scholarly journals Regional and monthly and clear-sky aerosol direct radiative effect (and forcing) derived from the GlobAEROSOL-AATSR satellite aerosol product

2013 ◽  
Vol 13 (1) ◽  
pp. 393-410 ◽  
Author(s):  
G. E. Thomas ◽  
N. Chalmers ◽  
B. Harris ◽  
R. G. Grainger ◽  
E. J. Highwood

Abstract. Using the GlobAEROSOL-AATSR dataset, estimates of the instantaneous, clear-sky, direct aerosol radiative effect and radiative forcing have been produced for the year 2006. Aerosol Robotic Network sun-photometer measurements have been used to characterise the random and systematic error in the GlobAEROSOL product for 22 regions covering the globe. Representative aerosol properties for each region were derived from the results of a wide range of literature sources and, along with the de-biased GlobAEROSOL AODs, were used to drive an offline version of the Met Office unified model radiation scheme. In addition to the mean AOD, best-estimate run of the radiation scheme, a range of additional calculations were done to propagate uncertainty estimates in the AOD, optical properties, surface albedo and errors due to the temporal and spatial averaging of the AOD fields. This analysis produced monthly, regional estimates of the clear-sky aerosol radiative effect and its uncertainty, which were combined to produce annual, global mean values of (−6.7 ± 3.9) W m−2 at the top of atmosphere (TOA) and (−12 ± 6) W m−2 at the surface. These results were then used to give estimates of regional, clear-sky aerosol direct radiative forcing, using modelled pre-industrial AOD fields for the year 1750 calculated for the AEROCOM PRE experiment. However, as it was not possible to quantify the uncertainty in the pre-industrial aerosol loading, these figures can only be taken as indicative and their uncertainties as lower bounds on the likely errors. Although the uncertainty on aerosol radiative effect presented here is considerably larger than most previous estimates, the explicit inclusion of the major sources of error in the calculations suggest that they are closer to the true constraint on this figure from similar methodologies, and point to the need for more, improved estimates of both global aerosol loading and aerosol optical properties.

2012 ◽  
Vol 12 (7) ◽  
pp. 18459-18497 ◽  
Author(s):  
G. E. Thomas ◽  
N. Chalmers ◽  
B. Harris ◽  
R. G. Grainger ◽  
E. J. Highwood

Abstract. Using the GlobAEROSOL-AATSR dataset, estimates of the instantaneous, clear-sky, direct aerosol radiative effect and radiative forcing have been produced for the year 2006. Aerosol Robotic Network sun-photometer measurements have been used to characterise the random and systematic error in the GlobAEROSOL product for 22 regions covering the globe. Representative aerosol properties for each region have been derived from the results of a wide range of literature sources and, along with the de-biased GlobAEROSOL AODs, were used to drive an offline version of the Met Office unified model radiation scheme. In addition to the mean AOD, best-estimate run of the radiation scheme, a range of additional calculations were done to propagate uncertainty estimates in the AOD, optical properties, surface albedo and errors due to the temporal and spatial averaging of the AOD fields. This analysis produced monthly, regional estimates of the clear-sky aerosol radiative effect and its uncertainty, which produce annual, global mean values of (−6.7 ± 3.9) W m−2 at the top of atmosphere (TOA) and (−12 ± 6) W m−2 at the surface. These results were then used to produce estimates of regional, clear-sky aerosol direct radiative forcing, using modelled pre-industrial AOD fields for 1750 calculated for the AEROCOM PRE experiment. However, as it was not possible to quantify the uncertainty in the pre-industrial aerosol loading, these figures can only be taken as indicative and their uncertainties as lower bounds on the likely errors. Although the uncertainty on aerosol radiative effect presented here is considerably larger than most previous estimates, the explicit inclusion of the major sources of error in the calculations suggest that they are closer to the true constraint on this figure from similar methodologies, and point to the need for more, improved estimates of both global aerosol loading and aerosol optical properties.


2017 ◽  
Vol 10 (1) ◽  
pp. 433-452 ◽  
Author(s):  
Bjorn Stevens ◽  
Stephanie Fiedler ◽  
Stefan Kinne ◽  
Karsten Peters ◽  
Sebastian Rast ◽  
...  

Abstract. A simple plume implementation of the second version (v2) of the Max Planck Institute Aerosol Climatology, MACv2-SP, is described. MACv2-SP provides a prescription of anthropogenic aerosol optical properties and an associated Twomey effect. It was created to provide a harmonized description of post-1850 anthropogenic aerosol radiative forcing for climate modeling studies. MACv2-SP has been designed to be easy to implement, change and use, and thereby enable studies exploring the climatic effects of different patterns of aerosol radiative forcing, including a Twomey effect. MACv2-SP is formulated in terms of nine spatial plumes associated with different major anthropogenic source regions. The shape of the plumes is fit to the Max Planck Institute Aerosol Climatology, version 2, whose present-day (2005) distribution is anchored by surface-based observations. Two types of plumes are considered: one predominantly associated with biomass burning, the other with industrial emissions. These differ in the prescription of their annual cycle and in their optical properties, thereby implicitly accounting for different contributions of absorbing aerosol to the different plumes. A Twomey effect for each plume is prescribed as a change in the host model's background cloud-droplet population density using relationships derived from satellite data. Year-to-year variations in the amplitude of the plumes over the historical period (1850–2016) are derived by scaling the plumes with associated national emission sources of SO2 and NH3. Experiments using MACv2-SP are performed with the Max Planck Institute Earth System Model. The globally and annually averaged instantaneous and effective aerosol radiative forcings are estimated to be −0.6 and −0.5 W m−2, respectively. Forcing from aerosol–cloud interactions (the Twomey effect) offsets the reduction of clear-sky forcing by clouds, so that the net effect of clouds on the aerosol forcing is small; hence, the clear-sky forcing, which is more readily measurable, provides a good estimate of the total aerosol forcing.


2018 ◽  
Vol 18 (6) ◽  
pp. 4131-4152 ◽  
Author(s):  
James P. Sherman ◽  
Allison McComiskey

Abstract. Aerosol optical properties measured at Appalachian State University's co-located NASA AERONET and NOAA ESRL aerosol network monitoring sites over a nearly four-year period (June 2012–Feb 2016) are used, along with satellite-based surface reflectance measurements, to study the seasonal variability of diurnally averaged clear sky aerosol direct radiative effect (DRE) and radiative efficiency (RE) at the top-of-atmosphere (TOA) and at the surface. Aerosol chemistry and loading at the Appalachian State site are likely representative of the background southeast US (SE US), home to high summertime aerosol loading and one of only a few regions not to have warmed during the 20th century. This study is the first multi-year ground truth DRE study in the SE US, using aerosol network data products that are often used to validate satellite-based aerosol retrievals. The study is also the first in the SE US to quantify DRE uncertainties and sensitivities to aerosol optical properties and surface reflectance, including their seasonal dependence.Median DRE for the study period is −2.9 W m−2 at the TOA and −6.1 W m−2 at the surface. Monthly median and monthly mean DRE at the TOA (surface) are −1 to −2 W m−2 (−2 to −3 W m−2) during winter months and −5 to −6 W m−2 (−10 W m−2) during summer months. The DRE cycles follow the annual cycle of aerosol optical depth (AOD), which is 9 to 10 times larger in summer than in winter. Aerosol RE is anti-correlated with DRE, with winter values 1.5 to 2 times more negative than summer values. Due to the large seasonal dependence of aerosol DRE and RE, we quantify the sensitivity of DRE to aerosol optical properties and surface reflectance, using a calendar day representative of each season (21 December for winter; 21 March for spring, 21 June for summer, and 21 September for fall). We use these sensitivities along with measurement uncertainties of aerosol optical properties and surface reflectance to calculate DRE uncertainties. We also estimate uncertainty in calculated diurnally-averaged DRE due to diurnal aerosol variability. Aerosol DRE at both the TOA and surface is most sensitive to changes in AOD, followed by single-scattering albedo (ω0). One exception is under the high summertime aerosol loading conditions (AOD  ≥  0.15 at 550 nm), when sensitivity of TOA DRE to ω0 is comparable to that of AOD. Aerosol DRE is less sensitive to changes in scattering asymmetry parameter (g) and surface reflectance (R). While DRE sensitivity to AOD varies by only ∼ 25 to 30 % with season, DRE sensitivity to ω0, g, and R largely follow the annual AOD cycle at APP, varying by factors of 8 to 15 with season. Since the measurement uncertainties of AOD, ω0, g, and R are comparable at Appalachian State, their relative contributions to DRE uncertainty are largely influenced by their (seasonally dependent) DRE sensitivity values, which suggests that the seasonal dependence of DRE uncertainty must be accounted for. Clear sky aerosol DRE uncertainty at the TOA (surface) due to measurement uncertainties ranges from 0.45 (0.75 W m−2) for December to 1.1 (1.6 W m−2) for June. Expressed as a fraction of DRE computed using monthly median aerosol optical properties and surface reflectance, the DRE uncertainties at TOA (surface) are 20 to 24 % (15 to 22 %) for March, June, and September and 49 (50 %) for DEC. The relatively low DRE uncertainties are largely due to the low uncertainty in AOD measured by AERONET. Use of satellite-based AOD measurements by MODIS in the DRE calculations increases DRE uncertainties by a factor of 2 to 5 and DRE uncertainties are dominated by AOD uncertainty for all seasons. Diurnal variability in AOD (and to a lesser extent g) contributes to uncertainties in DRE calculated using daily-averaged aerosol optical properties that are slightly larger (by ∼ 20 to 30 %) than DRE uncertainties due to measurement uncertainties during summer and fall, with comparable uncertainties during winter and spring.


2021 ◽  
Author(s):  
Jonas Witthuhn ◽  
Anja Hünerbein ◽  
Hartwig Deneke ◽  
Florian Filipitsch ◽  
Stefan Wacker

<p>The radiation budget of the earth and its climate system is driven by the solar radiation, which interacts with gases, aerosol particles and clouds. Focusing on aerosol, a fundamental measure is the radiative forcing resulting from aerosol-radiation interactions (RFari) which is also known as the aerosol direct radiative effect. Quantifying the surface RFari on regional scales aids the understanding of the role of aerosol in the climate system and is important for the planning of solar energy systems.</p><p>This study is based on a one year dataset (2015) of shortwave broadband global and diffuse horizontal irradiance measured with shaded and unshaded pyranometers at 26 station across Germany within the German Weather Service (DWD) observational network. A variety of clear-sky models are utilized to quantify RFari with a clear sky fitting technique. Clear sky models used are MMAC, MRM v.6.1, METSTAT, ESRA, Heliosat-1, CEM and the simplified Solis model. As these models have not been designed to estimate the clear sky irradiance without the presence of aerosol, we evaluated the accuracy of RFari with an reference simulation.</p><p>The reference RFari is simulated using the TROPOS (Leibniz Institute of Tropospheric Research) Cloud and Aerosol Radiative Simulator (T-CARS) utilizing the offline version of the ECMWF radiation scheme (ecRad) with input data of meteorological state of the atmosphere, trace-gases and aerosol from CAMS reanalysis.</p><p>The clear sky fitting approach for this set of clear sky models agrees well with T-CARS, showing an RMSE of 6.7 Wm<sup>-2</sup> and an correlation of 0.75. The annual mean of surface RFari over the observation stations in Germany shows a value of -13.2 Wm<sup>-2</sup> as an average over all clear sky models, compared to -13.4 Wm<sup>-2</sup> from T-CARS. Out of this set of clear sky models, best performance is shown by the ESRA and MRM v6.1 models. Although, the accuracy of the annual mean RFari from the clear sky fitting approach is strongly depended on the number available clear-sky irradiance measurements and its distribution over the year. Therefore, this approach is not recommended for climatological studies, but may serve as valuable information for e.g. the evaluation of power generation and the influence by aerosol of photo-voltaic power plants.</p>


2017 ◽  
Author(s):  
James P. Sherman ◽  
Allison McComiskey

Abstract. Aerosol optical properties measured at Appalachian State University's co-located NASA AERONET and NOAA ESRL aerosol network monitoring sites over a nearly four-year period (June 2012 thru February 2016) are used, along with satellite-based surface reflectance measurements, to study the seasonal variability of diurnally averaged clear sky aerosol direct radiative effect (DRE) and radiative efficiency (RE) at the top-of-atmosphere (TOA) and at the surface. Aerosol chemistry and loading at the Appalachian State site are likely representative of the background southeast U.S. (SE U.S.), home to high summertime aerosol loading and one of only a few regions not to have warmed during the 20th century. This study is the first multi-year ground truth DRE study in the SE U.S., using aerosol network data products that are often used to validate satellite-based aerosol retrievals. The study is also the first in the SE U.S. to quantify DRE uncertainties and sensitivities to aerosol optical properties and surface reflectance, including their seasonal dependence. Median DRE for the study period is −2.9 W m−2 at the TOA and −6.1 Wm−2 at the surface. Monthly median and monthly mean DRE at the TOA (surface) are −1 to −2 W m−2 (−2 to −3 W m−2) during winter months and −5 to −6 W m−2 (−10 W m−2) during summer months. The DRE cycles follow the annual cycle of aerosol optical depth (AOD), which is 9 to 10 times larger in summer than in winter. Aerosol RE is anti-correlated with DRE, with winter values 1.5 to 2 times more negative than summer values. Due to the large seasonal dependence of aerosol DRE and RE, we quantify the sensitivity of DRE to aerosol optical properties and surface reflectance, using a calendar day representative of each season (21 December for winter; 21 March for spring, 21 June for summer, and 21 September for fall). We use these sensitivities along with measurement uncertainties of aerosol optical properties and surface reflectance to calculate DRE uncertainties. Aerosol DRE at both the TOA and surface is most sensitive to changes in AOD, followed (in order) by single-scattering albedo (ω0), scattering asymmetry parameter (g), and surface reflectance (R). One exception is under the high summertime aerosol loading conditions, when sensitivity of TOA DRE to ω0 is comparable to that of AOD. While DRE sensitivity to AOD varies by only ~ 25 to 30 % with season, DRE sensitivity to ω0, g, and R vary by factors of 10 to 20 with season. Since the measurement uncertainties of AOD, ω0, g, and R are comparable at Appalachian State, their relative contributions to DRE uncertainty are roughly proportional to their (seasonally dependent) DRE sensitivity values, which suggests that the seasonal dependence of DRE uncertainty must be accounted for. Clear sky aerosol DRE uncertainty at the TOA (surface) ranges from 0.44 W m−2 (0.73 W m−2) for December to 0.90 W m−2 (1.3 W m−2) for June. Expressed as a fraction of DRE computed using monthly median aerosol optical properties and surface reflectance, the DRE uncertainties at TOA (surface) are 16 to 20 % (12 to 20 %) for March, June, and September and 48 % (49 %) for December. The relatively low DRE uncertainties are largely due to the low uncertainty in AOD measured by AERONET. Use of satellite-based AOD measurements by MODIS in the DRE calculations increases DRE uncertainties by a factor of 2.5 to 5 and DRE uncertainties are dominated by AOD uncertainty for all seasons.


2016 ◽  
Vol 16 (9) ◽  
pp. 5933-5948 ◽  
Author(s):  
Emily Gleeson ◽  
Velle Toll ◽  
Kristian Pagh Nielsen ◽  
Laura Rontu ◽  
Ján Mašek

Abstract. The direct shortwave radiative effect of aerosols under clear-sky conditions in the Aire Limitee Adaptation dynamique Developpement InterNational – High Resolution Limited Area Model (ALADIN-HIRLAM) numerical weather prediction system was investigated using three shortwave radiation schemes in diagnostic single-column experiments: the Integrated Forecast System (IFS), acraneb2 and the hlradia radiation schemes. The multi-band IFS scheme was formerly used operationally by the European Centre for Medium Range Weather Forecasts (ECMWF) whereas hlradia and acraneb2 are broadband schemes. The former is a new version of the HIRLAM radiation scheme while acraneb2 is the radiation scheme in the ALARO-1 physics package. The aim was to evaluate the strengths and weaknesses of the numerical weather prediction (NWP) system regarding aerosols and to prepare it for use of real-time aerosol information. The experiments were run with particular focus on the August 2010 Russian wildfire case. Each of the three radiation schemes accurately (within ±4 % at midday) simulates the direct shortwave aerosol effect when observed aerosol optical properties are used. When the aerosols were excluded from the simulations, errors of more than +15 % in global shortwave irradiance were found at midday, with the error reduced to +10 % when standard climatological aerosols were used. An error of −11 % was seen at midday if only observed aerosol optical depths at 550 nm, and not observation-based spectral dependence of aerosol optical depth, single scattering albedos and asymmetry factors, were included in the simulations. This demonstrates the importance of using the correct aerosol optical properties. The dependency of the direct radiative effect of aerosols on relative humidity was tested and shown to be within ±6 % in this case. By modifying the assumptions about the shape of the IFS climatological vertical aerosol profile, the inherent uncertainties associated with assuming fixed vertical profiles were investigated. The shortwave heating rates in the boundary layer changed by up to a factor of 2 in response to the aerosol vertical distribution without changing the total aerosol optical depth. Finally, we tested the radiative transfer approximations used in the three radiation schemes for typical aerosol optical properties compared to the accurate DISORT model. These approximations are found to be accurate to within ±13 % even for large aerosol loads.


2018 ◽  
Vol 37 ◽  
pp. 03004
Author(s):  
Abdelouahid Tahiri ◽  
Mohamed Diouri

The atmospheric aerosol contributes to the definition of the climate with direct effect, the diffusion and absorption of solar and terrestrial radiations, and indirect, the cloud formation process where aerosols behave as condensation nuclei and alter the optical properties. Satellites and ground-based networks (solar photometers) allow the terrestrial aerosol observation and the determination of impact. Desert aerosol considered among the main types of tropospheric aerosols whose optical property uncertainties are still quite important. The analysis concerns the optical parameters recorded in 2015 at Ouarzazate solar photometric station (AERONET/PHOTONS network, http://aeronet.gsfc.nasa.gov/) close to Saharan zone. The daily average aerosol optical depthτaer at 0.5μm, are relatively high in summer and less degree in spring (from 0.01 to 1.82). Daily average of the Angstrom coefficients α vary between 0.01 and 1.55. The daily average of aerosol radiative forcing at the surface range between -150W/m2 and -10 W/m2 with peaks recorded in summer, characterized locally by large loads of desert aerosol in agreement with the advections of the Southeast of Morocco. Those recorded at the Top of the atmosphere show a variation from -74 W/m2 to +24 W/m2


2014 ◽  
Vol 7 (5) ◽  
pp. 2503-2516 ◽  
Author(s):  
K. Klingmüller ◽  
B. Steil ◽  
C. Brühl ◽  
H. Tost ◽  
J. Lelieveld

Abstract. The modelling of aerosol radiative forcing is a major cause of uncertainty in the assessment of global and regional atmospheric energy budgets and climate change. One reason is the strong dependence of the aerosol optical properties on the mixing state of aerosol components, such as absorbing black carbon and, predominantly scattering sulfates. Using a new column version of the aerosol optical properties and radiative-transfer code of the ECHAM/MESSy atmospheric-chemistry–climate model (EMAC), we study the radiative transfer applying various mixing states. The aerosol optics code builds on the AEROPT (AERosol OPTical properties) submodel, which assumes homogeneous internal mixing utilising the volume average refractive index mixing rule. We have extended the submodel to additionally account for external mixing, partial external mixing and multilayered particles. Furthermore, we have implemented the volume average dielectric constant and Maxwell Garnett mixing rule. We performed regional case studies considering columns over China, India and Africa, corroborating much stronger absorption by internal than external mixtures. Well-mixed aerosol is a good approximation for particles with a black-carbon core, whereas particles with black carbon at the surface absorb significantly less. Based on a model simulation for the year 2005, we calculate that the global aerosol direct radiative forcing for homogeneous internal mixing differs from that for external mixing by about 0.5 W m−2.


2016 ◽  
Author(s):  
Simone Dietmüller ◽  
Patrick Jöckel ◽  
Holger Tost ◽  
Markus Kunze ◽  
Cathrin Gellhorn ◽  
...  

Abstract. The Modular Earth Submodel System (MESSy) provides an interface to couple submodels to a basemodel via a highly flexible data management facility (Jöckel et al., 2010). In the present paper we present the four new radiation related submodels RAD, AEROPT, CLOUDOPT and ORBIT. The submodel RAD (with shortwave radiation scheme RAD_FUBRAD) simulates the radiative transfer, the submodel AEROPT calculates the aerosol optical properties, the submodel CLOUDOPT calculates the cloud optical properties, and the submodel ORBIT is responsible for Earth orbit calculations. These submodels are coupled via the standard MESSy infrastructure and are largely based on the original radiation scheme of the general circulation model ECHAM5, however, expanded with additional features. These features comprise, among others, user-friendly and flexibly controllable (by namelists) on-line radiative forcing calculations by multiple diagnostic calls of the radiation routines. With this, it is now possible to calculate radiative forcing (instantaneous as well as stratosphere adjusted) of various greenhouse gases simultaneously in only one simulation, as well as the radiative forcing of cloud perturbations. Examples of on-line radiative forcing calculations in the ECHAM/MESSy Atmospheric Chemistry (EMAC) model are presented.


2021 ◽  
Author(s):  
Oscar Rojas ◽  
Marjolaine Chiriaco ◽  
Sophie Bastin ◽  
Justine Ringard

Abstract. Local temperature variations at the surface are mainly dominated by small-scale processes coupled through the surface energy budget terms, which depend mostly on radiation availability and thus cloud processes. A method to determine each of these terms based almost exclusively on observations is presented in this paper, with the main objective to estimate their importance in hourly surface temperature variations at the SIRTA observatory, near Paris. Almost all terms are estimated from the multi-year dataset SIRTA-ReOBS, following a few parametrizations. The four main terms acting on temperature variations are radiative forcing (separated into clear-sky and cloud radiation), atmospheric heat exchange, ground heat exchange, and advection. Compared to direct measurements of hourly temperature variations, it is shown that the sum of the four terms gives a good estimate of the hourly temperature variations, allowing a better assessment of the contribution of each term to the variation, with an accurate diurnal and annual cycles representation, especially for the radiative terms. A random forest analysis shows that whatever the season, clouds are the main modulator of the clear sky radiation for 1-hour temperature variations during the day, and mainly drive these 1-hour temperature variations during the night. Then, the specific role of clouds is analyzed exclusively in cloudy conditions considering the behavior of some classical meteorological variables along with lidar profiles. Cloud radiative effect in shortwave and longwave and lidar profiles show a consistent seasonality during the daytime, with a dominance of mid- and high-level clouds detected at the SIRTA observatory, which also affects surface temperatures and upward sensible heat flux. During the nighttime, despite cloudy conditions and having a strong cloud longwave radiative effect, temperatures are the lowest and are therefore mostly controlled by larger-scale processes at this time.


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