scholarly journals К расчету оптических характеристик и размерных сдвигов поверхностных плазмонов сферических биметаллических наночастиц

2021 ◽  
Vol 63 (1) ◽  
pp. 120
Author(s):  
А.В. Коротун ◽  
В.В. Погосов

Formulas are obtained for the effective relaxation time when the electron mean free path is less or comparable with the characteristic dimensions of the metallic regions. The frequency dispersion of the optical characteristics of spherical bimetallic particles near plasma resonances is calculated in the absence of quantum-size effects. Maintaining the style of the generally accepted description of monometallic particles based on the theories of Drude and Mie, the frequency dependence of the electric dipole polarizability of a two-layer metal nanosphere is analyzed. The appearance of two maxima of polarizability is a consequence of the difference between the metals of the core and the shell. The calculations were performed for Au @ Ag, Ag @ Au, Au @ Pt, Pt @ Au, and Pt @ Pd particles immersed in Teflon. The possibility of controlling the optical characteristics of bimetallic particles by changing their composition and volumetric content of metals has been demonstrated. The calculations of the absorption and scattering cross sections, as well as the optical radiation efficiency of particles in a wide spectral range, have been performed. The possible temperature of bimetallic particles upon absorption of an electromagnetic wave (for the purposes of photothermal therapy of malignant tumors) has been estimated. Key words: bimetallic nanoparticle, surface plasmon, polarizability, absorption cross section, scattering cross section, relaxation time.

Author(s):  
P.A. Crozier

Absolute inelastic scattering cross sections or mean free paths are often used in EELS analysis for determining elemental concentrations and specimen thickness. In most instances, theoretical values must be used because there have been few attempts to determine experimental scattering cross sections from solids under the conditions of interest to electron microscopist. In addition to providing data for spectral quantitation, absolute cross section measurements yields useful information on many of the approximations which are frequently involved in EELS analysis procedures. In this paper, experimental cross sections are presented for some inner-shell edges of Al, Cu, Ag and Au.Uniform thin films of the previously mentioned materials were prepared by vacuum evaporation onto microscope cover slips. The cover slips were weighed before and after evaporation to determine the mass thickness of the films. The estimated error in this method of determining mass thickness was ±7 x 107g/cm2. The films were floated off in water and mounted on Cu grids.


1996 ◽  
Vol 74 (7-8) ◽  
pp. 505-508 ◽  
Author(s):  
R. M. Finch ◽  
Á. Kövér ◽  
M. Charlton ◽  
G. Laricchia

Differential cross sections for elastic scattering and ionization in positron–argon collisions as a function of energy (40–150 eV) are reported at 60°. Of particular interest is the energy range 55–60 eV, where earlier measurements by the Detroit group found a drop in the elastic-scattering cross section of a factor of 2. This structure has been tentatively attributed to a cross channel-coupling effect with an open inelastic-scattering channel, most likely ionization. Our results indicate that ionization remains an important channel over the same energy range and only begins to decrease at an energy above 60 eV.


1988 ◽  
Vol 128 ◽  
Author(s):  
N. R. Parikh ◽  
Z. H. Zhang ◽  
M. L. Swanson ◽  
N. Yu ◽  
W. K. Chu

ABSTRACTElastic scattering of protons with energies from 1.5 MeV to 2 MeV was used to determine the concentration of oxygen in Y-Ba-Cu-O compound, nitrogen in GaN films, and boron in B-Si glass and other materials. Proton scattering from light elements in this energy range exhibits non-Rutherford scattering cross section, which are enhanced by a factor of 3 to 6 or more relative to the Rutherford scattering cross sections. Thus the sensitivity for the light clement detection is considerably larger than that obtained by He ion scattering.Quantitative analysis by proton scattering is discussed and compared with other methods.


2011 ◽  
Vol 10 (3) ◽  
pp. 672-694
Author(s):  
Lorella Fatone ◽  
Maria Cristina Recchioni ◽  
Francesco Zirilli

AbstractAcoustic scattering cross sections of smart furtive obstacles are studied and discussed. A smart furtive obstacle is an obstacle that, when hit by an incoming field, avoids detection through the use of a pressure current acting on its boundary. A highly parallelizable algorithm for computing the acoustic scattering cross section of smart obstacles is developed. As a case study, this algorithm is applied to the (acoustic) scattering cross section of a “smart” (furtive) simplified version of the NASA space shuttle when hit by incoming time-harmonic plane waves, the wavelengths of which are small compared to the characteristic dimensions of the shuttle. The solution to this numerically challenging scattering problem requires the solution of systems of linear equations with many unknowns and equations. Due to the sparsity of these systems of equations, they can be stored and solved using affordable computing resources. A cross section analysis of the simplified NASA space shuttle highlights three findings: i) the smart furtive obstacle reduces the magnitude of its cross section compared to the cross section of a corresponding “passive” obstacle; ii) several wave propagation directions fail to satisfactorily respond to the smart strategy of the obstacle; iii) satisfactory furtive effects along all directions may only be obtained by using a pressure current of considerable magnitude. Numerical experiments and virtual reality applications can be found at the website: http://www.ceri.uniromal.it/ceri/zirilli/w7.


2019 ◽  
Vol 219 ◽  
pp. 10005
Author(s):  
Kenji Mishima ◽  
Toshiya Otomo ◽  
Kazutaka Ikeda ◽  
Hidetoshi Ohshita

Due to their large coherent scattering cross section, diamond nanoparticles (DNPs) are considered as a promising candidate material for a new neutron reflector. For investigation of scattering cross sections of packed samples, we have developed a technique for mechanical compression of DNP powder. Application of 220 MPa allowed us to increase the bulk density from 0.40 g/cm3 to 1.1 g/cm3. The differential cross sections of uncompressed and packed samples were measured using the high-intensity total diffractometer instrument NOVA at J-PARC, covering transfer wavenumbers (q) from 0.6 to 100 nm−1. The q dependence for the compressed sample agreed with the theoretical expectation derived from the Born approximation applied to homogeneous spheres with inclusion of a hard-sphere model to account for the inter-particle structure, whereas the results obtained from the powder sample disagreed. This implies that the theoretical description does not well represent the mesoscopic structure of the DNP powder sample.


2020 ◽  
Vol 239 ◽  
pp. 14007
Author(s):  
Vaibhav Jaiswal ◽  
Luiz Leal ◽  
Alexander I. Kolesnikov

Thermal neutron scattering cross-section data for light water available in the major nuclear data libraries observes significant differences especially at reactor operating temperatures. During the past few years there has been a renewed interest in reviewing the existing thermal scattering models and generating more accurate and reliable thermal scattering cross sections using existing experimental data and in some cases based on Molecular Dynamics (MD) simulations. There is a need for performing new time-of-flight experiments at high temperatures and pressures, to have a better understanding of the physics involved in the scattering process that could help improve the existing TSL data. Lack of experimental thermal scattering data for light water at high temperatures led to a new measurement campaign within the INSIDER project at the Institut de radioprotection et de sûreté nucléaire (IRSN). Double differential scattering cross section for light water have been measured at the SEQUOIA spectrometer based at the Spallation Neutron Source (SNS), Oak Ridge National Laboratory, United States. Several measurements have been carried out at different temperatures and pressures corresponding to liquid light water. Measurements at five different incident neutron energies Ei (8, 60, 160, 280 and 800 meV) have been carried out to help exploring different regions of the frequency spectrum. This paper presents the analysis of the dynamic structure factor and the derived frequency spectrum of light water. The analysis of the experimental data would provide one with better confidence, the behavior of thermal scattering cross sections for light water at high temperatures, knowledge of which is very important for the design of novel reactors as well as existing pressurized water reactors.


1968 ◽  
Vol 46 (24) ◽  
pp. 2755-2763 ◽  
Author(s):  
Chin-Lin Chen

The problem of the scattering of a plane wave by a long, thin, perfectly conducting wire is studied. The scatterer is loaded at its center by a lumped element. The effects of the loading on the scattering of waves are investigated. Numerical results are obtained for the case of normal incidence. The results show that for relatively short wires, the back-scattering cross sections may be modified effectively by central loading, while for longer wires, the modification is rather difficult to achieve. To nullify the back-scattering cross section completely, it is necessary to use active loading if kh > 3.6. A physical explanation is also presented.


1975 ◽  
Vol 53 (17) ◽  
pp. 1672-1686 ◽  
Author(s):  
H. C. Chow ◽  
G. M. Griffiths ◽  
T. H. Hall

The cross section for the direct radiative capture of protons by 16O has been measured relative to the proton elastic scattering cross section for energies from 800 to 2400 keV (CM). The elastic scattering cross section was normalized to the Rutherford scattering cross section at 385.5 keV. The capture cross section for the reaction 16O(p,γ)17F, which plays a role in hydrogen burning stars, has been extrapolated to stellar energies using a theoretical model which gives a good fit to the measured cross sections. The model involves calculation of electromagnetic matrix elements between initial and final state wave functions evaluated for Saxon–Woods potentials with parameters adjusted to fit both elastic scattering data and binding energies for the ground and first excited states of 17F. Cross sections for capture to the 5/2+ ground and 1/2+ first excited states of 17F in terms of astrophysical S factors valid for energies ≤ 100 keV have been found to be: S5/2+ = (0.317 + 0.0002E) keV b (± 8%); S1/2+ = (8.552 − 0.353E + 0.00013E2) keV b (± 5%).


Differential cross-sections have been measured for the scattering of photons of mean energy 87 MeV by uranium at eight angles in the range from 1.18 to 4.48 mrad and by aluminium, silver, tungsten, lead and uranium at angles of 1.89 and 4.24 mrad, using a narrowly collimated bremsstrahlung beam from the Oxford 110 MeV synchrotron as the primary source of photons. A biased total-absorption Čerenkov counter was used to detect photons with energies near the peak energy of the bremsstrahlung spectrum, and absolute differential cross-sections were measured by comparing counting rates for photons in the primary and scattered beams. The experimental results, with the differential Compton scattering cross-sections of Klein and Nishina subtracted, were analyzed in terms of their variation with angle and atomic number, and can be described as consisting of a sharply peaked angular distribution with absolute cross-sections varying from element to element as Z 4 , together with a uniform distribution varying nearly as Z 2 ; these distributions were identified with Delbruck scattering and with bremsstrahlung from secondary electrons in the scattering target, respectively. The Delbruck scattering cross-section thus determined is slightly more sharply peaked than the cross-section predicted by an approximate theory of Bethe & Rohrlich.


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