pulsed pump-probe lasers are the preferred instruments for characterizing periodic multilayer stacks from common vacuum deposition techniques, but the detection mechanism requires the injected sound wave to maintain coherence during propagation. Beyond acoustic Bragg mirrors, frequency-domain studies using a tandem Fabry–Perot interferometer (TFPI) find dispersions of two- and three-dimensional phononic crystals (PnCs) even for highly disordered samples, but with the caveat that PnCs must be transparent. Here, we demonstrate a hybrid technique for overcoming the limitations that time- and frequency-domain approaches exhibit separately. Accordingly, we inject coherent phonons into a non-transparent PnC using a pulsed laser and acquire the acoustic transmission spectrum on a TFPI, where pumped appear alongside spontaneously excited (i.e. incoherent) phonons. Choosing a metallic Bragg mirror for illustration, we determine the bandgap and compare with conventional time-domain spectroscopy, finding resolution of the hybrid approach to match that of a state-of-the-art asynchronous optical sampling setup. Thus, the hybrid pump–probe technique retains key performance features of the established one and going forward will likely be preferred for disordered samples.


2008 ◽  
Vol 1 ◽  
pp. 121301 ◽  
Author(s):  
Shigemi Mizukami ◽  
Hiroyuki Abe ◽  
Daisuke Watanabe ◽  
Mikihiko Oogane ◽  
Yasuo Ando ◽  
...  

Author(s):  
Д.И Хусяинов ◽  
А.М. Буряков ◽  
В.Р. Билык ◽  
Е.Д. Мишина ◽  
Д.С. Пономарев ◽  
...  
Keyword(s):  

Методами оптического зондирования при фемтосекундной лазерной накачке (optical pump-probe) и терагерцевой спектроскопии во временной области исследовано влияние эпитаксиальных напряжений на динамику неравновесных носителей заряда, а также спектр терагерцевого излучения в пленках InyGa1-yAs. Продемонстрировано снижение времени жизни неравновесных носителей заряда и увеличение ширины спектра терагерцевого излучения для пленки InyGa1-yAs с большим механическим напряжением. DOI: 10.21883/PJTF.2017.22.45260.16958


Author(s):  
Joshua Alper ◽  
Aaron Schmidt ◽  
Kimberly Hamad-Schifferli

To facilitate analysis of nanoscale heat transfer in nanoparticle systems the thermal properties of ligand layers must be understood. To this end, we use an optical pump-probe technique to study the thermal transport across ligands on gold nanorods and into the solvent. We find that varying properties of the ligand can have large impacts on the thermal decay of a nanorod after exposure to a laser pulse. By raising the concentration of free CTAB from 1 mM and 10 mM in solutions, the CTAB layer’s effective thermal interface conductance increases three fold. The transition occurs near the CTAB critical micelle concentration. Similar results are found for other ligand layers.


2004 ◽  
Author(s):  
Verner K. Thorsmølle ◽  
R D. Averitt ◽  
J Demsar ◽  
X Chi ◽  
S Tretiak ◽  
...  

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