scholarly journals Systematic satellite observations of the impact of aerosols from passive volcanic degassing on local cloud properties

2014 ◽  
Vol 14 (19) ◽  
pp. 10601-10618 ◽  
Author(s):  
S. K. Ebmeier ◽  
A. M. Sayer ◽  
R. G. Grainger ◽  
T. A. Mather ◽  
E. Carboni

Abstract. The impact of volcanic emissions, especially from passive degassing and minor explosions, is a source of uncertainty in estimations of aerosol indirect effects. Observations of the impact of volcanic aerosol on clouds contribute to our understanding of both present-day atmospheric properties and of the pre-industrial baseline necessary to assess aerosol radiative forcing. We present systematic measurements over several years at multiple active and inactive volcanic islands in regions of low present-day aerosol burden. The time-averaged indirect aerosol effects within 200 km downwind of island volcanoes are observed using Moderate Resolution Imaging Spectroradiometer (MODIS, 2002–2013) and Advanced Along-Track Scanning Radiometer (AATSR, 2002–2008) data. Retrievals of aerosol and cloud properties at Kīlauea (Hawai'i), Yasur (Vanuatu) and Piton de la Fournaise (la Réunion) are rotated about the volcanic vent to be parallel to wind direction, so that upwind and downwind retrievals can be compared. The emissions from all three volcanoes – including those from passive degassing, Strombolian activity and minor explosions – lead to measurably increased aerosol optical depth downwind of the active vent. Average cloud droplet effective radius is lower downwind of the volcano in all cases, with the peak difference ranging from 2–8 μm at the different volcanoes in different seasons. Estimations of the difference in Top of Atmosphere upward Short Wave flux upwind and downwind of the active volcanoes from NASA's Clouds and the Earth's Radiant Energy System (CERES) suggest a downwind elevation of between 10 and 45 Wm−2 at distances of 150–400 km from the volcano, with much greater local (< 80 km) effects. Comparison of these observations with cloud properties at isolated islands without degassing or erupting volcanoes suggests that these patterns are not purely orographic in origin. Our observations of unpolluted, isolated marine settings may capture processes similar to those in the pre-industrial marine atmosphere.

2014 ◽  
Vol 14 (2) ◽  
pp. 2675-2716
Author(s):  
S. K. Ebmeier ◽  
A. M. Sayer ◽  
R. G. Grainger ◽  
T. A. Mather ◽  
E. Carboni

Abstract. The impact of volcanic emissions is a significant source of uncertainty in estimations of aerosol indirect radiative forcing, especially with respect to emissions from passive degassing and minor explosions. Understanding the impact of volcanic emissions on indirect radiative forcing is important for assessing present day atmospheric properties and also to define the pre-industrial baseline to assess anthropogenic perturbations. We present observations of the time-averaged indirect aerosol effect within 200 km downwind of isolated island volcanoes in regions of low present-day aerosol burden using MODIS and AATSR data. Retrievals of aerosol and cloud properties at Kīlauea (Hawai'i), Yasur (Vanuatu) and Piton de la Fournaise (Réunion) are rotated about the volcanic vent according to wind direction, so that retrievals downwind of the volcano can be averaged to improve signal to noise ratio. The emissions from all three volcanoes, including those from passive degassing, strombolian activity and minor explosions lead to measurably increased aerosol optical depth downwind of the active vent. Average cloud droplet effective radius is lower downwind of the volcano in all cases, with the peak difference in effective radius of 4–8 μm at the different volcanoes. A comparison of these observations with cloud properties at isolated islands with no significant source of aerosol suggests that these patterns are not purely orographic in origin. This approach sets out a first step for the systematic measurement of the effects of present day low altitude volcanic emissions on cloud properties. Our observations of unpolluted, isolated marine settings may also capture processes similar to those in the pre-industrial marine atmosphere.


2021 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Daniel T. McCoy ◽  
Ewan Crosbie ◽  
Richard H. Moore ◽  
Graeme J. Nott ◽  
...  

Abstract. Cloud droplet number concentration (Nd) is of central importance to observation-based estimates of aerosol indirect effects, being used to quantify both the cloud sensitivity to aerosol and the base state of the cloud. However, the derivation of Nd from satellite data depends on a number of assumptions about the cloud and the accuracy of the retrievals of the cloud properties from which it is derived, making it prone to systematic biases. A number of sampling strategies have been proposed to address these biases by selecting the most accurate Nd retrievals in the satellite data. This work compares the impact of these strategies on the accuracy of the satellite retrieved Nd, using a selection of insitu measurements. In stratocumulus regions, the MODIS Nd retrieval is able to achieve a high precision (r2 of 0.5–0.8). This is lower in other cloud regimes, but can be increased by appropriate sampling choices. Although the Nd sampling can have significant effects on the Nd climatology, it produces only a 20 % variation in the implied radiative forcing from aerosol-cloud interactions, with the choice of aerosol proxy driving the overall uncertainty. The results are summarised into recommendations for using MODIS Nd products and appropriate sampling.


2020 ◽  
Vol 20 (1) ◽  
pp. 613-623 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Johannes Mülmenstädt ◽  
Andrew Gettelman ◽  
Florent F. Malavelle ◽  
Hugh Morrison ◽  
...  

Abstract. The radiative forcing from aerosols (particularly through their interaction with clouds) remains one of the most uncertain components of the human forcing of the climate. Observation-based studies have typically found a smaller aerosol effective radiative forcing than in model simulations and were given preferential weighting in the Intergovernmental Panel on Climate Change (IPCC) Fifth Assessment Report (AR5). With their own sources of uncertainty, it is not clear that observation-based estimates are more reliable. Understanding the source of the model and observational differences is thus vital to reduce uncertainty in the impact of aerosols on the climate. These reported discrepancies arise from the different methods of separating the components of aerosol forcing used in model and observational studies. Applying the observational decomposition to global climate model (GCM) output, the two different lines of evidence are surprisingly similar, with a much better agreement on the magnitude of aerosol impacts on cloud properties. Cloud adjustments remain a significant source of uncertainty, particularly for ice clouds. However, they are consistent with the uncertainty from observation-based methods, with the liquid water path adjustment usually enhancing the Twomey effect by less than 50 %. Depending on different sets of assumptions, this work suggests that model and observation-based estimates could be more equally weighted in future synthesis studies.


2008 ◽  
Vol 65 (6) ◽  
pp. 1773-1794 ◽  
Author(s):  
Zachary A. Eitzen ◽  
Kuan-Man Xu

Abstract A two-dimensional cloud-resolving model (CRM) is used to perform five sets of simulations of 68 deep convective cloud objects identified with Clouds and the Earth’s Radiant Energy System (CERES) data to examine their sensitivity to changes in thermodynamic and dynamic forcings. The control set of simulations uses observed sea surface temperatures (SSTs) and is forced by advective cooling and moistening tendencies derived from a large-scale model analysis matched to the time and location of each cloud object. Cloud properties, such as albedo, effective cloud height, cloud ice and snow path, and cloud radiative forcing (CRF), are analyzed in terms of their frequency distributions rather than their mean values. Two sets of simulations, F+50% and F−50%, use advective tendencies that are 50% greater and 50% smaller than the control tendencies, respectively. The increased cooling and moistening tendencies cause more widespread convection in the F+50% set of simulations, resulting in clouds that are optically thicker and higher than those produced by the control and F−50% sets of simulations. The magnitudes of both longwave and shortwave CRF are skewed toward higher values with the increase in advective forcing. These significant changes in overall cloud properties are associated with a substantial increase in deep convective cloud fraction (from 0.13 for the F−50% simulations to 0.34 for the F+50% simulations) and changes in the properties of non–deep convective clouds, rather than with changes in the properties of deep convective clouds. Two other sets of simulations, SST+2K and SST−2K, use SSTs that are 2 K higher and 2 K lower than those observed, respectively. The updrafts in the SST+2K simulations tend to be slightly stronger than those of the control and SST−2K simulations, which may cause the SST+2K cloud tops to be higher. The changes in cloud properties, though smaller than those due to changes in the dynamic forcings, occur in both deep convective and non–deep convective cloud categories. The overall changes in some cloud properties are moderately significant when the SST is changed by 4 K. The changes in the domain-averaged shortwave and longwave CRFs are larger in the dynamic forcing sensitivity sets than in the SST sensitivity sets. The cloud feedback effects estimated from the SST−2K and SST+2K sets are comparable to prior studies.


2012 ◽  
Vol 12 (10) ◽  
pp. 27111-27172
Author(s):  
J. L. Petters ◽  
H. Jiang ◽  
G. Feingold ◽  
D. L. Rossiter ◽  
D. Khelif ◽  
...  

Abstract. The impact of changes in aerosol and cloud droplet concentration (Na and Nd) on the radiative forcing of stratocumulus-topped boundary layers (STBLs) has been widely studied. How these impacts compare to those due to variations in meteorological context has not been investigated in a systematic fashion. In this study we examine the impact of observed variations in meteorological context and aerosol state on daytime, non-drizzling stratiform evolution, and determine how resulting changes in cloud properties compare. We perturb aerosol and meteorological properties within an observationally-constrained LES and determine the cloud response, focusing on changes in liquid water path (LWP), bulk optical depth (τ) and cloud radiative forcing (CRF). We find that realistic variations in meteorological context (i.e. jump properties) can elicit responses in τ and shortwave (SW) CRF that are on the same order of magnitude as, and at times larger than, those responses found due to similar changes in aerosol state (i.e Nd). Further, we find that one hour differences in the timing of SW radiative heating can lead to substantial changes in LWP and τ. Our results suggest that, for observational studies of aerosol influences on the radiative properties of stratiform clouds, consistency in meteorological context (the cloud top jump properties in particular) and time of observations from day-to-day must be carefully considered.


2012 ◽  
Vol 12 (3) ◽  
pp. 8009-8051 ◽  
Author(s):  
A. Schmidt ◽  
K. S. Carslaw ◽  
G. W. Mann ◽  
A. Rap ◽  
K. J. Pringle ◽  
...  

Abstract. Observations and models have shown that continuously degassing volcanoes have a potentially large effect on the natural background aerosol loading and the radiative state of the atmosphere. Here, we use a global aerosol microphysics model to quantify the impact of these volcanic emissions on the cloud albedo radiative forcing under pre-industrial (PI) and present-day (PD) conditions. We find that volcanic degassing increases global annual mean cloud droplet number concentrations by 40% under PI conditions, but by only 10% under PD conditions. Consequently, volcanic degassing causes a global annual mean cloud albedo effect of −1.06 W m−2 in the PI era but only −0.56 W m−2 in the PD era. This non-equal effect is explained partly by the lower background aerosol concentrations in the PI era, but also because more aerosol particles are produced per unit of volcanic sulphur emission in the PI atmosphere. The higher sensitivity of the PI atmosphere to volcanic emissions has an important consequence for the anthropogenic cloud radiative forcing because the large uncertainty in volcanic emissions translates into an uncertainty in the PI baseline cloud radiative state. Assuming a −50/+100% uncertainty range in the volcanic sulphur flux, we estimate the annual mean anthropogenic cloud albedo forcing to lie between −1.16 W m−2 and −0.86 W m−2. Therefore, the volcanically induced uncertainty in the PI baseline cloud radiative state substantially adds to the already large uncertainty in the magnitude of the indirect radiative forcing of climate.


2019 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Johannes Mülmenstädt ◽  
Andrew Gettelman ◽  
Florent F. Malavelle ◽  
Hugh Morrison ◽  
...  

Abstract. The radiative forcing from aerosols (particularly through their interaction with clouds) remains one of the most uncertain components of the human forcing of the climate. Observation-based studies have typically found a smaller aerosol effective radiative forcing than in model simulations and were given preferential weighting in the IPCC AR5 report. With their own sources of uncertainty, it is not clear that observation-based estimates are more reliable. Understanding the source of the model-observational difference is thus vital to reduce uncertainty in the impact of aerosols on the climate. These reported discrepancies arise from the different decompositions of the aerosol forcing used in model and observational studies. Applying the observational decomposition to global climate model output, the two different lines of evidence are surprisingly similar, with a much better agreement on the magnitude of aerosol impacts on cloud properties. Cloud adjustments remain a significant source of uncertainty, particularly for ice clouds. However, they are consistent with the uncertainty from observation-based methods, with the liquid water path adjustment usually enhancing the Twomey effect by less than 50 %. Depending on different sets of assumptions, this work suggests that model and observation-based estimates could be more equally weighted in future synthesis studies.


2012 ◽  
Vol 12 (16) ◽  
pp. 7321-7339 ◽  
Author(s):  
A. Schmidt ◽  
K. S. Carslaw ◽  
G. W. Mann ◽  
A. Rap ◽  
K. J. Pringle ◽  
...  

Abstract. Observations and models have shown that continuously degassing volcanoes have a potentially large effect on the natural background aerosol loading and the radiative state of the atmosphere. We use a global aerosol microphysics model to quantify the impact of these volcanic emissions on the cloud albedo radiative forcing under pre-industrial (PI) and present-day (PD) conditions. We find that volcanic degassing increases global annual mean cloud droplet number concentrations by 40% under PI conditions, but by only 10% under PD conditions. Consequently, volcanic degassing causes a global annual mean cloud albedo effect of −1.06 W m−2 in the PI era but only −0.56 W m−2 in the PD era. This non-equal effect is explained partly by the lower background aerosol concentrations in the PI era, but also because more aerosol particles are produced per unit of volcanic sulphur emission in the PI atmosphere. The higher sensitivity of the PI atmosphere to volcanic emissions has an important consequence for the anthropogenic cloud radiative forcing because the large uncertainty in volcanic emissions translates into an uncertainty in the PI baseline cloud radiative state. Assuming a −50/+100% uncertainty range in the volcanic sulphur flux, we estimate the annual mean anthropogenic cloud albedo forcing to lie between −1.16 W m−2 and −0.86 W m−2. Therefore, the volcanically induced uncertainty in the PI baseline cloud radiative state substantially adds to the already large uncertainty in the magnitude of the indirect radiative forcing of climate.


2017 ◽  
Vol 14 (2) ◽  
pp. 27
Author(s):  
NFN Rosida ◽  
Indah Susanti

The direct effects of aerosols on radiation budget in Indonesia have been analyzed based on radiation flux net data from the Clouds and the Earth's Radiant Energy System (CERES) instrument and aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra. Radiation budget calculated including short wave and long-wave radiation. Data from March 2000 until February 2010, processed using Grads version 2 to obtain aerosol radiative forcing value. Net radiation in clean sky, estimated using slope method. The analysis showed high temporal variation of aerosols density in the atmosphere with a value AODmax> 2, which generally causes decreases net radiation flux, so providing a cooling effect. The influence of aerosols on the net radiation flux can be very clearly seen in the case of forest fires. AOD in 2006 increased and caused radiation flux anomalies ranging from -9 watt/m-2 to -14 watts/m-2, with the largest decline occurred in the surface. From all the data period, aerosol radiative forcing at TOA level (ARFTOA) on Indonesia was -0.49 watt/m-2 and aerosol radiative forcing at the surface level (ARFSurf) on Indonesia was -17.72 watt/m-2, that influence to the Indonesian climate condition.


2004 ◽  
Vol 43 (12) ◽  
pp. 1818-1833 ◽  
Author(s):  
Maria João Costa ◽  
Vincenzo Levizzani ◽  
Ana Maria Silva

Abstract A method based on the synergistic use of low earth orbit and geostationary earth orbit satellite data for aerosol-type characterization and aerosol optical thickness (AOT: τa) retrieval and monitoring over the ocean is presented in Part I of this paper. The method is now applied to a strong dust outbreak over the Atlantic Ocean in June 1997 and to two other relevant transport events of biomass burning and desert dust aerosol that occurred in 2000 over the Atlantic and Indian Oceans, respectively. The retrievals of the aerosol optical properties are checked against retrievals from sun and sky radiance measurements from the ground-based Aerosol Robotic Network (AERONET). The single-scattering albedo values obtained from AERONET are always within the error bars presented for Global Ozone Monitoring Experiment (GOME) retrievals, resulting in differences lower than 0.041. The retrieved AOT values are compared with the independent space–time-collocated measurements from the AERONET, as well as to the satellite aerosol official products of the Polarization and Directionality of the Earth Reflectances (POLDER) and the Moderate Resolution Imaging Spectroradiometer (MODIS). A first estimate of the AOT accuracy derived from comparisons with AERONET data leads to ±0.02 ± 0.22τa when all AOT values are retained or to ±0.02 ± 0.16τa for aerosol transport events (AOT &gt; 0.4). The upwelling flux at the top of the atmosphere (TOA) was computed with radiative transfer calculations and used to estimate the TOA direct shortwave aerosol radiative forcing; a comparison with space–time-collocated measurements from the Clouds and the Earth's Radiant Energy System (CERES) TOA flux product was also done. It was found that more than 90% of the values differ from CERES fluxes by less than ±15%.


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