Effect of gas flow rate and discharge volume on CO2 methanation with plasma catalysis

Author(s):  
Susumu Toko ◽  
Masashi Ideguchi ◽  
Taiki Hasegawa ◽  
Takamasa Okumura ◽  
Kunihiro KAMATAKI ◽  
...  

Abstract CO2 methanation can be a key technology for realizing a sustainable society. CH4 is used as an energy carrier and raw material for chemical products, thereby contributing to the reduction of CO2 emissions. Methanation with plasma catalysis lower the process temperature, which can improve the throughput and stability. In this study, we investigated the effect of the gas flow rate and the discharge volume on CO2 methanation, using a low- pressure CCP reactor. Higher gas flow rates can increase the rate of CO2 throughput, but the CH4 selectivity decreases owing to the reduced transportation rate of the reactants to the catalyst surface. Increasing the discharge volume is effective in improving the transportation rate. This study suggested that the structure of the reactor significantly affect the CH4 generation rate.

2012 ◽  
Vol 443-444 ◽  
pp. 637-642
Author(s):  
Yao Chun Yao ◽  
Takayuki Watanabe ◽  
Kazuyuki Yatsuda

A stable 12-phase AC arc was successfully generated and applied in the field of glass in-flight melting, the arc behavior was characterized by image analysis. The effects of electrode configuration and sheath gas flow rate on arc and melting behavior of granulated glass raw material were investigated. Results show that different electrode configurations leads to various arc discharge and high-temperature region. The luminance area with high-temperature region and its fluctuation reflect the change of arc discharge behavior. The vitrification degree of glass raw material is mostly dependent on the center temperature of arc. As the sheath gas flow rate increases, the ratio of luminance area decreases and the center temperature of arc increases.


2010 ◽  
Vol 82 (6) ◽  
pp. 1337-1351 ◽  
Author(s):  
Takayuki Watanabe ◽  
Kazuyuki Yatsuda ◽  
Yaochun Yao ◽  
Tetsuji Yano ◽  
Tsugio Matuura

A stable 12-phase AC arc was generated by transformers at a commercial electric power system, and the arc behavior was characterized by image analysis. For the unique advantages, the multiphase AC arc was developed to apply to in-flight glass melting for the purpose of energy-saving and emission reduction. The effects of electrode configuration and sheath gas flow rate on the arc and melting behavior of granulated glass raw material were investigated. Results show that the discharge behavior and the high-temperature region can be controlled by the electrode configuration. The luminance area of the high-temperature region and its fluctuation reflect the discharge behavior. The vitrification degree of glass raw material is mostly dependent on the center temperature of arc. As sheath gas flow rate increases, the ratio of luminance area decreases and the center temperature of arc increases.


2012 ◽  
Vol 479-481 ◽  
pp. 615-618
Author(s):  
Yao Chun Yao ◽  
Takayuki Watanabe ◽  
Kazuyuki Yatsuda

A stable 12-phase AC arc was successfully developed and applied in the field of glass in-flight melting, and the arc discharge behavior was characterized by image analysis. The effects of sheath gas flow rate on arc discharge and melting behavior of granulated glass raw material were investigated. Results show that different sheath gas flow rates lead to various arc discharge and high-temperature region. The fluctuation of luminance area ratio and coefficient of variation reflects the change of arc discharge behavior. As the sheath gas flow rate increases, the ratio of luminance area decreases and the center temperature of arc increases. The vitrification degree of glass raw material is mostly dependent on the center temperature of arc, higher center temperature and more vitrification degree.,A stable 12-phase AC arc was successfully developed and applied in the field of glass in-flight melting, and the arc discharge behavior was characterized by image analysis. The effects of sheath gas flow rate on arc discharge and melting behavior of granulated glass raw material were investigated. Results show that different sheath gas flow rates lead to various arc discharge and high-temperature region. The fluctuation of luminance area ratio and coefficient of variation reflects the change of arc discharge behavior. As the sheath gas flow rate increases, the ratio of luminance area decreases and the center temperature of arc increases. The vitrification degree of glass raw material is mostly dependent on the center temperature of arc, higher center temperature and more vitrification degree.


2012 ◽  
Vol 485 ◽  
pp. 185-188
Author(s):  
Yao Chun Yao ◽  
Takayuki Watanabe ◽  
Kazuyuki Yatsuda

Thermal plasma of 12-phase AC arc was successfully developed and applied in the field of glass in-flight melting, and the arc discharge behavior was characterized by image analysis. The effects of sheath gas flow rate on arc discharge and melting behavior of granulated glass raw material were investigated. Results show that different sheath gas flow rates lead to various arc discharge and high-temperature region. The fluctuation of luminance area ratio and coefficient of variation reflects the change of arc discharge behavior. As the sheath gas flow rate increases, the ratio of luminance area decreases and the center temperature of arc increases. The vitrification degree of glass raw material is mostly dependent on the center temperature of arc, higher center temperature and more vitrification degree.


Author(s):  
B.S. Soroka ◽  
V.V. Horupa

Natural gas NG consumption in industry and energy of Ukraine, in recent years falls down as a result of the crisis in the country’s economy, to a certain extent due to the introduction of renewable energy sources along with alternative technologies, while in the utility sector the consumption of fuel gas flow rate enhancing because of an increase the number of consumers. The natural gas is mostly using by domestic purpose for heating of premises and for cooking. These items of the gas utilization in Ukraine are already exceeding the NG consumption in industry. Cooking is proceeding directly in the living quarters, those usually do not meet the requirements of the Ukrainian norms DBN for the ventilation procedures. NG use in household gas stoves is of great importance from the standpoint of controlling the emissions of harmful components of combustion products along with maintenance the satisfactory energy efficiency characteristics of NG using. The main environment pollutants when burning the natural gas in gas stoves are including the nitrogen oxides NOx (to a greater extent — highly toxic NO2 component), carbon oxide CO, formaldehyde CH2O as well as hydrocarbons (unburned UHC and polyaromatic PAH). An overview of environmental documents to control CO and NOx emissions in comparison with the proper norms by USA, EU, Russian Federation, Australia and China, has been completed. The modern designs of the burners for gas stoves are considered along with defining the main characteristics: heat power, the natural gas flow rate, diameter of gas orifice, diameter and spacing the firing openings and other parameters. The modern physical and chemical principles of gas combustion by means of atmospheric ejection burners of gas cookers have been analyzed from the standpoints of combustion process stabilization and of ensuring the stability of flares. Among the factors of the firing process destabilization within the framework of analysis above mentioned, the following forms of unstable combustion/flame unstabilities have been considered: flashback, blow out or flame lifting, and the appearance of flame yellow tips. Bibl. 37, Fig. 11, Tab. 7.


1998 ◽  
Vol 63 (6) ◽  
pp. 881-898
Author(s):  
Otakar Trnka ◽  
Miloslav Hartman

Three simple computational techniques are proposed and employed to demonstrate the effect of fluctuating flow rate of feed on the behaviour and performance of an isothermal, continuous stirred tank reactor (CSTR). A fluidized bed reactor (FBR), in which a non-catalytic gas-solid reaction occurs, is also considered. The influence of amplitude and frequency of gas flow rate fluctuations on reactant concentrations at the exit of the CSTR is shown in four different situations.


Author(s):  
Pengju Huo ◽  
Xiaohong Li ◽  
Yang Liu ◽  
Haiying Qi

AbstractThe influences of loose gas on gas-solid flows in a large-scale circulating fluidized bed (CFB) gasification reactor were investigated using full-loop numerical simulation. The two-fluid model was coupled with the QC-energy minimization in multi-scale theory (EMMS) gas-solid drag model to simulate the fluidization in the CFB reactor. Effects of the loose gas flow rate, Q, on the solid mass circulation rate and the cyclone separation efficiency were analyzed. The study found different effects depending on Q: First, the particles in the loop seal and the standpipe tended to become more densely packed with decreasing loose gas flow rate, leading to the reduction in the overall circulation rate. The minimum Q that can affect the solid mass circulation rate is about 2.5% of the fluidized gas flow rate. Second, the sealing gas capability of the particles is enhanced as the loose gas flow rate decreases, which reduces the gas leakage into the cyclones and improves their separation efficiency. The best loose gas flow rates are equal to 2.5% of the fluidized gas flow rate at the various supply positions. In addition, the cyclone separation efficiency is correlated with the gas leakage to predict the separation efficiency during industrial operation.


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